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1.
The aerosol longwave radiative forcing of the atmosphere and heating rate of the near-surface aerosol layer are estimated for the extreme smoke conditions in the Moscow region in summer 2010. Thermal radiation fluxes in the atmosphere are determined using the integral transmission function and semiempirical aerosol model developed on the basis of standard aerosol models and measurements at the Zvenigorod Scientific Station, Obukhov Institute of Atmospheric Physics, Russian Academy of Sciences. The aerosol radiative forcing reached 33 W/m2 at the lower atmospheric boundary and ranged between–1.0 and 1.0 W/m2 at the upper atmospheric boundary. The heating rate of the 10-m atmospheric layer near surface was up to 0.2 K/h during the maximum smoke conditions on August 7–9. The sensitivity of the aerosol longwave radiative forcing to the changes in the aerosol absorption coefficient and aerosol optical thickness are estimated.  相似文献   

2.
The shortwave radiative forcings of smoke aerosol in the cloudless atmosphere during the summer fires of 2010 in European Russia were quantitatively estimated for the land surface and the atmospheric upper boundary from measurement data obtained at the Zvenigorod Scientific Station of the Obukhov Institute of Atmospheric Physics (OIAP ZSS), Russian Academy of Sciences. Variations in the temperature of the surface air layer due to the smoke-induced attenuation of incoming solar radiation were estimated. The most intensive smoke generation in the atmosphere was observed on August 7–9, 2010, when the maximum aerosol optical thickness amounted to more than 4.0 at a wavelength of 550 nm. In this case, the albedo of single aerosol scattering amounted to ∼0.95–0.96 and the asymmetry factor amounted to ∼0.69–0.70. The maximum shortwave radiative forcing of aerosol amounted to about −360 W/m2 for the land surface and almost −150 W/m2 for the atmospheric upper boundary. During the period of intensive smoke generation, the cooling of the atmospheric surface layer over daylight hours (12 h) amounted, on average, to ∼6°C. The power character of the dependence of the shortwave radiative forcing of aerosol for the land surface on aerosol optical thickness up to its values exceeding 4.0, which was revealed earlier on the basis of data on aerosol optical thickness (up to 1.5) obtained at the OIAP ZSS during the summer forest and peatbog fires of 2002 in the region of Moscow, was supported.  相似文献   

3.
Temperature and radiation effects of the 2010 summer fires are estimated on the basis of measurements at the Zvenigorod Scientific Station (ZSS) of the Obukhov Institute of Atmospheric Physics, Russian Academy of Sciences (RAS), in the Moscow region. The surface air temperature during the 2010 summer smoke varied in antiphase with the aerosol mass concentration, and the thermal radiation balance in the surface layer of the atmosphere varied in phase. Under extreme smoke of the surface layer in August 2010, the reduction in surface air temperature at ZSS has been found to reach 4 K with an increase in the downward flux of thermal radiation by an average of 20 W/m2 and a decrease in the difference between upward and downward fluxes of thermal radiation by an average of 24 W/m2.  相似文献   

4.
Relations between short-term variations in the concentrations of aerosol (PM10) and carbon monoxide (CO) and meteorological characteristics are considered for the episodes of severe atmospheric pollution in the region of Moscow in the summer of 2010. The assumption is made and substantiated that the observed (in late June) severe aerosol pollution of the atmosphere over Moscow was caused by air masses arrived from soil-drought regions of southern Russia. In August, during the episodes of advection of forest-fire products, the maximum surface concentrations of pollutants were observed in Moscow mainly at 11:00–12:00 under a convective burst into the atmospheric boundary layer and at night in the presence of local wind-velocity maxima or low-level jet streams within the inversion layer. On the basis of results from an analysis of these air-pollution episodes before and after fires, it is concluded that the shearing instability of wind velocity favors the surface-air purification under ordinary conditions and an increase in the surface concentrations of pollutants during their advection (long-range transport, natural-fire plumes, etc.). It is shown that the pollution of the air basin over the megapolis with biomass-combustion products in 2010 led to an increase in the thermal stability of the atmospheric surface layer and in the duration of radiation inversions, as well as to an attenuation of the processes of purification in the urban heat island.  相似文献   

