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1.
Assuming spheroidal and spherical particle shapes for mineral dust aerosols, the effect of particle shape on dust aerosol optical depth retrievals, and subsequently on instantaneous shortwave direct radiative forcing (SWDRF) at the top of the atmosphere (TOA), is assessed based on Moderate Resolution Imaging Spectroradiometer (MODIS) data for a case study. Specifically, a simplified aerosol retrieval algorithm based on the principle of the Deep Blue aerosol retrieval method is employed to retrieve dust aerosol optical depths, and the Fu-Liou radiative transfer model is used to derive the instantaneous SWDRF of dust at the TOA for cloud-free conditions. Without considering the effect of particle shape on dust aerosol optical depth retrievals, the effect of particle shape on the scattering properties of dust aerosols (e.g., extinction efficiency, single scattering albedo and asymmetry factor) is negligible, which can lead to a relative difference of at most 5% for the SWDRF at the TOA. However, the effect of particle shape on the SWDRF cannot be neglected provided that the effect of particle shape on dust aerosol optical depth retrievals is also taken into account for SWDRF calculations. The corresponding results in an instantaneous case study show that the relative differences of the SWDRF at the TOA between spheroids and spheres depend critically on the scattering angles at which dust aerosol optical depths are retrieved, and can be up to 40% for low dust-loading conditions. 相似文献
2.
Soil dust aerosol is the largest contributor to aerosol mass concentrations in the troposphere and has considerable effects on air quality and climate. Arid and semi-arid areas of East Asia are one of the important dust source regions thus it is crucial to understand dust mobilization and accurately estimate dust emissions in East Asia. However, present dust models still contain large uncertainties with dust emissions that remain a significant contributor to the overall uncertainties in the model. In this study, we attempt to reduce these uncertainties by using an inverse modeling technique and obtain optimized dust emissions. We use Moderate Resolution Imaging Spectrometer (MODIS) aerosol optical depths (AODs) and groundbased mass concentrations of particles less than 10 μm in aerodynamic diameter (PM10) observations over East Asia in May 2007. The MODIS AODs are validated with AErosol RObotic NETwork (AERONET) AODs. The inversion uses the maximum a posteriori method and the GEOS-Chem chemical transport model (CTM) as a forward model. The model error is large over dust source regions including the Gobi Desert and Mongolia. We find that inverse modeling analyses from the MODIS and PM10 observations consistently result in decrease of dust emissions over Mongolia and the Gobi Desert. Whereas over the Taklamakan Desert and Manchuria, the inverse modeling analyses from both observations yield contrast results such as increase of dust sources using MODIS AODs, while decrease of those using PM10 observations. We discuss some limitations of both observations to obtain the optimized dust emissions and suggest several strategies for the improvement of dust emission estimates in the model. 相似文献
3.
河西走廊夏季强沙尘暴数值模拟试验 总被引：1，自引：0，他引：1
影响我国的沙尘暴灾害性天气多发生在春季,很少在夏季发生。文章利用我国科学家自主研发的GRAPES-DAM沙尘气溶胶模式对2005年7月一次罕见的影响河西走廊地区的群发性强沙尘暴进行了数值模拟,对夏季小概率强沙尘暴灾害天气的可预报性进行了个例研究。试验结果表明:模式对此次过程的地面大风、沙尘暴的范围、移动等均能做出较好的模拟;对于夏季群发性强沙尘暴过程,基于数值预报方法的沙尘气溶胶模式在天气模式预报准确的条件下,可以对这种小概率事件做出有应用意义的预报结果。 相似文献
4.
