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Shelton Jenna L. Jubb Aaron M. Saxe Samuel W. Attanasi Emil D. Milkov Alexei V. Engle Mark Freeman Philip A. Shaffer Christopher A. Blondes Madalyn S. 《Natural Resources Research》2021,30(6):4147-4163
Natural Resources Research - Understanding the geochemistry of waters produced during petroleum extraction is essential to informing the best treatment and reuse options, which can potentially be... 相似文献
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Aaron M. Jubb Mark A. Engle Jessica M. Chenault Madalyn S. Blondes Cloelle G. Danforth Colin Doolan Tanya J. Gallegos Dan Mueller Jenna L. Shelton 《Geostandards and Geoanalytical Research》2020,44(2):385-397
Waters co‐produced during petroleum extraction are the largest waste streams from oil and gas development. Reuse or disposal of these waters is difficult due to their high salinities and the sheer volumes generated. Produced waters (PWs) may also contain valuable mineral commodities. While an understanding of produced water trace element composition is required for evaluating the associated resource and waste potential of these materials, measuring trace elements in brines is challenging due to the dilution requirements of typical methods. Alternatively, inductively coupled plasma‐optical emission spectrometry (ICP‐OES) has shown promise as being capable of direct measurements of trace elements within PWs with minimal dilution. Here, we evaluate direct ICP‐OES trace element quantification in PWs for seventeen trace elements (As, Al, Ba, Be, Cd, Cr, Co, Cu, Hg, Mo, Ni, Pb, Rb, Sb, U, V and Zn) within fifteen PWs from five U.S. continuous reservoirs. The total analytical uncertainties associated with the trace element levels determined using ICP‐OES were estimated to be better than ± 30% (2s) except for Rb, which could not be determined due to ionisation interferences. The ICP‐OES results are compared with trace element levels determined using inductively coupled plasma‐mass spectrometry from the same samples. Our results demonstrate the potential for direct analysis of high‐salinity waters using ICP‐OES with minimal dilution and provide trace element concentrations in waters from several important U.S. petroleum‐generating reservoirs where available data are sparse. 相似文献
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Commodities such as oil and gas occur in isolated reservoirs or accumulations, more generically called basic units here. To understand a study area’s economic potential and to craft plans for exploration and development, resource analysts often aggregate (sum, accumulate) basic unit magnitudes in distinct spatial subsets of the study area and then appraise the total area’s potential by summing these intermediate sums. In a probabilistic approach, magnitudes are modeled as random variables. Some have asked, “Do different methods of partitioning basic units into subsets lead to different probability distributions for the sum of all basic unit magnitudes?” Any method of aggregation of basic unit magnitudes which obeys the rules of probability leads to the same probability distribution of the sum of all unit magnitudes as that computed by direct summation of all basic unit magnitudes. A Monte Carlo simulation of a synthetic example in which the magnitude of resource in each unit is marginally lognormal and pairwise correlations among basic unit magnitudes are specified illustrates key features of probabilistic aggregation. The joint distribution of certain pairs of aggregates are closely approximated by a bivariate lognormal distribution. 相似文献
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Madalyn S. Blondes Peter W. Reiners Mihai N. Ducea Brad S. Singer John Chesley 《Earth and Planetary Science Letters》2008,269(1-2):140-154
Primitive basaltic single eruptions in the Big Pine Volcanic Field (BPVF) of Owens Valley, California show systematic temporal–compositional variation that cannot be described by simple models of fractional crystallization, partial melting of a single source, or crustal contamination. We targeted five monogenetic eruption sequences in the BPVF for detailed chemical and isotopic measurements and 40Ar/39Ar dating, focusing primarily on the Papoose Canyon sequence. The vent of the primitive (Mg# = 69) Papoose Canyon sequence (760.8 ± 22.8 ka) produced magmas with systematically decreasing (up to a factor of two) incompatible element concentrations, at roughly constant MgO (9.8 ± 0.3 (1σ) wt.%) and Na2O. SiO2 and compatible elements (Cr and Ni) show systematic increases, while 87Sr/86Sr systematically decreases (0.7063–0.7055) and εNd increases (− 3.4 to − 1.1). 187Os/188Os is highly radiogenic (0.20–0.31), but variations among four samples do not correlate with other chemical or isotopic indices, are not systematic with respect to eruption order, and thus the Os system appears to be decoupled from the dominant trends. The single eruption trends likely result from coupled melting and mixing of two isotopically distinct sources, either through melt-rock interaction or melting of a lithologically heterogeneous source. The other four sequences, Jalopy Cone (469.4 ± 9.2 ka), Quarry Cone (90.5 ±17.6 ka), Volcanic Bomb Cone (61.6 ± 23.4 ka), and Goodale Bee Cone (31.8 ± 12.1 ka) show similar systematic temporal decreases in incompatible elements. Monogenetic volcanic fields are often used to decipher tectonic changes on the order of 105–106 yr through long-term changes in lava chemistry. However, the systematic variation found in Papoose Canyon (100–102 yr) nearly spans that of the entire volcanic field, and straddles cutoffs for models of changing tectonic regime over much longer time-scales. Moreover, ten new 40Ar/39Ar ages combined with chemistry from all BPVF single eruption sequences show the long-term trend of BPVF evolution comprises the overlapping, temporal–compositional trends of the monogenetic vents. This suggests that the single eruption sequences contain the bulk of the systematic chemical variation, whereas their aggregate compositions define the long-term trend of volcanic field evolution. 相似文献
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