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南极大气臭氧和温度垂直结构及其季节变化的研究 总被引：1，自引：0，他引：1
利用南极中山站2008年2月至2009年2月臭氧和温度探空等资料,对中山站上空大气臭氧和温度的垂直结构及季节变化特征进行了研究.结果表明,在中山站上空热对流层顶和臭氧对流层顶的高度相近,年平均高度分别为7.9和7.4km.对流层顶的气压和温度都存在位相相反一波型季节变化.春季和冬季对流层顶的温度转折没有夏季和秋季明显,而依据臭氧变化恰能更好地确定对流层顶高度.在对流层臭氧垂直分布的季节变化不显著;而平流层却十分明显.春季下平流层臭氧严重耗损,14km处的臭氧最小分压仅为1.57MPa,最大分压出现在上平流层,其他季节下平流层臭氧随高度增加而升高.春季下平流层臭氧的严重损耗,与极夜过后低温条件和平流层冰晶云表面消耗臭氧的光化学过程有密切关系.大气臭氧和温度的垂直结构及季节变化特征,对春季南极臭氧洞的形成和发展具有重要意义. 相似文献
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副热带急流对中国南部地区对流层中上层臭氧浓度的影响程度及地理范围目前还研究较少,且缺乏综合使用常规气象资料及卫星资料来判识对流层中上层臭氧浓度增高的方法.本文利用NCEP再分析与最终分析资料、日本GMS-5地球静止卫星水汽云图资料,以2001年3月27~29日中国南部的临安、昆明、香港臭氧探测个例为基础,结合1996年3月29日香港与2001年4月13日临安对流层中上层高浓度臭氧分布个例对副热带急流对中国南部对流层中上层臭氧浓度的影响进行了详细分析,提出根据气象要素场判识春季中国南部对流层中上层臭氧浓度增高的充分条件为根据卫星水汽图像上的暗区、高空急流入口区的左侧辐合区、高空锋区、对流层中上层≥1 PVU的向下伸展的舌状高位涡区来综合判断.本文的分析结果表明,本文个例中对流层中上层高浓度臭氧来自平流层;香港对流层中上层低浓度臭氧来自热带海洋地区.不仅臭氧垂直廓线的多个极小与极大值表明臭氧垂直分布的多尺度变化特征,而且对流层中上层PV分布以及卫星水汽图像分析也表明大气中的多尺度运动对臭氧垂直分布特征有显著影响.本文的结果表明与副热带高空急流相联系的平流层空气侵入不仅发生在中国大陆的较高纬度地区,较低纬度的昆明与香港地区也有平流层空气侵入导致对流层中上层臭氧浓度升高. 相似文献
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利用1958~2001年共44年的ECMWF资料及参数化方法,计算了对流层顶上、下3 km气层间的臭氧含量及其吸收太阳辐射加热率的时空分布.结果表明: (1) 臭氧分布的空间梯度从赤道指向两极,而加热率则是分别由高纬和低纬指向副热带,这样的经向梯度可能是驱动对流层顶结构变化的一种重要因素;两者空间分布的季节变化显著,但其对应关系并不完全一致,1月和4月的空间结构与7月和10月的相反,随季节调整具有突变现象;东亚及青藏高原是季节变化相对稳定的区域.(2) 在热带对流层顶控制区加热率与臭氧含量呈正相关,而极地对流层顶控制区各季节有所不同,还与太阳赤纬变化相关联;各纬度间加热率季节变化的位相和变率都存在差异,但南半球相对较为一致,最大距平为±2×10-4 K·d-1,北半球则较复杂,最大正距平为4×1010-4 K·d-1;两半球的季节周期位相趋于相反.(3) 除赤道外,臭氧距平的季节变化位相超前于加热率距平2~3月,并且发生在季节变化的调整期;最大距平出现在南极的8月大于0.4 DU,3~4月则小于-0.2 DU,而北极为±0.2 DU.(4) 臭氧含量和加热率的年际与年代际演变关系对应一致,并具有多尺度的结构特征;但两半球及赤道的时空演变差异明显,30° S~30° N间副热带控制区的加热率变幅剧烈,最大距平为±2.5×10-4 K·d-1,高纬和两极的变幅在不同演变期各不相同;臭氧的变幅结构与之相反,北极的最大距平分别大于0.25 DU和小于-0.35 DU.(5) 20世纪70年代以前及70年代中期,两半球的正负距平具有相反的演变结构,而90年代是负距平演变最剧烈的时期. 相似文献
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利用1958~2001年的臭氧混合比和ECMWF(European Centre for Medium_range Weather Forecast)资料,采用Wei诊断模型定量计算了穿越全球对流层顶的臭氧质量通量.结果表明:(1)臭氧通量场存在纬向型和经向型的空间波列结构,这些空间波列均未能跨越对流层顶断裂带到达热带对流层顶控制区,其中南北两极的极区、地中海-伊朗高原-青藏高原-日本南部-北太平洋和南半球对流层顶断裂带中沿纬圈完整的空间波列最为显著.海洋上空臭氧通量的性质较为均匀一致,大陆上空的空间结构多变.北半球向下与向上的局地平均最大臭氧通量分别是-4μg.m-2.s-1和2.5μg.m-2.s-1,南半球的对应值为-2.5μg.m-2.s-1和1.5μg.m-2.s-1.