准确获取气溶胶光学厚度对于气候变化研究和大气环境监测具有重要意义。通过波长插值和时空匹配方法,利用气溶胶自动观测站网（AERONET）观测的气溶胶光学厚度（AOD）对风云3A/中分辨率光谱成像仪（FY-3A/MERSI）、Terra（Aqua）/MODIS的C5.1（Collections 5.1）和C6（Collections 6）气溶胶光学厚度产品在中国区域的反演精度进行验证分析。结合一次发生在中国境内的沙尘天气与一次严重雾霾天气个例,分析上述卫星气溶胶光学厚度的分布特征。研究结果表明,（1）FY-3A/MERSI AOD的反演精度较高（R=0.887,RMSE=0.234）,其值低于AERONET的观测值（Bias=-0.293）。（2）在不同的下垫面下,各种卫星暗像元算法AOD产品反演精度有差异,植被覆盖情况越好,反演精度越高,而植被很少的地区,即亮地表甚至没有反演值。（3）MODIS C5.1深蓝算法产品能在亮地表地区反演AOD,但效果不佳。MODIS C6中的深蓝算法产品在不同下垫面的反演精度都很高（RMSE为0.096-0.127）。（4）在不同季节的对比中,各种卫星AOD产品在夏季的反演精度最差,而反演最好的季节各有不同。（5）在一次沙尘天气污染与一次严重雾霾天气个例中,中国西部与北部区域,MODIS C6深蓝算法AOD的监测效果优于其他算法AOD;MERSI AOD产品在此区域的分布不连续。总体而言,MODIS C6 AOD分布比MODIS C5.1产品连续,MODIS 3 km产品在相同区域的AOD值高于其他产品。以上结论可为卫星AOD产品在中国区域的使用提供参考。 相似文献
5.
Reported in this article are the results of the analysis of extensive observations of aerosol optical, micro-physical characteristics, and precipitable water content (PWC) that have been carried out using compact, multi-band solar radiometers, over a semi-arid station, Agra (27°10′N, 78°05′E, 169 m AMSL) during winter 2004. The aerosol optical depth (AOD), Angstrom wavelength exponent (α), and PWC show, higher values on hazy- and foggy-days and lower values on clear-days. The turbidity coefficient (β) shows higher values for smaller values of α and vice versa. The aerosol size spectra exhibit bi-modal distribution with abundance of accumulation-mode particles during fog and haze occasions, and relatively coarse-mode particles on clear-days. The above features have been explained with co-located PWC and surface-level meteorological parameters. The NOAA HYSPLIT five-day back trajectories indicate the influence of trans-boundary pollution transport over the experimental station during the study period. 相似文献
6.
Aerosol optical depth(AOD) is the most basic parameter that describes the optical properties of atmospheric aerosols,and it can be used to indicate aerosol content. In this study, we assimilated AOD data from the Fengyun-3 A(FY-3 A) and MODIS meteorological satellite using the Gridpoint Statistical Interpolation three-dimensional variational data assimilation system. Experiments were conducted for a dust storm over East Asia in April 2011. Each 0600 UTC analysis initialized a24-h Weather Research and Forecasting with Chemistry model forecast. The results generally showed that the assimilation of satellite AOD observational data can significantly improve model aerosol mass prediction skills. The AOD distribution of the analysis field was closer to the observations of the satellite after assimilation of satellite AOD data. In addition, the analysis resulting from the experiment assimilating both FY-3 A/MERSI(Medium-resolution Spectral Imager) AOD data and MODIS AOD data had closer agreement with the ground-based values than the individual assimilation of the two datasets for the dust storm over East Asia. These results suggest that the Chinese FY-3 A satellite aerosol products can be effectively applied to numerical models and dust weather analysis. 相似文献
7.