5.
The results of measurements of surface ozone in central European Russia in 2004–2010 are presented. The variation coefficient for hourly, monthly, and annual mean ozone concentrations is 78, 26, and 12%, respectively. The measurements established a link between increased (>60 μg/m3) and minimum (<12 μg/m3) hourly mean ozone concentrations with the existence of a temperature inversion in the lower 300-m atmospheric layer. Sixty-seven percent of the total number of increased hourly mean ozone concentrations over the 2004–2010 period took place in 2010. A maximum hourly mean ozone concentration of 218.5 μg/m3 was recorded at 17:00 on August 1, 2010. The annual mean ozone concentration in a climatically significant range of hourly mean concentrations from 12 to 60 μg/m3 increased by 45% in a linear approximation over the period of record. The spectral analysis of monthly mean concentrations of surface ozone identified composite oscillations with periods from 3 to 60 months. To approximate the temporal dynamics of ozone, a statistical model was used. This model satisfactorily describes the experimental monthly and annual mean concentrations.  相似文献   

6.
The volatile organic compounds (VOCs) emitted from vegetation into the atmosphere play an important role in atmospheric chemistry and participate in the formation and growth of aerosol particles that affect the atmospheric radiation balance and the earth’s climate. A number of VOCs, such as isoprene, monoterpene, methylvinylketone, and methacrolein, whose surface concentrations were measured between Moscow and Vladivostok in the course of the Transcontinental Observations into the Chemistry of the Atmosphere (TROICA-12) experiment in July–August 2008, are considered. For the first time in Russia, a PTR-MS proton mass-spectrometer was used to measure the VOC concentrations. The continuous series of VOC concentrations in the atmosphere over the Trans-Siberian Railway were obtained, and the characteristic features of their variations were determined. The spatial distribution of the concentrations of biogenic VOC was compared with a map of Russia’s forests. It was found that the maximum concentrations of isoprene between Moscow and Vladivostok correspond to the zones of broad-leaved forests in the Far East and Primorskii Krai, and the maximum concentrations of monoterpene correspond to coniferous forests in Siberia. The obvious correlation between the concentrations of isoprene and the total concentration of methylvinylketone and methacrolein was revealed.  相似文献   

7.
Estimates of some aerosol and radiation characteristics of the atmosphere in the summer of 2010 are obtained according to the results of the measurements made at the Meteorological Observatory (MO) at Moscow State University and are compared with the results of the measurements performed in 2002 and 1972 during the forest and peat fires. In contrast to 1972 and 2002, the period under study in 2010 is characterized by a greater frequency of the highest class of fire danger according to Nesterov, higher aerosol optical depths of the atmosphere up to 4.6, and a more significant weakening of solar radiation in different spectrum regions. In 2010 the smoke aerosol caused losses of the total shortwave radiation of 33%, visible radiation of 39%, ultraviolet radiation of 300–380 nm of 51%, and erythemal radiation of 63%. At the same time, an increase in the downward long-wave radiation to 40–50 W/m2 under extreme aerosol optical depths is recorded.  相似文献   

8.
The evolution of smoke plume over European Russia (ER) during the massive forest and peatbog fires of summer 2010 has been studied using observations of aerosol optical depth (AOD) from MODIS instruments (both Aqua and Terra platforms), objective analysis of meteorological fields performed at the Russian Hydrometeorological Research Center, NCEP/NCAR reanalysis, as well as upper air data. A relation between the structure inhomogeneities of the AOD field and regional atmospheric circulation has been found. It is shown that, on August 5–9, 2010, the maximum of smoke pollution did complete turn around Moscow, while remaining at a distance of 200 to 650 km from the megacity. Both regionally averaged shortwave aerosol radiative forcings (ARFs) at the top and the bottom of the atmosphere are estimated for the period of extreme smoke pollution over ER. The spatial distributions of ARF values over the territory of the region and the estimates of the local and spatially distributed thermal effects of smoke aerosol are given. It is shown that, on August 5–9, 2010, the spatial distribution of AOD and the calculated thermal effects of smoke aerosol were in agreement with the spatial distributions of air-temperature anomalies observed in the lower 1.5-km layer of the atmosphere. MODIS’s AOD data obtained during the wildfires were validated by AOD observations from the CIMEL sun photometer operated at the AERONET station Zvenigorod.  相似文献   

