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1.
The authors used a high-resolution regional climate model(RegCM3) coupled with a chemistry/aerosol module to simulate East Asian climate in 2006 and to test the climatic impacts of aerosols on regionalscale climate.The direct radiative forcing and climatic effects of aerosols(dust,sulfate,black carbon,and organic carbon) were discussed.The results indicated that aerosols generally produced negative radiative forcing at the top-of-the-atmosphere(TOA) over most areas of East Asia.The radiative forcing induced by aerosols exhibited significant seasonal and regional variations,with the strongest forcing occurring in summer.The aerosol feedbacks on surface air temperature and precipitation were clear.Surface cooling dominated features over the East Asian continental areas,which varied in the approximate range of-0.5 to-2°C with the maximum up to-3-C in summer over the deserts of West China.The aerosols induced complicated variations of precipitation.Except in summer,the rainfall generally varied in the range of-1 to 1 mm d-1 over most areas of China.  相似文献   

2.
There are many indicators that human activity may change climate conditions all around the globe through emissions of greenhouse gases. In addition, aerosol particles are emitted from various natural and anthropogenic sources. One important source of aerosols arises from biomass burning, particularly in low latitudes where shifting cultivation and land degradation lead to enhanced aerosol burden. In this study the counteracting effects of greenhouse gases and aerosols on African climate are compared using climate model experiments with fully interactive aerosols from different sources. The consideration of aerosol emissions induces a remarkable decrease in short-wave solar irradiation near the surface, especially in winter and autumn in tropical West Africa and the Congo Basin where biomass burning is mainly prevailing. This directly leads to a modification of the surface energy budget with reduced sensible heat fluxes. As a consequence, temperature decreases, compensating the strong warming signal due to enhanced trace gas concentrations. While precipitation in tropical Africa is less sensitive to the greenhouse warming, it tends to decrease, if the effect of aerosols from biomass burning is taken into account. This is partly due to the local impact of enhanced aerosol burden and partly to modifications of the large-scale monsoon circulation in the lower troposphere, usually lagging behind the season with maximum aerosol emissions. In the model equilibrium experiments, the greenhouse gas impact on temperature stands out from internal variability at various time scales from daily to decadaland the same holds for precipitation under the additional aerosol forcing. Greenhouse gases and aerosols exhibit an opposite effect on daily temperature extremes, resulting in an compensation of the individual responses under the combined forcing. In terms of precipitation, daily extreme events tend to be reduced under aerosol forcing, particularly over the tropical Atlantic and the Congo basin. These results suggest that the simulation of the multiple aerosol effects from anthropogenic sources represents an important factor in tropical climate change, hence, requiring more attention in climate modelling attempts.  相似文献   

3.
The coupled climate model EC-Earth2 is used to investigate the impact of direct radiative effects of aerosols on stationary waves in the northern hemisphere wintertime circulation. The direct effect of aerosols is simulated by introducing prescribed mixing ratios of different aerosol compounds representing pre-industrial and present-day conditions, no indirect effects are included. In the EC-Earth2 results, the surface temperature response is uncorrelated with the highly asymmetric aerosol radiative forcing pattern. Instead, the anomalous extratropical temperature field bears a strong resemblance to the aerosol-induced changes in the stationary-wave pattern. It is demonstrated that the main features of the wave pattern of EC-Earth2 can be replicated by a linear, baroclinic model forced with latent heat changes corresponding to the anomalous convective precipitation generated by EC-Earth2. The tropical latent heat release is an effective means of generating stationary wave trains that propagate into the extratropics. Hence, the results of the present study indicate that aerosol-induced convective precipitation anomalies govern the extratropical wave-field changes, and that the far-field temperature response dominates over local effects of aerosol radiative forcing.  相似文献   