(2)纬向平均的臭氧净通量依赖于纬度变化,北半球与南半球具有显著的非对称特性,总效应是平流层臭氧向对流层输运注入.臭氧通量有着显著的季节变化,可随不同季节在地理分布上发生空间转移现象,而且其控制机制不仅受对流层顶的季节运动影响,也随大气环境的季节调整而发生改变.(3)南北半球臭氧净通量的变化趋势相反,南半球为双峰结构,表现为非对称振幅的季节波动结构.全球臭氧通量振幅的年际变化表现出明显的QBO(Quasi_Biennial Oscillation)特性,年代际演变的结构形态(向下的臭氧净通量)可划分为4个阶段:1960年代是平稳变化期,1970年代为增强期,1980年代是又一个相对平稳期,1990年代为剧烈变化期.向下的臭氧净通量主极大值出现在1977、1990年和1998年,极小值在1993年和1996年. 相似文献
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亚洲地区是物质由对流层向平流层输送的主要通道,在平流层-对流层交换中扮演着积极的角色. 本文主要利用卫星资料和欧洲中心ERA40再分析资料,借助Wei诊断模式研究亚洲地区夏季上对流层-下平流层(UTLS)水汽分布和平流层-对流层水汽交换特征,重点着眼于水汽交换的年际变化,并探讨其与亚洲夏季风的联系. 结果表明,季风区UTLS水汽较赤道地区偏多,且通过磁带记录信号的传播,可穿越对流层顶影响下平流层水汽的多寡. 夏季平流层-对流层水汽交换表现出明显的年际特征,其年际变化与亚洲季风强弱变化有密切联系,尤其与南亚夏季风的关系更为显著. 在亚洲夏季风影响下,亚洲地区出现异常的大气环流和垂直运动,从而影响平流层-对流层之间水汽的交换. 这些结果对认识其它大气成分的输送过程也具有重要的指示意义. 相似文献
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青藏高原和热带西北太平洋大气热源在亚洲地区夏季平流层-对流层水汽交换的年代际变化中的作用 总被引：5，自引：0，他引：5
利用欧洲中期天气预报中心ERA40资料,借助Wei诊断模式研究平流层一对流层水汽交换过程,重点分析亚洲地区夏季平流层．对流层水汽交换的年代际特征,探讨青藏高原和热带西北太平洋大气热源在其变化中的作用．气候学特征表明,北半球夏季“亚洲南部半岛-印度洋-太平洋交汇区”为全球最强的对流层向平流层输送的通道,它能将亚洲季风区丰富的水汽源源不断地输送到平流层,影响平流层水汽的分布和变化．北半球夏季亚洲地区穿越对流层顶水汽交换整体上都具有明显的年代际变化,且在近44a可以分为三段比较稳定的时段：1958～1977年、1978～1992年和1993。2001年．在这三个时段中,孟加拉湾．东亚大陆及南海海域的水汽交换通道作用在逐渐减弱,而西北太平洋地区在水汽交换中扮演着越来越重要的角色．进一步研究发现,青藏高原、热带西北太平洋热源的年代际异常是亚洲地区平流层．对流层水汽交换年代际变化的主要原因．44a来青藏高原和热带西北太平洋的热力作用均发生了重大调整,在年代际尺度上两者的综合作用决定了亚洲夏季风的年代际变异,从而影响平流层．对流层水汽交换的年代际异常．然而不同时段不同地区两者的贡献有所不同,尤其是1992年以后,高原热源影响明显减弱,而热带西北太平洋热源在影响平流层．对流层水汽交换中起主要作用．这些结果对深入认识其他大气成份输送过程和正确评估人类活动（排放）对全球气候的影响也具有重要的指示意义． 相似文献
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根据Aura卫星微波临边探测(MLS)2.2,3.3版水汽和臭氧廓线,采用线性内插方法,将夏季在青藏高原(西藏的那曲和拉萨)及其周边地区(云南腾冲)通过冷冻霜点仪(CFH)和电化学反应池型(ECC)探空仪分别测得的水汽和臭氧数据插值到与卫星产品规定的气压高度进行比较分析,以检验MLS水汽和臭氧廓线产品.结果表明:MLS 2.2和3.3版水汽相对误差在100 h Pa的对流层顶附近分别为(9.8±46.0)%(n=18),(23.0±45.8)%(n=17);在小于并包含82.5h Pa在内的下平流层则分别为(-2.2±15.7)%(n=74),(0.3±14.9)%(n=75);而在对流层316~121h Pa高度则分别为(21.5±90.6)%(n=104),(6.0±83.4)%(n=99).相应MLS 2.2,3.3版臭氧的误差分别为:(-3.5±54.4)%(n=27),(-8.7±41.6)%(n=38)(100 h Pa);(-11.7±16.3)%(n=135),(15.6±24.2)%(n=305)(下平流层);(18.0±79.1)%(n=47),(34.2±76.6)%(n=160)(对流层上层).MLS水汽和臭氧的误差垂直分布在对流层上层-平流层低层振荡和离散分布明显,部分误差可能由于此高度层水汽和臭氧浓度梯度大和比较用线性插值探空数据引起."臭氧低谷"期间,拉萨地区70 h Pa高度以下MLS卫星臭氧浓度误差明显增加;腾冲、那曲与拉萨三地的MLS臭氧误差的垂直分布特征较一致.卫星产品与探空测值的初步关系表明,MLS廓线的灵敏度与水汽和臭氧在大气中垂直分布有密切联系,3.3版水汽产品的灵敏度在82.5 h Pa以上高度略有提高,臭氧产品灵敏度没有明显变化.文中还讨论了导致MLS水汽和臭氧廓线产品误差的可能因素. 相似文献
