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1.
Transfer rule of 137C3 and 60Co in seawater and an arrificial food web which made up of Platy-monas, Arca, tenaeus and Tilapia were studied.The results showed that the transfer of nuclide could be realized in a longer food chain in which seawater contained radioactivity, the transfer along food chain alone was slight, the pathway of nuclide uptaken by organism was mainly from seawater,but the pressnce of the food was helpful to the transfer of the nuclide, the transfer efficiency of 60Co by every member in the marine food chain was greater than that of 137C3. 相似文献
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As part of a broad research program on the behavior of critical radionuclides to be discharged into the sea by the first Brazilian nuclear powerplant, the uptake accumulation and loss of 137Cs, 60Co and 125I by locally abundant seaweed species was studiedUptake in static 12 liter aquarium experiments reached apparent steady-state in 2–7 days (60Co and 125I) or 2–3 weeks (137Cs). Elimination followed a reverse pattern, being comparatively fast for 137Cs and slow for 60Co and 125I. Dry weight bioaccumulation factors (BFs) were variable, falling in the 101 range for 137Cs, 103 for 125I and 103–104 for 60Co. Various short-term experiments performed over a 16 month period, showed marked temporal variations of 60Co BFs for all species.The results demonstrated that the studied species may play an important role in the transfer of the critical radionuclides through local food webs and can be employed as useful monitors for routine or accidental radionuclide releases. 相似文献
3.
The transfer of 137C3, 60Co along Platymonas sp., Brachionus plieatilis Muller and Tilapia mos-sambica Peters was studied by using the tracer methods of both 137C3 and 60Co with Ge (Li) Gamma ray detector and S-80 type multichannel-analyser for measuring the radioactivity of the sample. The experiment was carried out in four groups and the period of the experiment was fifteen days. It was found that 60Co could be transferred along seawater→Platymonas→Brackionus→Tilapia, and that 137C3 could only be transferred from seawater to Platymonas. 137C3 was not accumulated by Brachionus in any group of the experiment. Brachionus ingested 60Co mainly from Platymonas, when 60Co was ingested by Tilapia; Brachionus played an important role in the transfer and the Tilapia ingested 137C3 mainly from seawater. 相似文献
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The effects of three photoperiods (24 hr illumination, 12 hr illumination + 12 hr darkness and 24 hr darkness) and three salinities (20‰, 30‰ and 35‰) on the uptake of 60Co and 137Cs for Chlorella sp. and on the growth of its algae are studied. The uptake of 60Co for the algae is two orders of magnitude higher than that of 137Cs. Of factorial effects, the effect of photoperiod is most significant either on the uptake of the radionuclides or on the growth of the algae; the effect of salinity comes next in order and that of their interaction remains with the last. The uptake of the two radionuclides increases with extended photoperiod while the uptake of 137Cs declines with increasing of salinity. The growth of the algae appears to be the best under the conditions of 24 hr illumination and 30‰ salinity. 相似文献
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D.S. Swan M.S. Baxter I.G. McKinley W. Jack 《Estuarine, Coastal and Shelf Science》1982,15(5):515-536
Analysis of 210Pb, 226Ra, 137Cs and 134Cs in short sediment cores provide first estimates of deposition rates in some Clyde sea lochs. The radio-caesium nuclides originate mainly in the liquid effluent released at distance from the Clyde by the Windscale nuclear fuel reprocessing plant and their concentrations in Clyde sediments provide information on (a) enrichment factors onto particulate matter, (b) surficial mixing coefficients and (c) sedimentation rates. A radiocaesium residence time in coastal waters of ca. 103 years reflects the importance of scavenging by the high nearshore particulate flux. 210Pb levels in sediments are controlled, in the unsupported fraction, by a major input sorbed on catchment particulates and, in the supported component, by 226Ra activities occasionally perturbed by unusually high surface values probably of planktonic origin. In one loch, detectable levels of 134Cs and 60Co are attributed to their discharge by nuclear submarines. 相似文献
7.
