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1.
East China (23.6°–38.4°N, 113.6°–122.9°E) is the largest developed region in China. Based on CO2 products retrieved from the Greenhouse Gases Observing Satellite (GOSAT), the spatial and temporal distributions of CO2 mixing ratios in East China during 2014–17 are discussed, and the retrieved CO2 from AIRS (Atmospheric Infrared Sounder) and OCO-2 (Orbiting Carbon Observatory-2), as well as WLG (Waliguan) background station observations, are compared with those of GOSAT. The annual CO2 retrieved from GOSAT in East China ranged from 398.96 ± 0.24 ppm in 2014 to 407.39 ± 0.20 ppm in 2017, with a growth rate of 2.82 ± 0.15 ppm yr?1, which were higher than in other regions of China. The seasonal cycle presented a maximum in spring and a minimum in summer or autumn. Higher values were mainly concentrated in the coastal areas of Zhejiang Province, and lower values were concentrated in Jiangxi and the north of Fujian Province. CO2 observed in Fujian and parts of Jiangxi increased by less than 1.0 ppm during 2014–15, but enhanced significantly by more than 5.0 ppm during 2015–16, perhaps influenced by local emissions and global impacts. We calculated year-to-year CO2 enhancements in the Yangtze River Delta region during 2014–17 that were relatively low and stable, due to the region’s carbon emissions control and reduction policies. The annual and seasonal amplitudes of CO2 retrieved from AIRS were lower than those from GOSAT in East China, probably owing to the CO2 retrieved from AIRS better reflecting the characteristics of the mid-troposphere, while GOSAT is more representative of near-surface CO2. The spatial and temporal distribution characteristics of CO2 retrieved from OCO-2 were close to those from GOSAT in East China.  相似文献   

2.
Measurements of column-averaged dry-air mole fractions of carbon dioxide and carbon monoxide, CO2 (XCO2) and CO (XCO), were performed throughout 2019 at an urban site in Beijing using a compact Fourier Transform Spectrometer (FTS) EM27/SUN. This data set is used to assess the characteristics of combustion-related CO2 emissions of urban Beijing by analyzing the correlated daily anomalies of XCO and XCO2 (e.g., ΔXCO and ΔXCO2). The EM27/SUN measurements were calibrated to a 125HR-FTS at the Xianghe station by an extra EM27/SUN instrument transferred between two sites. The ratio of ΔXCO over ΔXCO2 (ΔXCO:ΔXCO2) is used to estimate the combustion efficiency in the Beijing region. A high correlation coefficient (0.86) between ΔXCO and ΔXCO2 is observed. The CO:CO2 emission ratio estimated from inventories is higher than the observed ΔXCO:ΔXCO2 (10.46 ± 0.11 ppb ppm?1) by 42.54%–101.15%, indicating an underestimation in combustion efficiency in the inventories. Daily ΔXCO:ΔXCO2 are influenced by transportation governed by weather conditions, except for days in summer when the correlation is low due to the terrestrial biotic activity. By convolving the column footprint [ppm (μmol m–2 s–1)–1] generated by the Weather Research and Forecasting-X-Stochastic Time-Inverted Lagrangian Transport models (WRF-X-STILT) with two fossil-fuel emission inventories (the Multi-resolution Emission Inventory for China (MEIC) and the Peking University (PKU) inventory), the observed enhancements of CO2 and CO were used to evaluate the regional emissions. The CO2 emissions appear to be underestimated by 11% and 49% for the MEIC and PKU inventories, respectively, while CO emissions were overestimated by MEIC (30%) and PKU (35%) in the Beijing area.  相似文献   

3.
Space-borne measurements of atmospheric greenhouse gas concentrations provide global observation constraints for top-down estimates of surface carbon flux.Here,the first estimates of the global distribution of carbon surface fluxes inferred from dry-air CO_2 column (XCO_2) measurements by the Chinese Global Carbon Dioxide Monitoring Scientific Experimental Satellite (Tan Sat) are presented.An ensemble transform Kalman filter (ETKF) data assimilation system coupled with the GEOS-Chem global chemistry transport model is used to optimally fit model simulations with the Tan Sat XCO_2 observations,which were retrieved using the Institute of Atmospheric Physics Carbon dioxide retrieval Algorithm for Satellite remote sensing (IAPCAS).High posterior error reduction (30%–50%) compared with a priori fluxes indicates that assimilating satellite XCO_2 measurements provides highly effective constraints on global carbon flux estimation.Their impacts are also highlighted by significant spatiotemporal shifts in flux patterns over regions critical to the global carbon budget,such as tropical South America and China.An integrated global land carbon net flux of 6.71±0.76 Gt C yr~(-1) over12 months (May 2017–April 2018) is estimated from the Tan Sat XCO_2 data,which is generally consistent with other inversions based on satellite data,such as the JAXA GOSAT and NASA OCO-2 XCO_2 retrievals.However,discrepancies were found in some regional flux estimates,particularly over the Southern Hemisphere,where there may still be uncorrected bias between satellite measurements due to the lack of independent reference observations.The results of this study provide the groundwork for further studies using current or future Tan Sat XCO_2 data together with other surfacebased and space-borne measurements to quantify biosphere–atmosphere carbon exchange.  相似文献   

