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1.
Establishment of water quality criteria to guide catchment sediment management is required by the European Union (EU) Water Framework Directive. The topic, however, is hotly contested among scientists and policy makers. Existing legislation with regard to fine sediment was set by the EU Freshwater Fish Directive. Its guideline, i.e. mean annual suspended sediment concentration, is 25 mg l−1. Such a static target fails to capture the episodic nature of sediment transport. Furthermore, application of such global standards is inappropriate for a pollutant that is strongly controlled by spatial variation in key catchment drivers. Paleolimnology offers an approach for assessing background sediment pressures on watercourses, enabling determination of values for times pre-dating agricultural intensification. We propose that Modern Background Sediment Delivery to Rivers (MBSDR) across England and Wales can be determined using paleolimnology to quantify maximum feasible sediment reduction. No management programme should aim to reduce sediment loss to values below those resulting from background, natural physiographic and/or hydrological controls. Lacking generic tools to quantify process linkages between sediment pressures and biological impact, we propose that MBSDR could be taken to represent ecological demand for sediment inputs into watercourses required to support healthy aquatic habitats. In situations where generic tools exist for coupling sediment pressures and ecological impacts, assessment of MBSDR could be used to correct the gap between current or future projected sediment loss and biological condition. Existing paleolimnological data on sediment yields across England and Wales are presented to illustrate the approach and provide preliminary national estimates of MBSDR. We briefly consider the basis for reconstructing sediment yields using a paleolimnological approach and analyse temporal trends in published sediment yield, inferred for a range of landscape types. We also attempt to correlate sediment accumulation rates (SARs) with sediment yields to extend the MBSDR data base. Preliminary maps were generated to identify regions where further sediment yield data are needed to produce a more robust estimate of the spatial distribution of MBSDR across England and Wales.  相似文献   

2.
Groundwater dominance has important effects on the hydrological and geomorphological characteristics of river systems. Low suspended sediment concentrations and high water clarity are expected because significant inputs of sediment-free spring water dilute the suspended sediment generated by storms. However, in many Mediterranean rivers, groundwater dominance is characterised by seasonal alternations of influent and effluent discharge involving significant variability on the sediment transport regimes. Such areas are often subject to soil and water conservation practices over the centuries that have reduced the sediment contribution from agricultural fields and favour subsurface flow to rivers. Moreover, urbanisation during the twentieth century has changed the catchment hydrology and altered basic river processes due to its ‘flashy’ regime. In this context, we monitored suspended sediment fluxes during a two-year period in the Na Borges River, a lowland agricultural catchment (319 km2) on the island of Mallorca (Balearic Islands). The suspended sediment concentration (SSC) was lower when the base flow index (i.e., relative proportion of baseflow compared to stormflow, BFI) was higher. Therefore, strong seasonal contrasts explain the high SSC coefficient of variation, which is clearly related to dilution effects associated with different groundwater and surface water seasonal interactions. A lack of correlation in the Q-SSC rating curves shows that factors other than discharge control sediment transport. As a result, at the event scale, multiple regressions illustrate that groundwater and surface water interactions are involved in the sedimentary response of flood events. In the winter, the stability of baseflow driven by groundwater contributions and agricultural and urban spills causes hydraulic variables (i.e., maximum discharge) to exert the most important control on events, whereas in the summer, it is necessary to accumulate important volumes of rainfall, creating a minimum of wet conditions in the catchment to activate hydrological pathways and deliver sediment to the drainage network. The BFI is also related to sediment delivery processes, as the loads are higher with lower BFI, corroborating the fact that most sediment movement is caused by stormflow and its related factors. Overall, suspended sediment yields were very low (i.e., < 1 t km− 2 yr− 1) at all measuring sites. Such values are the consequence of the limited sediment delivery attributable to soil conservation practices, low surface runoff coefficients and specific geomorphic features of groundwater-dominated rivers, such as low drainage density, low gradient, steep valley walls and flat valley floors.  相似文献   