The impact of several chemical poisons on the Arca granosa absorbing 45Ca was studied. The results showed that the absorption of 45Ca in the blood and the soft tissue by Arca granosa was inhibited by the inorganic compounds of Cu, Zn, Pd, Cd, Hg and so on, among which the inhibition of Cd was the strongest, next was that of Cu and Hg. But the inhibition of the absorption of 45Ca in the shell of Arca granosa was little. The impact of three kinds of energy metabolism inhibitory substances on the absorption of 45Ca by the Area granosa showed that the absorption was an active transfer process. 相似文献
8.
本文报道2015年9月和2016年5月期间天然放射性核素224Ra和223Ra在吕宋海峡及周边海域表层和垂向水体的分布特征。为理解日本福岛核事故的影响,本文亦分析研究区域内人工放射性核素137Cs的分布特征。结果表明,224,223Ra和137Cs比活度水平均处于我国南海海洋天然放射性本底变化范围之内。224Ra在吕宋海峡以西南海北部海域比活度较高,在吕宋海峡以东菲律宾海域比活度较低。137Cs没有明显的分布趋势。基于三站位（LS3,LS5和LS8）224Ra、137Cs以及温盐的垂向分布特征,本文揭示224Ra和137Cs在热带表层水、次表层水和中-深层水中比活度水平和梯度变化的差异特征。彩虹台风事件扭转了整个吕宋海峡及周边海域的海流循环过程。大量以低水平224Ra为特征的西太平洋海水涌入南海,降低水体224Ra比活度水平。但是,西太平洋和南海北部海域水体137Cs比活度水平没有明显差异,台风导致的海流变化对水体137Cs比活度没有明显影响。 相似文献
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历次核试验进入海洋的~(137)Cs对中国近海影响的模拟研究 总被引：1，自引：0，他引：1
1945年以来,世界各主要核国家进行了数千次核试验,这些核试验产生的绝大部分放射性物质通过多种途径进入海洋,对海洋环境造成放射性污染。本文建立了一个准全球海洋的放射性物质输运和扩散数值模式,通过数值模拟手段评估了历史核试验释放的放射性物质137 Cs对中国近海海洋环境的影响。本文借助前人工作评估了核试验释放137Cs进入海洋的途径和总量;通过比较模拟结果与观测资料,表明本文建立的放射性物质模式能够较好地模拟出137Cs在中国近海及其邻近海域的分布情况和随时间演变特征;模拟结果表明中国近海里的137Cs浓度在20世纪50年代中期达到最大,其中吕宋海峡海域137Cs浓度最高,达80.99Bq/m3;进一步分析了2011年3月份日本福岛核事故前中国近海137Cs浓度分布状况,2011年整个中国近海137Cs浓度介于1.0~1.6Bq/m3间,且其浓度垂向分布较均匀,相对封闭的南海浓度略高于其他海域。 相似文献
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几种近海沉积物吸附137Cs的初步研究 总被引：1，自引：0，他引：1
在对青岛近海放射性污染调查研究中发现,该海区与对照海区(石岛海区和连云港海区)海水中~(137)Cs的含量处于同一水平,而所取沉积物中~(l37)Cs的含量却存在明显差异。同 相似文献
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Contents of90Sr,137Cs and60Co in surface sediments were investigated in and around Urazoko Bay, Fukui Prefecture, where a nuclear power plant has been operating since 1969 and the waste effluent has been released into the sea. The main source of90Sr and137Cs was recognized to be radioactive fallout, whereas60Co was considered to originate from the nuclear power plant. Using the137Cs concentration as an indicator of sorption capacity of the sediment, the behaviour of60Co was investigated. No seasonal variation was observed in the distribution pattern of60Co/137Cs ratio and the retention of the heavy initial discharge in 1969 was considered to dominate the radionuclide level in the sediment. Correlation of60Co/137Cs ratio in the sediment and the distance from the discharge outlet was expressed by a simple exponential function of the distance. It was suggested that the contamination is spreading out gradually to the outer region of Urazoko Bay. 相似文献
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The Fukushima nuclear accident in 2011 released large amounts of radionuclides, including ~(137)Cs, into the Pacific Ocean. A quasi-global ocean radioactive transport model with horizontal grid spacing of 0.5°×0.5° and 21 vertical layers was thereafter established to study the long-term transport of the Fukushima-derived ~(137)Cs in the ocean.The simulation shows that the plume of ~(137)Cs would be rapidly transported eastward alongside the Kuroshio Current and its extensions. Contaminated waters with concentrations lower than 2 Bq/m3 would reach the west coast of North America 4 or 5 years after the accident. The ~(137)Cs tends to be carried, despite its very low concentration, into the Indian and South Pacific Oceans by 2016 via various branches of ocean currents.Meanwhile, the ~(137)Cs concentrations in the western part of the North Pacific Ocean decrease rapidly with time. Up to now the highly contaminated waters have remained in the upper 400 m, showing no evidence of significant penetration to deeper layers. 