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利用北半球40°N～50°N纬度带上HALOE实验测量的O3和H2O廓线资料,根据示踪成分O3和H2O空间分布的化学寿命以及输运特征时间常数等性质,在等熵坐标中构建了对流层顶附近及最低平流层300～390 K等熵面间,O3/H2O混合关系的结构形态和季节特征.结果表明: (1) 在对流层顶转换层的320～380 K等熵面间O3混合比廓线的斜率具有空间转折"突变",而H2O混合比廓线的斜率则出现空间渐变转折.在对流层顶附近O3和H2O的源分别是平流层与对流层,使O3混合比和H2O混合比在320～380 K等熵面的两侧显现出截然不同的垂直分布梯度.(2) 在对流层顶附近O3/H2O达到最小二乘意义上的最佳拟合时,两者参考关系的对流层支与平流层支呈现出非规则"L"结构形态的季节与季节内变化,其中对流层支的斜率为负,而平流层支的斜率可随季节出现正负变化.同时,由"L"形态的转角处可确定随季节变化的化学对流层顶(chemopause)特征.(3) 由O3/H2O混合关系反映出对流层不同区域空气携带的物质成分分别与平流层空气混合而形成混合层,而且可使混合层的混合线不恒定.混合层的表现在2003年、2005年1月和2003年4月的混合程度相当,混合的等熵厚度大约是30 K,即在320～350 K等熵面间.2005年11月的混合高度有所增高,进入平流层的H2O混合比要比2003年和2005年1月的小,混合的等熵厚度大约为30 K,在330～360 K等熵面间.不同季节混合的等熵厚度变化较小,但高度可随季节而变化.O3/H2O混合关系的平流层支随季节的变化很明显,1月最低平流层空气脱水是引起平流层支季节变化的重要原因. 相似文献
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By using 2-D chemical model, the trend of total column ozone over the Tibetan Plateau is simulated. The results show that from 1980 to 1993, the total column ozone over the Tibetan Plateau decreases; after 1995, it starts to recover. But until 2050, it will not still reach the level of 1980 total column ozone. Under Tibetan special circulation, its total column ozone recovers more rapidly than zonal mean. Therefore, the Tibetan special meridional circulation is not a main reason why the total column ozone over the Tibetan Plateau decreases more strongly than zonal mean.
相似文献12.
《Journal of Atmospheric and Solar》2003,65(11-13):1235-1243
The aim of the present paper is to study the solar response in the vertical structure of ozone and temperature over the Indian tropical region and a search for any mutual relationship between their solar coefficients on a decadal scale in the lower stratosphere. For the purpose, the data obtained by ozonesonde and Umkehr methods for the lower stratospheric ozone and that of the total ozone amount from Dobson spectrophotometer during the period 1979–2001 have been analyzed. These data are analyzed using the multi-functional regression model, which takes into account most of the known natural and anthropogenic signals. The NCEP- and MSU-satellite