Synchronous pattern of moisture availability on the southern Tibetan Plateau since 17.5 cal. ka BP – the Tangra Yumco lake sediment record     

Marieke Ahlborn  Torsten Haberzettl  Junbo Wang  Karoline Henkel  Thomas Kasper  Gerhard Daut  Liping Zhu  Roland Mäusbacher 《Boreas: An International Journal of Quaternary Research》2017,46(2):229-241

A possible asynchronicity of the spatial and temporal moisture availability on the Tibetan Plateau has been a controversial subject of discussion in recent years. Here we present the first attempt to systematically investigate possible spatial and temporal variations in moisture availability by examining two lakes, Tangra Yumco and Nam Co, on an east–west transect on the southern Tibetan Plateau using identical proxies for palaeoenvironmental reconstruction. In this study, an independent record from Tangra Yumco was analysed applying a multi‐proxy approach to reconstruct variations in moisture availability since the Lateglacial. Results were subsequently compared with previously published records from Nam Co and additional records from Tso Moriri (northwestern Himalaya) and Naleng Co (southeastern Tibetan Plateau). Our results show that Tangra Yumco was at least partially ice covered prior to 17.1 cal. ka BP. A temperature rise after 17.1 cal. ka BP probably resulted in thawing of the permafrost. At 16.0 cal. ka BP moisture availability increased, representing an initial monsoonal intensification. Warmer conditions between 13.0 and 12.4 cal. ka BP and cooler conditions between 12.4 cal. ka BP and the onset of the Holocene reflect the Bølling‐Allerød and Younger Dryas. At the onset of the Holocene moisture availability rapidly increased, with moisture highest prior to 8.5 cal. ka BP when temperatures were also highest. After 8.5 cal. ka BP the moisture availability gradually decreased and showed only minor amplitude variations. These findings are consistent with the records from large lakes like Nam Co, Tso Moriri, and Naleng Co, revealing a synchronous pattern of moisture availability on the southern Tibetan Plateau.  相似文献   

The respective roles of surface temperature driven feedbacks and tropospheric adjustment to CO2 in CMIP5 transient climate simulations     

Lorenzo Tomassini  Olivier Geoffroy  Jean-Louis Dufresne  Abderrahmane Idelkadi  Chiara Cagnazzo  Karoline Block  Thorsten Mauritsen  Marco Giorgetta  Johannes Quaas 《Climate Dynamics》2013,41(11-12):3103-3126

An overview of radiative climate feedbacks and ocean heat uptake efficiency diagnosed from idealized transient climate change experiments of 14 CMIP5 models is presented. Feedbacks explain about two times more variance in transient climate response across the models than ocean heat uptake efficiency. Cloud feedbacks can clearly be identified as the main source of inter-model spread. Models with strong longwave feedbacks in the tropics feature substantial increases in cloud ice around the tropopause suggestive of changes in cloud-top heights. The lifting of the tropical tropopause goes together with a general weakening of the tropical circulation. Distinctive inter-model differences in cloud shortwave feedbacks occur in the subtropics including the equatorward flanks of the storm-tracks. Related cloud fraction changes are not confined to low clouds but comprise middle level clouds as well. A reduction in relative humidity through the lower and mid troposphere can be identified as being the main associated large-scale feature. Experiments with prescribed sea surface temperatures are analyzed in order to investigate whether the diagnosed feedbacks from the transient climate simulations contain a tropospheric adjustment component that is not conveyed through the surface temperature response. The strengths of the climate feedbacks computed from atmosphere-only experiments with prescribed increases in sea surface temperatures, but fixed CO₂ concentrations, are close to the ones derived from the transient experiment. Only the cloud shortwave feedback exhibits discernible differences which, however, can not unequivocally be attributed to tropospheric adjustment to CO₂. Although for some models a tropospheric adjustment component is present in the global mean shortwave cloud feedback, an analysis of spatial patterns does not lend support to the view that cloud feedbacks are dominated by their tropospheric adjustment part. Nevertheless, there is positive correlation between the strength of tropospheric adjustment processes and cloud feedbacks across different climate models.  相似文献   

Homogeneous freezing of single sulfuric and nitric acid solution drops levitated in an acoustic trap     

Karoline Diehl  Matthias Ettner-Mahl  Anke Hannemann  Subir K. Mitra   《Atmospheric Research》2009,94(2):356-361