4.
利用2004年以来东亚地区10个本底观测站大气φ(CO2)观测资料,分析了各站大气φ(CO2)的变化特征及其各站之间的差异,讨论了下垫面特征、源汇作用等对φ(CO2)变化的影响.结果表明:10个本底站大气月均φ(CO2)有明显的季节变化,高值多出现在冬春等寒冷季节,而低值则多出现在6—9月,属于北半球的夏季;大气φ(CO2)日变化趋势较为一致,15时(当地时间)前后达到全天最低,随后φ(CO2)升高,并在日落后继续积累,至清晨7时(当地时间)前后达到全天最高,之后φ(CO2)随着太阳辐射的增强而逐渐降低,且平均φ(CO2)水平与下垫面植被量成反比,φ(CO2)日变化的幅度与下垫面植被量成反比.作为全球基准站之一的瓦里关山站,2004—2008年φ(CO2)年均值逐年增加,年增长率为2.28×10-6/a.  相似文献   

5.
China’s first carbon dioxide(CO2) measurement satellite mission, TanSat, was launched in December 2016. This paper introduces the first attempt to detect anthropogenic CO2 emission signatures using CO2 observations from TanSat and NO2 measurements from the TROPOspheric Monitoring Instrument(TROPOMI) onboard the Copernicus Sentinel-5 Precursor(S5P) satellite. We focus our analysis on two selected cases in Tangshan, China and Tokyo, Japan.We found that t...  相似文献   

6.
Cloud radiative kernels were built by BCC_RAD(Beijing Climate Center radiative transfer model) radiative transfer code. Then, short-term cloud feedback and its mechanisms in East Asia(0.5°S-60.5°N, 69.5°-150.5°E) were analyzed quantitatively using the kernels combined with MODIS satellite data from July 2002 to June 2018. According to the surface and monsoon types, four subregions in East Asia—the Tibetan Plateau, northwest, temperate monsoon(TM), and subtropical monsoon(SM)—were selected. The average longwave, shortwave, and net cloud feedbacks in East Asia are-0.68 ± 1.20, 1.34 ± 1.08, and 0.66 ± 0.40 W m~(-2) K~(-1)(±2σ), respectively, among which the net feedback is dominated by the positive shortwave feedback. Positive feedback in SM is the strongest of all subregions, mainly due to the contributions of nimbostratus and stratus. In East Asia, short-term feedback in spring is primarily caused by marine stratus in SM, in summer is primarily driven by deep convective cloud in TM, in autumn is mainly caused by land nimbostratus in SM, and in winter is mainly driven by land stratus in SM. Cloud feedback in East Asia is chiefly driven by decreases in mid-level and low cloud fraction owing to the changes in relative humidity, and a decrease in low cloud optical thickness due to the changes in cloud water content.  相似文献   

7.
During two measuring campaigns in early spring 1994 and 1995 (March/April) and one campaign in summer 1994, measurements of ozone, PAN, sulfur dioxide, nitric acid, and particulate nitrate, sulfate, and ammonium (only 1995) were recorded in the Arctic. Observations were made by aircraft at various sites in the eastern and western Arctic. Ozone concentrations showed a steady increase with altitude both in spring and summer. During five flights in springtime, low ozone events (LOEs) could be observed near the surface and up to altitudes of 2000 m. SO2 background concentrations, ranging from detection limit (0.5 nmol/m3) to 5 nmol/m3, were observed during both spring and summer. Distinct maxima up to 55 nmol/m3 in lower altitudes were only obtained in springtime. Concentrations of the organic nitrate PAN were within a similar range as those of the inorganic nitrate HNO3 during spring campaigns. In contrast, concentrations of particulate nitrate were one half an order of magnitude lower. HNO3 concentrations increased significantly with altitude. Evidently, HNO3 was intruded from the stratosphere into the troposphere. Sulfate concentrations ranged between 5 and 30 nmol/m3; ammonium concentrations were obtained within a range from 10 to 50 nmol/m3.  相似文献   