相似文献
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对赣北黄茅潭近代湖泊沉积岩芯进行了~(137)Cs、~(210)Pb测试和SCP(球状碳粒)计数分析,阐述了~(137)Cs蓄积特征,结合SCP计数、粒度指标及降水记录厘定了一些事件性沉积层位。研究表明,1986年前后是沉积环境中~(137)Cs行为的转折点;在这之前,~(137)Cs以大气散落为主,其蓄积行为大致与降水存在正相关关系,在这之后,~(137)Cs以流域侵蚀为主,其蓄积行为与降水呈负相关关系。1953—1954年、1974—1975年、1998—1999年,流域降水丰沛,相应沉积层位~(137)Cs比活度低,这与流域强烈侵蚀稀释了进入湖泊的~(137)Cs有关。1963—1964年沉积层位~(137)Cs蓄积峰稳定而显著,与高通量的大气散落有关,也与当时降水量低,大雨、暴雨次数少,流域侵蚀强度低造成较低的沉积速率等密切相关,是可靠的定年时标。1986年存在同样的气候环境特点,其蓄积峰可能也是存在的,但需要进一步确认。基于~(210)Pb方法,利用多种计年模式计算了沉积岩芯的年代,发现与这些事件性沉积层位具有较大差异。研究认为,在长江中游这种降水高、流域侵蚀强度高的较为复杂的沉积环境中,~(210)Pb计年存在较大误差。复杂沉积环境中近代沉积的定年,有必要深度挖掘~(137)Cs环境行为,在全面阐述其蓄积特点的基础上,辅以SCP计数、粒度指标及降水等识别事件性沉积层位,矫正~(210)Pb计年,是精确建立近代沉积时标的必要方法。 相似文献
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The observed distribution of 137Cs resulting from known sources in the Severn Estuary permits the testing of simple predictive models for the one-dimensional distribution of non-conservative substances in an estuary. These models either use a known distribution of salinity to infer corresponding ones for other substances, or else directly solve mass balance equations utilizing previously determined dispersion coefficients. Both methods are shown to previously determined dispersion coefficients. Both methods are shown to provide results comparing favorably with observations.Stokes drift plays an important role in the circulation of the Severn. A modified densimetric Froude number, including this drift, is therefore used to estimate the circulation and stratification of the estuary.A new equation is used for calculating the 137Cs distribution from the observed salinity distribution. It generalizes previous formulations to permit variation of the net runoff with position along the estuary. 相似文献
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According to the principle of photosythesis with sunlight and CO2 by phytoplankton supplying food for marine organisms, while the nitrogenous compounds excreted by marine animals are transferred by bacteria into the nitrate for the use of phytoplankton, an artificial microhabitat is built to investigate comprehensively distributive relationship of 127Cs, 134Cs, 65Zn, 60Co, 50Fe, 54Mn In the parts of the microhabitat. The results show that 78% of the 134Cs and 137Cs in ion state are present in sea water, with 28 % of them nearly homogenous envolved in the exchanging processes of the suspensates and organisms, and that 80% of 59Fe, 54Mn, 65Zn, 60Co were concentrated by solid substance, whose motion was mainly controlled by biological processes. The factors affecting the distribution of nuclides in each composition are discussed. As another type of research on the controlled ecological system which is a subject currently studied in the world, the present paper is of reference value for studying quantitativ 相似文献
17.