The freezing temperatures of single supercooled drops of binary and ternary sulfuric and nitric acid solutions were measured while varying the acid concentration. An acoustic levitator was used which allows to freely suspend single solution drops in air without electrical charges thereby avoiding any electrical influences which may affect the freezing process. The drops of typically 500 µm in radius were monitored by a video camera during cooling cycles down to − 85 °C to simulate the upper tropospheric and stratospheric temperature range. The present data confirm that liquid solution droplets can be supercooled far below the equilibrium melting point by approximately 35 °C. They follow the general trend of the expected freezing temperatures for homogeneous ice nucleation.  相似文献   

Laboratory studies about the interaction of ammonia with ice crystals at temperatures between 0 and −20°C     

Ines Hoog  Subir K. Mitra  Karoline Diehl  Stephan Borrmann 《Journal of Atmospheric Chemistry》2007,57(1):73-84

In laboratory experiments the interactions of ammonia with ice crystals were studied within the temperature range between 0 and −20°C. In a first series of experiments dendritic ice crystals were grown from water vapor in presence of ammonia gas in various concentrations between 4 and 400 ppbv. In a second series of experiments pure ice crystals were exposed to a humidified ammonia–air mixture inside a horizontal flow tube. The influence of temperature, ammonia gas concentration (0.6, 1.5, and 10 ppmv), exposure time, and the presence of impurities such as sulfate on the ammonia uptake by the ice surface was investigated by determining the ammonium content in the melt water of the ice crystals by ion chromatography. During the growth of ice crystals significant amounts of ammonia (around 200 μg/l) were taken up even at small gas concentrations. In contrast, even at high gas concentrations the uptake of ammonia by non-growing ice crystals was lower by approximately one order of magnitude. The presence of sulfate on the ice surface affected an enhanced uptake of ammonia by a factor of 5–10. A model is presented which describes the uptake of ammonia by ice considering the chemical processes occurring in the ice surface layer and simultaneous diffusion of ammonia into bulk ice. Even the increased uptake of ammonia by growing ice is rather small compared to the uptake by water droplets; thus, the major process for scavenging of ammonia from the atmosphere via the ice phase might not be the direct uptake by ice crystals but the riming involving super-cooled droplets containing ammonia.  相似文献   

The retention of ammonia and sulfur dioxide during riming of ice particles and dendritic snow flakes: laboratory experiments in the Mainz vertical wind tunnel     

Nadine v. Blohn  Karoline Diehl  Anke Nölscher  Alexander Jost  Subir K. Mitra  Stephan Borrmann 《Journal of Atmospheric Chemistry》2013,70(2):131-150

Laboratory experiments were carried out in the Mainz vertical wind tunnel to determine the retention of the trace gases ammonia and sulfur dioxide dissolved in supercooled cloud droplets during riming. The conditions during riming were similar to the ones in atmospheric mixed phase clouds: temperatures from ?18 °C to ?5 °C, liquid water contents between 1 and 1.5 g m^?3, liquid drop radii between 10 and 20 μm, liquid phase concentrations from 1 to 22 mg/l. As collectors, floating ice particles and snow flakes with diameters between 6 mm and 1.5 cm were used. After riming the retention coefficients, i.e. the fractions of the species which remained in the ice phase after freezing were determined. Retention coefficients lying between 0.1 and 1.0 were measured depending on the solubility and dissociation of the trace gas, liquid phase concentration, ambient air temperature, and shape of rimed collector. This can be explained from the chemists’ point of view by the effective Henry’s law constant of the species and physically with the rate of latent heat removal from the rimed collector during freezing. Parameterizations derived from the different experimental cases describe the retention coefficients as a function of temperature. In general, an average retention of ammonia of 92?±?21 % was determined independently of liquid phase concentration while mean values for sulfur dioxide were 53?±?10 % at low liquid phase concentrations and 29?±?7 % at high liquid phase concentrations.  相似文献   

The ice nucleating ability of pollen: Part III: New laboratory studies in immersion and contact freezing modes including more pollen types     

Nadine von Blohn  Subir K. Mitra  Karoline Diehl  Stephan Borrmann   《Atmospheric Research》2005,78(3-4):182-189

Based on earlier experimental studies, the ice nucleating abilities of further pollen types were investigated in the immersion and contact freezing modes. The studies were carried out at the Mainz vertical wind tunnel with freely floating supercooled droplets down to − 28 °C. The pollen had diameters between 26 and 28 μm and correspondingly low sink velocities around 2.5 cm s^{− 1}. The radii of the studied drops were calculated from the recorded wind velocity and for both freezing modes the radii of the observed droplets varied between 315 and 380 μm. Immersion freezing experiments were conducted with pollen particles added to the droplets while in contact freezing experiments supercooled droplets were subjected to a burst of pollen particles. The median freezing temperatures found in the immersion freezing mode were: − 13.5 °C (alder), − 21.5 °C (lombardy poplar), − 21.0 °C (redtop grass) and − 19.8 °C (kentucky blue). The median freezing temperatures in the contact freezing mode were found as: − 12.6 °C (alder), − 17.9 °C (lombardy poplar), − 18.7 °C (redtop grass) and − 16.1 °C (kentucky blue). The results show that the ice nucleating ability of pollen is not restricted to single pollen types but seems to be a general pollen property.  相似文献   