8.
Cirrus clouds related to transported dust layers were identified on 22 occasions with ground-based polarization lidar from December 2012 to February 2018 over Wuhan (30.5°N, 114.4°E), China. All the events occurred in spring and winter. Cirrus clouds were mostly located above 7.6 km on top of the aloft dust layers. In-cloud relative humidity with respect to ice (RHi) derived from water vapor Raman lidar as well as from ERA5 reanalysis data were used as criteria to determine the possible ice nucleation regimes. Corresponding to the two typical cases shown, the observed events can be classified into two categories: (1) category A (3 cases), in-cloud peak RHi ≥ 150%, indicating competition between heterogeneous nucleation and homogeneous nucleation; and (2) category B (19 cases), in-cloud peak RHi < 150%, revealing that only heterogeneous nucleation was involved. Heterogeneous nucleation generally took place during instances of cirrus cloud formation in the upper troposphere when advected dust particles were present. Although accompanying cloud-top temperatures ranged from –51.9°C to –30.4°C, dust-related heterogeneous nucleation contributed to primary ice nucleation in cirrus clouds by providing ice nucleating particle concentrations on the order of 10?3 L?1 to 102 L?1. Heterogeneous nucleation and subsequent crystal growth reduced the ambient RHi to be less than 150% by consuming water vapor and thus completely inhibited homogeneous nucleation.  相似文献   

9.
The CO2 concentrations and fluxes over an urban forest site (Namsan) and an urban residential region (Boramae) in Seoul, Korea, during the non-growing season (2–4 March 2011), the growing season (10–12 June 2011), and the late-growing season (22–24 September 2011) were analyzed. The CO2 concentrations of two sites showed nearly the same diurnal variation, with a maximum value occurring during the night and a minimum value occurring during daytime, as well as the same seasonal variation, with a maximum value during the non-growing season (early spring) and a minimum value during the growing season (summer). The CO2 flux over the urban forest did not show any typical diurnal variation during the non-growing season, but did show diurnal variation with a small positive value during the night and a large negative value during daytime in the growing and late-growing seasons due to photosynthesis in the urban forest. The CO2 flux over the urban residential region showed a positive daily mean value for all periods, with large values during the non-growing season and small values during the growing season, and it also showed diurnal variation with two maxima at 0600–1000 LST and 1800–2400 LST, and two minima at 0300-0600 LST and 1100-1500 LST, and was strongly correlated with the use of liquefied natural gas for cooking and heating by surrounding houses.  相似文献   

10.
Surface ozone (O3) and fine particulate matter (PM2.5) are dominant air pollutants in China. Concentrations of these pollutants can show significant differences between urban and nonurban areas. However, such contrast has never been explored on the country level. This study investigates the spatiotemporal characteristics of urban-to-suburban and urban-to-background difference for O3 (Δ[O3]) and PM2.5 (Δ[PM2.5]) concentrations in China using monitoring data from 1171 urban, 110 suburban, and 15 background sites built by the China National Environmental Monitoring Center (CNEMC). On the annual mean basis, the urban-to-suburban Δ[O3] is ?3.7 ppbv in Beijing–Tianjin–Hebei, 1.0 ppbv in the Yangtze River Delta, ?3.5 ppbv in the Pearl River Delta, and ?3.8 ppbv in the Sichuan Basin. On the contrary, the urban-to-suburban Δ[PM2.5] is 15.8, ?0.3, 3.5 and 2.4 μg m?3 in those areas, respectively. The urban-to-suburban contrast is more significant in winter for both Δ[O3] and Δ[PM2.5]. In eastern China, urban-to-background differences are also moderate during summer, with ?5.1 to 6.8 ppbv for Δ[O3] and ?0.1 to 22.5 μg m?3 for Δ[PM2.5]. However, such contrasts are much larger in winter, with ?22.2 to 5.5 ppbv for Δ[O3] and 3.1 to 82.3 μg m?3 for Δ[PM2.5]. Since the urban region accounts for only 2% of the whole country’s area, the urban-dominant air quality data from the CNEMC network may overestimate winter [PM2.5] but underestimate winter [O3] over the vast domain of China. The study suggests that the CNEMC monitoring data should be used with caution for evaluating chemical models and assessing ecosystem health, which require more data outside urban areas.  相似文献   

