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1.
Mani  A.  Sreedharan  C. R. 《Pure and Applied Geophysics》1973,106(1):1180-1191
The latitudinal and temporal variations in the vertical profiles of ozone over the Indian subcontinent are discussed. In the equatorial atmosphere represented by Trivandrum (8°N) and Poona (18°N), while tropospheric ozone shows marked seasonal variations, the basic pattern of the vertical distribution of ozone in the stratosphere remains practically unchanged throughout the year, with a maximum at about 28 to 26 km and a minimum just below the tropopause. The maximum total ozone occurs over Trivandrum in the summer monsoon season and the latitudinal anomaly observed over the Indian monsoon area at this time is explained as arising from the horizontal transport of ozone-rich stratospheric air from over the thermal equator to the southern regions.In the higher latitudes represented by New Delhi (28°N), the maximum occurs at 23 km. Delhi, which lies in the temperate regime in winter, shows marked day-to-day variations in association with western disturbances and the strong westerly jet stream that lies over north and central India at this time.Although the basic pattern of the vertical distribution of ozone in the equatorial atmosphere is generally the same in all seasons, significant though small changes occur in the lower stratosphere and in the troposphere. There are small perturbations in the ozone and temperature structures, distinct ozone maxima being always associated with temperature inversions. There are also large perturbances not related to temperature, ozone-depleted regions normally reflecting a stratification of either destructive processes or materials such as dust layers or clouds at these levels. Particularly interesting are the upper tropospheric levels just below the tropopause where the ozone concentration is consistently the smallest, in all seasons and at all places where soundings have been made in India.  相似文献   

2.
Summary Calculations of the covariance between ozone amounts and meridional wind in the lower stratosphere are presented for all stations in the northern hemisphere for the IGY-IGC. Northward ozone transport occurs by large-scale quasi-horizontal transient and standing eddies and the transport is a maximum early in the year. It is suggested that the transport is governed by the exchange of energy between the troposphere and stratosphere and data are presented on the energy transformations within the lower stratosphere and the transfer of energy into the region which support this suggestion. The vertical flux of energy is also calculated from tropospheric data and its seasonal changes are seen to be in the correct phase to explain the spring maximum in ozone amount.The research reported in this article was sponsored by the Atomic Energy Commission under Contract AT (30-1)2241.  相似文献   

3.
Aboard commercial airliners twenty registrations of the ozone concentration of the upper troposphere were carried out within a period of 14 months between Europe and South Africa. Nearly each of these meridional ozone profiles shows an approximately constant ozone content between 25°S and 25°N with a pronounced seasonal variation. Most of these profiles show two marked peaks of the ozone concentration at about 30°N and between 40° and 45°N. Though the number of these registrations is not sufficient for statistical computations, the first results confirm the meridional ozone distribution, which was expected from studies with ozone-radiosonde soundings. Moreover a strong asymmetry of the northern and southern hemisphere is confirmed by these ozone measurements.  相似文献   

4.
Mani  A.  Sreedharan  C. R.  Joseph  P. V.  Sinha  S. S. 《Pure and Applied Geophysics》1973,106(1):1192-1199
A series of ozone soundings were made at New Delhi (77°E 28°N) from 21 to 30 January 1969 and 10 to 22 February 1972 to study the changes in the vertical distribution of atmospheric ozone associated with western disturbances. The sonde used was the Indian ozonesonde made in the Instruments Laboratories at Poona.In February 1972, two western disturbances moved eastwards in quick succession across the western Himalayas, the first between the 11th and 13th and the second between the 13th and 15th. Associated with the first tropospheric trough was a high-speed jet stream with wind speeds reaching 180 knots, when the tropopause descended to 304 mb over Delhi. The second trough had no high-speed jet associated with it and the tropopause was at 227 mb. Ozone maxima were observed at 350, 180 and 125 mb in addition to the main peak at 35 mb in association with the upper tropospheric troughs over Delhi and its neighbourhood. A similar lowering of the tropopause and the influx of ozone in shallow layers was observed during the passage of two upper air troughs in January 1969. The study shows that with the approach of upper tropospheric troughs and the simultaneous lowering of the tropopause there is an increased influx in shallow layers of middle latitude ozone-rich air through breaks in the tropopause, replacing the subropical ozone-poor air over the station.  相似文献   