Structural and thermal controls of rockfall frequency and magnitude within rockwall–talus systems (Swiss Alps)          下载免费PDF全文

Karoline Messenzehl  Richard Dikau 《地球表面变化过程与地形》2017,42(13):1963-1981

Both from a systemic and natural hazard perspective, it is essential to understand the causes and frequency of rockfalls in mountain terrain and to predict the block sizes deposited at specific locations. Commonly, rockfalls are studied either retrospectively, using talus slopes, or directly by rockwall surveys. Nevertheless, our understanding of rockfall activity, particularly at the lower magnitude spectrum, is still incomplete. Moreover, the explanatory framework is rarely addressed explicitly. In this study, we investigate two rockwall–talus systems in the Swiss Alps to estimate the rockfall frequency–magnitude pattern and their key controls. We present a holistic approach that integrates deductive geotechnical and thermal investigations of the source rockwalls with abductive talus‐based explanations of rockfall volume and frequency. The rockwalls' three‐dimensional (3D) joint pattern indicates that 75% of the blocks may be released as debris fall (< 14 m³) and boulder falls (14–61 m³), which is mirrored in the corresponding talus material. Using two‐year records of near‐surface rockwall temperatures as input for a 1D heat conduction model underlines the destabilizing role of seasonal ice segregation. Deepest frost cracking of 300 cm may occur on the north‐northeast (NNE)‐exposed, snow‐rich rockwall, with peaks at the outermost surface. The synthesis of all data suggests that infrequent, large planar slides (approximately every 250 years) overlain by smaller, more frequent wedge and toppling failures (approximately every 17–50 years) as well as high‐frequency flake‐like clasts (3–6 events/year) characterize the rockfall frequency–magnitude pattern at Hungerli Peak. Here, we argue that small‐size rockfalls need more scientific attention, particularly in discontinuous permafrost zones. Our study emphasizes that future frequency–magnitude research should ideally incorporate site‐specific structural and thermal properties, rather than just focusing on climatic or meteorological triggers. We discuss how holistic rockwall–talus approaches, as proposed here, could help to increase our process understanding of rockfalls in mountain environments. Copyright © 2017 John Wiley & Sons, Ltd.  相似文献   

Origins and genesis of loess deposits in central Spain,as indicated by heavy mineral compositions and grain‐size variability     

Daniel Wolf  Karoline Ryborz  Thomas Kolb  Ruben Calvo Zapata  Jesús Sanchez Vizcaino  Ludwig Zller  Dominik Faust 《Sedimentology》2019,66(3):1139-1161

The formation of loess deposits strongly depends on the availability of deflatable dust‐sized material. Identification of source areas and mechanisms of dust production is essential for an appropriate characterization of related palaeoenvironmental conditions. So far, little research has been done on loess deposits in the Mediterranean region and information about mechanisms of dust production is very rare. In this context, it is not clear from where the loess deposits from the upper Tagus Basin in central Spain originated. The main objective of this study was to find out whether these loess deposits were formed primarily by mountain processes and fluvial comminution, or whether they have their origin in the weathering of Tertiary marls in the centre of the Madrid Basin. A further concern was to link the determined source areas with loess formation mechanisms and concomitant environmental contexts. Following a comprehensive approach using heavy minerals and grain‐size data, together with information on stratigraphic features and geomorphic positions, different local loess sources could be identified. This study shows that during the last 35 kyr a major proportion of the Tagus loess deposits was deflated from river floodplains, while the mountain region of the Iberian Range was identified as a significant source of respective floodplain sediments. Based on heavy mineral compositions and dating results, it was found that during Heinrich Stadial 3, sediment supply from the Iberian Range strongly increased, suggesting an environmental shift from initially warmer towards colder temperatures in late Marine Isotope Stage 3. Furthermore, it was found that grain‐size patterns clearly indicate maximum wind strengths during Heinrich Stadial 3, followed by Heinrich Stadial 2 and Heinrich Stadial 1. These results demonstrate that the formation of dust‐sized particles in this part of the Mediterranean operated similar to many other places in temperate and continental regions, and that weathering processes linked to hot and dry environments were only of minor importance.  相似文献