11.
根据1985—2004年NCEP/NCAR再分析资料,采用HYSPLIT扩散模式和虚拟源方法,模拟分析了珠江三角洲大气污染物的空间和时间分布状况,初步讨论了珠江三角洲大气输送和扩散的季节特征,及其长期变化趋势。结果表明:珠江三角洲大气的输送和扩散有明显的季节变化特征,春、夏季大气污染物汇聚区位于珠江三角洲的西北侧,秋、冬季位于偏西侧;春、夏季的汇聚区明显强于秋、冬季。春、夏季大气分别向珠江三角洲西北和偏北方向的山区输送和扩散,而秋、冬季则沿着较为平坦的粤西海岸,向西南偏西方向输送和扩散。秋、冬季大气污染物的滞留时间明显比春、夏季短。1985—2004年大气输送和扩散能力存在年际差异,其中以2004年的输送和扩散能力最弱、1996年最强。  相似文献   

12.
Hydrofluorocarbons(HFCs) have been widely used in China as substitutes for ozone-depleting substances,the production and use of which are being phased out under the Montreal Protocol.China is a major consumer of HFCs around the world,with its HFC emissions in CO_2-equivalent contributing to about 18% of the global emissions for the period2012-16.Three methods are widely used to estimate the emissions of HFCs-namely,the bottom-up method,top-down method and tracer ratio method.In this study,the tracer ratio method was adopted to estimate HFC emissions in the Yangtze River Delta(YRD),using CO as a tracer.The YRD region might make a significant contribution to Chinese totals owing to its rapid economic growth.Weekly flask measurements for ten HFCs(HFC-23,HFC-32,HFC-125,HFC-134 a,HFC-143 a,HFC-152 a,HFC-227 ea,HFC-236 fa,HFC-245 fa and HFC-365 mfc) were conducted at Lin'an Regional Background Station in the YRD over the period 2012-16,and the HFC emissions were 2.4±1.4 Gg yr~(-1) for HFC-23,2.8±1.2 Gg yr~(-1) for HFC-32,2.2±1.2 Gg yr~(-1) for HFC-125,4.8±4.8 Gg yr~(-1) for HFC-134 a,0.9±0.6 Gg yr~(-1) for HFC-152 a,0.3±0.3 Gg yr~(-1) for HFC-227 ea and 0.3±0.2 Gg yr~(-1) for HFC-245 fa.The YRD total HFC emissions reached 53 Gg CO_2-e yr~(-1),contributing 34% of the national total.The per capita HFC CO_2-equivalent emissions rate was 240 kg yr-1,while the values of per unit area emissions and per million GDP emissions reached 150 Mg km~(-2)yr~(-1) and 3500 kg yr~(-1)(million CNY GDP)-1,which were much higher than national or global levels.  相似文献   

13.
The Puelo River is a watershed shared between Chile and Argentina with a mean annual streamflow of 644 m3 s?1. It has a high ecologic and economic importance, including introduced farmed salmon, tourism, sports fishing and projected hydroelectricity. Using Austrocedrus chilensis and Pilgerodendron uviferum tree-ring records we reconstructed summer–fall (December–May) Puelo River streamflow, which is the first of such reconstructions developed in the Pacific domain of South America. The reconstruction goes back to 1599 and has an adjusted r 2 of 0.42. Spectral analysis of the reconstructed streamflow shows a dominant 84-year cycle which explains 25.1% of the total temporal variability. The Puelo River summer–fall streamflow shows a significant correlation (P?>?0.95, 1943–2002) with hydrological records throughout a vast geographic range within the Valdivian eco-region (35 to 46°S). Seasonal Puelo River interannual streamflow variability is related to large-scale oceanic and atmospheric circulation features. Summer–fall streamflows showed a significant negative correlation with the Antarctic Oscillation (AAO), whereas winter–spring anomalies appear to be positively connected with sea surface temperature variations in the tropical Pacific. In general, above- and below-average discharges in winter–spring are related to El Niño and La Niña events, respectively. The temporal patterns of the observed and reconstructed records of the Puelo River streamflow show a general decreasing trend in the 1943–1999 period. Projected circulation changes for the next decades in the Southern Hemisphere would decrease summer–fall Puelo River streamflows with significant impacts on salmon production, tourism and hydropower generation.  相似文献   