5.
Using a modified Brewer bubbler ozone sensor, continuous measurements of the ozone concentration near the ground were made at Poona (18°N, 73°E) for one year 1969–1970. The surface ozone concentration shows a pronounced seasonal variation, with a minimum during the monsoon months and a maximum during the pre-monsoon summer months. There is also a marked diurnal variation in surface ozone concentration which clearly follows the diurnal variation of temperature and is again a maximum during the summer months and a minimum during the monsoon. A secondary maximum in ozone concentration occurs in the forenoon during the winter months, associated with the temperature inversions that occur near the ground in this season.Both ozone and radioactive tracers, such as Cs-137 both in air and in precipitation show variations indicating that they have identical source regions and sinks. The latitudinal anomaly of surface ozone and Cs-137 observed in the low latitudes over India is explained as arising from the reduction in the rate of transfer of these tracers from the stratosphere to the troposphere, as a result of the reversed circulation at the upper levels in this season.From continuous measurements of surface ozone made with three electrochemical sensors exposed at three levels, 0, 15 and 35 m above the ground, the ozone flux has been directly calculated for the first time in the tropics. The ozone flux was calculated using both the rate of decay method used by Kroening and Ney and Regener's profile method. The profile method gives values of the order of 1.71 to 7.04×1011 mol/cm2/sec and that obtained by the rate of decay method is found to be 4.2 to 5.6×1011 mol/cm2/sec and are in good agreement with the flux values reported by other investigators.  相似文献   

6.
Temperature structures in the height range of 0–30 km over Pan Chiao (25°N, 121°E) in northern Taiwan were studied for the period 1990–1995 using radiosonde data. The purpose of this study is to see the annual variation of tropopause temperature and height and also to study local temperature perturbations caused by the series of volcanic eruptions at Mount Pinatubo in June 1991. While the annual variation in the tropopause height and temperature is clearly observed, we found a large increase in the temperature at the tropopause and in the lower stratospheric region during the year 1992. The tropopause is warm during the year 1992 and temperature increase at the tropopause is nearly 6°C in January 1992. The annual average temperature at the lower stratosphere during 1992 shows an increase of 2°C from the normal trend. The effects of Pinatubo are in general different in the troposphere and stratosphere.  相似文献   

7.
副热带急流对中国南部地区对流层中上层臭氧浓度的影响程度及地理范围目前还研究较少,且缺乏综合使用常规气象资料及卫星资料来判识对流层中上层臭氧浓度增高的方法.本文利用NCEP再分析与最终分析资料、日本GMS-5地球静止卫星水汽云图资料,以2001年3月27~29日中国南部的临安、昆明、香港臭氧探测个例为基础,结合1996年3月29日香港与2001年4月13日临安对流层中上层高浓度臭氧分布个例对副热带急流对中国南部对流层中上层臭氧浓度的影响进行了详细分析,提出根据气象要素场判识春季中国南部对流层中上层臭氧浓度增高的充分条件为根据卫星水汽图像上的暗区、高空急流入口区的左侧辐合区、高空锋区、对流层中上层≥1 PVU的向下伸展的舌状高位涡区来综合判断.本文的分析结果表明,本文个例中对流层中上层高浓度臭氧来自平流层;香港对流层中上层低浓度臭氧来自热带海洋地区.不仅臭氧垂直廓线的多个极小与极大值表明臭氧垂直分布的多尺度变化特征,而且对流层中上层PV分布以及卫星水汽图像分析也表明大气中的多尺度运动对臭氧垂直分布特征有显著影响.本文的结果表明与副热带高空急流相联系的平流层空气侵入不仅发生在中国大陆的较高纬度地区,较低纬度的昆明与香港地区也有平流层空气侵入导致对流层中上层臭氧浓度升高.  相似文献   

8.
A study is presented of a possible correlation between ozone and Aitken nuclei concentration measured between 6 km and 19 km by the instruments installed on the WB-57F aircraft. Samples were taken between 48°N and 9°S latitudes over the U.S., the Gulf of Mexico, and Central and South America between March 1974 and February 1975.A weak negative correlation between AN and ozone concentrations was found at altitudes higher than the tropical tropopause. Scattering of the signs and magnitudes of correlation coefficients was found below the tropopause. Largest variations of the coefficient values were related to the stratospheric pollution following the eruption of the Guatemalan volcano Fuego.  相似文献   