It is nontrivial to extract the dust top height(DTH) accurately from passive instruments over land due to the complexity of the surface conditions. The Moderate Resolution Imaging Spectroradiometer(MODIS) deep blue(DB) algorithm can be used to infer the aerosol optical depth(AOD) over high-reflective surfaces. The Atmospheric Infrared Sounder(AIRS) can simultaneously obtain the DTH and optical depth information. This study focuses on the synergistic use of AIRS observations and MODIS DB results for improving the DTH by using a stable relationship between the AIRS infrared and MODIS DB AODs. A one-dimensional variational(1DVAR) algorithm is applied to extract the DTH from AIRS. Simulation experiments indicate that when the uncertainty of the dust optical depth decreases from 50% to 20%, the improvement of the DTH retrieval accuracy from AIRS reaches 200 m for most of the assumed dust conditions. For two cases over the Taklimakan Desert, the results are compared against Cloud-Aerosol Lidar with Orthogonal Polarization(CALIOP) measurements. The results confirm that the MODIS DB product could help extract the DTH over land from AIRS. 相似文献
8.
9.
沙尘暴影响下北京沙尘气溶胶的垂直分布及溯源分析 总被引：2，自引：0，他引：2
采用云-大气气溶胶激光雷达红外探索卫星观测系统(Cloud-Aerosol Lidarand Infrared Pathfinder Satellite Observations,CALIPSO)资料,得出了2013年3月8-11日的一次途经新疆、甘肃、内蒙古等地的沙尘暴,对造成北京的沙尘天气影响下的沙尘气溶胶的空间垂直分布图。在此基础上研究了衰减后向散射系数、退偏振比、色比等光学特性参数。结果表明:在此次沙尘暴影响下造成的北京地区沙尘天气过程中,气溶胶的退偏振比在0.1~0.4之间,色比大于0.3。3月10-11日北京地区的沙尘气溶胶分布高度从3km以下被抬升至约4km。再利用欧拉-拉格朗日混合单粒子轨道模型(Hybrid Single Particle Lagrangian Integrated Trajectory Model)和NAAPS全球气溶胶模式,模拟分析了这次沙尘的来源和传输过程,表明此次沙尘起源于南疆盆地和内蒙古中西部,影响甘肃大部、内蒙古中西部、宁夏、山西北部和河北西北部、北京等地区。并用双波长迭代反演法初步反演了3月10、11日北京地区处于沙尘天气情况下的气溶胶光学厚度,分别为0.334和0.621。 相似文献
10.
近年来华东地区大气气溶胶的时空特征 总被引：4，自引：1，他引：3
利用2000年2月—2008年12月的AERONET（AErosol RObotic NETwork）地基观测数据对MODIS/TERRA Collection 005气溶胶光学厚度（aerosol optical thickness;AOT）在华东区域的适用性进行了验证,并利用验证后的MODIS气溶胶产品对华东区域气溶胶光学厚度和尺度分布特征进行了分析。结果表明,（1）通过验证比较,MODIS的AOT在华东区域与AERONET站陆基观测到的AOT具有非常好的一致性,满足美国NASA的设计要求。（2）华东区域的气溶胶光学厚度存在明显的时空分布特征。时间上,在春季和夏季达到最大,而在秋季和冬季最小,表现出明显的季节变化规律。空间上,气溶胶光学厚度受地形影响明显。其高值区主要分布在平原地区,而低值区主要在海拔较高的山区。（3）该区域的气溶胶尺度分布也存在显著的变化特征。在冬、春由于沙尘输送的影响,整个华东区域气溶胶粒子的尺度都比较大,主要以自然生成的沙尘粒子为主。而在夏、秋季由于夏季风和降水的影响,气溶胶粒子的尺度都比较小,以工业排放的人为气溶胶粒子为主。 相似文献
11.