data for the temperature over this region have been used. Results indicate an in-phase correlation of around 0.5 between ozone and solar flux (F10.7) in the vertical structure over the equatorial station, Trivandrum (8.3°N) but no significant correlation over Pune (18.3°N). The solar components of ozone and temperature indicate an in-phase but poor correlation in the lower stratospheric altitudes over both stations. However, when total ozone content data is analyzed, it indicates a very high correlation (⩾0.9) between the solar components of ozone and temperature. The solar trend in the vertical distribution of ozone is found to be of the order of 5–25% per 100 units of F10.7 solar flux for Trivandrum but it is relatively smaller (1.6–15.2%) over Pune. The solar dependence of temperature is found to be quite significant for the entire Indian tropical region with not much latitudinal variation. 相似文献
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Using the improved CCM1 dynamic climate model, the impact of abnormal heat source and sink over the Tibetan Plateau in winter on the abnormal zonal wind over the Pacific Ocean is studied in this paper. The following new-findings are obtained: (1) When the at mospheric cold source during January—March on the Tibetan Plateau gets intensified, an abnormal anticyclone around the Tibetan Plateau will appear in lower troposphere. Abnormal northerly wind at the coastal area of the mainland of China and an abnormal cyclone will appear on the West Pacific in the following months. Then, abnormal west wind will appear over the equator of the West Pacific and extends to the East Pacific. (2) When the atmospheric cold source during January—March over the Tibetan Plateau is unusually weak, an abnormal cyclone around the Tibetan Plateau will appear at lower levels first, then abnormal anticyclone will appear on the West Pacific and move to the south and result in abnormal easterly wind over the equator of the West Pacific, which will extend to the east. Furthermore, abnormal changes of zonal wind on equatorial Indian Ocean can be caused by the intensity change of atmospheric cold source in winter and early spring over the Tibetan Plateau.
相似文献14.