14.
Measurements of carbon dioxide(CO2), methane(CH4), and carbon monoxide(CO) are of great importance in the Qinghai-Tibetan region, as it is the highest and largest plateau in the world affecting global weather and climate systems. In this study, for the first time, we present CO2, CH4, and CO column measurements carried out by a Bruker EM27/SUN Fourier-transform infrared spectrometer(FTIR) at Golmud(36.42°E, 94.91°N, 2808 m) in August 2021. The mean and...  相似文献   

15.
Near real-time measurements of PM2.5 ionic compositions were performed at the summit of the highest mountain in the central-eastern plains in the spring and summer of 2007 in order to characterize aerosol composition and its interaction with clouds. The average concentrations of total water soluble ions were 27.5 and 36.7 μg?m?3, accounting for 44% and 62% of the PM2.5 mass concentration in the spring and summer, respectively. A diurnal pattern of SO 4 2- , NH 4 + and NO 3 - was observed in both campaigns and attributed to the upslope/downslope transport of air mass and the development of the planetary boundary layer (PBL). The average SO2 oxidation ratio (SOR) in summer was 57% (±27%), more than twice that in spring 24% (±16%); the fine nitrate oxidation ratio (NOR) was comparable in the two seasons (9?±?6% and 11?±?10% in summer and spring, respectively). This result indicates strong summertime production of sulfate aerosol. A principal component analysis shows that short-range and long-range transport of pollution, cloud processing, and crustal source were the main factors affecting the variability of the measured ions (and other trace gases and aerosols) at Mt. Tai. Strong indications of biomass burning were observed in summer. Cloud scavenging rates showed larger variations for different ions and in different cloud events. The elevated concentrations of the water soluble ions at Mt. Tai indicate serious aerosol pollution over the North China plain of eastern China.  相似文献   

16.
In order to correctly use the column-averaged atmospheric CO2 dry-air mole fraction (XCO2) data in the CO2 flux studies, XCO2 measurements retrieved from the Orbiting Carbon Observatory-2 (OCO-2) in 2015 were compared with those obtained from the global ground-based high-resolution Fourier Transform Spectrometer (FTS) participating in the Total Carbon Column Observing Network (TCCON). The XCO2 retrieved from three observing modes adopted by OCO-2, i.e., nadir, target, and glint, were separately validated by the FTS measurements at up to eight TCCON stations located in different areas. These comparisons show that OCO-2 glint mode yields the best qualitative estimations of CO2 concentration among the three operational approaches. The overall results regarding the glint mode show no obvious systematic biases. These facts may indicate that the glint concept is appropriate for not only oceans but also land regions. Negative systematic biases in nadir and target modes have been found at most TCCON sites. The standard deviations of XCO2 retrieved from target and nadir modes within the observation period are similar, and larger than those from glint mode. We also used the FTS site in Beijing, China, to assess the OCO-2 XCO2 in 2016. This site is located in a typical urban area, which has been absent in previous studies. Overall, OCO-2 XCO2 agrees well with that from FTS at this site. Such a study will benefit the validation of the newly launched TanSat products in China.  相似文献   

17.
海表温度和地表温度与中国东部夏季异常降水   总被引：18，自引：2，他引：16  
主要研究太平洋与印度洋海表温度和地表温度场与中国东部夏季降水的相关关系,以及异常大降水产生的下垫面条件.研究结果表明:(1)夏季黑潮区海温与同期长江流域的降水存在明显正相关,北方地区夏季降水与靠近非洲东岸的印度洋海域存在明显负相关.(2)夏季海温异常与同期中国降水异常场之间的相关分析(SVDI)表明,20世纪70年代后期当海温由La Nina多发期向El Nino多发期转变后,长江流域向异常多雨转变,而其北方和南方地区则向异常少雨方向发展.(3)中国东部区域降水与陆面温度的明显相关区有:(a)春,夏季热带非洲和夏季亚洲大陆部分地区地表温度与当年长江流域夏季降水存在显著正相关;(b)春季4、5月份部分亚洲大陆地表温度与当年华北地区夏季降水有明显负相关.(4)通过对比分析发现:长江(1954,1998和1999年)或江淮(1991年)流域几次特大异常降水的下垫面条件是黑潮区为海温正距平,同期欧亚大陆主要为正地表温度距平场.  相似文献   

18.

