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1.
A new two-dimensional zonal model of the stratosphere, based on a formulation in an isentropic framework, with complete chemistry has been coupled with a high resolution detailed microphysical model for polar stratospheric clouds (PSCs). The 2D model chemistry includes all presently known heterogeneous processes on sulfate aerosols and PSCs. The coupling of these two models, with inherently different time scales, is discussed. It is demonstrated that in order to obtain a realistic interrelationship between NOy and N2O an accurate simulation of the sedimentation by PSC particles is necessary. A good agreement of model PSC presence and observations is found for the Antarctic polar winter without the need to impose additional artificial temperature variations in the model. The calculated occurrence of polar stratospheric clouds and resulting heterogeneous chemistry during the Antarctic winter are discussed. Sensitivity of the polar stratospheric chemical composition and cloud formation for different perturbations is investigated by studying the effects of transport across the polar vortex boundary and heterogeneous processing by an enhanced sulfate aerosol load. The importance of including sedimentation for all cases is also discussed.  相似文献   

2.
The comprehensive chemistry module CHEM has been developed for application in general circulation models (GCMs) describing tropospheric and stratospheric chemistry, including photochemical reactions and heterogeneous reactions on sulphate aerosols and polar stratospheric clouds. It has been coupled to the spectral atmospheric GCM ECHAM3. The model configuration used in the current study has been run in an –off-line mode, i.e. the calculated chemical species do not affect the radiative forcing of the dynamic fields. First results of a 15-year model integration indicate that the model ECHAM3/CHEM runs are numerically efficient and stable, i.e. that no model drift can be detected in dynamic and chemical parameters. The model reproduces the main features regarding ozone, in particular intra- and interannual variability. The ozone columns are somewhat higher than observed (approximately 10%), while the amplitude of the annual cycle is in agreement with observations. A comparison with HALOE data reveals, however, a serious model deficiency regarding lower-stratosphere dynamics at high latitudes. Contrary to what is concluded by observations, the lower stratosphere is characterized by slight upward motions in the polar regions, so that some of the mentioned good agreements must be considered as fortuitous. Nevertheless, ECHAM3/CHEM well describes the chemical processes leading to ozone reduction. It has been shown that the mean fraction of the northern hemisphere, which is covered by polar stratospheric clouds (PSCs) as well as the temporal appearance of PSCs in the model, is in fair agreement with observations. The model results show an activation of chlorine inside the polar vortex which is stronger in the southern than in the northern winter hemisphere, yielding an ozone hole over the Antarctic; this hole, however, is also caused to a substantial degree by the dynamics. Interhemispheric differences concerning reformation of chlorine reservoir species HCl and ClONO2 in spring have also been well reproduced by the model.  相似文献   

3.
During the past decades, concurrent with global warming, most of global oceans, particularly the tropical Indian Ocean, have become warmer. Meanwhile, the Southern Hemispheric stratospheric polar vortex (SPV) exhibits a deepening trend. Although previous modeling studies reveal that radiative cooling effect of ozone depletion plays a dominant role in causing the deepening of SPV, the simulated ozone-depletion-induced SPV deepening is stronger than the observed. This suggests that there must be other factors canceling a fraction of the influence of the ozone depletion. Whether the tropical Indian Ocean warming (IOW) is such a factor is unclear. This issue is addressed by conducting ensemble atmospheric general circulation model (AGCM) experiments. And one idealized IOW with the amplitude as the observed is prescribed to force four AGCMs. The results show that the IOW tends to warm the southern polar stratosphere, and thus weakens SPV in austral spring to summer. Hence, it offsets a fraction of the effect of the ozone depletion. This implies that global warming will favor ozone recovery, since a warmer southern polar stratosphere is un-beneficial for the formation of polar stratospheric clouds (PSCs), which is a key factor to ozone depletion chemical reactions. Supported by National Natural Science Foundation of China (Grant Nos. 40775053 and 90711004), National Basic Research Program of China (Grant No. 2009CB421401), and Innovation Key Program of Chinese Academy of Sciences (Grant Nos. KZCXZ-YW-Q11-03, KZCZ2-YW-Q03-08)  相似文献   