Due to increase in population and economic development, the mega-cities are facing increased haze events which are causing important effects on the regional environment and climate. In order to understand these effects, we require an in-depth knowledge of optical and physical properties of aerosols in intense haze conditions. In this paper an effort has been made to analyze the microphysical and optical properties of aerosols during intense haze event over mega-city of Lahore by using remote sensing data obtained from satellites (Terra/Aqua Moderate-resolution Imaging Spectroradiometer (MODIS) and Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO)) and ground based instrument (AErosol RObotic NETwork (AERONET)) during 6-14 October 2013. The instantaneous highest value of Aerosol Optical Depth (AOD) is observed to be 3.70 on 9 October 2013 followed by 3.12 on 8 October 2013. The primary cause of such high values is large scale crop residue burning and urban-industrial emissions in the study region. AERONET observations show daily mean AOD of 2.36 which is eight times higher than the observed values on normal day. The observed fine mode volume concentration is more than 1.5 times greater than the coarse mode volume concentration on the high aerosol burden day. We also find high values (~0.95) of Single Scattering Albedo (SSA) on 9 October 2013. Scatter-plot between AOD (500 nm) and Angstrom exponent (440-870 nm) reveals that biomass burning/urban-industrial aerosols are the dominant aerosol type on the heavy aerosol loading day over Lahore. MODIS fire activity image suggests that the areas in the southeast of Lahore across the border with India are dominated by biomass burning activities. A Hybrid Single-Particle Lagrangian Integrated Trajectory (HYSPLIT) model backward trajectory showed that the winds at 1000 m above the ground are responsible for transport from southeast region of biomass burning to Lahore. CALIPSO derived sub-types of aerosols with vertical profile taken on 10 October 2013 segregates the wide spread aerosol burden as smoke, polluted continental and dust aerosols. 相似文献
12.
该文提出了一种简单快速反演气溶胶光学厚度的方法,该算法对地表反照率的处理与MODIS V5.2算法相同,但气溶胶谱分布假定为Junge谱,设置了新的气溶胶参数。应用2006年9月6日—2008年6月10日太湖MODIS观测资料和2008年5月20日—2009年7月6日香河MODIS观测资料进行反演,并将反演结果与AERONET (AErosol RObotic NETwork) 站点资料进行对比,以检验算法的适用性和精度。对比结果显示:该算法在太湖的反演结果与AERONET太湖站反演结果对比的标准偏差为0.429,而MODIS卫星AOD产品与AERONET太湖站反演结果对比的标准偏差为0.693;相应在香河的两种反演结果与地面观测对比的标准偏差分别为0.493和0.542。该算法的反演误差小于MODIS现行算法,反演结果合理,具有较好的适用性,说明这种方法在这两个区域具有更高的反演精度。 相似文献
13.
The importance of specifying realistic lateral boundary conditions in the regional modeling of mineral aerosols has not been examined previously. This study examines the impact of assigning values for mineral aerosol (dust) concentrations at the lateral boundaries of Regional Climate Model version 3 (RegCM3) and its aerosol model over Southwest Asia. Currently, the dust emission module of RegCM3 operates over the interior of the domain, allowing dust to be transported to the boundaries, but neglecting any dust emitted at these points or from outside the domain. To account for possible dust occurring at, or entering from the boundaries, mixing ratios of dust concentrations from a larger domain RegCM3 simulation are specified at the boundaries of a smaller domain over Southwest Asia. The lateral boundary conditions are monthly averaged concentration values (μg of dust per kg of dry air) resolved in the vertical for all four dust bin sizes within RegCM3’s aerosol model. RegCM3 simulations with the aerosol/dust model including lateral boundary conditions for dust are performed for a five year period and compared to model simulations without prescribed dust concentrations at the boundaries. Results indicate that specifying boundary conditions has a significant impact on dust loading across the entire domain over Southwest Asia. More specifically, a nearly 30% increase in aerosol optical depth occurs during the summer months from specifying realistic dust boundary conditions, bringing model results closer to observations such as MISR. In addition, smaller dust particles at the boundaries have a more important impact than large particles in affecting the dust loading within the interior of this domain. Moreover, increases in aerosol optical depth and dust concentrations within the interior domain are not entirely caused by inflow from the boundaries; results indicate that an increase in the gradient of concentration at the boundaries causes an increase of diffusion from the boundaries. Lastly, experiments performed using a climatology of dust concentrations yield similar results to those using actual monthly values. Therefore, using a climatology of dust mixing ratios is sufficient in implementing lateral boundary conditions for mineral aerosols. In short, this work concludes that realistic specification of lateral boundary conditions for mineral aerosols can be important in modeling the dust loading over arid regional climates such as Southwest Asia. 相似文献
14.
