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1.
本文阐明了长江下游水体中的主要溶解组分,主要是由蒸发岩和碳酸盐经化学风化作用所提供的。其中,SO_4部分由化石燃料燃烧后生成的SO_2在大气中氧化成SO_3,并随降雨生成H_2SO_4而进入河水,同时还分析了长江在入海过程中,各溶解组分的浓度受物理混合的影响以及可能发生的转移和溶出作用。 相似文献
2.
Accumulation of petroleum hydrocarbons and heavy metals in clams （Ruditapes philippinarum） in Jiaozhou Bay, China 总被引：2，自引：0，他引：2
Accumulation and distributions of aliphatic and polyaromatic hydrocarbons (PAHs) and heavy metals were measured in tissues
of the clam Ruditapes philippinarum collected from 5 sites in Jiaozhou Bay, Qingdao, China. The concentrations of total aliphatic hydrocarbon and PAHs ranged
from 570 to 2 574 ng/gdw (gram dry weight) and from 276 to 939 ng/gdw, in the most and least polluted sites, respectively.
The bio-accumulation of hydrocarbons and PAHs in the clams appeared to be selective. Aliphatic hydrocarbons were predominantly
represented by short chain (<nC23) n-alkanes, suggesting that petroleum hydrocarbons were likely the major contamination source. The selective uptake of 3 and
4 ring PAHs, such as naphthalene, fluorene, phenanthrene, fluoranthene and pyrene, by the clams was probably related to the
physiological and bio-kinetic processes that were energetically favorable for uptake of compounds with fewer rings. Accumulation
of the metals Cd, Cu, Zn, Pb, Cr, Hg, and As in the clam tissues also showed high variability, ranging from 0.043 to 87 μg/gdw.
Among the 7 detected metals, Zn, Cd, Cu, and As had a particularly high potential of accumulation in R. philippinarum. In general, a positive correlation was found between the tissue concentrations and sediment concentrations of hydrocarbons
and of some metals. Our study suggests that moderate contamination with polyaromatic hydrocarbons, and low to moderate contamination
with metals, currently exists for clam R. philippinarum in Jiaozhou Bay, in comparison with other regional studies. A long-term monitoring program is certainly needed for assessment
of the potential ecological influence and toxicity of these contaminants of R. philippinarum in Jiaozhou Bay. 相似文献
3.
Black carbon and polycyclic aromatic hydrocarbons (PAHs) in surface sediments of China’s marginal seas 总被引：8，自引：0，他引：8
This study investigates the distribution of black carbon (BC) and its correlation with total polycyclic aromatic hydrocarbons (ΣPAH) in the surface sediments of China’s marginal seas. BC content ranges from <0.10 to 2.45 mg/g dw (grams dry weight) in the sediments studied, and varied among the different coastal regions. The Bohai Bay sediments had the highest BC contents (average 2.18 mg/g dw), which comprises a significant fraction (27%–41%) of the total organic carbon (TOC) preserved in the sediments. In ... 相似文献
4.
Decomposition of algal lipids in clay-enriched marine sediment under oxic and anoxic conditions 总被引：1，自引：1，他引：0
A series of laboratory incubation experiments were conducted to examine the decomposition of algal organic matter in clay-enriched
marine sediment under oxic and anoxic conditions. During the 245-day incubation period, changes in the concentrations of TOC,
major algal fatty acid components (14:0, 16:0, 16:1, 18:1 and 20:5), and n-alkanes (C16–C23) were quantified in the samples. Our results indicate that the organic matters were degraded more rapidly in oxic than anoxic
conditions. Adsorption of fatty acids onto clay minerals was a rapid and reversible process. Using a simple G model, we calculated
the decomposition rate constants for TOC, n-alkanes and fatty acids which ranged from 0.017–0.024 d−1, 0.049–0.103 d−1 and 0.011 to 0.069 d−1, respectively. Algal organic matter degraded in two stages characterized by a fast and a slow degradation processes. The
addition of clay minerals montmorillonite and kaolinite to the sediments showed significant influence affecting the decomposition
processes of algal TOC and fatty acids by adsorption and incorporation of the compounds with clay particles. Adsorption/association
of fatty acids by clay minerals was rapid but appeared to be a slow reversible process. In addition to the sediment redox
and clay influence, the structure of the compounds also played important roles in affecting their degradation dynamic in sediments. 相似文献
5.
王旭晨 《中国海洋大学学报(自然科学版)》2020,(3):I0001-I0002
化学化工学院是中国海洋大学历史最悠久的院系之一,其前身是始建于1930年的国立青岛大学化学系。1959年创建海洋化学系,1982年和1986年建立全国首批海洋化学硕士点和博士点。1993年被批准为全国唯一的海洋科学国家理科基础科学研究和教学人才培养基地(海洋化学点)。2002年改名为化学化工学院。2005年依托化学化工学院的海洋化学理论与工程技术教育部重点实验室批准立项建设,2009年5月通过验收并正式成立。 相似文献
6.
