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Size distribution of colloidal trace metals and organic carbon during a coastal bloom in the Baltic Sea 总被引：1，自引：0，他引：1
Johan Ingri Susanna Nordling Jenny Larsson Jenny Rnnegrd Nina Nilsson Ilia Rodushkin Ralf Dahlqvist Per Andersson
rjan Gustafsson 《Marine Chemistry》2004,91(1-4):117-130
The physico-chemical speciation of organic carbon and selected metals was measured during a coastal bloom in Ekhagen Bay, Baltic Sea, using ultrafiltration.One important objective with the study was to see if any depletion of trace metals could be measured in the directly bioavailable fraction (<1000 Da, the soluble low molecular weight fraction, LMW) during a plankton bloom. Filters with five different cut-offs were used (1 kD (1000 Da), 5 kD, 10 kD, 100 kD and 0.22 μm) in order to delineate the size distribution of colloidal organic carbon (COC) and trace metals.During the bloom in May, LMW Al, Co, Cu, Mn and Ni concentrations decreased although the colloidal and particulate concentrations were relatively high. Data show that desorption of colloidal and particulate bound trace metals to the LMW fraction was slower than the process depleting the LMW fraction.Estimates of the maximum active uptake of Cu, Ni and Mn by the phytoplankton, and the loss of non-bioactive Al from the LMW fraction, indicate that processes other than active uptake by phytoplankton must contribute to the observed depletion of trace metals in the LMW fraction. Hence, in order to estimate the bioavailable pool of trace metals for plankton during bloom conditions, these other processes must be understood and quantified.Transparent Exopolymeric Particles (TEP, reflecting sugar-rich phytoplankton exudates) increased around eight times during the plankton bloom. We hypothesize that the formation of TEP is a process that might be important for the transfer of trace metals from the LMW to the particulate fraction during the phytoplankton bloom, but the significance of TEP for this depletion in Baltic Sea surface water remains to be shown. 相似文献
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Anja Engel Lynn Abramson Jennifer Szlosek Zhanfei Liu Gillian Stewart David Hirschberg Cindy Lee 《Deep Sea Research Part II: Topical Studies in Oceanography》2009,56(18):1408-1419
The quantitative relationship between organic carbon and mineral contents of particles sinking below 1800 m in the ocean indicates that organisms with mineral shells such as coccolithophores are of special importance for transporting carbon into the deep sea. Several hypotheses about the mechanism behind this relationship between minerals and organic matter have been raised, such as mineral protection of organic matter or enhanced sinking rates through ballast addition. We examined organic matter decomposition of calcifying and non-calcifying Emiliania huxleyi cultures in an experiment that allowed aggregation and settling in rotating tanks. Biogenic components such as particulate carbon, particulate nitrogen, particulate volume, pigments, transparent exopolymer particles (TEP), and particulate amino acids in suspended particles and aggregates were followed over a period of 30 d. The overall pattern of decrease in organic matter, the amount of recalcitrant organic matter left after 30 d, and the compositional changes within particulate organic matter indicated that cells without a shell are more subject to loss than calcified cells. It is suggested that biogenic calcite helps in the preservation of particulate organic matter (POM) by offering structural support for organic molecules. Over the course of the experiment, half the particulate organic carbon in both calcifying and non-calcifying cultures was partitioned into aggregates and remained so until the end of the experiment. The partial protection of particulate organic matter from solubilization by biominerals and by aggregation that was observed in our experiment may help explain the robustness of the relationship between organic and mineral matter fluxes in the deep ocean. 相似文献
3.
透明胞外聚合颗粒物（TEP）是凝聚网的重要组成部分甚至核心,在微尺度范围上形成了水环境结构的重要梯度,对于元素地球化学生物循环、碳沉降以及食物网有着举足轻重的作用。本文研究了东海典型断面PN透明胞外聚合颗粒物的分布特征及来源。结果表明:东海典型断面PN透明胞外聚合颗粒物含量介于28~376 μg Xeq./L之间,平均值为（115±67）μg Xeq./L;呈现出明显的夏季 > 冬季 > 秋季 > 春季的季节变化特征以及近岸 > 外海和底层 > 表层的分布趋势。通过对比透明胞外聚合颗粒物分布趋势和硅藻、甲藻分布趋势以及统计分析得出,东海典型断面PN透明胞外聚合颗粒物主要来源于硅藻,甲藻贡献不大;而外海TEP的来源可能主要由超微型浮游植物贡献。 相似文献
4.