3.
Dissolved and total organic and inorganic carbon in some British rivers   总被引：2，自引：0，他引：2  
Rivers transport both organic and inorganic carbon from their sources to the sea. Results of ~800 organic and inorganic analyses from various British rivers of contrasting size and land use are presented here: (1) the headwater River Tern, a rural river of 852 km2 catchment; (2) the Ouseburn, a small urban 55 km2 catchment; (3) the River Tyne, a larger river system of ~3000 km2 catchment; (4) a spatial survey from 205 sample sites on ~60 rivers from SW England. We found that, with the exception of peat-rich headwaters, DIC concentration is always greater than DOC. DIC is primarily in the form HCO3 − , with DIC concentrations highest in highly urbanised catchments, typically greater than those observed in catchments with carbonate bedrock, demonstrating a significant and previously unrecognised anthropogenic inorganic carbon input to urban rivers.  相似文献   

4.
Suspended sediment concentration (SSC) in the Ova da Morteratsch, Switzerland, measured during July 2007 was closely associated with discharge (Q) and showed statistically significant relationships at the p < 0.001 level at the proximal and distal ends of the 600 m pro‐glacial zone. SSC predicted from 10‐minute turbidity records gives a much more detailed insight into SSC fluctuations and identified SSC peaks which do not coincide with discharge peaks. Net (proximal – distal) 10‐minute suspended sediment loads (SSL) are predominantly positive (i.e. suspended sediment is being stored in the reach) for most of the 7–19 July 2007 record. Net (proximal – distal) SSLs correlate closely with discharge for the first part of the record (7–13 July) but from 14 to 19 July suspended sediment exhaustion is in evidence and discrete phases of negative net SSL (i.e. sediment flushing) are likely for up to six hours on three separate days which coincide with phases of high discharge and exhaustion of the glacial suspended sediment sources. Analysis of Q at the Berninabach–Pontresina gauging station (5 km downstream) for the past five years revealed that maximum monthly discharges capable of generating sediment flushing events occur in an average of four months each year. The study emphasises the rapid change in suspended sediment transport and yields with distance from the glacier snout and highlights the importance of measurements as close to the glacier snout as possible if data are to be representative of the glaciated land up‐valley. A better understanding of the processes of sediment exchange and the colonisation and stabilisation of sediment stores by vegetation in such pro‐glacial zones is essential if we are to improve predictions of the impacts of climate change on river sediment dynamics and the subsequent effects on aquatic ecology.  相似文献   

5.
The global cycling of anthropogenic trace metals intensified during the twentieth century, impacting aquatic systems throughout the world. There are, however, few quantitative records showing the history of this contamination in large rivers. Here we present a well-dated sedimentary record of trace metal accumulation in Lake St. Croix, a natural riverine lake on the St. Croix River (Minnesota and Wisconsin, USA), revealing the history of heavy metal inputs to the river over the past 200 years. Concentrations of Hg, Pb, Ag, Cd, Cr and Zn and stable Pb isotopes were measured in eight 210Pb-dated sediment cores collected from profundal depositional areas throughout the lake. Time trends of trace metal concentrations and accumulation rates differed greatly between the upper lake (above Valley Creek) and the lower lake, reflecting contrasting sediment sources along the flow axis of the lake. For most of the study period (1800–2000 AD), sediment deposited throughout the lake derived almost exclusively from the suspended sediment load carried by the main-stem river into the lake. From 1910 through 1970, however, large inputs of eroded soils and stream channel sediments from side-valley tributaries resulted in greatly increased sediment and trace metal accumulation in the lower lake. Anthropogenic accumulation rates of Hg, Pb, Cd, Zn, and Ag in the upper lake correlate well with those from Square Lake, a small, relatively undisturbed nearby lake that has received trace metal inputs almost exclusively via atmospheric deposition. The similarity of these records suggests that atmospheric deposition was primarily responsible for trace metal accumulation trends in upper Lake St. Croix. Trace metal accumulation in the lower lake was also strongly influenced by atmospherically derived inputs, but metal contributions from native soils were important, as well, during the period of elevated sediment inputs from side-valley tributaries. Concentrations and accumulation rates of trace metals in both upper and lower lake sediments have decreased substantially since the 1970s due to decreased atmospheric inputs and sediment loadings, but accumulation rates remain well above pre-settlement values. Metal inputs to Lake St. Croix have been far lower than those to nearby Lake Pepin, located on the Mississippi River downstream of the Minneapolis-St. Paul metropolitan area, but there nevertheless remains a clear record of anthropogenic impact on the relatively pristine St. Croix River.  相似文献   