4.
Climate forcing by carbonaceous and sulfate aerosols   总被引:3,自引:0,他引:3  
 An atmospheric general circulation model is coupled to an atmospheric chemistry model to calculate the radiative forcing by anthropogenic sulfate and carbonaceous aerosols. The latter aerosols result from biomass burning as well as fossil fuel burning. The black carbon associated with carbonaceous aerosols is absorbant and can decrease the amount of reflected radiation at the top-of-the-atmosphere. In contrast, sulfate aerosols are reflectant and the amount of reflected radiation depends nonlinearly on the relative humidity. We examine the importance of treating the range of optical properties associated with sulfate aerosol at high relative humidities and find that the direct forcing by anthropogenic sulfate aerosols can decrease from −0.81 W m-2 to −0.55 Wm-2 if grid box average relative humidity is not allowed to increase above 90%. The climate forcing associated with fossil fuel emissions of carbonaceous aerosols is calculated to range from +0.16 to +0.20 Wm-2, depending on how much organic carbon is associated with the black carbon from fossil fuel burning. The direct forcing of carbonaceous aerosols associated with biomass burning is calculated to range from −0.23 to −0.16 Wm-2. The pattern of forcing by carbonaceous aerosols depends on both the surface albedo and the presence of clouds. Multiple scattering associated with clouds and high surface albedos can change the forcing from negative to positive. Received: 29 September 1997 / Accepted: 10 June 1998  相似文献   

5.
Anthropogenic aerosols play an important role in the atmospheric energy balance. Anthropogenic aerosol optical depth (AOD) and its accompanying shortwave radiative forcing (RF) are usually simulated by nu- merical models. Recently, with the development of space-borne instruments and sophisticated retrieval algorithms, it has become possible to estimate aerosol radiative forcing based on satellite observations. In this study, we have estimated shortwave direct radiative forcing due to anthropogenic aerosols over oceans in all-sky conditions by combining clouds and the Single Scanner Footprint data of the Clouds and Earth’s Radiant Energy System (CERES/SSF) experiment, which provide measurements of upward shortwave fluxes at the top of atmosphere, with Moderate Resolution Imaging Spectroradiometer (MODIS) aerosol and cloud products. We found that globally averaged aerosol radiative forcing over oceans in the clear-sky conditions and all-sky conditions were -1.03±0.48 W m-2 and -0.34 ±0.16 W m-2, respectively. Direct radiative forcing by anthropogenic aerosols shows large regional and seasonal variations. In some regions and in particular seasons, the magnitude of direct forcing by anthropogenic aerosols can be comparable to the forcing of greenhouse gases. However, it shows that aerosols caused the cooling effect, rather than warming effect from global scale, which is different from greenhouse gases.  相似文献   

6.
The study investigated the effects of global direct radiative forcing due to carbonaceous aerosol on the climate in East Asia, using the CAM3 developed by NCAR. The results showed that carbonaceous aerosols cause negative forcing at the top of the atmosphere (TOA) and surface under clear sky conditions, but positive forcing at the TOA and weak negative forcing at the surface under all sky conditions. Hence, clouds could change the sign of the direct radiative forcing at the TOA, and weaken the forcing at the surface. Carbonaceous aerosols have distinct effects on the summer climate in East Asia. In southern China and India, it caused the surface temperature to increase, but the total cloud cover and precipitation to decrease. However, the opposite effects are caused for most of northern China and Bangladesh. Given the changes in temperature, vertical velocity, and surface streamflow caused by carbonaceous aerosol in this simulation, carbonaceous aerosol could also induce summer precipitation to decrease in southern China but increase in northern China.  相似文献   

7.
The air quality model system RAMS (Regional Atmospheric Modeling System)-CMAQ (Models-3 Community Multi-scale Air Quality) coupled with an aerosol optical/radiative module was applied to investigate the impact of different aerosol mixing states (i.e., externally mixed, half externally and half internally mixed, and internally mixed) on radiative forcing in East Asia. The simulation results show that the aerosol optical depth (AOD) generally increased when the aerosol mixing state changed from externally mixed to internally mixed, while the single scattering albedo (SSA) decreased. Therefore, the scattering and absorption properties of aerosols can be significantly affected by the change of aerosol mixing states. Comparison of simulated and observed SSAs at five AERONET (Aerosol Robotic Network) sites suggests that SSA could be better estimated by considering aerosol particles to be internally mixed. Model analysis indicates that the impact of aerosol mixing state upon aerosol direct radiative forcing (DRF) is complex. Generally, the cooling effect of aerosols over East Asia are enhanced in the northern part of East Asia (Northern China, Korean peninsula, and the surrounding area of Japan) and are reduced in the southern part of East Asia (Sichuan Basin and Southeast China) by internal mixing process, and the variation range can reach 5 W m-2. The analysis shows that the internal mixing between inorganic salt and dust is likely the main reason that the cooling effect strengthens. Conversely, the internal mixture of anthropogenic aerosols, including sulfate, nitrate, ammonium, black carbon, and organic carbon, could obviously weaken the cooling effect.  相似文献   