4.
This paper reports the study data on variations in the ozone content in the middle stratosphere over Moscow based on millimeter wavelength observations during a range of midwinter sudden stratospheric warmings that occurred in the past two decades. The relation of ozone with planetary waves and the intensity of the polar stratospheric vortex has been established. The ozone vertical distribution has been monitored with a highly sensitive spectrometer with a two-millimeter wave band. The discovered phenomena of a relatively long-term lower ozone content in December in the considered cold half-year periods are related to the higher amplitude of the planetary wave with n = 1. Such phenomena preceded the development of strong midwinter stratospheric warmings, which, in turn, were accompanied by a significant increase in the ozone content in January. This ozone enrichment was related to the lower amplitude of the wave with n = 1 and higher amplitude of the wave with n = 2 and was accompanied by geopotential H c.v. growth in the polar vortex center. Specific features of variations in the ozone content under the influence of the major atmospheric processes are observed not only in certain cold half-year periods but are also well seen in the general averaged pattern for winters with strong stratospheric warmings.  相似文献   

5.
Based on total ozone data from the World Ozone Data Center and stratospheric geopotential height data from the Meteorological Institute of Berlin Free University for the months of January through March for the time period of 1958–1996, the influence of the 11-year solar cycle and the equatorial quasi-biennial oscillation (QBO) on total ozone and the stratospheric circulation at 30 hPa over Northern Europe is investigated. The analysis is performed for different levels of solar activity. The relationship of the equatorial QBO with ozone and the stratospheric circulation over the study region exhibits unique features attributed to strong opposite connections between the equatorial zonal wind and ozone/stratospheric dynamics during periods of solar minimum and maximum. Using the Solar/QBO effect, a statistical extraction of the interannual variations of total ozone and stratospheric circulation over Northern Europe has been attempted. The variations extracted and observed for late winter show very good correspondence. The solar/QBO effect in total ozone and stratospheric dynamics over Northern Europe appears to be related to planetary wave activity.  相似文献   

6.
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7.
The Stratospheric Regular Sounding project was planned to measure regularly the vertical profiles of several tracers like ozone, water vapor, NOx, ClOx and BrOx radicals, aerosol, pressure and temperature, at three latitudes, to discriminate between the transport and photochemical terms which control their distribution. As part of this project, the “Istituto di Fisica dell’Atmosfera” launched nine laser backscattersondes (LABS) on board stratospheric balloons to make observations of background aerosol and PSCs. LABS was launched with an optical particle counter operated by the University of Wyoming. Observations have been performed in the arctic, mid-latitudes and tropical regions in different seasons. Polar stratospheric clouds have been observed in areas inside and outside the polar vortex edge. A background aerosol was observed both in mid-latitudes and in arctic regions with a backscattering ratio of 1.2 at 692 nm. Very stratified aerosol layers, possibly transported into the lower stratosphere by deep convective systems, have been observed in the lower stratosphere between 20 and 29 km in the tropics in the Southern Hemisphere.  相似文献   

8.
The stratosphere holds a variety of particulates like polar stratospheric clouds (PSCs) and sulphate aerosols which catalyse chemical reactions. These reactions cause changes in the composition of the stratosphere, including the redistribution of active chlorine which might lead to ozone destruction. As a result during recent years a lot of effort has been directed towards the quantification of the uptake of trace gases like ClONO2, HCl, etc. into these particulates. However, it has been observed that many of the two and three dimensional models used in such studies are constrained by the lack of adequate rate constant data. This paper describes a theoretical approach to estimate the reaction rate constants for 23 gases on both types of polar stratospheric clouds (type I and II). It is found that for gases like N2O5, ClONO2 and HCl, diffusional uptake is important and contributes significantly to the heterogeneous reaction rate. A complete Lennard-Jones calculation is used to accurately compute the trace gas diffusion coefficients.  相似文献   

9.
利用2003-2011年的SABER/TIMED温度数据观测发现,在2006年、2009年和2010年北半球高纬（70°N）的冬季（1-3月）发生了“平流层顶抬升”.在这3次事件中,1月末-2月初的~50 km和~80 km高度处分别出现了温度的极大值~260 K和~230 K,即平流层顶的高度突然由原来的50 km左右上升至80 km左右,这就是平流层顶抬升事件;随着时间的推移,抬升的平流层顶的高度逐渐下降直至恢复到原有位置,与此同时其温度由~230 K上升至~260 K.值得注意的是,虽然在极区的每年冬天都发生平流层突然增温事件,但是只在伴随着极涡分裂的平流层突然增温事件后出现平流层顶抬升.此外,在发生平流层顶抬升事件的冬季里,高纬的重力波活动在1月末-2月初的~80 km高度处突然增强,对应着平流层顶的抬升时间和高度;在2月份之后,重力波活动在75 km以下逐渐增强、在75 km以上逐渐减弱,同时抬升的平流层顶也不断下降.通过重力波活动与平流层顶抬升事件的相关性分析,表明重力波活动可能对平流层顶的抬升有重要影响.  相似文献   