6.
Erosion and sediment transport in High Arctic rivers, Svalbard   总被引：2，自引：0，他引：2  
This paper discusses sediment yield, sediment delivery and processes of erosion in rivers subject to High Arctic conditions in Svalbard. Long-term measurements reveal large variations between rivers and from year to year in each individual river. In the unglacierized catchment of Londonelva, annual sediment transport varied between 28 and 93 t/yr, with a mean sediment yield of 82.5 t/km2/yr. In the glacier-fed rivers Bayelva and Endalselva, the suspended sediment transport varied in the range of 5126 t/yr to 22797 t/yr during a 12-year period. A mean of 11 104 t/yr gave rise to a mean sediment yield of 359 t/km2/yr for the whole Bayelva catchment area. The sediment yield of the glacier and the moraine area was estimated at 586 t/km2/yr. A conceptual model used to interpret the long- and short-term patterns of sediment concentration in the meltwater from the glacier and erosion of the neoglacial moraines is proposed. Evidence is found that a proportion of the sediments are delivered by a network of englacial and subglacial channels that exist even in cold ice. Regression analyses of water discharge versus suspended sediment concentration gave significant correlations found to be associated with the stability of ice tunnels in cold ice. Large floods have been found to flush the waterways and exhaust the sediment sources. A long-term change in the exponent of regression lines is attributed to changes in sediment availability caused by flushing and expansion of tunnels and waterways by large floods and a subsequent slow deformation of them caused by the ice overburden and the glacier movement. A comparison of sediment yields from a number of polythermal and temperate glaciers in various areas showed large differences that were attributed primarily to bedrock susceptibility to erosion and, secondarily, to glaciological parameters.  相似文献   

7.
Slope–channel coupling and in-channel sediment storage can be important factors that influence sediment delivery through catchments. Sediment budgets offer an appropriate means to assess the role of these factors by quantifying the various components in the catchment sediment transfer system. In this study a fine (< 63 µm) sediment budget was developed for a 1.64-km2 gullied upland catchment in southeastern Australia. A process-based approach was adopted that involved detailed monitoring of hillslope and bank erosion, channel change, and suspended sediment output in conjunction with USLE-based hillslope erosion estimation and sediment source tracing using 137Cs and 210Pbex. The sediment budget developed from these datasets indicated channel banks accounted for an estimated 80% of total sediment inputs. Valley floor and in-channel sediment storage accounted for 53% of inputs, with the remaining 47% being discharged from the catchment outlet. Estimated hillslope sediment input to channels was low (5.7 t) for the study period compared to channel bank input (41.6 t). However an estimated 56% of eroded hillslope sediment reached channels, suggesting a greater level of coupling between the two subsystems than was apparent from comparison of sediment source inputs. Evidently the interpretation of variability in catchment sediment yield is largely dependent on the dynamics of sediment supply and storage in channels in response to patterns of rainfall and discharge. This was reflected in the sediment delivery ratios (SDR) for individual measurement intervals, which ranged from 1 to 153%. Bank sediment supply during low rainfall periods was reduced but ongoing from subaerial processes delivering sediment to channels, resulting in net accumulation on the channel bed with insufficient flow to transport this material to the catchment outlet. Following the higher flow period in spring of the first year of monitoring, the sediment supplied to channels during this interval was removed as well as an estimated 72% of the sediment accumulated on the channel bed since the start of the study period. Given the seasonal and drought-dependent variability in storage and delivery, the period of monitoring may have an important influence on the overall SDR. On the basis of these findings, this study highlights the potential importance of sediment dynamics in channels for determining contemporary sediment yields from small gullied upland catchments in southeastern Australia.  相似文献   

8.
Sediment supplied by continental sources is commonly suspected to have exerted a strong influence on the development of canyons and other morphological features on the continental slopes, but rarely is the sediment supply known sufficiently quantitatively to test this link. Here, we outline an area where offshore morphology, in the western Ionian Sea, may be linked to estimated sediment fluxes produced by subaerial erosion in NE Sicily and SW Calabria. Shelves in this area are narrow (<1 km), and the bathymetry shows that rivers and adjacent submarine channels are almost directly connected with each other. Integrated topographic analyses were performed on a merged digital elevation model (DEM) of ASTER data for subaerial topography and multibeam sonar data for submarine bathymetry. Spatial variations in sediment fluxes from onshore erosion were assessed using a variety of methods, namely: long‐term sediment flux from Pleistocene uplift rates, decadal sediment flux from landslide occurrences and published long‐term exhumation rates from 10Be cosmogenic nuclide concentrations. Submarine channels associated with rivers delivering larger sediment fluxes have broad channels, high relief and smooth concave‐upward longitudinal profiles. Conversely, submarine channels that lie offshore small‐flux rivers have straight longitudinal profiles, low relief and steep gradients. Where river catchments supply a greater sediment flux offshore, shelves tend to be wider (ca. 400 m) and submarine channels have gentler gradients. In contrast, where catchments supply less sediment flux, shelves are narrow (250–300 m) and offshore channel gradients are steeper. The variation of submarine morphology with tectonic uplift rate was also studied, but we find that, unlike onshore terrains where tectonics is commonly an important factor influencing channel morphology, in the submarine landscapes, sediment flux appears to dominate here.  相似文献   