9.
Total ozone anomalies (deviation from the long-term mean) are created by anomalous circulation patterns. The dynamically produced ozone anomalies can be estimated from known circulation parameters in the layer between the tropopause and the middle stratosphere by means of statistics. Satellite observations of ozone anomalies can be compared with those expected from dynamics. Residual negative anomalies may be due to chemical ozone destruction. The statistics are derived from a 14 year data set of TOMS (Total Ozone Mapping Spectrometer January 1979-Dec. 1992) and corresponding 300 hPa geopotential (for the tropopause height) together with 30 hPa temperature (for stratospheric waves) at 60°N. The correlation coefficient for the linear multiple regression between total ozone (dependent variable) and the dynamical parameters (independent variables) is 0.88 for the zonal deviations in the winter of the Northern Hemisphere. Zonal means are also significantly dependent on circulation parameters, besides showing the known negative trend function of total ozone observed by TOMS. The significant linear trend for 60°N is 3 DU/year in the winter months taking into account the dependence on the dynamics between the tropopause region and the mid-stratosphere. The highest correlation coefficient for the monthly mean total ozone anomalies is reached in November with 0.94.  相似文献   

10.
Summary The average change in height of several constant pressure levels in the troposphere and lower stratosphere after a strong solar flare is described. The analysis covers the northern hemisphere north of 10°N and is based on a sample of 81 carefully selected flares from the period July 1957 through December 1959.The statistical significance of the results is tested by drawing a comparison with the results obtained when one applies exactly the same analysis to three samples of 81 random key-dates selected from the same period.Properties of the reaction pattern are (1) it is pronounced at high as well as low latitudes, (2) it consists of alternating cells of positive and negative height change, (3) it is established within six hours after the flare, and (4) the maximum response occurs near the tropopause.It appears more likely that the atmospheric reaction pattern can be attributed to very energetic solar particles rather than to enhanced ultraviolet radiation.  相似文献   

11.
Fabian  P. 《Pure and Applied Geophysics》1973,106(1):1044-1057
Summary Based on the global distribution of various surface types the mean tropospheric residence time of ozone is estimated as a function of latitude. Due to the land-sea distribution varies from 50 days in the northern hemisphere to 190 days in the southern hemisphere. For the stratospheric-tropospheric exchange a sinusoidal variation with season is assumed. The annual variation of tropospheric ozone thus gets a sine function from mean, amplitude and phase of whch the injection function for the particular latitude can be determined.  相似文献   

12.
利用1979~1992年卫星TOR对流层臭氧数据库资料,以及同期太阳辐照度数据序列,考察青藏高原对流层臭氧含量变化与太阳辐射周期变化之间的关系.分析表明,青藏高原对流层臭氧分布表现出与太阳辐照度相同的变化趋势,存在着明显的太阳周期变化特征.逐月线性回归分析表明,太阳辐照度增加导致青藏高原对流层臭氧增加的正效应.在太阳周期内,太阳辐射增加可使青藏高原对流层臭氧、平流层臭氧和臭氧总量分别增加1.31、4.97、6.628DU,或4.07%、2.04%、2.28%.该特征与赤道太平洋地区完全相反,分析产生差异的原因,至少应包括两方面因素:一是背景大气NOX和水汽含量的差异;二是青藏高原频繁发生的平流层-对流层大气物质交换和输送.  相似文献   