10.
冬季太阳11年周期活动对大气环流的影响   总被引：2，自引：0，他引：2       下载免费PDF全文
刘毅  陆春晖 《地球物理学报》2010,53(6):1269-1277
利用气象场的再分析资料和太阳辐射活动资料,对太阳11年周期活动影响北半球冬季(11月~3月)大气环流的过程进行了统计分析和动力学诊断.根据赤道平流层纬向风准两年振荡(QBO)的东、西风状态对太阳活动效应进行了分类讨论,结果表明：东风态QBO时,太阳活动效应主要集中在赤道平流层中、高层和南半球平流层,强太阳活动时增强的紫外辐射加热了赤道地区的臭氧层,造成平流层低纬明显增温,同时加强了南半球的Brewer-Dobson(B-D)环流,引起南极高纬平流层温度增加;而北半球中高纬的环流主要受行星波的影响,太阳活动影响很小.西风态QBO时,太阳活动效应在北半球更为重要,初冬时强太阳活动除了加热赤道地区臭氧层外,还抑制了北半球的B-D环流,造成赤道平流层温度增加和纬向风梯度在垂直方向的变化,从而改变了对流层两支行星波波导的强度;冬末时在太阳活动调制下,行星波向极波导增强,B-D环流逐渐恢复,造成北半球极地平流层明显增温,同时伴随着赤道区域温度的下降.  相似文献   

11.
The solid and liquid particles which constitute polar stratospheric clouds (PSCs) are of manifold importance to the meteorology of the stratosphere. The heterogeneous reactions which take place on and within these particles release halogens from relatively inert reservoir species into forms which can destroy ozone in the polar spring. In addition, solid PSC particles are instrumental in the physical removal of nitrogen oxides (denitrification) and water (dehydration) of regions of the polar stratosphere. Denitrification, in particular, allows extended ozone destruction by slowing the conversion of chlorine radicals back into reservoir species.We review the historical development of PSC studies, with particular emphasis on results from the last decade, encompassing developments in observations, in laboratory experiments, and in theoretical treatments. The technical challenge of measuring sufficient of the parameters describing any given PSC, to allow its microphysics to be understood, has driven forward balloon-borne, aircraft, and satellite instrumentation. The technical challenge of finding suitable laboratory proxies for PSCs, in order to observe the microphysics under controlled conditions, has resulted in a wide variety of experimental designs, some of which maximise the probability of observing phase change, others which mimic the surface–volume ratios of PSCs more closely. The challenge to theory presented by PSCs has resulted in improvements in the thermodynamics of concentrated inorganic solutions of volatile compounds, and a new general theory of freezing of water ice from concentrated aqueous solutions. Of the major processes involving PSCs, heterogeneous reaction probabilities for ternary HNO3/H2SO4/H2O solutions, and heterogeneous freezing to produce nitric-acid hydrates, are the least well understood.  相似文献   

12.
The transport mechanisms responsible for the seasonal behavior of total ozone are deduced from the comparison of model results to stratospheric data. The seasonal transport is dominated by a combination of the diabatic circulation and transient planetary wave activity acting on a diffusively and photochemically determined background state. The seasonal variation is not correctly modeled as a diffusive process. The buildup of total ozone at high latitudes during winter is dependent upon transient planetary wave activity of sufficient strength to cause the breakdown of the polar vortex. While midwinter warmings are responsible for enhanced ozone transport to high latitudes, the final warming marking the transition from zonal mean westerlies to zonal mean easterlies is the most important event leading to the spring maximum. The final warming is not followed by reacceleration of the mean flow; so that the ozone transport associated with this event is more pronounced than that associated with midwinter warmings.  相似文献   

13.
The planetary wave impact on the polar vortex stability, polar stratosphere temperature, and content of ozone and other gases was simulated with the global chemical–climatic model of the lower and middle atmosphere. It was found that the planetary waves propagating from the troposphere into the stratosphere differently affect the gas content of the Arctic and Antarctic stratosphere. In the Arctic region, the degree of wave activity critically affects the polar vortex formation, the appearance of polar stratospheric clouds, the halogen activation on their surface, and ozone anomaly formation. Ozone anomalies in the Arctic region as a rule are not formed at high wave activity and can be registered at low activity. In the Antarctic Regions, wave activity affects the stability of polar vortex and the depth of ozone holes, which are formed at almost any wave activity, and the minimal ozone values depend on the strong or weak wave activity that is registered in specific years.  相似文献   