9.
孙虎  甘枝茂  吴成基 《中国沙漠》1997,17(3):261-268
对黄河中游河口镇至龙门区间的产沙岩层与河流悬移质输沙进行了耦合平衡分析,确定了该区间各种产沙岩层的产沙数量,并推算出黄土、基岩和风沙对河流粗泥沙(d>0.05mm)的贡献率分别为61.2%、34.2%和4.6%。同时,分析了该区间侵蚀产粗泥沙的分布规律。  相似文献   

10.
基于多参数指标的长江口滨岸多环芳烃来源辨析   总被引：2，自引：0，他引：2  
在长江口滨岸及临近排污口、滨岸河流、城市中心城区采集悬浮颗粒物、表层沉积物、街道灰尘等样品, 分别利用GC-MS 和GC-C-IRMS 定量分析了不同环境介质中的多环芳烃 (PAHs) 与有机单体化合物稳定碳同位素(δ13C), 开展了基于PAH 环数、分子量特征比值和有机单体化合物稳定碳同位素组成等参数指标的长江口滨岸悬浮颗粒物与表层沉积物中PAHs 源解析研究。研究结果显示, 长江口滨岸悬浮颗粒物与表层沉积物中的PAH 化合物主要以3~4 环为主, 与吴淞排污口、石洞口污水处理厂、黄浦江、滨岸小河流以及上海中心城区等潜在来源区域不同环境介质中的PAHs 组成特征相似, 主要来源于汽油、柴油、煤炭和木材的不完全燃烧以及石油残余物的混合。其中, 木材和煤炭不完全燃烧形成的PAHs 以及石油残余物, 枯季经过滨岸河流及排污口直接输入, 洪季则为城市街道灰尘被暴雨冲刷, 随地表 径流最终汇入河口; 汽车排放(汽油、柴油不完全燃烧) 产生的PAHs 主要富集在城市交通区和商业区的街道灰尘中, 枯季借助区域盛行风迁移至河口区, 洪季则主要通过暴雨径流冲刷进入河口。  相似文献   

11.
滇池不同流域类型降雨径流对河流氮磷入湖总量的影响   总被引：25，自引：5，他引：20  
通过对滇池三种不同流域类型的雨季初始期三场降雨径流的汇水河道的入湖口水质和流量监测 ,重点分析了典型城市纳污河流、城乡结合型河道和农业重污染区河道的营养盐携带状况与特征。研究结果表明 :不同流域类型河流的氮磷营养盐入湖总量受降雨过程及特征、流域类型特征、降雨径流流量、径流水营养盐浓度综合控制。城乡结合型河道 (大清河 )有最高的TP、KN (凯氏N)、NH3 N、NO3 N和NO2 N入湖总量 ,三场降雨累积量分别为11374 3、 12 7971 7、 85 36 5 4、 92 3 4和 84 1 2kg ;城市纳污河流 (乌龙河 )有最高的单位面积入湖总量负荷 ,TP、KN、NH3 N和NO2 N分别为 5 35 7、 5 86 0 5、 382 1 9和 2 4 6kg/km2 。  相似文献   