13.
Examined are temperature and ozone variations in the Northern Hemisphere stratosphere during the period 1958–77, as estimated from radiosondes rocketsondes, ozonesondes, and Umkehr measurements. The temperature variation in the low tropical stratosphere is a combination of the variation associated with the quasi-biennial oscillation, and a variation nearly out of phase with the pronounced 3-yearly temperature oscillation (Southern Oscillation) present in the tropical troposphere since 1963. Based on radiosonde and rocketsonde data, the quasibiennial temperature oscillation can be traced as high as the stratopause, the phase varying with both height and latitude. However, the rocketsonde-derived temperature decrease of several degrees Celsius in the 25–55 km layer of the Western Hemisphere between 1969 (sunspot maximum) and 1976 (sunspot minimum) is not apparent in high-level radiosonde data, so that caution is advised with respect to a possible solar-terrestrial relation.There has been a strong quasi-biennial oscillation in ozone in the 8–16 km layer of the north polar region, with ozone minimum near the time of quasi-biennial west wind maximum at a height of 20 km in the tropics. A quasi-biennial oscillation in ozone (of similar phase) is also apparent from both ozonesonde data and Umkehr measurements in 8–16 and 16–24 km layers of north temperate latitudes, but not higher up. Both measurement techniques also suggest a slight overall ozone decrease in the same layers between 1969 and 1976, but no overall ozone change in the 24–32 km layer. Umkehr measurements indicate a significant 6–8% increase in ozone amount in all stratospheric layers between 1964 and 1970, and in 1977 the ozone amount in the 32–46 km layer was still 4% above average despite the predicted depletion due to fluorocarbon emissions. The decrease in ozone in the 32–46 km, layer of mid latitudes following the volcanic eruptions of Agung and Fuego is believed to be mostly fictitious and due to the bias introduced into the Umkehr technique by stratospheric aerosols of volcanic origin. Above-average water vapor amounts in the low stratosphere at Washington, DC, appear closely related to warm tropospheric temperatures in the tropics, presumably reflecting variations in strength of the Hadley circulation.  相似文献   

14.
The spatial and temporal distribution of total ozone over India and its vertical distribution in theatmosphere during 1964–1969 was studied using Dobson spectrophotometer data at a network of six stations in India, Srinagar (34°N), New Delhi (28°N), Varanasi (24°N), Ahmedabad (23°N), Dum Dum (22°N), and Kodaikanal (10°N). The annual and seasonal variations show a clear phase-shift in the occurrence of the ozone maxima and minima as one proceeds from higher to lower latitudes in the tropics. In the northern stations (north of 25°N) the increase in total ozone during the course of the annual variation is caused by the fractional increase in all layers from the ground to 28 km, the main contribution coming from 10–24 km. Above 28 km the concentration changes roughly in accordance with photochemical production.In lower latitudes (south of 25°N) an increase in total ozone amount during the annual cycle is caused by a gradual increase in all the layers from the ground to 36 km above which the variation is negligible.  相似文献   

15.
Spänkuch  D.  Döhler  W.  Kubasch  H. 《Pure and Applied Geophysics》1973,106(1):1208-1218
Summary The correlation matrix for the vertical ozone distribution and the temperature-ozone cross-correlation matrix, which was calculated from ozone soundings made over Berlin between 1967 and 1970, the statistical structure of the vertical ozone profile (correlation coefficients, average profiles, average standard deviation, relative variability) was derived for the three ozone seasons. The partial ozone pressure does not at all heights follow a normal distribution (e. g. at tropopause level). Generally, the correlation between tropospheric and stratospheric ozone is rather poor. In some layers the highest correlation coefficients, i.e. –0.3 and +0.4, occur in autumn (October to December) and in winter and spring (January to April). The correlation between the ozone amounts of various stratospheric layers is distinct in autumn, less distinct in summer (May to September) and entirely missing from January to April. Conspicuous cross-correlations between temperature and ozone have been found for all three seasons. a) With a negative correlation between tropospheric temperature and middle tropospheric to middle stratospheric ozone (maximum up to –0.8); b) with a rather strong positive correlation between the ozone amount and the temperature in the lower stratosphere (maximum up to +0.84); c) with a positive correlation between the ozone amount of the middle stratosphere and the temperature of the middle stratosphere (maximum up to +0.8). The highest correlation coefficients occur in autumn.  相似文献   

16.
Calculating the global mass exchange between stratosphere and troposphere   总被引:1,自引:0,他引:1  
Large-scale cross-tropopause mass fluxes are diagnosed globally from 1979 to 1989 for Northern Hemisphere winter conditions (December, January, and February). Results of different methods of approaches with regard to the definition of the tropopause and the way to calculate the mass fluxes are compared and discussed. The general pattern of the mass exchange from the tropopause into the stratosphere and vice versa agrees fairly well when using different methods, but the absolute values can differ up to 100%.An inspection of the temporal development of the mass fluxes for solstice conditions indicates a complex picture. Whereas a permanent significant downward flux from the stratosphere into the troposphere is detected for latitude regions nearly between 25°N and 40°N and between 30°S and 50°S (initiated by the poleward branches of the Hadley cells), a non-uniform behaviour is observed at higher latitude bands. Periods of strong mass exchange from the troposphere into the stratosphere are disrupted by periods of an opposite mass exchange. A comparison of the stratoshere-troposphere (ST) exchange with the exchange at higher altitudes through surfaces, quasi-parallel to the tropopause, excludes a general connection. Only a few strong upward directed ST mass exchange events have counterparts at higher altitudes. The composition of the stratosphere may be influenced directly by the ST exchange only in a thin layer above the tropopause.  相似文献   