Size-segregated aerosol particles were collected using a high volume MOUDI sampler at a coastal urban site in Xiamen Bay, China, from March 2018 to June 2020 to examine the seasonal characteristics of aerosol and water-soluble inorganic ions (WSIIs) and the dry deposition of nitrogen species. During the study period, the annual average concentrations of PM1, PM2.5, PM10, and TSP were 14.8?±?5.6, 21.1?±?9.0, 35.4?±?14.2 μg m?3, and 45.2?±?21.3 μg m?3, respectively. The seasonal variations of aerosol concentrations were impacted by the monsoon with the lowest value in summer and the higher values in other seasons. For WSIIs, the annual average concentrations were 6.3?±?3.3, 2.1?±?1.2, 3.3?±?1.5, and 1.6?±?0.8 μg m?3 in PM1, PM1-2.5, PM2.5–10, and PM>10, respectively. In addition, pronounced seasonal variations of WSIIs in PM1 and PM1-2.5 were observed, with the highest concentration in spring-winter and the lowest in summer. The size distribution showed that SO42?, NH4+ and K+ were consistently present in the submicron particles while Ca2+, Mg2+, Na+ and Cl? mainly accumulated in the size range of 2.5–10 μm, reflecting their different dominant sources. In spring, fall and winter, a bimodal distribution of NO3? was observed with one peak at 2.5–10 μm and another peak at 0.44–1 μm. In summer, however, the fine mode peak disappeared, likely due to the unfavorable conditions for the formation of NH4NO3. For NH4+ and SO42?, their dominant peak at 0.25–0.44 μm in summer and fall shifted to 0.44–1 μm in spring and winter. Although the concentration of NO3–N was lower than NH4–N, the dry deposition flux of NO3–N (35.77?±?24.49 μmol N m?2 d?1) was much higher than that of NH4–N (10.95?±?11.89 μmol N m?2 d?1), mainly due to the larger deposition velocities of NO3–N. The contribution of sea-salt particles to the total particulate inorganic N deposition was estimated to be 23.9—52.8%. Dry deposition of particulate inorganic N accounted for 0.95% of other terrestrial N influxes. The annual total N deposition can create a new productivity of 3.55 mgC m?2 d?1, accounting for 1.3–4.7% of the primary productivity in Xiamen Bay. In light of these results, atmospheric N deposition could have a significant influence on biogeochemistry cycle of nutrients with respect to projected increase of anthropogenic emissions from mobile sources in coastal region.

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19.
This paper reports aerosol chemical properties for the first time over a Korean Global Atmosphere Watch (GAW) supersite, Anmyeon (36°32′N; 126° 19′E), during 2003–2004 period. Total suspended Particulates (TSP) showed significant seasonal variation with consistent higher mass concentrations during spring season (average of up to 230?±?190 μg/m3). PM10 also followed similar trend with higher concentrations during spring (average of up to 170?±?130 μg/m3) and showed reduced concentrations during summer. PM2.5 showed a significant increase during summer (average of up to 60?±?25 μg/m3), which could be due to the influx of fine mode sea salt aerosols associated with the Changma front (summer monsoon). Chemical composition analysis showed enhanced presence of acidic fractions, majorly contributed by sulphates (SO 4 2- ) and nitrates (NO 3 - ) in TSP, PM10 and PM2.5 during different seasons. Enhanced presence of Calcium (Ca2+) was observed during sand storm days during spring. The high correlation obtained on matrix analysis between crustal ions and acidic ions suggests that the ionic compositions over the site are mainly contributed by terrestrial sources of similar origin. The neutralization factors has been estimated to find the extend of neutralization of acidicity by main basic components, and found to have higher value for Ammonium (up to 1.1) in different seasons, indicating significant neutralization of acidic components over the region by NH 4 + . Back trajectory analysis has been performed during different seasons to constrain the possible sources of aerosol origin and the results are discussed in detail.  相似文献   

20.
In this study, ideal but realistic numerical experiments are performed to explore the relative effects of changes in land use and emission distribution on air quality in the Pearl River Delta (PRD) region in winter. The experiments are accomplished using the Lagrangian particle transport and dispersion model FLEXPART coupled with the Weather Research and Forecasting model under different scenarios. Experiment results show that the maximum changes in daily mean air pollution concentration (as represented by SO2 concentration) caused by land use change alone reaches up to 2?×?10?6 g m?3, whereas changes in concentrations due to the anthropogenic emission distribution are characterized by a maximum value of 6?×?10?6 g m?3. Such results reflect that, although the impacts of land use change on air quality are non-negligible, the emission distribution exerts a more significant influence on air quality than land use change. This provides clear implications for policy makers to control urban air pollution over the PRD region, especially for the urban planning in spatial arrangements for reasonable emissions.  相似文献   

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