14.
Ozone depression in the polar stratosphere during the energetic solar proton event on 4 August 1972 was observed by the backscattered ultraviolet (BUV) experiment on the Nimbus 4 satellite. Distinct asymmetries in the columnar ozone content, the amount of ozone depressions and their temporal variations above 4 mb level (38 km) were observed between the two hemispheres. The ozone destroying solar particles precipitate rather symmetrically into the two polar atmospheres due to the geomagnetic dipole field These asymmetries can be therefore ascribed to the differences mainly in dynamics and partly in the solar illumination and the vertical temperature structure between the summer and the winter polar atmospheres. The polar stratosphere is less disturbed and warmer in the summer hemisphere than the winter hemisphere since the propagation of planetary wave from the troposphere is inhibited by the wind system in the upper troposphere, and the air is heated by the prolonged solar insolation. Correspondingly, the temporal variations of stratospheric ozone depletion and its recovery appear to be smooth functions of time in the (northern) summer hemisphere and the undisturbed ozone amount is slighily, less than that of its counterpart. On the other hand, the tempotal variation of the upper stratospheric ozone in the winter polar atmosphere (southern hemisphere) indicates large amplitudes and irregularities due to the disturbances produced by upward propagating waves which prevail in the polar winter atmosphere. These characteristic differences between the two polar atmospheres are also evident in the vertical distributions of temperature and wind observed by balloons and rocker soundings.  相似文献   

15.
As a result of the long-term observations lead in region of Kola Peninsula, connection between character of variations of the ozone content in a stratosphere of Arctic regions and behavior and structure of a winter polar vortex is established. During winter seasons with well developed cyclone and duration of stable existence not less than 1.5–2 months were observed extremely low ozone number density at heights 20–25 km connected, apparently, with its chemical destruction. On the other hand, during disturbances of the vortex, accompanied strong stratospheric warming, was registered almost double increase of ozone amount in a high-altitude interval from 20 up to 40 km. Comparison of results of ground-based microwave monitoring of an ozone layer to data of the satellite instrument EOS MLS installed on satellite AURA is lead. In most cases comparison has shown satisfactory within the limits of an error of measurements coincidence of results. However in conditions of atmospheric disturbances when arose significant spatial heterogeneity, the discrepancy of results of comparison was marked. The possible reasons which cause the detected disagreement in results are discussed.  相似文献   

16.
Based on radiative transfer calculations, it is studied whether polar stratospheric clouds (PSCs) can be detected by the new Global Ozone Monitoring Experiment (GOME) on board the second European Research Satellite (ERS-2) planned to be launched in 1995. It is proposed to identify PSC-covered areas by use of an indicator, the Normalized Radiance Difference (NRD), which relates the difference of two spectral radiances at 0.515 µm and 0.67 µm to one radiance measured in the centre of the oxygen A-band at 0.76 µm. Simulations are carried out for two solar zenith angles, =78.5° and =86.2°. They indicate that, in presence of PSCs and with increasing solar zenith angles above =80°, the NRD decrease to values clearly below those derived under conditions of a cloud-free stratosphere. Results for =86.2° show that the method is successful independent of existing tropospheric clouds, of different tropospheric aerosol loadings, and of surface albedos. Results for =78.5° illustrate that PSC detection under conditions of smaller solar zenith angles <80° needs additional information about tropospheric clouds.  相似文献   

17.
Based on the daily NCEP/DOE reanalysis II data,dates of the boreal spring Stratospheric Final Warming(SFW) events during 1979–2010 are defined as the time when the zonal-mean zonal wind at the central latitudes(65°–75°N) of the westerly polar jet drops below zero and never recovers until the subsequent autumn.It is found that the SFW events occur successively from the mid to the lower stratosphere and averagely from the mid to late April with a temporal lag of about 13 days from 10 to 50 hPa.Over the past 32 years,the earliest SFW occurs in mid March whereas the latest SFW happens in late May,showing a clear interannual variability of the time of SFW.Accompanying the SFW onset,the stratospheric circulation transits from a winter dynamical regime to a summertime state,and the maximum negative tendency of zonal wind and the strongest convergence of planetary-wave are observed.Composite results show that the early/late SFW events in boreal spring correspond to a quicker/slower transition of the stratospheric circulation,with the zonal-mean zonal wind reducing about 20/5 m s-1 at 30 hPa within 10 days around the onset date.Meanwhile,the planetary wave activities are relatively strong/weak associating with an out-of-/in-phase circumpolar circulation anomaly before and after the SFW events in the stratosphere.All these results indicate that,the earlier breakdown of the stratospheric polar vortex(SPV),as for the winter stratospheric sudden warming(SSW) events is driven mainly by wave forcing;and in contrast,the later breakdown of the SPV exhibits more characteristics of its seasonal evolution.Nevertheless,after the breakdown of SPV,the polar temperature anomalies always exhibit an out-of-phase relationship between the stratosphere and the troposphere for both the early and late SFW events,which implies an intimate stratosphere–troposphere dynamical coupling in spring.In addition,there exists a remarkable interdecadal change of the onset time of SFW in the mid 1990s.On average,the SFW onset time before the mid 1990s is 11 days earlier than that afterwards,corresponding to the increased/decreased planetary wave activities in late winter-early spring before/after the 1990s.  相似文献   