In this study, results of source identification and apportionment for ambient volatile organic compounds (VOCs) from a previous work were used to estimate ozone‐forming potentials (OFPs) of effective sources for developing proper strategies for reduction of tropospheric ozone pollution. The source identification and apportionment of ambient VOC pollution within Yildiz Technical University's Davutpasa Campus (Istanbul, Turkey) was done by positive matrix factorization (PMF). The results suggested five effective source groups with the emissions related with paint use and solvent use having the highest contributions (36.8 and 28.2%). The results from PMF were used along with maximum incremental reactivities to estimate potentials of individual sources for ozone formation. It was found that biogenic emissions (3.78) and traffic related emissions (gasoline and diesel vehicle exhaust) (3.83 and 3.15, respectively) have the highest potential for ozone formation in terms of grams O3/g VOC emitted. The results were used to suggest proper source‐based reduction strategies for OFP. 相似文献
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Harry van Loon Gerald A. Meehl Julie M. Arblaster 《Journal of Atmospheric and Solar》2004,66(18):1767-1778
The availability of global gridded precipitation and outgoing long-wave radiation (OLR) data after 1978 makes possible an investigation of the influence of the decadal solar oscillation in the tropics during three solar maxima and two solar minima. The NCEP/NCAR reanalyses starting in the 1950s allows the inclusion of an additional two solar maxima and minima to look for consistency of response across a longer time period. In the northern summer (July–August), the major climatological tropical precipitation maxima are intensified in solar maxima compared to solar minima during the period 1979–2002. The regions of this enhanced climatological precipitation extend from the Indian monsoon to the West Pacific oceanic warm pool and farther eastwards in the Intertropical Convergence Zone of the North Pacific and North American Monsoon, to the tropical Atlantic and greater rainfall over the Sahel and central Africa. The differences between solar maxima and minima in the zonal mean temperature through the depth of the troposphere, OLR, tropospheric vertical motion, and tropopause temperature are consistent with the differences in the rainfall. The upward vertical motion is stronger in regions of enhanced tropical precipitation, tropospheric temperatures are higher, tropopause temperatures are lower, and the OLR is reduced due to higher, colder cloud tops over the areas of deeper convective rainfall in the solar maxima than in the minima. These differences between the extremes of the solar cycle suggest that an increase in solar forcing intensifies the Hadley and Walker circulations, with greater solar forcing resulting in strengthened regional climatological tropical precipitation regimes. These effects are as strong or even more pronounced when warm and cold extremes in the Southern Oscillation are removed from the analyses. Additionally, lower stratospheric temperatures and geopotential heights are higher with greater solar forcing suggesting ozone interactions with solar forcing in the upper stratosphere. 相似文献
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Evaluations of radiosonde soundings over North America and Europe, measurements aboard commercial airlines, and permanent ozone registrations at nineteen ground-based stations between Tromsö, Norway, and Hermanus, South Africa, yield three belts of higher ozone intrusion from the stratosphera and maximum values of the annual means at about 30°N, at between 40°–45°N and at about 60°N. A marked decrease of the annual mean values of the tropospheric ozone is detected towards the equator and the pole, respectively.In the northen hemisphere the maximum of the annual cycle of the tropospheric ozone concentration occurs in spring at high latitudes and in summer at mid-latitudes.For the tropical region from 30°S to 30°N a strong asymmetry of the northern and southern hemisphere occurs. This fact is discussed in detail. The higher troposphere of the tropics seems to be a wellmixed reservoir and mainly supplied with ozone from the tropopause gap region in the northern hemisphere. The ozone distribution in the lower troposphere of the whole tropics seems to be controlled by the up and down movements of the Hadley cell. The features of large-scale and seasonal variation of tropospheric ozone are discussed in connection with the ozone circulation in the stratosphere, the dynamic processes near the tropopause and the destruction rate at the earth's surface. 相似文献