8.
通过比较EMAC模式模拟结果和卫星观测结果证实了模式的可信性,进而利用模拟结果分析研究了2010~2012年青藏高原上空气溶胶光学厚度及其直接辐射强迫的时空分布规律。结果表明:所有气溶胶组分中,沙尘、水溶性气溶胶和气溶胶中液态水是高原的主要消光物质,三者年平均消光占比分别为0.27、0.20和0.49。2011年夏季纳布罗火山爆发,高空气溶胶消光在海拔14 km以上显著增强。青藏高原气溶胶在大气顶和地表的直接辐射强迫分布总体上由北向南递减,沙尘气溶胶在高原北部边缘大气顶产生正辐射强迫,气溶胶大气层直接辐射强迫对大气有增温效应,主要出现在沙尘含量高的地区。此外,受纳布罗火山爆发的影响,平流层气溶胶在2011年秋、冬季产生了明显较强的负辐射强迫,相比于无火山爆发的2010年和 2012年,青藏高原上空平流层气溶胶负辐射强迫在2011年秋季和冬季分别增加了55.50%和52.38%。  相似文献   

9.
Effects of aerosol radiative forcing on the diurnal and seasonal cycles of precipitation over West Africa and eastern Atlantic Ocean are investigated for the boreal summer season: June–July–August. An eight year (2000–2007) average of GCM simulated rainfall data is compared with the corresponding TRMM rainfall data. The comparison shows that the amplitude of the diurnal cycles of rainfall over land and ocean are reasonably well simulated. Over land, the phase of the simulated diurnal cycle of precipitation peaks several hours earlier than that of the TRMM data. Corresponding differences over the ocean(s) are relatively smaller. Some of the key features of the aerosol induced model simulated field anomalies are: (a) aerosol direct radiative forcing which increases the atmospheric stability and reduces the daytime moist convection and convective precipitation; (b) the aerosol induced changes in the diurnal cycle of precipitation are out of phase with those of the TRMM data over land, but are in-phase over the ocean; (c) aerosols reduce the amplitude of the diurnal cycle of precipitation over land and enhance it over ocean. However, the phase of the diurnal cycle is not affected much by the aerosol radiative forcing both over land and ocean. During the boreal summer, aerosol radiative forcing and induced circulation and precipitation cool the Sahel and the southern part of Sahara desert more than the adjacent areas to the north and south, thereby shifting the peak meridional temperature gradient northward. Consequently, an anomalous easterly jet is found north of its climatological location. This anomalous jet is associated with increased cyclonic circulation to the south of its axis, resulting in an anomalous monsoon rain belt in the Sahel.  相似文献   

10.
We examine the simulated future change of the North Atlantic winter climate influenced by anthropogenic greenhouses gases and sulfate aerosol. Two simulations performed with the climate model ECHAM4/OPYC3 are investigated: a simulation forced by greenhouse gases and a simulation forced by greenhouse gases and sulfate aerosol. Only the direct aerosol effect on the clear-sky radiative fluxes is considered. The sulfate aerosol has a significant impact on temperature, radiative quantities, precipitation and atmospheric dynamics. Generally, we find a similar, but weaker future climate response if sulfate aerosol is considered additionally. Due to the induced negative top-of-the-atmosphere radiative forcing, the future warming is attenuated. We find no significant future trends in North Atlantic Oscillation (NAO) index in both simulations. However, the aerosol seems to have a balancing effect on the occurence of extreme NAO events. The simulated correlation patterns of the NAO index with temperature and precipitation, respectively, agree well with observations up to the present. The extent of the regions influenced by the NAO tends to be reduced under strong greenhouse gas forcing. If sulfate is included and the warming is smaller, this tendency is reversed. Also, the future decrease in baroclinicity is smaller due to the aerosols’ cooling effect and the poleward shift in track density is partly offset. Our findings imply that in simulations where aerosol cooling is neglected, the magnitude of the future warming over the North Atlantic region is overestimated, and correlation patterns differ from those based on the future simulation including aerosols.  相似文献   