9.
This is a comprehensive study of the physicochemical characterization of multicomponent aerosols in the smoky atmosphere of Moscow during the extreme wildfires of August 2010 and against the background atmosphere of August 2011. Thermal–optical analysis, liquid and ion chromatography, IR spectroscopy, and electron microscopy were used to determine the organic content (OC) and elemental content (EC) of carbon, organic/inorganic and ionic compounds, and biomass burning markers (anhydrosaccharides and the potassium ion) and study the morphology and elemental composition of individual particles. It has been shown that the fires are characterized by an increased OC/EC ratio and high concentrations of ammonium, potassium, and sulfate ions in correlation with an increased content of levoglucosan as a marker of biomass burning. The organic compounds containing carbonyl groups point to the process of photochemical aging and the formation of secondary organic aerosols in the urban atmosphere when aerosols are emitted from forest fires. A cluster analysis of individual particles has indicated that when the smokiest atmosphere is characterized by prevailing soot/tar ball particles, which are smoke-emission micromarkers.  相似文献   

10.
Variations in the concentrations of both primary (PM10, CO, and NOx) and secondary (ozone) pollutants in the atmosphere over the Moscow and Kirov regions, Kiev, and Crimea under the conditions of the anomalously hot summer of 2011 are given and analyzed. The concentrations of ozone, PM10, CO, and NOx in the atmosphere over the Moscow region exceeded their maximum permissible levels almost continuously from late July to late August 2010. The highest level of atmospheric pollution was observed on August 4–9, when the Moscow region was within a severe plume of forest and peatbog fires. The maximum single concentrations of ozone, which exceeded its maximum permissible level two-three times, were accompanied by high concentrations of combustion products: the concentrations of PM10 and CO were also three-seven times higher than their maximum permissible concentrations. The maximum levels of air pollution were observed under the meteorological conditions that were unfavorable for pollution scattering, first of all, at a small vertical temperature gradient in the lower atmospheric boundary layer. The number of additional cases of mortality due to the exceeded maximum permissible concentrations of PM10 and ozone in the atmosphere over Moscow was estimated. Under the weather conditions that were close to those for the Moscow region, the air quality remained mainly satisfactory in the Kirov region, Kiev, and Crimea, which were almost not affected by fires.  相似文献   

11.
Dimethylsulfide in coastal zone of the East China Sea   总被引：1，自引：0，他引：1  
Dimethylsulfide (DMS) in seawater were observed four times from February 1993 to August 1994 along a fixed section (PN line) in the East China Sea. The DMS concentrations showed remarkable temporal and spatial variations. The DMS concentrations were generally higher in the upper euphotic layer of the continental shelf zone in summer. The spatial variation, however, was more pronounced even in well mixed winter water, where the concentration of DMS varied widely from 3 to 106 ng-S/l in the continental shelf zone while the salinity was vertically almost uniform. This means that DMS in seawater is rapidly produced and decomposed with a time scale less than one month in the water column. The largest value of 376 ng-S/l was obtained at 5 m depth near the mouth of Changjiang River in August 1994. The mean concentrations in the surface 30 m layer in the continental shelf zone were 21, 54, 126 and 57 ng-S/l in February, October, June and August, respectively, which were about twice as large as those in the Kuroshio region. The mean fluxes of DMS from the East China Sea to the atmosphere are estimated to be 49 g-S/m2/day in winter and 194 g-S/m2/day in summer in the continental shelf zone, and to be 32 and 107 g-S/m2/day in the Kuroshio region.  相似文献   

12.
Variations in the surface aerosol over the arid steppe zone of Southern Russia have been measured. The parameters of atmospheric aerosol (mass concentration, both dispersed and elemental compositions) and meteorological parameters were measured in Tsimlaynsk raion (Rostov oblast). The chemical composition of aerosol particles in the atmospheric surface layer has been determined, and the coefficients of enrichment of elements with respect to clarkes in the Earth’s crust have been calculated. It is shown that, in summer, arid aerosols are transported from both alkaline and sandy soils of Kalmykia to the air basin over the observation zone. Aerosol particles in the surface air layer over this region have been found to contain the products of combustion of oil, coal, and ethylized fuel. These combustion products make a small contribution to the total mass concentration of atmospheric aerosol; however, they are most hazardous to the health of people because of their sizes and heavy-metal contents. A high concentration of submicron sulfur-containing aerosol particles of chemocondensation nature has been recorded. Sources of aerosol of both natural and anthropogenic origins in southern Russia are discussed.  相似文献   

