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Zhongwu Li Hao Peng Binggeng Xie Chun Liu Xiaodong Nie Danyang Wang Mei Huang Haibing Xiao Lin Shi Xuqin Zhang Jieyu Jiang 《水文研究》2020,34(6):1446-1459
Exploring the chemical characterization of dissolved organic matter (DOM) is important for understanding the fate of laterally transported organic matter in watersheds. We hypothesized that differences in water-extractable organic matter (WEOM) in soils of varying land uses and rainfall events may significantly affect the quality and the quantity of stream DOM. To test our hypotheses, characteristics of rainfall-runoff DOM and WEOM of source materials (topsoil from different land uses and gullies, as well as typical vegetation) were investigated at two adjacent catchments in the Loess Plateau of China, using ultraviolet–visible absorbance and excitation emission matrix fluorescence with parallel factor analysis (PARAFAC). Results indicated that land-use types may significantly affect the chemical composition of soil WEOM, including its aromaticity, molecular weight, and degree of humification. The PARAFAC analysis demonstrated that the soils and stream water were dominated by terrestrial/allochthonous humic-like substances and microbial transformable humic-like fluorophores. Shifts in the fluorescence properties of stream DOM suggested a pronounced change in the relative proportion of allochthonous versus autochthonous material under different rainfall patterns and land uses. For example, high proportions of forestland could provide more allochthonous DOM input. This study highlights the relevance of soils and hydrological dynamics on the composition and fluxes of DOM issuing from watersheds. The composition of DOM in soils was influenced by land-use type. Precipitation patterns influenced the proportion of terrestrial versus microbial origins of DOM in surface runoff. Contributions of allochthonous, terrestrially derived DOM inputs were highest from forested landscapes. 相似文献
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本文以全国化工产业密集区——长三角地区为例,基于规模以上中国工业企业详细数据,从化工企业入园率的视角出发,综合运用均值中心、标准差椭圆、核密度分析及空间自相关等分析方法,分析并揭示了1998—2013年长三角地区化工产业时空格局演化规律及影响因素。研究结果表明：1998—2013年长三角地区化工企业总体上呈现不断增长趋势,入园率由6.19%提升到36.98%;化工企业“西北-东南”方向分布明显,且近似呈“先东南,后西北”的路径迁移规律,较之全部企业,入园企业具有更高的离散度、更大的迁移幅度,入园企业与全部企业逐步由空间失配演变为空间匹配;中心集聚与外围扩散态势并存,发育并逐渐形成了环太湖集聚区、沿杭州湾集聚区、沿长江密集带及沿海密集带四大化工产业集聚片区,化工产业的区域空间结构趋于复杂化、有序化与稳定化;地级尺度上化工企业入园率不断提升,2003年与2013年呈显著的空间正相关,热点区逐渐由浙江东南转移到苏皖北部,冷点区从安徽北部迁移到浙江西北,基本完成了空间格局上的对称反转变换,但化工企业入园率与空间密度分布一直处于错配失衡状态。通过结合化工产业特性与长三角区域特征,定性探讨了长三角地区化工产业时空格局演化的影响因素,特别是阐述了化工产业“园区化”进程的作用机制。 相似文献
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DDM波形是GNSS-R技术用于反演地球物理参量的基本观测量,其仿真结果的可靠性直接影响GNSS-R的理论研究及项目工程参数设计。利用GREEPS仿真软件分析了时延间隔与多普勒间隔对DDM波形仿真结果可靠性的影响,得到了用于获取可靠DDM仿真波形的时延与多普勒间隔参数。研究表明,时延和多普勒间隔越小,DDM仿真波形与理论波形吻合度越高;当时延间隔取1/16个GPS L1 C/A码元、多普勒间隔取50 Hz时,DDM仿真波形与理论波形几乎完全吻合,二者的相关系数大于0.99;时延间隔对DDM仿真波形峰值位置的影响远大于对峰值信噪比的影响;而多普勒间隔对DDM仿真波形峰值位置与信噪比的影响相当。 相似文献
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通过对比星载DPR雷达与地基CINRAD雷达的降雨测量值,评估星地雷达联合应用的潜力。为了提高对比的准确性,在尽可能高的时空分辨率下,以几何匹配与格点匹配相结合的方式,提取星地雷达降水样本数据。2015年6月30日降水过程的对比分析结果表明:泰州、常州CINRAD雷达反射率因子在两站中分剖面的平均值偏差0.94 dB,地基雷达之间有很好的一致性;在DPR雷达与常州、泰州CINRAD雷达同时覆盖的降雨区域,星地之间雷达反射率因子的平均值偏差分别为-1.2 dB和-1.6 dB,显示星地雷达也有较好的一致性;现有DPR雷达陆上衰减订正算法在缩小星地雷达偏差方面起到一定作用,平均订正量0.4 dB,只要回波覆盖充分,匹配样本的高度以及其到地基雷达的距离对对比结果没有明显影响,而衰减订正和匹配样本区回波覆盖率是影响星地雷达对比结果的重要因素。 相似文献
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Danyang Li Minfang Zheng Yusheng Qiu Limin Lai Nengwang Chen Hongmei Jing Run Zhang Min Chen 《海洋学报(英文版)》2023,42(1):75-82
Nitrogen fixation is one of the most important sources of new nitrogen in the ocean and thus profoundly affects the nitrogen and carbon biogeochemical processes. The distribution, controlling factors, and flux of N2 fixation in the global ocean remain uncertain, partly because of the lack of methodological uniformity. The 15N2 tracer assay (the original bubble method → the 15N2-enriched seawater method → the modified bubble method) is the mainstream method for field measurements of N2 fixation rates (NFRs), among which the original bubble method is the most frequently used. However, accumulating evidence has suggested an underestimation of NFRs when using this method. To improve the availability of previous data, we compared NFRs measured by three 15N2 tracer assays in the South China Sea. Our results indicate that the relationship between NFRs measured by the original bubble method and the 