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The characteristics of spatial and temporal distribution of tropospheric NO2 column density concentration over China are presented, on the basis of measurements from the satellite instruments GOME and SCIAMACHY. From these observations, monthly averaged tropospheric NO2 variations are determined for the period of 1997 to 2006. The trend and seasonal cycle are also investigated. The possible source of tropospheric NO2 over megacity area is discussed in this paper. The results show a large growth of tropospheric NO2 over eastern China, especially above the industrial areas with a fast economical growth, such as, Yangtze Rive Delta region and Pearl River Delta region because of the prominent anthropogenic activity. There is a rapid increase of tropospheric NO2 over megacities in China. For instance, Shanghai had a linear significant increase in NO2 columns of ～20% per year (reference year 1997) in the period of 1997-2006, which is the rapidest increase among all the selected cities. The seasonal pattern of the NO2 concentration shows a difference between the east and west in China. In the eastern part of China, an expected winter maximum in seasonal cycle is found because of the prominent anthropogenic activity and meteorological conditions. In the western part this cycle shows a NO2 maximum in summer time, which is attributed to natural emissions, especially soil emissions and lightning. A quickly increasing vehicle population may contribute to the increase of tropospheric NO2 over megacities in China for the remarkable correlation for vehicle population with tropospheric NO2. 相似文献
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The Tibetan Plateau has one of the most complex climates in the world. Analysis of the climate in this region is important for understanding the climate change worldwide. In this study, climate patterns and trends in the Tibetan Plateau were analysed for the period from 1961 to 2001. Air temperature and precipitation were analysed on monthly and annual time scales using data collected from the National Meteorological Centre, China Meteorological Administration. Nonlinear slopes were estimated and analysed to investigate the spatial and temporal trends of air temperature and precipitation in the Tibetan Plateau using a Mann–Kendall method. Spatial analysis of air temperature and precipitation variability across the Tibetan Plateau was undertaken. While most trends are local in nature, there are general basinwide patterns. Temperature during the last several decades showed a long‐term warmer trend, especially the areas around Dingri and Zogong stations, which formed two increasing centres. Only one of the stations investigated exhibited decreasing trend, and this was not significant. Precipitation in the Tibetan Plateau has increased in most regions of the study area over the past several decades, especially in the eastern and central part, while the western Tibetan Region exhibited a decreased trend over the same period. Copyright © 2007 John Wiley & Sons, Ltd. 相似文献
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本文基于1979—2014年臭氧总量的卫星遥感数据,利用多元线性回归模型对臭氧总量数据序列进行模拟计算,考察了北太平洋上空臭氧总量长期变化趋势及其影响因素的作用.结果表明,北太平洋地区大气臭氧总量长期变化呈现减少趋势,但是减少速率随季节和纬度带表现出差异性,在各纬度带臭氧峰值季节臭氧下降趋势最为显著.在0°—15°N地区臭氧高值出现在夏秋季节并在8月达到峰值,峰值月份臭氧年均下降率约为0.2DU/a;15°—30°N亚热带地区臭氧高值出现在春夏季并在5月达到峰值,峰值月份臭氧年均下降速率约为0.22DU/a;而在30°—45°N中纬度地区臭氧高值出现在冬春季并在2月达到峰值,峰值月份臭氧年均下降率0.75DU/a.在臭氧分布年平均态基础上,影响臭氧总量分布变化的因素主要有臭氧损耗物质(EESC)、太阳辐射周期(Solar)、准两年振荡(QBO)和厄尔尼诺-南方涛动(ENSO)等.其中,EESC导致臭氧损耗效应随着纬度升高而增大,在从低到高的三个纬度带损耗最大值分别为11DU、16DU和66DU;Solar增强导致臭氧增加,在三个纬度带的增加效应最大值分别为16DU、17DU和19DU;QBO@10hPa和QBO@30hPa对臭氧影响幅度基本在±10DU内波动,只有QBO@10hPa对30°—45°N区域的影响作用达到14DU,值得注意的是QBO影响作用随着纬度变化存在相位差异,在0°—15°N区域臭氧变化与QBO呈现相同相位,而在15°—30°N和30°—45°N区域臭氧变化与QBO呈现相反相位;ENSO对各个纬度带臭氧影响幅度也在±10DU内,ENSO影响作用在不同纬度带也存在相位差异,臭氧总量变化在0°—15°N、15°—30°N区域与ENSO相位相反,在30°—45°N区域与ENSO相位一致. 相似文献