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1.
连霍高速郑商段路旁土壤重金属积累初探 总被引：2，自引：1，他引：1
以连霍高速郑州-商丘段路旁土壤为研究对象,在野外调查采样和实验室分析的基础上,探讨了公路交通对周围土壤中Ni、Pb、Cr、Cu、Zn和Cd 6种重金属含量与分布的影响,计算了表层土壤的重金属元素积累速率与积累通量.结果表明:Cu、Pb和Cd是典型的交通源重金属,其含量在公路两侧随着距离的增加,呈先增加后减少的趋势,含量峰值出现在离路基25-50 m之间.公路运营时间越长,交通源重金属含量就越高.两断面绝大部分样点Pb、Cu和Cd的积累速率和通量均为正值,且Cu＞Pb＞Cd,小王庄断面大于湾刘断面,Cu和Pb的通量远远超过国际上正常土壤标准. 相似文献
2.
在西安、南京采集111个气溶胶样品，测定了虚折射率ni和分析了粒子中Si、Al、Ca、Fe、K、Mg、Mn、Na、Ti、S、P、Pb和Zn的含量。统计分析表明，ni与S和Pb的相关系数r最高，分别为0.36和0.30，统计检验也表明，这一相关性是显著的。其它11种元素与ni的相关性较差，且并不显著。西安气溶胶S含量明显高于南京，它与ni之间的相关系数高出南京近一倍。这些结果表明，除碳C之外，气溶胶中的S和Pb及其化合物对辐射的吸收不能忽视。 相似文献
3.
基于ECMWF再分析数据的大气波导分布规律研究 总被引：2，自引：0，他引：2
大气波导对电磁波传播有显著的影响,大气波导特征参量分布研究对于分析电磁波传播乃至雷达、通信等电子设备效能具有重要意义,利用ERA-Interim数据计算大气波导特征参量,并用海洋调查期间的低空探空火箭数据计算的大气波导进行了验证,在此基础上用2011—2016年ERA-Interim温度、湿度分层数据统计分析了全球大气波导的发生概率、强度、高度,得出的结论是:大洋东部、大陆西部的信风带是大气波导的高发区,大洋上大气波导的高发区（发生概率＞50%）主要有6个,分别是北太平洋海区、南太平洋海区、北大西洋海区、南大西洋海区、北印度洋海区、南印度洋澳大利亚西部海区;同时,存在3个大气波导低发区或无大气波导区（热带辐合带区、北半球中高纬度区、南半球中高纬度区）。这些大气波导高发和低发区的位置、范围、发生概率具有季节变化,北半球MAM季（3—5月）发生概率最高,出现的范围最大,SON季（9—11月）概率最低,出现的范围最小,DJF（12、1、2月）、JJA（6—8月）季节介于两者之间;南半球SON季发生概率最高,出现的范围最大,MAM季概率最低,出现的范围最小。北半球大气波导强度总体上强于南半球大气波导强度,北半球MAM季大气波导较强海域范围最大,强度最强,其次为JJA季,SON季大气波导较强海域范围最小,强度最弱;南太平洋大气波导强度季节变化不明显,强度与北太平洋比均较弱,南大西洋SON季大气波导较强海域范围最大,强度最强,DJF季大气波导较强海域范围最小,强度最弱;北印度洋MAM季大气波导强度强,是大洋上波导最强的海域,大气波导较强海域范围大,JJA季基本没有大气波导。大气波导高度在信风带靠近大陆西岸海域高度较低,随着向西离岸距离增大高度升高,大气波导高发区的波导高度季节变化特征是:北半球在SON、DJF季高度高,波导高度高的区域面积大,MAM、JJA季高度低,波导高度高的区域面积小;南半球在MAM、JJA季高度高,波导高度高的区域面积大,SON、DJF季高度低,波导高度高的区域面积小;其他中低纬度近岸海域大气波导高度较低,大陆包围的内海大气波导高度最低。 相似文献
4.
大伙房水库是辽河流域典型水库饮用水源地。由于汇水区周边工矿废水的排放,重金属污染问题一直比较突出。为研究水库受重金属污染影响的情况,采用Hakanson潜在生态风险指数法对大伙房水库表层沉积物中重金属Cr、Cu、Zn、Cd、Pb的含量及分布进行分析,并对其污染程度及潜在生态风险危害进行评价,评价结果用地累积指数法进行验证。结果表明：大伙房水库表层沉积物中潜在生态危害最大的重金属元素为Cd,5种重金属元素潜在生态风险危害程度由大到小的顺序为Cd＞Cu＞Pb＞Cr＞Zn。 相似文献
5.
全球水循环的海洋分量研究 总被引：22，自引：2，他引：20
利用ＮＣＥＰ／ＮＣＡＲ再分析月平均和逐日资料,采用“余差”方法,计算了１９８４～１９９４年全球海气淡水通量,分析了全球水汽输送的特点。主要结果有：（１）在全球水循环中,副热带大洋是重要的水汽辐散区,热带辐合带、南太平洋辐合带和南太平洋东南海域是集中的水汽辐合区,赤道东风带是夏季印度洋季风环流的主要水汽通道;（２）再现了全球海气淡水通量的分布,例如副热带“海洋沙漠”带、热带辐合带和南太平洋辐合带净降水区等;展示了细节特征,如黑潮区的净蒸发特点等;（３）发现了北大西洋中高纬度地区存在一东北—西南向的净蒸发带,而前人结果中则为净降水带;（４）分析了各大洋海气淡水通量的季节、年际变化特征,讨论了太平洋相对于大西洋作为水汽汇的特点;指出热带辐合带和南太平洋辐合带是海气淡水通量变率最大的海域 相似文献
6.
