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1.
To determine if Cu mediated reactions on atmospheric particles are important to HO2 chemistry in the ambient atmosphere, Cu molalities were calculated from measured Cu aerosol particle concentrations, mass and number size distribution data from a site in central Sweden. A comparison of characteristic times indicates that at low relative humidities the reaction is limited by the mass transport of gas phase HO2 to the particle surface and not by the chemical kinetics of the aqueous reaction. Comparison of half-lives for particle reactions and the gas phase destruction of HO2 to form H2O2 indicate that heterogeneous reactions on aerosol particles may have important consequences on the chemistry of HO2 and H2O2 in the troposphere. 相似文献
2.
气溶胶的光学厚度与反射率比的处理方法 总被引:2,自引:0,他引:2
气溶胶光学厚度与气溶胶反射率比都是大气校正所需的重要大气参数,同时也是海洋水色卫星主要的数据产品,它们的测量精度将直接到卫星数据产品正演的精度和卫星数据产品的应用。文章在简述气溶胶光学厚度与气溶胶反射率比的基本测量原理和处理方法的基础上,结合多次试验数据结果进行简要的评价。 相似文献
3.
Qian Fenlan Yu Hongjian Lan Youchang Chen Zhi Zhou Mingyu Farn Parungo Wu Peiming 《海洋学报(英文版)》1996,15(1):69-84
AtmosphericinputoftraceelementstothewesternPacificOceanandtheKuroshiooceanarea¥QianFenlan;YuHongjian;LanYouchang;ChenZhi;Zhou... 相似文献
4.
Effect of emersion and immersion on the porewater nutrient dynamics of an intertidal sandflat in Tokyo Bay 总被引:2,自引:0,他引:2
Tomohiro Kuwae Eiji Kibe Yoshiyuki Nakamura 《Estuarine, Coastal and Shelf Science》2003,57(5-6):929-940
Porewater nutrient dynamics during emersion and immersion were investigated during different seasons in a eutrophic intertidal sandflat of Tokyo Bay, Japan, to elucidate the role of emersion and immersion in solute transport and microbial processes. The water content in the surface sediment did not change significantly following emersion, suggesting that advective solute transport caused by water table fluctuation was negligible. The rate of change in nitrate concentration in the top 10 mm of sediments ranged from −6.6 to 4.8 μmol N l−1 bulk sed. h−1 during the whole period of emersion. Steep nutrient concentration gradients in the surface sediment generated diffusive flux of nutrients directed downwards into deeper sediments, which greatly contributed to the observed rates of change in porewater nutrient concentration for several cases. Microbial nitrate reduction within the subsurface sediment appeared to be strongly supported by the downward diffusive flux of nitrate from the surface sediment. The stimulation of estimated nitrate production rate in the subsurface layer in proportion to the emersion time indicates that oxygenation due to emersion caused changes in the sediment redox environment and affected the nitrification and/or nitrate reduction rates. The nitrate and soluble reactive phosphorus pools in the top 10 mm of sediment decreased markedly during immersion (up to 68% for nitrate and up to 44% for soluble reactive phosphorus), however, this result could not be solely explained by molecular diffusion. 相似文献
5.
The interstitial water composition (
, alkalinity, Ca2+, Mg2+, Sr2+, Na+, K+) and the cation exchange capacity (CEC) were determined for the muddy sediments of the continental shelf off the Gironde Estuary (France), in the area where the sediment represents the deposit of the muddy suspension of the river. In comparison with seawater concentrations, the pore waters below 10 cm depth, show depletions of
and Ca2+ and below a 30 cm depth show depletions of Mg2+. Inversely, the upper 10 cm an enrichment of Ca2+ concentration, and an increase of K+ concentration to a 40 cm depth. High values of
are observed at the top 4 cm. Alkalinity enrichment is observed along the length of the core. Applying the alkalinity models for the sediment below a 10 cm depth demonstrates generally that calculated alkalinities are higher than the measured ones. Ca2+ dissolution occurs at the first 10 cm and authigenic carbonate precipitation starts beneath that level. Mg2+ depletion is accompanied by bicarbonate loss. This proves that Mg2+ depletion is due to a Mg-silicate reaction. The result of the CEC does not confirm the Mg2+ uptake by clay minerals in exchangeable site, under reducing conditions. Diffusion and bioturbation play an important role in the pore water concentration at the top of the core. 相似文献
6.
离子色谱分析在黄土和粉尘研究中的应用 总被引:1,自引:0,他引:1
黄土中存在着大量的碱金属及碱土金属,以往的测试方法多为原子吸收和ICP—MS,离子色谱法在测试黄土样品的碱金属和碱土金属元素含量中应用不多。将黄土地质标准样品进行消解后用离子色谱进行测试,测试效果良好,重复测试的相对标准偏差小于5%,与推荐值的相对误差小于5%,准确度和精密度符舍相关的质量控制要求。本实验方法测试的离子含量都在仪器响应呈线性的最佳测试范围之内,标准曲线经回归后相关系数均达到0.9999。黄土样品的分析结果与粉尘气溶胶样品的离子分析结果对比表明,此方法对于探讨粉尘起源以及沙尘暴天气的研究具有重要意义。 相似文献
7.
8.
REEdistributioninwater-sedimentinterfacesystematdeepoceanfloor¥ZhangLijie;LiuJihuaandYaoDe(ReceivedFebruary1,1994;acceptedMay... 相似文献
9.
本文通过环境背景值、风化壳地球化学、对流层(大气气溶胶)地球化学和人为地球化学异常,初步探讨了南极长城站地区的现代环境地球化学特征。分析表明:环境要素固有的地球化学性质、区域环境条件和自然环境演变之间具有深刻的内在联系。 相似文献
10.