Under the artificial condition the 59Fe morphology in sea water, its concentration in sediment and phytoplankton, its distribution and metabolism in tissue organs of marine animals were studied. The results showed that the morphology of 59Fe was in a particulate state in sea water. The adsorption rule of 59Fe by three kinds of sediments was similar. The concentration ability of 59Fe by phytoplankton was very strong. The critical concentration organs of S9Fe by marine animals were viscera. The gross radioactivity of 59Fe was mainly concentrated in protein. The concentration factor of 59Fe by DNA was the highest one. After excretion experiment, 59Fe of all the tissue organs was not detected. Small part of59Fe remained in the organic acid and protein state. There was a redistribution process in sediment for59Fe. 相似文献
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Shigeyoshi Otosaka 《Journal of Oceanography》2017,73(5):559-570
Temporal changes in cesium-137 (137Cs) concentrations in the surface (0–10 cm) layer of seabed sediment were quantified from continuous observation data at 71 stations within a 150-km radius of the Fukushima Daiichi Nuclear Power Plant, and the primary processes affecting temporal changes were identified. From March 2011 to the end of 2015, about 80% of the initially deposited 137Cs in the surface sediment in the coastal region (bottom depth ≤100 m) region has dissipated (radioactive decay is not included). Such a remarkable change in the 137Cs concentration was not observed in the offshore (>100 m) region. This paper focuses on the following three processes that affected the decrease in the 137Cs concentrations, and assesses their relative importance; (1) resuspension and transport of 137Cs-bound sediment, (2) desorption of 137Cs from the sediment, and (3) dilution of 137Cs by vertical mixing of sediment. Consequently, it was estimated that the first two processes together have potentially contributed to reduce the 137Cs inventory in the top 10 cm of the coastal region by at most 35%. Furthermore, by applying a pulse input sediment mixing model to the observed vertical distribution of sedimentary 137Cs, it was also estimated that more than 43% of the 137Cs in the surface sediment was transported to deeper sediment layers by vertical mixing of the sediment. This indicates that the decrease of 137Cs concentrations in coastal sediments was mainly affected by mixing of 137Cs-bound surface sediment with less contaminated sediment in the deeper layers. 相似文献
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Further studies on the transport in sea water and accumulation in marine sediment of the radionuclides, released from a nuclear power plant, on Urazoko Bay, Fukui Prefecture were reported.The partition of radionuclides among the particle size fractions of a sediment sample indicated that the accumulation of60Co,137Cs and54Mn in the sediment were dominated substantially by the sorption on the particle surface in sea water, and the patterns of their sorption were considerably similar to each other.In regard to the60Co contamination of marine sediments in an area of about 13 km2 around the nuclear power plant, 60% of the60Co contamination were retained in Urazoko Bay, which occupies only 7% of the bottom surface of the region.It is clear that a part of60Co accumulated in the sediment of Urazoko Bay gradually moved to the outerward. 相似文献
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Barnacles (Balanus sp) were used to examine the uptake and release of chromium-51 added to sea water in two different valence states, 51Cr(VI) and 51Cr(III).Hexavalent chromium-51 (sodium chromate) forms a true ionic solution in filtered sea water and barnacles were able to accumulate chronium in soft tissues 543 times the levels found in sea water. The experiment showed that incorporated Cr(VI), is released to the water in such way that only 20%% of maximum uptake was lost by the organisms after 26 days. Addition of the hexavalent form to non filtered sea water showed that 2% of the total radioactivity was attached to the suspended particles. Here again chromium is mainly concentrated in soft tissues, showing a concentration factor of 380 related to total chromium available in aquarium (solution + suspended particles). From the total radioactivity incorporated by the organisms, 20 % was released after 56 days in the clearance experiment.Chromium, as trivalent chromic chloride, when added to sea water precipitates and is quickly removed from the water by the filter activity of the barnacles. Unlike the hexavalent form, trivalent chromium is not concentrated in soft tissues of the barnacles and is quickly released to the water through the organisms digestive system. 相似文献