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1.
Characterization of carbonaceous aerosols including CC (carbonate carbon), OC (organic carbon), and EC (elemental carbon) were investigated at Xi'an, China, near Asian dust source regions in spring 2002. OC varied between 8.2 and 63.7 μg m-3, while EC ranged between 2.4 and 17.2 μ m-3 during the observation period. OC variations followed a similar pattern to EC and the correlation coeflcient between OC and EC is 0.89 (n=31). The average percentage of total carbon (TC, sum of CC, OC, and EC) in PM2.5 during dust storm (DS) events was 13.6%, which is lower than that during non-dust storm (NDS) periods (22.7%). CC, OC, and EC accounted for 12.9%, 70.7%, and 16.4% of TC during DS events, respectively. The average ratio of OC/EC was 5.0 in DS events and 3.3 in NDS periods. The OC-EC correlation (R2=0.76, n=6) was good in DS events, while it was stronger (R2=0.90, n=25) in NDS periods. The percentage of water-soluble OC (WSOC) in TC accounted for 15.7%, and varied between 13.3% and 22.3% during DS events. The distribution of eight carbon fractions indicated that local emissions such as motor vehicle exhaust were the dominant contributors to carbonaceous particles. During DS events, soil dust dominated the chemical composition, contributing 69% to the PM2.5 mass, followed by organic matter (12.8%), sulfate (4%), EC (2.2%), and chloride (1.6%). Consequently, CC was mainly entrained by Asian dust. However, even in the atmosphere near Asian dust source regions, OC and EC in atmospheric dust were controlled by local emission rather than the transport of Asian dust.  相似文献   

2.
Aerosol particles can directly alter the radiation balance by scattering and absorbing incident solar radiation, thus decreasing the amount of light reaching the surface and increasing the fraction of diffuse radiation—the so-called ‘aerosol direct radiative effect'. Using the Moderate Resolution Imaging Spectroradiometer aerosol products, the aerosol direct radiative effects under all-sky conditions in Beijing and Shanghai in 2007 were explored in this study. The total shortwave radiation was calculated using the Fu-Liou radiative transfer model, with the influence of clouds taken into account through sunshine-duration data, and the diffuse radiation was calculated with radiation decomposition models. Good correlation between measured and calculated total radiation was obtained at both cities, with an R greater than 0.9, and thus this calculation method was adopted to derive aerosol direct radiative effects. The presence of aerosols caused the mean total and diffuse solar radiation reaching the surface to change by-19.9% and +27.4% in Beijing, respectively, and by-18.4% and +6.5% in Shanghai. It was also found that, despite the strong negative correlation between aerosol optical depth and total radiation change, the diffuse radiation changes were determined predominantly by clouds. The effects of such changes induced by aerosols on plant productivity should be further studied.  相似文献   

3.
Based on daily observation data at 222 meteorological stations in China,the characteristics of dust storms between 1997 and 2007 were examined.Next,the relationship between dust events and chlorophyll (Chl) a concentration in the Yellow Sea was investigated.There were six regions with high annual frequencies of dust storms.The seasonal distribution of dust storms showed spatiotemporal variation.The six regions with highest annual frequencies also exhibited high frequencies of dust storms in spring.Dust storms in most regions occurred in spring.Of all dust storms in China,sixty-five percent of all dust storms occurred during the spring.The area and frequency of dust storms were smaller in fall and winter than in spring and summer.A significant correlation was found between dust events and Chl a concentration in the Yellow Sea.High correlation regions included Qinghai-Xizang region,part of the Hexi Corridor,the western Inner Mongolia and Hetao Regions,and the Hunshandake Desert.The high correlation may be induced by the high ratio of dust storms in the abovementioned regions that arrive over the Yellow Sea,as inferred through a forward trajectory analysis;especially notable is dust transported at a lower altitude (< 3 km).  相似文献   