17.
An observation by UHF ST radar of a subsidence pattern on the right side of the exit region of a jet streak is reported. The onset of the subsidence pattern occurred at 23:30 UTC on the 29 November 1991, when a downward motion was initiated above 14 km. The injections of stratospheric air in this region seem to have an intermittent nature; they occur during at least three intervals during the lifetime of the subsidence pattern. Comparison of these results with an ECMWF analysis suggests that it is an unfolding case. However, observation of turbulent intensities w’ greater than 60 cm s−1 at the tropopause level also suggests the existence of a turbulent flux between the stratosphere and the troposphere. From the turbulence characteristics measured by the radar and the potential temperature profile obtained by radiosonde data, the eddy diffusivity at the tropopause level has been calculated. An eddy diffusion coefficient ranging between 5 and 7 m2 s−1 is found. From these values, and with the assumption of a climatological gradient of the volume mixing ratio of ozone in the lower stratosphere, it is possible to deduce a rough estimate of the amount of ozone injected from the stratosphere into the troposphere during this event. A rate of transfer of 1.5×1020 molecules of ozone per day and per square meter is found.  相似文献   

18.
The availability of global gridded precipitation and outgoing long-wave radiation (OLR) data after 1978 makes possible an investigation of the influence of the decadal solar oscillation in the tropics during three solar maxima and two solar minima. The NCEP/NCAR reanalyses starting in the 1950s allows the inclusion of an additional two solar maxima and minima to look for consistency of response across a longer time period. In the northern summer (July–August), the major climatological tropical precipitation maxima are intensified in solar maxima compared to solar minima during the period 1979–2002. The regions of this enhanced climatological precipitation extend from the Indian monsoon to the West Pacific oceanic warm pool and farther eastwards in the Intertropical Convergence Zone of the North Pacific and North American Monsoon, to the tropical Atlantic and greater rainfall over the Sahel and central Africa. The differences between solar maxima and minima in the zonal mean temperature through the depth of the troposphere, OLR, tropospheric vertical motion, and tropopause temperature are consistent with the differences in the rainfall. The upward vertical motion is stronger in regions of enhanced tropical precipitation, tropospheric temperatures are higher, tropopause temperatures are lower, and the OLR is reduced due to higher, colder cloud tops over the areas of deeper convective rainfall in the solar maxima than in the minima. These differences between the extremes of the solar cycle suggest that an increase in solar forcing intensifies the Hadley and Walker circulations, with greater solar forcing resulting in strengthened regional climatological tropical precipitation regimes. These effects are as strong or even more pronounced when warm and cold extremes in the Southern Oscillation are removed from the analyses. Additionally, lower stratospheric temperatures and geopotential heights are higher with greater solar forcing suggesting ozone interactions with solar forcing in the upper stratosphere.  相似文献   

19.
Bischof  W.  Fabian  P. 《Pure and Applied Geophysics》1973,106(1):1041-1043
Ozone measurements aboard commercial airliners over Scandinavia and on transpolar flights were analyzed for tropospheric ozone concentration. The results confirm a region of enhanced stratospheric-tropospheric exchange around 60° latitude which was expected from Sr-90 fallout measurements.  相似文献   

20.
Regular measurements of the atmospheric ozone in the Brazilian sector were started at Cachoeira Paulista (22.7°S, 45.0°W), and Natal (5.8°S, 35.2°W) in May 1974 and November 1978, respectively. The results of the total ozone measurements carried out at these two stations up to 1981 are presented in this communication and compared with other low-and mid-latitude stations. Although Natal is an equatorial station, it presents a prominent annual variation, and the average total ozone content is high compared to satellite measurements. During 1977–78, abnormally low values of total ozone were observed at Cachoeira Paulista. Some preliminary results about the QBO 9quasi-biennial oscillation) during 1974–81 are also presented.  相似文献   

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