11.
利用耦合化学过程的区域气候模式RegCM3,模拟研究3种主要人为排放气溶胶(硫酸盐、黑碳、有机碳)对东亚区域气候的影响.计算分析近20 a来3种气溶胶的时空分布、综合辐射强迫作用及其对地面气温和降水的影响.模拟结果表明:3种气溶胶冬夏季分布有所不同,冬季气溶胶大值区主要分布在南方地区,而夏季大值区北移;气溶胶短波辐射强迫在大气层顶和地面均为负值;气溶胶的加入对东亚地区地表气温有明显影响,冬季降温中心位于四川盆地,夏季降温大值区位于华北地区.气溶胶直接气候效应使得冬季东亚大部分地区降水减少,夏季东亚地区降水与中国南方地区夏季气溶胶浓度有较好的相关关系,中国东部雨带有南移趋势.  相似文献   

12.
 The atmospheric general circulation model ECHAM-4 is coupled to a chemistry model to calculate sulfate mass distribution and the radiative forcing due to sulfate aerosol particles. The model simulates the main components of the hydrological cycle and, hence, it allows an explicit treatment of cloud transformation processes and precipitation scavenging. Two experiments are performed, one with pre-industrial and one with present-day sulfur emissions. In the pre-industrial emission scenario SO2 is oxidized faster to sulfate and the in-cloud oxidation via the reaction with ozone is more important than in the present-day scenario. The atmospheric sulfate mass due to anthropogenic emissions is estimated as 0.38 Tg sulfur. The radiative forcing due to anthropogenic sulfate aerosols is calculated diagnostically. The backscattering of shortwave radiation (direct effect) as well as the impact of sulfate aerosols on the cloud albedo (indirect effect) is estimated. The model predicts a direct forcing of −0.35 W m-2 and an indirect forcing of −0.76 W m-2. Over the continents of the Northern Hemisphere the direct forcing amounts to −0.64 W m-2. The geographical distribution of the direct and indirect effect is very different. Whereas the direct forcing is strongest over highly polluted continental regions, the indirect forcing over sea exceeds that over land. It is shown that forcing estimates based on monthly averages rather than on instantaneous sulfate pattern overestimate the indirect effect but have little effect on the direct forcing. Received: 16 October 1996/Accepted: 24 October 1996  相似文献   

13.
本文应用WRF-Chem(Weather Research and Forecasting—Chemistry)模式研究中国东部地区气溶胶及其部分组分(硫酸盐、硝酸盐和黑碳气溶胶)在天气尺度下的辐射强迫和对地面气温的影响。5个无明显降水时间段(2006年8月23~25日、2008年11月10~12日、2008年12月16~18日、2009年1月15~17日和2009年4月27~29日)的模拟显示,气溶胶浓度呈现显著的白天低,夜间高的日变化特征,且北方区域(29.8°~42.6°N,110.2°~120.3°E)平均PM2.5近地面浓度(40~80 μg m-3)高于南方区域(22.3°~29.9°N,109.7°~120.2°E,30~47 μg m-3)。气溶胶对地面2 m温度(地面气温)有明显的降温效果,在早上08:00(北京时,下同)和下午17:00左右最为显著,最高可降低约0.2~1 K,同时气溶胶的参与改善了模式对地面气温的模拟。本文还通过对2006年8月23~25日一次个例的模拟,定量分析了气溶胶及其部分组分(硫酸盐、硝酸盐和黑碳气溶胶)的总天气效应(直接效应+间接效应)、直接效应和间接效应分别对到达地面的短波辐射和地面气温的影响。北方区域平均气溶胶直接效应所造成的短波辐射强迫要高于南方区域,分别为-11.3 W m-2和-5.8 W m-2,导致地面气温分别降低了0.074 K和0.039 K。南方区域平均气溶胶间接效应所产的短波辐射强迫高于北方区域,分别为-14.4 W m-2和-12.4 W m-2,引起的地面气温的改变分别为-0.094 K和-0.035 K。对于气溶胶组分,硫酸盐气溶胶的直接效应和间接效应的作用相当,其总效应在北方和南方区域平均短波辐射强迫分别为-7.0 W m-2和-10.5 W m-2,对地面气温的影响为-0.062 K和-0.074 K,而硝酸盐气溶胶的作用略小。黑碳气溶胶使得北方和南方区域平均到达地表的太阳短波辐射分别减少了6.5 W m-2和5.8 W m-2,而地表气温则分别增加了0.053 K和0.017 K,相比于间接效应,黑碳气溶胶的直接效应的影响更加显著。  相似文献   