4.
Dust aerosol optical depth （AOD） and its accompanying shortwave radiative forcing （RF） are usually simulated by numerical models. Here, by using 9 months of Moderate Resolution Imaging Spectroradiometer （MODIS） aerosol product data in combination with Clouds and the Earth＇s Radiant Energy System Single Scanner Footprint （CERES/SSF） data, dust AOD and its shortwave RF were estimated over the cloud-free northwest （NW） Pacific Ocean in the springs of 2004, 2005, and 2006. The results showed that in this region, the mean dust AOD and its shortwave RF were 0.10 and -5.51 W m^-2, respectively. In order to validate the dust AOD derived by MODIS, results from the Goddard Global Ozone Chemistry Aerosol Radiation and Transport （GOCART） model were also used here. The correlation coefficient between the monthly averaged dust AOD derived by MODIS measurements and the model simulation results was approximately 0.53. Since the estimates of the dust AOD and its shortwave RF obtained in this study are based mainly on satellite data, they offer a good reference for numerical models.  相似文献   

5.
The spatial distributions and interannual variations of aerosol concentrations,aerosol optical depth(AOD) ,aerosol direct radiative forcings,and their responses to heterogeneous reactions on dust surfaces over East Asia in March 2006-10 were investigated by utilizing a regional coupled climate-chemistry/aerosol model. Anthropogenic aerosol concentrations(inorganic+carbonaceous) were higher in March 2006 and 2008,whereas soil dust reached its highest levels in March 2006 and 2010,resulting in stronger aerosol radiative forcings in these periods.The domain and five-year(2006-10) monthly mean concentrations of anthropogenic and dust aerosols,AOD,and radiative forcings at the surface(SURF) and at the top of the atmosphere(TOA) in March were 2.4μg m-3,13.1μg m-3,0.18,-19.0 W m-2,and-7.4 W m-2,respectively.Heterogeneous reactions led to an increase of total inorganic aerosol concentration;however,the ambient inorganic aerosol concentration decreased,resulting in a smaller AOD and weaker aerosol radiative forcings.In March 2006 and 2010,the changes in ambient inorganic aerosols,AOD,and aerosol radiative forcings were more evident.In terms of the domain and five-year averages,the total inorganic aerosol concentrations increased by 13.7%(0.17μg m-3) due to heterogeneous reactions,but the ambient inorganic aerosol concentrations were reduced by 10.5%(0.13μg m-3) .As a result,the changes in AOD,SURF and TOA radiative forcings were estimated to be-3.9%(-0.007) ,-1.7%(0.34 W m-2) ,and-4.3%(0.34 W m-2) ,respectively,in March over East Asia.  相似文献   

6.
The present study investigates the characteristics of turbulent transfer and the conditions for dust emission and transport using the dust concentration and micrometeorological data obtained during dust events occurring in the spring of 2004 over the Hunshandake desert area. The turbulent exchange coefficients and turbulent fluxes of momentum and heat are calculated. The relationships between dust flux, friction velocity, and wind speed are also explored. The results show that thermal turbulence is dominant during daytime of non-dusty days. The dynamic turbulence increases obviously and the sensible heat flux reduces by different degrees during dust events. There is an efficient downward transfer of momentum before duststorm occurrence, and both the dynamic turbulence and the thermal turbulence are important in the surface layer. The dynamic turbulence even exceeds the thermal turbulence during severe duststorm events. The values of dust flux vary in the range of -5 5, -30 30, and -200-300 μg m^-2 s^-1 during non-dusty days, blowing dust, and duststorm events, respectively. A slight upward transport of dust is observed during non-dusty days. The dust flux gradually varies from positive to negative during duststorm periods, which indicates the time evolution of dust events from dust rising to stably suspending and then deposition. The dust flux is found to be proportional to u＊^3. The threshold values of wind speed and friction velocity are about 6 and 0.4 m s^-1, respectively.  相似文献   