N. Ramaiah V. V. S. S. Sarma Mangesh Gauns M. Dileep Kumar M. Madhupratap 《Journal of Earth System Science》2000,109(4):443-451
Bacterial abundance and production, numbers, sizes and concentrations of transparent exopolymer particles (TEP) and total
organic carbon (TOC) were measured during the 1996 summer monsoon to understand the relationship between TEP, the most labile
particulate organic carbon, and bacteria. While high regional variability in the vertical distribution of TOC was discernible,
TEP concentrations were high in surface waters at 18–20°N along 64°E with concentrations well over 25 mg alginic acid equivalents
I−1 due to upwelling induced productivity. Their concentrations decreased with depth and were lower between 200 and 500 m. Bacterial
concentrations were up to 1.99 × 108 I–1 in the surface waters and decreased by an order of magnitude or more at depths below 500 m. A better relationship has been
found between bacterial abundance and concentrations of TEP than between bacteria and TOC, indicating that bacterial metabolism
is fueled by availability of TEP in the Arabian Sea. Assuming a carbon assimilation of 33%, bacterial carbon demand (BCD)
is estimated to be 1.017 to 4.035 g C m–2 d–1 in the surface waters. The observed TEP concentrations appear to be sufficient in meeting the surface and subsurface BCD
in the northern Arabian Sea. 相似文献
5.
Characterization of the proteinaceous matter in marine aerosols 总被引：1，自引：0，他引：1
Marine aerosols play a dominant role in the transfer of oceanic material to the atmosphere. Most marine aerosol originates when air bubbles burst at the sea surface ejecting material from the sea surface microlayer and bubble surface layers into the air. Concentrations of chemical compounds in these surface layers often differ from their concentrations in bulk water. We examined the enrichment of aerosols with proteinaceous matter and attempted to characterize the physical nature and sources of this matter. We measured concentrations of dissolved free (DFAA), dissolved combined (DCAA), and particulate (PAA) amino acids, transparent stainable particles (TSP), and bacteria and virus-like particles as carriers of protein, in natural and simulated aerosols. We also evaluated D/L ratios certain amino acids in all amino acid fractions.DFAA and DCAA enriched the aerosols we sampled by 1.2–20 times compared to bulk seawater; PAA enrichment was usually higher (up to 50-fold). Aerosols contained particles typical of seawater, e.g., microorganisms, organic debris, inorganic particles with adsorbed organic matter, but also a large number of semitransparent gel-like particles, which all contained amino acids. Some of these particles were probably scavenged from bulk water, but new particles produced as bubbles burst at the surface comprised at least 10% of total proteinaceous matter in the aerosol. D/L ratios of certain amino acid suggested that the particles were most likely made from dissolved polymers secreted by phytoplankton that were concentrated on bubble surfaces and in the microlayer. Examination with Alcian Blue (a dye that targets carbohydrates) and Coomassie Blue (a dye that targets proteins) showed that most TSP in the aerosols contained both proteins and polysaccharides. Microorganisms enriched the aerosols by up to two orders of magnitude, but contributed less than 4% to the total protein pool. 相似文献
6.
北白令海透明胞外聚合颗粒物的含量与来源 总被引：2，自引：1，他引：1
透明胞外聚合颗粒物(TEP)是海水中大量存在的黏性颗粒物质,它对于海洋颗粒物的聚集、有机碳的埋藏、食物网物质的传递、痕量金属的清除与迁出等均起着重要作用。本研究开展了夏季北白令海陆架、陆坡和海盆区透明胞外聚合颗粒物含量和分布的研究。结果表明,北白令海TEP含量介于34~628 mg/m3(Xeq)之间,其中陆架、陆坡和海盆区TEP的平均含量分别为240, 145和83 mg/m3(Xeq),整体呈现由陆架向外海降低的趋势。在陆坡和海盆区,TEP含量随着深度的增加而降低,但在陆架近底层水中,观察到TEP高含量的特征,与近底层水高的TSM, POC相对应。TEP与荧光强度、TSM、POC等的关系分析显示,研究海域TEP存在两个来源,其一为海洋上层水体的浮游生物,其主要贡献于陆架上层、陆坡和海盆水体;其二为陆架沉积物的底栖生物,其通过沉积物再悬浮贡献于陆架近底层水。 相似文献
7.