12.
Samples of suspended particulate matters (SPMs), surface sediment and road dust were collected from the Yangtze estuarine and nearby coastal areas, coastal rivers, and central Shanghai. The samples were analyzed for the presence of 16 polycyclic aromatic hydrocarbons (PAHs) in the USEPA priority-controlled list by GC-MS. The compound-specific stable carbon isotopes of the individual PAHs were also analyzed by GC-C-IRMS. The sources of PAHs in the SPMs and surface sediments in the Yangtze estuarine and nearby coastal areas were then identified using multiple source identification techniques that integrated molecular mass indices with organic compound-specific stable isotopes. The results revealed that 3-ring and 4-ring PAH compounds were dominant in the SPMs and surface sediments, which are similar to the PAH compounds found in samples from the Wusong sewage discharge outlet, Shidongkou sewage disposal plant, Huangpu River, coastal rivers and central Shanghai. Principal component analysis (PCA) integrated with molecular mass indices indicated that gasoline, diesel, coal and wood combustion and petroleum-derived residues were the main sources of PAHs in the Yangtze Estuary. The use of PAH compound- specific stable isotopes also enabled identification of the PAHs input pathways. PAHs derived from wood and coal combustion and petroleum-derived residues were input into the Yangtze Estuary and nearby coastal areas by coastal rivers, sewage discharge outlets during the dry season and urban storm water runoff during the flood season. PAHs derived from vehicle emissions primarily accumulated in road dust from urban traffic lines and the commercial district and then entered the coastal area via the northwest prevailing winds in the dry season and storm water runoff during flood season.  相似文献   

13.
A revised typology of Australian tropical rivers was applied to the complete channel network (named and major rivers) shown on 1:250 000 topographic maps for three large drainage basins in northern Australia (Daly River, NT; Fitzroy River, WA; Flinders River, Qld). Reach mapping and classification were conducted using the revised typology. The 12 major river types proposed were: (1) bedrock rivers; (2) bedrock‐confined and ‐constrained rivers; (3) low sinuosity (straight) rivers; (4) meandering rivers; (5) wandering rivers; (6) anabranching rivers; (7) chains of ponds; (8) gullies; (9) floodouts; (10) lakes, swamps, billabongs and wetlands; (11) non‐channelized valley floors; and (12) estuarine rivers. The 12 major river types were developed based on river reach mapping for more than 264 000 km2 of tropical Australian catchments. At scales larger than 1:250 000, subdivision of each major river type is recommended. In the Daly and Fitzroy catchments, confined and constrained rivers dominate, whereas in the Flinders and Fitzroy catchments, anabranching rivers dominate. The dominant river types need benchmarking with adequate numbers of control reaches so that channel changes induced by human and natural impacts can be measured by reference to the stability of these controls. Wandering rivers, floodouts and non‐channelized valley floors were rare for the 1:250 000 channel network in northern Australia but need inclusion in national parks.  相似文献   

14.
A quantitative assessment is made of suspended sediment load, including particulate organic matter and organic carbon, in 2014 for the small streams of the Northern Yenisei region, in the taiga–tundra transition zone (near the city of Igarka, Krasnoyarsk krai). It was found that the suspended sediment concentration (SSC) of the streams under investigation fluctuated between 2 and 18 mg/L during the summer–autumn low-water period of 2014. The proportion of dissolved organic matter (DOM) in the total sediment yield varied from 16.4% to 74.1%, depending on landscape-geomorphological conditions for suspended sediment formation: it is higher for streams with tundra catchments and lower on forest watersheds underlain by sandy and clayey loams. The DOM content varies from catchment to catchment from 1.63 to 2.42 mg/L, and the mean concentration of dissolved organic carbon (DOC) is estimated at 0.73 to 1.09 mg C/L. It is shown that the local channel transformations serve as the main source of POM and DOC input to the water of two out of three streams under study. Surface runoff or fast subsurface flow in the organic soil horizon is the external source of DOM input to the water of the third stream during flooding. Regional empirical dependencies were obtained, which correlate the water discharge, total SSC and the proportion of DOM are obtained. The long-term proportion of DOM in the annual suspended sediment flow of the Graviika river makes up 25% and DOC, 11%, or, in absolute values, 406 and 183 t/year, and in units of layer 1.26 and 0.57 t/km2, respectively.  相似文献   