7.
Characterization of carbonaceous aerosols including CC （carbonate carbon）, OC （organic carbon）, and EC （elemental carbon） were investigated at Xi＇an, China, near Asian dust source regions in spring 2002. OC varied between 8.2 and 63.7μgm^- 3, while EC ranged between 2.4 and 17.2 μ m^-3 during the observation period. OC variations followed a similar pattern to EC and the correlation coefficient between OC and EC is 0.89 （n=31）. The average percentage of total carbon （TC, sum of CC, OC, and EC） in PM2.5 during dust storm （DS） events was 13.6%, which is lower than that during non-dust storm （NDS） periods （22.7%）. CC, OC, and EC accounted for 12.9%, 70.7%, and 16.4% of TC during DS events, respectively. The average ratio of OC/EC was 5.0 in DS events and 3.3 in NDS periods. The OC-EC correlation （R^2=0.76, n=6） was good in DS events, while it was stronger （R^2=0.90, n=25） in NDS periods. The percentage of watersoluble OC （WSOC） in TC accounted for 15.7%, and varied between 13.3% and 22.3% during DS events. The distribution of eight carbon fractions indicated that local emissions such as motor vehicle exhaust were the dominant contributors to carbonaceous particles. During DS events, soil dust dominated the chemical composition, contributing 69% to the PM2.5 mass, followed by organic matter （12.8%）, sulfate （4%）, EC （2.2%）, and chloride （1.6%）. Consequently, CC was mainly entrained by Asian dust. However, even in the atmosphere near Asian dust source regions, OC and EC in atmospheric dust were controlled by local emission rather titan the transport of Asian dust.  相似文献   

8.
A continuous measurement of number size distributions and chemical composition of aerosol particles was conducted in Beijing in a dust storm event during 21-26 March 2001. The number concentration of coarse particles （ 〉2μm） increased more significantly than fine particles （ 〈2μm） during the dust storm due to dust weather, while the anthropogenic aerosols collected during the non-dust-storm period tended to be associated with fine particles. Elemental compositions were analyzed by using proton-induced X-ray emission （PIXE）. The results show that 20 elements in the dust storm were much higher than in the non-dust-storm period. The calculated soil dust concentration during the dust storm was, on average, 251.8μg m^-3, while it was only 52.1μg m^-3 on non-dust-storm days. The enrichment factors for Mg, A1, P, K, Ca, Ti, Mn, Fe, C1, Cu, Pb, and Zn show small variations between the dust storm and the non-dust-storm period, while those for Ca, Ni and Cr in the dust storm were much lower than those in the non-dust-storm period due to significant local emission sources. A high concentration and enrichment factor for S were observed during the dust storm, which implies that the dust particles were contaminated by aerosol particles from anthropogenic emissions during the long-range transport. A statistical analysis shows that the elemental composition of particles collected during the dust storm in Beijing were better correlated with those of desert soil colleted from desert regions in Inner Mongolia. Air mass back-trajectory analysis further confirmed that this dust storm event could be identified as streaks of dust plumes originating from Inner Mongolia.  相似文献   

9.
The emission of dust particles into the atmosphere is governed by the aerodynamic and resistant factors,which are quantified by the friction velocity u＊ and the threshold friction velocity u＊t, respectively. The threshold friction velocity u＊t influences the vertical dust flux and dust transport. Based on the micrometeorological data obtained in the springs of 2004 and 2006 over Hunshandake desert area, Loess Plateau,and Gobi desert area, the relationship between dust concentration and friction velocity for the dust events that occurred over Hunshandake desert area was investigated, and the threshold friction velocities over the three different dust source areas were estimated. The results show that the value of dust concentration is low during the preemission stage of a dust storm event, and the rapid increase of friction velocity provides favorable dynamic conditions for dust emission. During the dust emission stage, the dust concentration increases sharply due to mechanical and thermal turbulent mixing. At the calm-down stage, the dust concentration drops nearly linearly with the decreasing friction velocity, on account of the gravitational deposition of larger dust particles. When the dust concentration is higher than 200 μg m-3, it is considered as a dust emission process. According to the criteria, the values of threshold friction velocity over Hunshandake desert area and Gobi region are 0.6 and 0.45 m s-1, respectively. The threshold friction velocity over Loess Plateau depends on the wind direction, due to the complex terrain and inhomogeneous surface. The northwest wind shows the effects of the Mu Us desert in the northwest. The corresponding u＊t is 0.35 m s-1. The south wind exhibits the characteristics of the Loess hilly dunes in the south, and the u＊t is 0.7 m s-1.The large roughness length of the Loess hilly dunes and the large inter-particle cohesion for the clay soil texture increases the local friction velocity. Different threshold friction velocities and occurrence frequencies of strong wind account for different dust emission capabilities for various source areas.  相似文献   