20世纪80年代中国地区大气气溶胶光学厚度的平均状况分析 总被引：29，自引：3，他引：29
利用中国北京等 41个甲种日射站 1 979～ 1 990年太阳直接辐射日总量和日照时数等资料 ,配合同期 TOMS version - 7臭氧观测资料 ,反演了 41个站逐年、逐月 0 .75μm大气气溶胶的平均光学厚度值 (Aerosol Optical Depth,AOD) ,据此分析了 1 2 a来中国大气气溶胶的变化和时空平均分布特征。结果表明 :中国大气气溶胶光学厚度 AOD的多年平均分布是以四川盆地为中心向四周减少 ,南疆盆地和长江中游武汉附近为另两个大值中心 ;长江中下游大部分地区、山东半岛以及广东沿海等 ,AOD值亦较大 ;而东北大部、西北大部、云南和福建沿海等地 AOD较小。AOD各月平均分布有所不同。中国绝大部分地区春季 AOD值最大 ,最小值则各地不同。 1 979～ 1 990年 ,青藏高原、四川盆地西部、贵州北部、长江中下游大部分地区、山东半岛和南疆盆地西部等 ,AOD呈增长趋势。而东北地区、西北地区大部、云贵高原和广西西部以及华东沿海等地 AOD呈减小势态。中国地区 AOD的季节变化曲线大体可分为单峰、一峰一谷、两峰一谷和多峰等 4种类型 相似文献
15.
利用全球自动观测网（AERONET）纳木错观测点（90．962°E,30．773°N）2009年1～12月的地基观测数据,对青藏高原中部气溶胶光学厚度的分布进行了分析研究,并利用观测结果对MODIS气溶胶光学厚度（AOD）产品进行检验。结果表明,2009年1～12月期间,气溶胶光学厚度月平均值呈现双峰双谷状分布,3月的值最大。9月以后的波长指数a较小,这一时期气溶胶粒子的粒径较大。混浊系数卢的平均值为0．063,说明该地区的空气较为清洁。利用该地基观测资料对MODISAOD产品进行检验,结果表明两者的相关系数平方为0．14,没有通过95％的置信度检验,适用性不显著,需要进一步订正该地区的MODIS气溶胶光学厚度产品。 相似文献
16.
尝试以单星多角度卫星观测数据同时反演晴空陆地的气溶胶光学厚度和地表反射率,并选取2009年5月的MODIS(Moderate Resolution Imaging Spectroradiometer)1B资料进行了反演试验.结果表明:单星多角度法反演得到的气溶胶光学厚度结果与MODIS气溶胶产品(MOD04)平均值的相关系数为0.7914;反演的地表反射率结果与MODIS地表反射率产品(MOD09)也具有较好的一致性.对直接利用单星多角度观测数据反演获得一段时间内平均的气溶胶光学厚度进行了有益的尝试. 相似文献
17.
This study evaluates the spatial and temporal variation of the aerosol optical depth (AOD), the particle size characteristics (Ångström coefficients) and single scattering albedos during selected episodes over the Mediterranean area in 2006, based on independent observational datasets. We compare the satellite data of MODIS and MISR with those of the ground-based AERONET and in situ measurements. In general the yearly mean MODIS and MISR AODs as well as their temporal variation are in good agreement with AERONET. The highest AODs are caused by mineral dust outbreaks and the accumulation of anthropogenic aerosols during stagnant meteorological conditions. The comparison of MODIS with MISR aerosol optical properties for June corroborates that the AODs, Ångström coefficients and single scattering albedos agree well, and indicates the presence of high dust loads over the Mediterranean. Later in summer, however, MISR AOD is generally lower than MODIS, which is consistent with previous studies that show that MISR tends to underestimate and MODIS tends to overestimate AOD over land when compared to AERONET observations. Comparing MODIS Aqua Deep Blue with MISR for June over the Saharan desert reveals some differences in the location and the maxima of the AODs. Over the eastern Mediterranean highest dust loads occur during spring and autumn. Biomass burning activities around the Black Sea during July and August cause high AODs (e.g. by agricultural waste burning), and the particulate pollution is transported to the eastern Mediterranean and the Middle East by the prevailing northerly Etesian winds. 相似文献
18.