15.
This study contrasts the effects of human disturbances on two very different lake/catchment systems: Hatch Pond and Beaver Lake, New Hampshire. Hatch is in a steep mountain catchment remote from urban/industrial centers, and is a small, relatively deep, primarily seepage lake with moderate flushing rate. The catchment has been continuously forested, but disturbed by partial loggings and a forest fire. Beaver’s more extensive and gently sloping catchment is much closer to urban/industrial centers, and has been agricultural and recently suburban. Beaver is a larger but shallower drainage lake with much more rapid flushing than Hatch. We compared the sedimentary records and inferred limnological responses to catchment land uses and air pollution inputs of these mesotrophic lakes, and interpreted differing responses as a function of basic differences between the lakes and their catchments. Some chemical and biological variables in the sediment of both lakes respond sensitively to the first disturbances of the catchments by Euro-American settlers. Diatom-inferred Cl at both lakes indicates a modest increase of salinity at this time. Hatch sediment contains a record of soil erosion starting 1810 with first logging and fire. For ~125 years, erosion was largely of upper eluviated soil, but by 1935 it reached deeper into the illuviated (enriched) horizon. Maximal lake trophic state based on diatom-inferred limnological variables occurred in the mid-1900’s period of maximum sedimentation of illuviated soil. The sediment record since 1964 reflects forest maturation, and soil stabilization and acidification, but not lake acidification. At Beaver, the limnological effects of forest clearance and agriculture starting ~1700 were relatively mild due to gentleness of slopes and soil characteristics favoring stability. A near doubling of earth elements, and major increases in trace metal pollutants and coal combustion particles (CCP) occurred in sediment dating around 1900. Landscape analysis as well as historical and sedimentary records preclude the catchment as the major source of these increases. The most likely source is atmospheric fallout of CCP with its metal load. Despite controls on CCP and other emissions starting 1960, concentrations of earth elements and trace metals in Beaver sediment remain high due to soil mobilization by residential development of the catchment. The trophic state of Beaver Lake has increased, but the relative increase has been smaller than at Hatch, despite more intensive land uses and greater aerial inputs at Beaver. We propose that this lesser eutrophication is due to rapid flushing of Beaver Lake with stream water from relatively undeveloped parts of the extensive catchment, and lower sensitivity to nutrient inputs of this naturally more eutrophic lake. A major shift from unicellular to colonial chrysophytes at Hatch starts in the late-1800’s, and at Beaver in the early 1900’s. Colonial taxa in lesser quantities appear at the time of first settlement of the Beaver catchment. At both lakes the shifts are correlated with increasing metal fluxes from the opening of catchment biogeochemical cycles, as with the aforementioned erosional sequence at Hatch. But at Hatch aerial inputs of trace metals, and at Beaver aerial inputs major and trace metals associated with CCP are also correlated with the major chrysophyte shift. It appears that the chrysophytes have responded to stressors associated with both catchment disturbance and regional atmospheric inputs.  相似文献   

16.
洞庭湖年径流泥沙的演变特征及其动因   总被引：18，自引：2，他引：16  
通过对洞庭湖1951~1998年径流泥沙演变过程及其驱动力的全面分析表明, 径流泥沙关系密切, 其相关系数r = 0.9013。年径流量、年输沙量总体均呈同步减少趋势, 在演变过程中表现出明显的阶段性。由于湘、资、沅、澧四水流域产水量大, 森林覆盖率达52%以上, 连年兴建的水利工程及工农业、生活用水量的增加, 未能对四水河流水文特征产生根本性的影响, 其入湖径流泥沙基本处于稳定状态, 故没有对湖泊径流泥沙的演变造成深刻影响。而由长江中游河段的调弦口堵口, 下荆江系统裁弯和葛洲坝截流所引起的3次江湖水沙关系调整, 即是导致洞庭湖径流泥沙缓减速减的主动因子。  相似文献   

17.
Samples of suspended particulate matters(SPMs),surface sediment and road dust were collected from the Yangtze estuarine and nearby coastal areas,coastal rivers,and central Shanghai.The samples were analyzed for the presence of 16 polycyclic aromatic hydrocarbons(PAHs)in the USEPA priority-controlled list by GC-MS.The compound-specific stable carbon isotopes of the individual PAHs were also analyzed by GC-C-IRMS.The sources of PAHs in the SPMs and surface sediments in the Yangtze estuarine and nearby coastal...  相似文献   