10.
The temperature anomaly and dust concentrations recorded from central Antarctic ice core records display a strong negative correlation. The dust concentration recorded from an ice core in central Antarctica is 50-70 times higher during glacial periods than interglacial periods. This study investigated the impact of dust aerosol on glacial-interglacial climate, using a zonal energy balance model and dust concentration data from an Antarctica ice core. Two important effects of dust, the direct radiative effect and dust-albedo feedback, were considered. On the one hand, the direct radiative effect of dust significantly cooled the climate during the glacial period, with cooling during the last glacial maximum being as much as 2.05℃ in Antarctica. On the other hand, dust deposition onto the ice decreased the surface albedo over Antarctica, leading to increased absorption of solar radiation, inducing a positive feedback that warmed the region by as much as about 0.9℃ during the glacial period. However, cooling by the direct dust effect was found to be the controlling effect for the glacial climate and may be the major influence on the strong negative correlation between temperature and dust concentration during glacial periods.  相似文献   

11.
Deposition of atmospheric mineral particles in the North Pacific Ocean   总被引：5，自引：0，他引：5  
Total deposition of atmospheric mineral particles (wet plus dry) has been measured during consecutive two-week sampling intervals from January, 1981 to March, 1982 at four island stations (Midway, Oahu, Enewetak, and Fanning) of the SEAREX Asian Dust Study Network in the North Pacific. The total deposition of mineral aerosol during the period from February to June is higher than that during the period from July to January at most of the stations. A systematic geographical trend is apparent in the dust flux, with greater fluxes at higher latitudes. The deposition values are correlated with the atmospheric mineral particle concentrations at these stations. The mineral particles are transported from arid regions in Asia to the North Pacific, and the annual dust deposition to the ocean appears to be dominated by sporadic dust events of short duration. Wet deposition dominates the removal of dust particles from the atmosphere over the North Pacific. The total deposition of atmospheric mineral material to the central North Pacific is estimated to be 20×1012 g yr-1.  相似文献   

12.
高玮  屈文军 《山东气象》2018,38(4):81-92
研究了非洲地区大气气溶胶光学厚度（AOD）的时空变化及沙尘气溶胶越大西洋海区的传输。结果表明：1）源于撒哈拉沙漠的沙尘及其随赤道东风向西输送使得沙尘气溶胶成为非洲沙漠地区和紧邻的大西洋海区的主要气溶胶组分;AOD高值区和沙尘气溶胶光学厚度高值区在1—7月随赤道辐合带北移同步向北移动,而在8—12月则向南回撤。2）刚果盆地大气气溶胶主要为热带雨林和稀树草原排放的有机碳（OC）和黑碳（BC）气溶胶;其中与生物质燃烧源排放有关的OC、BC高值主要集中在干季（6—9月）的后半段（8—9月）;而生物源OC排放全年连续,其排放峰值出现于雨季开始时;生物质燃烧排放高值期与生物源排放高值期前后相继,形成干季（尤其是后半段）时期的OC、BC光学厚度高值。3）亚马逊河入海口地区主要气溶胶组分为海盐气溶胶,9—11月该区风力输送增强,风向由东南风转变为东风,海盐进入亚马逊河入海口处,形成AOD和海盐气溶胶光学厚度高值区。4）撒哈拉沙漠沙尘气溶胶向大西洋传输的偏北月份为7—9月、偏南月份为1—3月;2000—2016年海区沙尘气溶胶的传输路径存在向南移动的变化趋势,与同期亚速尔高压的增强和沙尘传输路径以北北风分量的增强以及赤道辐合带的移动一致。上述研究结果揭示了利用大气气溶胶时空变化特征反映区域大气环流和气候变化的可能性。  相似文献   