A one-year field study was conducted to determine the conversion ratio of phytoplankton biomass carbon (Phyto-C) to chlorophyll-a (Chl-a) in Jiaozhou Bay, China. We measured suspended particulate organic carbon (POC) and phytoplankton Chl-a samples collected in surface water monthly from March 2005 to February 2006. The temporal and spatial variations of Chl-a and POC concentrations were observed in the bay. Based on the field measurements, a linear regression model II was used to
generate the conversion ratio of Phyto-C to Chl-a. In most cases, a good linear correlation was found between the observed POC and Chl-a concentrations, and the calculated conversion ratios ranged from 26 to 250 with a mean value of 56 μg μg−1. The conversion ratio in the fall was higher than that in the winter and spring months, and had the lowest values in the
summer. The ratios also exhibited spatial variations, generally with low values in the near shore regions and relatively high
values in offshore waters. Our study suggests that temperature was likely to be the main factor influencing the observed seasonal
variations of conversion ratios while nutrient supply and light penetration played important roles in controlling the spatial
variations. 相似文献
7.
利用中国历次北极科学考察航次在白令海北部陆坡及海盆等深水区所采集的沉积物样品,对其开展沉积学等研究,系统归纳该海域常见的异常沉积类型及特征,并初步探讨其可能成因。BR02孔出现至少3段浊积层,浊积层主要分布于末次冰消期至中全新世。B5-4孔存在至少2段火山碎屑沉积层,其沉积年代分别约为1.3 ka BP和13.2 ka BP。B5-7站表层沉积物中的硅藻组合以新近系硅藻化石Kisseleviella carina Sheshukova-Poretzkaya和Kisseleviella ezoensis Akib为主,且与附近海域其他表层沉积物的硅藻组合面貌差异明显,可能是沉积物再沉积结果,其初始沉积年代大约为早中新世。白令海北部陆缘/陆坡区附近遍布的海底大峡谷对该区沉积物沉积过程具有重要影响,可能是导致该区浊流沉积与再沉积物的主要原因。此外,白令海位于欧亚板块、太平洋板块及北美板块交汇区边缘,其独特的地理位置决定该区地震与火山等构造活动相对活跃,进而进一步促使该区海底异常沉积现象频发。 相似文献
8.
A series of laboratory incubation experiments were conducted to examine the decomposition of algal organic matter in clay-enriched marine sediment under oxic and anoxic conditions.During the 245-day incubation period,changes in the concentrations of TOC,major algal fatty acid components (14:0,16:0,16:1,18:1 and 20:5),and n-alkanes (C16-C23) were quantified in the samples.Our results indicate that the organic matters were degraded more rapidly in oxic than anoxic conditions.Adsorption of fatty acids onto cla... 相似文献
9.
为深入认识马里亚纳海沟溶解有机物的垂直变化特征,本文于2015年12月采集马里亚纳海沟从表层至深层的水样,分析其DOC含量和CDOM的光谱特征。研究结果表明,研究站位DOC含量范围为37.12~58.30μmol·L-1,以表层最高,2 000m次之,之后维持较低含量。CDOM吸收系数a(320)以8 727m处最高,为0.48m-1;4 000m处CDOM的a(320)最小为0.14m-1。CDOM相对含量从表层至4 000m层与DOC变化规律较为一致,底层则与DOC不同,呈现升高现象。根据CDOM荧光光谱解析出3种类腐殖质和4种类蛋白荧光组分,其中类腐殖质组分荧光强度从表层至底层相对稳定,类蛋白组分荧光信号变化较为显著,尤其2种短波激发类蛋白荧光组分荧光信号的变化与表层较高初级生产、2 000m有机物再生产,以及底层物质的缓慢降解和汇集作用相对应。 相似文献
10.
Sedimentary facies of the subaqueous Changjiang River delta since the late Pleistocene 总被引：1，自引：0，他引：1
The sedimentary facies of the subaqueous Changjiang(Yangtze) River delta since the late Pleistocene was studied based on lithology and foraminifera analysis for two boreholes,CJK07 and CJK11,along with14C dating.Four sedimentary facies were identified,namely fluvial,tidal flat,offshore,and prodelta facies.The fluvial sedimentary facies is comprised of fluvial channel lag deposits,fluvial point bar deposits,and floodplain deposits,showing a fining-upward sequence in general with no benthic foraminifera.A layer of stiff clay overlies the fluvial deposits in core CJK07,indicating a long-term exposure environment during the Last Glacial Maximum(LGM).During the postglacial sea-level rise around 13-7.5 cal ka BP,the tidal flat facies was deposited in core CJK11,characterized by abundant silt-clay couplets.Euryhaline species dominate the subtidal flat foraminiferal assemblages,while almost no foraminifera was found in the intertidal flat.The offshore environment was the major sedimentary environment when the sea level reached its highest level around 7.5 cal ka BP,with a maximum accumulation rate of 10 mm/a found in core CJK11.Prodelta sediments have been deposited in core CJK11 since ~3 cal ka BP,after the formation of the Changjiang River delta.The difference in sedimentary facies between core CJK07 and CJK11 is due to their location: core CJK07 was in an interfluve while core CJK11 was in an incised valley during the LGM.Furthermore,AMS14C dating of core CJK07 shows poor chronological order,indicating that the sediments were reworked by strong tidal currents and that sediment deposited since ~7.7 cal ka BP in core CJK07 was eroded away by modern hydrodynamic forces caused by the southward shift of the Changjiang River delta depocenter. 相似文献