利用MODIS可见光通道气溶胶光学厚度的卫星遥感和523 nm波长微脉冲激光雷达 (MPL LIDAR) 对气溶胶消光系数垂直分布的观测，分析了珠江三角洲地区2003年6月一次气溶胶污染过程中气溶胶光学厚度的分布特征、气溶胶消光系数廓线的演变，认为这次污染过程是弱高压控制下的区域性污染，而香港地区污染物浓度的上升与区域性输送有直接关系，结果表明卫星和激光雷达的光学遥感方法提供了研究大气污染的可行手段。 相似文献
19.
Kuwait was exposed to a severe dust storm on 19 March 2003, the eve of operation ??Iraqi Freedom??. Three days of dust events (19, 26, 27 March) were analyzed for their aerosol optical and physical properties using ground-based and satellite-retrieved measurements. Ground-based measurements of aerosol optical depth (or thickness; AOD or AOT) at 675?nm, ?? 657, ?ngstrom coefficient ?? 936/657, particulate matter of diameter 10???m or less, PM10 (??g/m3), and meteorological parameters were analyzed for March 2003. AOT exceeded 3 for the 3?days of interest and PM10 concentrations reached as high value as 2,457???g/m3 on 19 March dust storm day. Retrieved aerosol characteristics from space using Moderate Resolution Imaging Spectrometer (MODIS) on board Terra and Aqua satellite were examined against ground-based measurements. A strong correlation was found between ground-based measurements of ?? 675 and the Terra-MODIS retrieved AOD550. The synoptic of the dust storm were analyzed and source regions were identified using back trajectory analysis and Total Ozone Mapping Spectrometer Aerosol Index. 相似文献
20.
研究了非洲地区大气气溶胶光学厚度（AOD）的时空变化及沙尘气溶胶越大西洋海区的传输。结果表明：1）源于撒哈拉沙漠的沙尘及其随赤道东风向西输送使得沙尘气溶胶成为非洲沙漠地区和紧邻的大西洋海区的主要气溶胶组分;AOD高值区和沙尘气溶胶光学厚度高值区在1—7月随赤道辐合带北移同步向北移动,而在8—12月则向南回撤。2）刚果盆地大气气溶胶主要为热带雨林和稀树草原排放的有机碳（OC）和黑碳（BC）气溶胶;其中与生物质燃烧源排放有关的OC、BC高值主要集中在干季（6—9月）的后半段（8—9月）;而生物源OC排放全年连续,其排放峰值出现于雨季开始时;生物质燃烧排放高值期与生物源排放高值期前后相继,形成干季（尤其是后半段）时期的OC、BC光学厚度高值。3）亚马逊河入海口地区主要气溶胶组分为海盐气溶胶,9—11月该区风力输送增强,风向由东南风转变为东风,海盐进入亚马逊河入海口处,形成AOD和海盐气溶胶光学厚度高值区。4）撒哈拉沙漠沙尘气溶胶向大西洋传输的偏北月份为7—9月、偏南月份为1—3月;2000—2016年海区沙尘气溶胶的传输路径存在向南移动的变化趋势,与同期亚速尔高压的增强和沙尘传输路径以北北风分量的增强以及赤道辐合带的移动一致。上述研究结果揭示了利用大气气溶胶时空变化特征反映区域大气环流和气候变化的可能性。 相似文献