13.
近10年东亚沙尘气溶胶时空分布与起尘通量的数值研究   总被引：2，自引：0，他引：2  
宿兴涛  王汉杰 《高原气象》2012,31(3):676-687
利用一个耦合了沙尘模型的区域气候模式RegCM3和NCEP再分析资料,对近10年(2000-2009年)东亚地区沙尘气溶胶(直径≤20μm)时空分布特征和起尘通量进行了数值模拟。结果表明,(1)耦合模式能较好地模拟东亚地区沙尘气溶胶的时空分布特点。东亚地区沙尘气溶胶光学厚度、柱含量高值区主要位于塔克拉玛干沙漠和巴丹吉林沙漠。沙尘气溶胶柱含量的季节变化特征明显,春季最大,冬季次之,秋季最小。东亚地区110°E以东,沙尘主要以700hPa高度为中心向东传输。(2)东亚地区起沙源区主要位于塔克拉玛干沙漠、巴丹吉林沙漠、藏北沙漠化地区及蒙古国西南部,起沙强度存在明显的季节变化。2000-2009年东亚地区年平均起沙通量为1015.34mg.m-2.d-1,其中62.4%和2.3%分别通过干、湿过程重新沉降在东亚地区,其余35.3%被净释放进入大气或进行远距离传输。  相似文献   

14.
2006年一次沙尘活动的卫星定量遥感和分析研究   总被引：1，自引：0，他引：1  
针对MODIS监测的2006年3月我国新疆区域发生的一次沙尘活动,基于卫星红外窗区3通道(8.5、11和12 μm)方法,自动识别并同步物理反演了沙尘大气的光学厚度、粒子有效半径和垂直气柱沙尘总量,同时利用后向轨迹方法模拟计算的4种高度的气团轨迹对此次反演试验结果的合理性进行了分析和验证,结果表明两者相当一致.  相似文献   

15.
利用2006年3～5月天空辐射计观测数据反演得到北京地区春季大气气溶胶光学性质参数,包括大气气溶胶光学厚度(0.5μm)、Angstrm指数、单次散射反射比和粒子谱分布特征。结果表明:北京地区春季气溶胶平均光学厚度0.67,Angstrm指数0.54,单次散射比0.88,粒子吸收性质较弱,粒子谱呈双峰形,以粗粒子为主,粗、细模态粒子粒径分别集中在0.17μm和7.7μm左右。相比2004年此次观测期间气溶胶粒径较大,粒子体积浓度较高,散射作用在其消光特性中的比重略有下降。光学厚度日变化呈单峰型,日间单次散射比随时间逐渐递减,Angstrm指数在上午递减趋势明显,午后变得稳定。对同时观测的天空辐射计与CE-318不同波长光学厚度结果进行比较,结果显示两者得到的光学厚度相关性很好,各波长小时平均结果的相对误差小于7%。  相似文献   

16.
京津冀地区一次强沙尘天气过程的成因及特征   总被引：1，自引：0，他引：1       下载免费PDF全文
利用常规污染物监测资料、卫星资料和再分析资料等,对京津冀地区在2017年春季遭遇的一次强沙尘天气过程进行分析。结果表明,此次过程是由地面冷锋过境,高空槽后冷空气持续补充引起,沙源地主要位于巴丹吉林、腾格里沙漠,随后以西北路径输送至京津冀地区。前期沙源地感热通量迅速增大,与中低层冷平流叠加,导致不稳定层结增强,助于起沙;高空强风速带加强并向下延伸,中低层次级环流发展,不但使沙尘传输并下降至地面,而且使高层高动量和高位涡冷空气下传,促进低空急流形成、低层系统发展,使大风及沙尘天气维持;沙尘过境时,地面至4 km高度存在沙尘型气溶胶,PM_(2.5)和PM_(10)浓度变化趋势较一致并达到重度污染水平,且气溶胶光学厚度(Aerosol Optical Depth,AOD)与空气质量指数(Air Quality Index,AQI)具有较好的时空匹配关系,重污染时段AOD值大于1,污染减弱时AOD值降至0.6以下。  相似文献   