18.
The global structures of annual oscillation (AO) and semiannual oscillation (SAO) of stratospheric ozone are examined by applying spherical harmonic analysis to the ozone data obtained from the Nimbus-7 solar backscattered UV-radiation (SBUV) measurements for the period November 1978 to October 1980. Significant features of the results are: (1) while the stratospheric ozone AO is prevalent only in the polar regions, the ozone SAO prevails both in the equatorial and polar stratospheres; (2) the vertical distribution of the equatorial ozone SAO has a broad maximum of the order of 0.5 (mixing ratio in g/g) and the maximum appears earlier at high altitude (shifting from May [and November] at 0.3 mb [60 km] to November [and May] at 40 mb); (3) above the 40 km level, the maximum of the polar ozone SAO shifts upward towards later phase with altitude with a rate of approximately 10 km/month in both hemispheres; (4) vertical distributions of the polar ozone AOs and SAOs show two peaks in amplitude with a minimum (nodal layer) in between and a rapid phase change with altitude takes place in the respective nodal layers; and (5) the heights of the ozone AO- and SAO-peaks decrease with latitude. The main part of AOs and SAOs of stratospheric ozone including hemispheric asymmetries is ascribable to: (i) temperature dependent ozone photochemistry in the upper stratosphere and mesosphere, (ii) variations of radiation field in the lower stratosphere affected by the annual cycle of solar illumination and temperature in the upper stratosphere and (iii) meridional ozone transport by dynamical processes in the lower stratosphere.  相似文献   

19.
Using the monthly mean NCEP/NCAR reanalysis and NOAA Extended Reconstructed sea surface temperature (SST) datasets, strong correlations between the SST anomalies in the North Pacific and calculated three-dimensional Eliassen–Palm vertical fluxes are indicated in December 1958–1976 and 1992–2006. These correlations between the interannual variations of the SST anomalies and the penetration of planetary waves into the stratosphere are much less during the decadal sub-period 1976–1992 in the positive phase of the Pacific Decadal Oscillation (PDO) and the decadal cold SST anomalies in the North Pacific. Interannual variations of the polar jet in the lower stratosphere in January are strongly associated with SST anomalies in the Aleutian Low region in December for the years with positive PDO index. This sub-period corresponds well with that of the violation of the Holton–Tan relationship between the equatorial Quasi-Beinnial Oscillation (QBO) and the stratospheric circulation in the extra-tropics. It is shown that interannual and interdecadal variations of stratospheric dynamics, including stratospheric warming occurrences in January, depend strongly on changes of the upward propagation of planetary waves from the troposphere to the stratosphere over North Eurasia in preceding December. These findings give evidences of a large impact of the decadal SST variations in the North Pacific on wave activity in early winter due to changes of thermal excitation of planetary waves during distinct decadal periods. Possible causes of the decadal violation of the Holton–Tan relationship, its relation to the PDO and an influence of the 11-year solar cycle on the stratosphere are discussed.  相似文献   

20.
Total ozone anomalies (deviation from the long-term mean) are created by anomalous circulation patterns. The dynamically produced ozone anomalies can be estimated from known circulation parameters in the layer between the tropopause and the middle stratosphere by means of statistics. Satellite observations of ozone anomalies can be compared with those expected from dynamics. Residual negative anomalies may be due to chemical ozone destruction. The statistics are derived from a 14 year data set of TOMS (Total Ozone Mapping Spectrometer January 1979-Dec. 1992) and corresponding 300 hPa geopotential (for the tropopause height) together with 30 hPa temperature (for stratospheric waves) at 60°N. The correlation coefficient for the linear multiple regression between total ozone (dependent variable) and the dynamical parameters (independent variables) is 0.88 for the zonal deviations in the winter of the Northern Hemisphere. Zonal means are also significantly dependent on circulation parameters, besides showing the known negative trend function of total ozone observed by TOMS. The significant linear trend for 60°N is 3 DU/year in the winter months taking into account the dependence on the dynamics between the tropopause region and the mid-stratosphere. The highest correlation coefficient for the monthly mean total ozone anomalies is reached in November with 0.94.  相似文献   

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