14.
利用SBDART(Santa Barbara DISORT Atmospheric Radiative Transfer)辐射传输模式,结合AERONET(Aerosol Robotic Network)北京站观测的气溶胶光学特性数据,评估北京地区近十年气溶胶以及黑碳气溶胶的辐射强迫,主要研究结果如下:北京近十年气溶胶平均光学厚度(aerosol optical depth, AOD440nm)为0.61±0.56,?ngstr?m波长指数均值为1.09,单次散射反照率(single scattering albedo, SSA440nm)的均值为0.888±0.045;AOD呈现下降趋势,SSA呈上升趋势,表明该区域气溶胶污染有所改善。晴空条件下,大气层顶、地面和大气的气溶胶直接辐射强迫多年均值分别为?24.91±19.80 W m?2、?65.52±43.78 W m?2、40.61±28.62 W m?2,即气溶胶对大气层顶和地表为冷却效应,对大气产生加热作用。气溶胶和黑碳气溶胶的直接辐射强迫绝对值的年际变化表现为微弱的下降趋势,季节变化特征为春夏季高,冬季低,这与AOD的变化规律一致。并且黑碳气溶胶的直接辐射强迫下降趋势与SSA的上升趋势呈现较好的反位相关系。  相似文献   

15.
In this study, we examine the mass distributions, direct and semi-direct effects of different biomass burning aerosols (BBAs) over South Africa using the 12-year runs of the Regional Climate Model (RegCM4). The results were analyzed and presented for the main BB season (July–October). The results show that Mpumalanga, KwaZulu Natal and the eastern parts of Limpopo are the main local source areas of BBAs in South Africa. In comparison to carbonaceous aerosols, BB-induced sulfate aerosol mass loading and climatic effects were found to be negligible. All carbonaceous aerosols reduce solar radiation at the surface by enhancing local atmospheric radiative heating. The climatic feedback caused by BBAs, resulted in changes in background aerosol concentrations. Thus, on a regional scale, climatic effects of BBAs were also found in areas far away from the BBA loading zones. The feedback mechanisms of the climate system to the aerosol radiative effects resulted in both positive and negative changes to the low-level columnar averaged net atmospheric radiative heating rate (NAHR). Areas that experienced an NAHR reduction showed an increase in cloud cover (CC). During the NAHR enhancement, CC over arid areas decreased; whereas CC over the wet/semi-wet regions increased. The changes in surface temperature (ST) and surface sensible heat flux are more closely correlated with BBA semi-direct effects induced CC alteration than their direct radiative forcing. Furthermore, decreases (or increases) in ST, respectively, lead to the reductions (and enhancements) in boundary layer height and the vice versa on surface pressure. The direct and semi-direct effects of BBAs also jointly promoted a reduction and rise in surface wind speed that was spatially highly variable. Overall, the results suggest that the CC change induced by the presence of radiatively interactive BBAs is important to determine alterations in other climatic variables.  相似文献   