15N2-enriched seawater method varies obviously with area and season, which may be influenced by incubation time, diazotrophic composition, and environmental factors. In comparison, the relationship between NFRs measured by the original bubble method and the modified bubble method is more stable, indicating that the N2 fixation rates based on the original bubble methods may be underestimated by approximately 50%. Based on this result, we revised the flux of N2 fixation in the South China Sea to 40 mmol/(m2·a). Our results improve the availability and comparability of literature NFR data in the South China Sea. The comparison of the 15N2 tracer assay for NFRs measurements on a larger scale is urgently necessary over the global ocean for a more robust understanding of the role of N2 fixation in the marine nitrogen cycle. 相似文献
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2022年夏季长江流域遭受极端干旱,在此背景下,围绕长江荆江河段(松滋-城陵矶),东、西、南洞庭湖,松滋河、虎渡河、藕池河三口水系,湘江、资水、沅江、澧水四水尾间河段,以及环洞庭湖主要垸区,开展了原位监测和采样工作,测定了湖泊、河道、沟渠、池塘等各类水体中氮、磷、碳等生源要素和叶绿素a浓度,以及浮游植物种类和丰度。结果显示,东、西、南洞庭湖中,总氮、总磷、溶解态有机碳和叶绿素a浓度均值分别为0.57 mg/L、0.45 mg/L、38 mg/L和5.38μg/L,氮、磷分别以溶解态和颗粒态为主;浮游植物共检出6门37种,以硅藻和绿藻为主,藻类生物量约1.337 mg/L。就综合营养状态指数而言,洞庭湖处于中营养状态,并不显著高于长江和三口四水。极端干旱导致荆江-洞庭湖的水文连通削弱,洞庭湖来自三口的生源要素通量减少,来自四水和湖内自源生产的比重增加;洞庭湖垸区与外部自然河湖的阻隔限制垸内水体自由流动,导致生源要素累积,造成富营养化。2022年极端干旱气象条件下,洞庭湖总磷、叶绿素a、浮游植物数量相比历史阶段数据处于高位,但总氮浓度低于历史水平。恢复水文连通,改善江湖关系,削减内源污染释... 相似文献
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现代涂鸦发源于欧美国家,近些年来也在中国的城市街巷空间中大量出现,并带来了一定的社会问题。通过梳理国内外学界相关研究成果,阐明了涂鸦具有建构和改变地方意义的作用。在此基础上运用尺度政治理论分析香港著名涂鸦者“九龙皇帝”曾灶财的个案,探讨了3个时期中香港政府、文化精英和曾灶财本人对其涂鸦性质的不同界定,以及相互之间的博弈过程。分析认为：香港政府在曾灶财去世后对其涂鸦的保护并不意味着对这些涂鸦艺术品性质的承认,而是面对文化精英尺度上推策略的妥协。最后探讨了尺度政治理论在当前中国城市涂鸦问题中的应用前景。 相似文献
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The current lack of high-precision information on subsurface seawater is a constraint in fishery research. Based on Argo temperature and salinity profiles, this study applied the gradient-dependent optimal interpolation to reconstruct daily subsurface oceanic environmental information according to fishery dates and locations. The relationship between subsurface information and matching yellowfin tuna(YFT) in the western and central Pacific Ocean(WCPO) was examined using catch data from January 1... 相似文献
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Distribution of the Ordovician Fluid in the Tahe Oilfield and Dynamic Response of Cave System S48 to Exploitation 总被引：2，自引：1，他引：1
The Tahe Oilfield is a complex petroleum reservoir of Ordovician carbonate formation and made up of spatially overlapping fracture-cavity units. The oilfield is controlled by a cave system resulting from structure-karst cyclic sedimentation. Due to significant heterogeneity of the reservoir, the distribution of oil and water is complicated. Horizontally, a fresh water zone due to meteoric water can be found in the north part of the Akekule uplift. A marginal freshening zone caused by water released from mudstone compaction is found at the bottom of the southern slope. Located in a crossformational flow discharge zone caused by centripetal and the centrifugal flows, the main part of the Tahe Oilfield, featuring high salinity and concentrations of CI^- and K^＋＋Na^＋, is favorable for accumulation of hydrocarbon. Three types of formation water in the Tahe Ordovician reservoir are identified： （1） residual water at the bottom of the cave after oil and gas displacement, （2） residual water in fractures/pores around the cave after oil and gas displacement, and （3） interlayer water below reservoirs. The cave system is the main reservoir space, which consists of the main cave, branch caves and depressions between caves. Taking Cave System S48 in the Ordovician reservoir as an example, the paper analyzes the fluid distribution and exploitation performance in the cave system. Owing to evaporation of groundwater during cross-formational flow, the central part of the main cave, where oil layers are thick and there is a high degree of displacement, is characterized by high salinity and Br^- concentration. With high potential and a long stable production period, most wells in the central part of the main cave have a long water-free oil production period. Even after water breakthrough, the water content has a slow or stepwise increase and the hydrochemistral characteristics of the produced water in the central part of the main cave are uniform. From the center to the edge of the main cave, displacement and enri 相似文献