18.
We used statistical analyses to determine which subset of 36 environmental variables best explained variations in surface sediment δ13C and δ15N from 50 lakes in western Ireland that span a human-impact gradient. The factors controlling lake sediment δ13C and δ15N depended on whether organics in the lake sediment were mostly derived from the lake catchment (allochthonous) or from productivity within the lake (autochthonous). Lake sediments with a dominantly allochthonous organic source (high C:N ratio sediments) produced δ13C and δ15N measurements similar to values from catchment vegetation. δ13C and δ15N measurements from lake sediments with a dominantly autochthonous organic source (low C:N ratio sediments) were influenced by fractionation in the lake and catchment leading up to assimilation of carbon and nitrogen by lacustrine biota. δ13C values from lake sediment samples in agricultural catchments were more negative than δ13C values from lake sediment samples in non-impacted, bogland catchments. Hypolimnetic oxygen concentrations and methane production had a greater influence on δ13C values than fractionation due to algal productivity. δ15N from lake sediment samples in agricultural catchments were more positive than δ15N in non-impacted bogland catchments. Lower δ15N values from non-impacted lake catchments reflected δ15N values of catchment vegetation, while higher δ15N values in agricultural catchments reflected the high δ15N values of cattle manure and inorganic fertilisers. The influence of changing nitrogen sources and lake/catchment fractionation processes were more important than early diagenesis for lake sediment δ15N values in this dataset. The results from this study suggest a possible influence of bound inorganic nitrogen on the bulk sediment δ15N values. We recommend using a suitable method to control for bound inorganic nitrogen in lake sediments, especially when working with clay-rich sediments. This study confirms the usefulness of δ13C and δ15N from bulk lake sediments, as long as we are mindful of the multiple factors that can influence these values. This study also highlights how stable isotope datasets from lake surface sediments can complement site-specific isotope source/process studies and help identify key processes controlling lake sediment δ13C and δ15N in a study area.  相似文献   

19.
Information on post-fire sediment and nutrient redistribution is required to underpin post-fire catchment management decisions. Fallout radionuclide budgets (210Pbxs, 137Cs and 7Be) were derived to quantify soil redistribution and sediment yield in forested terrain following a moderately severe wildfire in a small (89 ha) water supply catchment in SE Australia. Application of these techniques in burnt terrain requires careful consideration of the partitioning of radionuclides between organic and mineral soil components. Beryllium-7 and 210Pbxs were shown to be closely associated with ash, litter and soil organic matter whereas 137Cs was more closely associated with subsurface coarse mineral soil. Comparison of the three tracer budgets indicated that the dominant sediment source areas were ridgetops and steep valley sideslopes, from which burnt surface material was conveyed to the stream network via pre-existing gullies. Erosion was predominantly driven by sheetwash, enhanced by soil water repellency, and modified by bioturbation which both supplies subsurface sediment and provides sinks for erosive overland flow. Footslope and riparian zones were not important sediment source areas. The estimated event-based (wildfire and subsequent rainfall) sediment yield is 58 ± 25 t km− 2, based on fallout 7Be measurements. The upper estimate of total particulate phosphorus yield (0.70 kg ha− 1) is more than 10 times that at equivalent unburnt sites. This illustrates that, soon after fire, burnt eucalypt forest can produce nutrient loads similar to those of agricultural catchments. The tracer budgets indicate that wildfire is an important control on sediment and phosphorus inputs to the stream network over the decadal timeframe and the pulsed nature of this release is an important concern for water quality management.  相似文献   

20.
Changes to the tectonic boundary conditions governing erosional dynamics in upland catchments have a significant effect on the nature and magnitude of sediment supply to neighbouring basins. While these links have been explored in detail by numerical models of landscape evolution, there has been relatively little work to quantify the timing, characteristics and locus of sediment release from upland catchments in response to changing tectonic boundary conditions that are well‐constrained independently. We address this challenge by quantifying the volume and granulometric characteristics of sediment exported from modern rivers draining across active normal faults in the Central Apennines in Italy. We demonstrate that catchments undergoing a transient response to tectonics are associated with significant volumetric export of material derived primarily from the zone upstream of the fault, producing bi‐modal grain‐size distributions with elevated D84 values within the transient reach. This is in direct contrast to the headwaters, where the fluvial capacity to transport sediment is low and the grain‐size distribution of material in transit is fine and uni‐modal. The grain‐size response is driven by landslides feeding coarse material directly into the channel, and we show the amplitude of the signal is modulated by the degree of tectonic perturbation, once the threshold for bedrock landsliding is exceeded. Additionally, we evaluate the length‐scale over which this transient grain‐size signal propagates downstream into the basin. We show that the coarse‐fraction sediment released is retained in the proximal hanging‐wall if rates of tectonic subsidence are high and if the axial river system is small or far from the fault‐bounded mountain front. Our results therefore provide some of the first quantitative data to evaluate how transient landscape responses affect the locus, magnitude and calibre of sediment supply to basins.  相似文献   

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