16.
Previous observational studies have estimated anthropogenic aerosol direct radiative forcing over oceans without due consideration of cloudy-sky aerosols.However,when interaction between clouds and aerosols located below or above the cloud level is taken into account,the aerosol direct radiative forcing is larger by as much as 5 W m-2 in most mid-latitude regions in the Northern Hemisphere.  相似文献   

17.
Why Is the Climate Forcing of Sulfate Aerosols So Uncertain?   总被引:2,自引:0,他引:2  
l. IntroductionAlthough the aerosol has been recognized as an important factor which has innuence onthe past, present and future climate for a long time, it still has much uncertainty in assessingits climate forcing. The direct radiative forcing of sulfate aerosols has been estimated rangingfrom --0.3 W/ m2 to --0.9 W/ m2 in recent publications (Charlson et al., l992, Kiehl andBriegleb l993; Taylor and Penner 1994, Boucher and Anderson l995, Kieh1 and Rodhe l995;Chuang et al., l997, Penne…  相似文献   

18.
The National Center for Atmospheric Research Community Atmosphere Model (version 3.5) coupled with the Morrison?CGettelman two-moment cloud microphysics scheme is employed to simulate the aerosol effects on clouds and precipitation in two numerical experiments, one representing present-day conditions (year?2000) and the other the pre-industrial conditions (year?1750) over East Asia by considering both direct and indirect aerosol effects. To isolate the aerosol effects, we used the same set of boundary conditions and only altered the aerosol emissions in both experiments. The simulated results show that the cloud microphysical properties are markedly affected by the increase in aerosols, especially for the column cloud droplet number concentration (DNC), liquid water path (LWP), and the cloud droplet effective radius (DER). With increased aerosols, DNC and LWP have been increased by 137% and 28%, respectively, while DER is reduced by 20%. Precipitation rates in East Asia and East China are reduced by 5.8% and 13%, respectively, by both the aerosol??s second indirect effect and the radiative forcing that enhanced atmospheric stability associated with the aerosol direct and first indirect effects. The significant reduction in summer precipitation in East Asia is also consistent with the weakening of the East Asian summer monsoon, resulting from the decreasing thermodynamic contrast between the Asian landmass and the surrounding oceans induced by the aerosol??s radiative effects. The increase in aerosols reduces the surface net shortwave radiative flux over the East Asia landmass, which leads to the reduction of the land surface temperature. With minimal changes in the sea surface temperature, hence, the weakening of the East Asian summer monsoon further enhances the reduction of summer precipitation over East Asia.  相似文献   

19.
温室气体和硫酸盐气溶胶的辐射强迫作用   总被引:9,自引:4,他引:5  
对GOALS4 .0海 陆 气耦合模式的相关部分进行了改进 ,主要改进包括温室气体的扩充和硫酸盐气溶胶“显式”方案的引入 ,并引入 2 0世纪温室气体的实际浓度变化以及硫循环模式模拟的硫酸盐气溶胶的三维全球浓度分布 ,模拟了温室气体和硫酸盐气溶胶造成的辐射强迫的空间分布和时间变化。全球平均的温室气体和硫酸盐气溶胶的辐射强迫分别为 2 .17W /m2 和 - 0 .2 9W /m2 ;温室气体造成的辐射强迫在空间上呈现明显的纬向结构 ,最大值 (大于 2 .5W/m2 )和最小值 (小于 1W /m2 )分别位于副热带和两极地区 ,在北半球主要工业区硫酸盐气溶胶的辐射强迫绝对值接近温室气体的辐射强迫值 (大于 - 2 .0W /m2 )。  相似文献   

20.
平流层气溶胶的辐射强迫及其气候响应的水平二维分析   总被引:7,自引:0,他引:7  
利用比较先进的辐射模式计算了平流层气溶胶的辐射强迫,并对之进行了参数化。结果发现平流层气溶胶的辐射强迫的水平分布不仅与其本身的水平变化有关,而且与下垫面的反照率有很大的关系。利用近期开发的二维能量平衡模式模拟了皮纳图博火山气溶胶对地面平衡温度的影响,结果表明:皮纳图博火山至喷发后1年半左右降温达最大,至喷发后第5年降温已很小。  相似文献   

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