13.
We report results from the first deployment of a buoy-mounted aerosol sampler on the Bermuda Testbed Mooring (BTM) in the Sargasso Sea, in which a time-series of 21 aerosol samples were collected over the period May 5–September 29, 2004. These aerosol samples were analyzed for iron and soluble sodium (as a proxy for sea salt). Also analyzed was a time-series of 22 aerosol samples collected over the same period at the Tudor Hill atmospheric sampling tower on Bermuda. The buoy sampler worked as intended and successfully collected a time-series of aerosol samples, thus demonstrating that moored buoys can be used as oceanic observatories to provide information on the temporal (weekly, monthly and seasonal) variability in the concentration of aerosol iron (and other trace elements) over the surface ocean. The magnitude and time variation of aerosol Fe concentrations calculated from the BTM buoy samples are in close agreement with the corresponding aerosol Fe record from the Tudor Hill tower, which is located approximately 80 km northwest of the mooring site. Both the BTM and Tudor Hill samples record periods of high aerosol iron loadings in late June and late July 2004, reflecting the transport of soil dust from North Africa, with the highest concentration of aerosol iron at the BTM site (0.83 μg m−3) measured in late June. Concentrations of sea-salt aerosol calculated from the BTM samples are comparable to values measured over the Sargasso Sea and for samples collected at the Tudor Hill tower. Sea-salt aerosols do not appear to impede the collection of mineral aerosols by the buoy-mounted sampler.  相似文献   

14.
Phytoplankton productivity, community composition and biomass were determined over a nine-month period in brackish waters of the lower Gunpowder River, a tributary of Chesapeake Bay. Primary productivity followed expected seasonal magnitudes for temperate estuaries with rates exceeding 142·4 mg C m?3 h?1 in July through September 1979 and minimum rates of 1·6 mg C m?3 h?1 in February 1980. Annual primary production was estimated at 45·5 gC m?2. Cell numbers were highest in August, September and November with cyanophytes dominating the planktonic algae. Primary productivity, chlorophyll concentrations and cell densities were dominated by nanoplanktonic forms (< 10 μm) through-out the study. Phytoplankton carbon calculated from cells volumes exceeded nutritional requirements of the pelagic herbivores in all months suggesting a mean daily export (to the bay or sediments) of 1607 mg C m?3 d?1.  相似文献   

15.
长江口及其邻近陆架区夏季网采浮游植物及其影响因素   总被引：3，自引：1，他引：2  
2009年6、8月长江口及其邻近陆架区的网采样品中检出浮游植物9门395种(含223种硅藻与125种甲藻)。浮游植物丰度8月(3 077.15×104 cells/m3)显著高于6月(107.80×104 cells/m3)。随长江冲淡水势力增强,位于长江口的丰度高值区8月较6月更偏外侧。种类丰富度8月高于6月,但多样性和均匀度指数略低于6月。6月尖刺伪菱形藻和三角角藻占绝对优势,8月优势种主要有尖刺伪菱形藻、笔尖形根管藻和铁氏束毛藻。骨条藻虽非优势种,但在长江冲淡水区丰度较高。相似性分析和多维尺度分析表明,浮游植物群落组成时空差异显著。典范对应分析表明,温度和盐度是分别影响6、8月群落分布的首要因子。根据水动力和化学参数,该区浮游植物群落分布与环流变化和水团消长密切相关。  相似文献   

16.
强壮箭虫是我国温带海域的浮游动物优势种。本文通过2009年7月至2010年6月在北黄海獐子岛海域的逐月综合调查,研究了大网浮游动物中强壮箭虫丰度的周年变化及其与环境因子的关系。结果显示,强壮箭虫年平均丰度为22.6 ind/m3,高峰值出现在12月（47.5 ind/m3）,最低值出现在8月（7.8 ind/m3）;在水平分布上,除了夏季的8月,全年近岸海域强壮箭虫丰度均高于外海海域,且在10月及次年2月差异显著（P<0.05）。相关性分析显示,作为肉食性浮游动物,强壮箭虫丰度时空变化除了受温度和盐度影响外,还与饵料生物（主要是桡足类）丰度有关。我们认为,这是其丰度周年变化规律在不同海域出现明显差异的主要原因。  相似文献   