17.
沙尘传输路径上气溶胶浓度与干沉降通量的粒径分布特征   总被引：1，自引：0，他引：1  
利用2002年春季中国北京、青岛和日本福冈3个地区的分级气溶胶浓度资料,结合改进的Wil-liams模型,分析了沙尘传输路径上空气动力学直径≤11μm气溶胶(PM11)浓度和干沉降通量的粒径分布特征,并估算了黄海海域春季PM11的干沉降通量及不同粒径气溶胶的贡献。结果表明:3个地区PM11浓度粒径分布在非沙尘时期呈双峰分布,两个峰值分别出现在细颗粒(<2.1μm)部分和粗颗粒(2.1～11μm)部分;沙尘时期,3个地区PM11浓度粒径分布均趋于单峰分布,峰值位于粗颗粒部分,并且越靠近沙尘源地,这种趋势越明显。较强沙尘天气时期,粗颗粒部分的浓度峰值粒径从沙尘源地附近到黄海西岸、东岸呈降低趋势,但在一般沙尘天气时期,这种现象并不明显。沙尘时期和非沙尘时期,3个地区粗颗粒的干沉降通量均随粒径增加而增大,细颗粒的干沉降通量随粒径的变化不明显。虽然沙尘时期粗颗粒沉降通量较非沙尘时期有明显增加,但粗颗粒对PM11干沉降通量的贡献与非沙尘时期相比,并没有明显的变化。较强沙尘天气时期,3个地区粗颗粒的干沉降通量明显高于一般沙尘天气时期;细颗粒的干沉降通量较一般沙尘天气时期略有增加。黄海海域春季沙尘时期PM11的干沉降通量约为31.70～58.59mg.m-2.d-1,非沙尘时期约为8.33～15.94mg.m-2.d-1。粗颗粒是黄海海域春季PM11干沉降通量的主要贡献者,约占PM11干沉降通量的94.2%以上。  相似文献   

18.
Inter-annual and regional variations in aerosol and cloud characteristics, water vapor and rainfall over six homogeneous rainfall zones in India during the core monsoon month of July from 2000 to 2010, and their correlations are analyzed. Aerosol optical depth (AOD) and aerosol absorbing index (AAI) in July 2002, a drought year are higher over India when compared to normal monsoon years. The drier conditions that existed due to deficient rainfall in July 2002 could be responsible for raising more dust and smoke resulting in higher AODs over India. In addition, over India precipitation is not uniform and large-scale interruptions occur during the monsoon season. During these interruptions aerosols can build up over a region and contribute to an increase in AODs. This finding is supported by the occurrence of higher anomalies in AOD, AAI and rainfall over India in July 2002. Aerosol characteristics and rainfall exhibit large regional variations. Cloud effective radius (CER), cloud optical thickness and columnar water vapor over India are the lowest in July 2002. CER decreases as AOD and AAI increase, providing an observational evidence for the indirect effect of aerosols. Eighty percent of CER in northwest India, and 30% of CER over All India in July 2002 are <14 μm, the precipitation threshold critical cloud effective radius. Northeast India shows contrasting features of correlation among aerosols, clouds and rainfall when compared to other regions. These results will be important while examining the inter-annual variation in aerosols, cloud characteristics, rainfall and their trends.  相似文献   

19.
Synergistic use of AIRS and MODIS for dust top height retrieval over land   总被引：1，自引：0，他引：1  
It is nontrivial to extract the dust top height(DTH) accurately from passive instruments over land due to the complexity of the surface conditions. The Moderate Resolution Imaging Spectroradiometer(MODIS) deep blue(DB) algorithm can be used to infer the aerosol optical depth(AOD) over high-reflective surfaces. The Atmospheric Infrared Sounder(AIRS) can simultaneously obtain the DTH and optical depth information. This study focuses on the synergistic use of AIRS observations and MODIS DB results for improving the DTH by using a stable relationship between the AIRS infrared and MODIS DB AODs. A one-dimensional variational(1DVAR) algorithm is applied to extract the DTH from AIRS. Simulation experiments indicate that when the uncertainty of the dust optical depth decreases from 50% to 20%, the improvement of the DTH retrieval accuracy from AIRS reaches 200 m for most of the assumed dust conditions. For two cases over the Taklimakan Desert, the results are compared against Cloud-Aerosol Lidar with Orthogonal Polarization(CALIOP) measurements. The results confirm that the MODIS DB product could help extract the DTH over land from AIRS.  相似文献   

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