3种光温指标在模拟设施黄瓜生长发育中的应用与比较 总被引：2，自引：0，他引：2
2011年9～12月间,以黄瓜“津优1号”（ Cucumis sativus linn. cv. Jingyoul ） 为试材,在南京信息工程大学试验温室进行分批栽培试验,测定温室气象要素和作物数据,分别用活动积温（AAT,Ac-tive accumulated temperature ）、有效积温（ EAT, Effective accumulated temperature） 和辐热积（TEP,Thermal effectiveness and photosynthesis active radiation）3种光温指标模拟温室黄瓜植株叶面积、株高和生育期,并利用独立试验数据对各个模型进行验证。结果表明：用辐热积指标分别模拟黄瓜各生育期（出苗期、开花期、坐果期、果实膨大期、成熟期）距播种日期的天数,其相对标准误差（RMSE）分别为0d,3d,4d,5d,4d,小于活动积温法（1d,6d,8d,11d,11d）和有效积温法（0d,4d,3d,8d,10d）。利用辐热积指标模拟叶面积和株高的相对标准误差（RMSE）分别为43．0cm^2和4．3cm,决定系数（R^2）分别为0．98和0．98,而用活动积温和有效积温指标模拟黄瓜单株叶面积的相对标准误差（RMSE）分别为61．3cm^2和54．6cm^2,模拟株高的相对标准误差（RMSE）分别为9．8cm和7．5cm。比较结果显示利用辐热积指标模拟温室黄瓜生育期、株高和叶面积的精度明显高于活动积温和有效积温,该研究为温室黄瓜生长指标和各生育期的预测以及环境调控提供参考。 相似文献
8.
Distributions of carbohydrate species in the Gulf of Mexico 总被引：2，自引：0，他引：2
Chin-Chang Hung Laodong Guo Peter H. Santschi Nicolas Alvarado-Quiroz Jennifer M. Haye 《Marine Chemistry》2003,81(3-4):119-135
In order to study the role of polysaccharides in the cycling of marine organic matter and transparent exopolymeric particles (TEP), the concentrations of total carbohydrates (p-TCHO), total uronic acids (URA) and total acid polysaccharides (APS) in suspended and sinking particles, as well as carbohydrates in the filter-passing “dissolved” phase (d-TCHO), were measured in vertical profiles along a N–S transect in the Gulf of Mexico, across a cold core (CCR) and a warm core (WCR) ring (eddy) during both July 2000 and May 2001. The concentrations of d-TCHO in 2000 ranged from 4 to 22 μM C, with a subsurface maximum, which was located slightly above the depth of chl a maximum, amounting to, on average, 34% of DOC in the CCR, and 13% in the WCR. The concentration of particulate carbohydrates (p-TCHO) in different size fractions (0.7–10, 10–53, and >53 μm) ranged from 0.04 to 1.1, 0.005 to 0.40, and 0.006 to 0.26 μM C, respectively, indicating that carbohydrates are mostly concentrated in small particles (0.7–10 μm). URA and APS were similarly concentrated in small particles, in which, on average, URA accounted for 87% and 57% of total URA, and APS for 92% and 88% of total APS in 2000 and 2001, respectively. URA accounted for 3–9% of carbohydrates in suspended particles, suggesting that URA are a minor component of the p-TCHO pool. Due to its surface-reactive nature, URA could play a major role in the coagulation of particles and macromolecules despite its relatively low abundance. While, on average, p-TCHO and total APS were more enriched in suspended particles than in sinking particles in both 2000 and 2001, the opposite was true for URA in both years. The greater contents of URA that are present in settling particles compared to suspended particles could indicate a mass flow in the direction of sinking particles, either caused by coagulation, by bacterial reworking of particulate and colloidal organic matter, or by their more refractory nature. 相似文献
9.
Effect of iron enrichment on the dynamics of transparent exopolymer particles in the western subarctic Pacific 总被引：1，自引：0，他引：1
Neelam Ramaiah Shigenobu Takeda Ken Furuya Takeshi Yoshimura Jun Nishioka Tatsuo Aono Yukihiro Nojiri Keiri Imai Isao Kudo Hiroaki Saito Atsushi Tsuda 《Progress in Oceanography》2005,64(2-4):253
Dynamics of transparent exopolymer particles (TEP) was studied during the first in situ iron-enrichment experiment conducted in the western subarctic Pacific in July–August 2001, with the goal of evaluating the contribution of TEP to vertical flux as a result of increased primary production following iron enrichment in open ocean ecosystems. Subsequent to the enhancement of phytoplankton production, we observed increase in TEP concentration in the surface layer and sedimentation of organic matter beneath it. Vertical profiles of TEP, chlorophyll a (Chl a) and particulate organic carbon (POC) were obtained from six depths between 5 and 70 m, from a station each located inside and outside the enriched patch. TEP and total mass flux were estimated from the floating sediment traps deployed at 200 m depth. Chl a and TEP concentrations outside the patch varied from 0.2 to 1.9 μg L−1 and 40–60 μg XG equiv. L−1, respectively. Inside the patch, Chl a increased drastically from day 7 reaching the peak of 19.2 μg L−1 on day 13, which coincided with the TEP peak of 189 μg XG equiv. L−1. TEP flux in the sediment trap increased from 41 to 88 mg XG equiv. m−2 d−1, with 8–14% contribution of TEP to total mass flux. This forms the basic data set on ambient concentrations of TEP in the western subarctic Pacific, and evaluation of the effect of iron enrichment on TEP. 相似文献
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