17.
Measurement results of downward longwave radiation (DLR) in a wavelength range of 3.5?C50 ??m are considered which have been obtained with the use of a precision IR radiometer (Eppley pyrgeometer) of the PIR model at the Meteorological Observatory of Moscow State University in 2008?C2010. The influence of air temperature and atmospheric moisture content on the DLR values has been analyzed; correlations between DLR and the above parameters have been found. The effect of clouds on DLR has been estimated: DLR increases by about 30% in daytime and by 25% in nighttime under overcast low clouds. The annual average DLR in Moscow is 305 W/m2, with a minimum in December?CMarch and a maximum in July?CAugust. Variations in DLR throughout a year can exceed 250 W/m2. The daily average amplitude is 18?C33 W/m2 in summer and 6?C13 W/m2 in winter. An increase in DLR by about 40 W/m2 is noted under conditions of haze from forest and peat-bog fires and an aerosol optical depth of about 4 at a wavelength of 500 nm.  相似文献   

18.
The East China Sea is a productive marginal sea with a wide continental shelf and plays an important role in absorbing atmospheric carbon dioxide and transferring terrigenous organic matter to the open ocean. To investigate the roles of heterotrophic bacteria in the biogeochemical dynamics in the East China Sea, bacterial biomasses(BB) and productions(BP) were measured in four cruises. The spatial distributions of the BB and the BP were highly season-dependent. Affected by the Changjiang River discharge, the BB and the BP were high in shelf waters(bottom depth not deeper than 50 m) and generally decreased offshore in August 2009. In December 2009 to January 2010, and November to December 2010, the BB and the BP were high in waters with medium bottom depth. The onshore-offshore decreasing trends of the BB and the BP also existed in May–June 2011, when the BB was significantly higher than in other cruises in shelf break waters(bottom depth deeper than 50 m but not deeper than 200 m). The results of generalized additive models(GAM) suggest that the BB increased with the temperature at a range of 8-20°C, increased with the chlorophyll concentration at a range of 0.02–3.00 mg/m3 and then declining, and decreased with the salinity from 28 to 35. The relationship between the temperature and the log-transformed bacterial specific growth rate(SGR) was linear. The estimated temperature coefficient(Q10) of the SGR was similar with that of the phytoplankton growth. The SGR also increased with the chlorophyll concentration. The ratio of the bacterial to phytoplankton production ranged from less than 0.01 to 0.40, being significantly higher in November–December 2010 than in May–June 2011. Calculated from the bacterial production and growth efficiency, the bacterial respiration consumed, on average, 59%, 72% and 23% of the primary production in August 2009, November–December 2010, and May–June 2011, respectively.  相似文献   

19.
The results of 2-year (2010–2012) measurements of the concentrations of organic carbon (OC) and elemental carbon (EC), which were taken at the Zotino Tall Tower Observatory (ZOTTO) Siberian background station (61° N, 89° E), are given. Despite the fact that this station is located far from populated areas and industrial zones, the concentrations of OC and EC in the atmosphere over boreal forests in central Siberia significantly exceed their background values. In winter and fall, high concentrations of atmospheric carbonaceous aerosol particles are caused by the long-range transport (~1000 km) of air masses that accumulate pollutants from large cities located in both southern and southwestern regions of Siberia. In spring and summer, the pollution level is also high due to regional forest fires and agricultural burning in the steppe zone of western Siberia in the Russian–Kazakh border region. Background concentrations of carbonaceous aerosol particles were observed within relatively short time intervals whose total duration was no more than 20% of the entire observation period. In summer, variations in the background concentrations of OC closely correlated with air temperature, which implies that the biogenic sources of organic-particle formation are dominating.  相似文献   

20.
Using the data obtained in 1999–2000 during the spring bloom of phytoplankton (late May–early June), the variability of the pigment concentrations, the phytoplankton biomass and species compositions, and the hydrological conditions on the eastern shelf of Sakhalin Island was studied. The study resulted in revealing 135 microalgae species belonging to eight divisions. The most diversely presented were the Dinophyta dinoflagellates and Bacillariophyta diatoms (70 and 53 species, respectively). The concentration of chlorophyll a in the euphotic zone amounted, on average, to 3.8 mg/m3 in 1999 and 2.4 mg/m3 in 2000. It was shown that, in the northern and southern parts of the coastal zone, the concentration of chlorophyll a and the phytoplankton density in the spring were considerably different and depended on the hydrological conditions. In the north, their maximum values were found in the area of the depth break and were determined by the tidal mixing. The increased algae concentrations and temperature inversions at depths of 400–600 m confirm the downslope sliding of the near-bottom shelf waters. In the southern part, the high phytoplankton concentrations in the surface layer in 1999 confirmed by the monthly averaged estimates from the SeaWiFS satellite color scanner were caused by the abnormal northward propagation of the Soya Current waters and by intense tidal mixing.  相似文献   

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