7.
冬季黑潮海域异常加热与北太平洋大气环流的耦合关系 总被引：1，自引：0，他引：1
利用NCEP/NCAR和OAFlux月平均资料,采用SVD方法分析冬季黑潮海域的热通量和北太平洋500 hPa位势高度场之间的关系。第1对奇异向量占总方差的86.24%,表现为黑潮北部海域异常多的放热和北太平洋中西部的500 hPa位势高度场异常低。将正负异常年的各气象要素的距平场进行合成分析后表明：当阿留申低压增强（减弱）时,黑潮海域上空的西北风增强（减弱）,导致近地面层大气温度降低（升高）,使得热通量异常释放增加（减少）,从而降低（升高）了海表面温度。在黑潮海域及其下游,温度场在纬向垂直方向是斜压结构,位势高度场是相当正压结构,反映的是冷低压（暖脊）结构。通过分析风场无旋分量和垂直速度的距平发现,在中纬度地区存在距平的纬向环流圈：大气在北太平洋中部的低层上升（下沉）,在对流层高层（低层）分别向西、向东运动,在黑潮海域和北美西部下沉（上升）,增强（减弱）了中纬度纬向环流圈（MZC）。 相似文献
8.
2018年3月27-28日,内蒙古中东部、中国东北地区、华北等地出现一次大范围沙尘天气。28日凌晨,沙尘进入北京,受此影响北京出现了严重的污染天气。本文利用中国气象局地面常规观测资料、气溶胶激光雷达、风廓线雷达资料、生态环境部大气成分等资料分析了北京沙尘天气前后边界层特征、沙尘来源以及沙尘天气前后大气污染特征。结果表明：此次沙尘天气期间,北京沙尘气溶胶退偏振比约为0.25-0.40,退偏振比数据显示此次沙尘首先从高空进入北京,比地面提前6 h。此次影响北京的沙尘主要来自于北路,东路沙尘有一定补充;沙尘影响时段,北京Ca、Fe、Na、K、Mn等元素浓度显著升高,与该物质地壳丰度相当,污染物元素Cu、Zn、Pb、Cd、As等浓度有所降低,丰度远大于该物质在地壳中丰度。 相似文献
9.
2017年春季（3—5月）大气环流特征为：北半球极涡呈单极型分布,主体位于北冰洋上空,中高纬西风带呈5波型分布。3月,地面冷高压偏强,冷空气活动频繁。4月,环流由纬向型向经向型逐渐调整,冷空气势力减弱。5月,东北气旋明显加强,冷暖势力相当,入海气旋增多。春季,我国近海海域主要有16次8级以上大风过程,其中冷空气大风过程有7次,冷空气和温带气旋共同影响的大风过程有1次,入海温带气旋过程有4次,东北冷涡影响大风过程有3次,强对流导致雷暴大风过程1次;且有8次明显的浪高在2 m以上的大浪过程。春季共有6次比较明显的海雾过程,分别为3月1次、4月2次、5月3次。西北太平洋和南海共生成1个台风“梅花”和1个热带低压,其他各大洋共有热带气旋15个,分别为大西洋1个、东太平洋1个、南太平洋5个、南印度洋6个、北印度洋2个。 相似文献
10.
太湖底泥中重金属污染及潜在生态危害评价 总被引：29，自引：0，他引：29
以太湖底泥为研究对象，分析太湖底泥中重金属的含量分布及富集状况，采用Lars HǎKanson潜在生态危害指数法对重金属的生态危害进行了评价。结果表明：各种重金属的含量分布呈现一定的区域特征，太湖湖岸区平均含量明显高于湖心区，从富集系数来看，Pb的富集程度最高，其次是Zn、Cu、As、Cr、Hg、Cd。太湖底泥重金属的潜在生态危害评价显示，除无锡片区犊山口Hg的污染属于中等生态危害外，其他各点重金属的生态危害都相对轻微，污染程度顺序为Hg〉Cd〉Pb〉As〉Cu〉Zn〉Cr． 相似文献
11.
Continental origin and industrial sources of trace metals in the Northwest Atlantic troposphere 总被引：1，自引：0，他引：1
A. Veron T. M. Church C. C. Patterson Y. Erel J. T. Merrill 《Journal of Atmospheric Chemistry》1992,14(1-4):339-351
Trace metals (Mn, Fe, Ni, Cu, Zn, Cd, Pb and stable lead isotopes) have been analyzed in precipitation and total aerosols collected in the northwest Atlantic troposphere in April and November 1989. According to stable lead isotope signatures we encountered two main air mass sources, Mediterranean easterlies (206Pb/207Pb=1.131) and US westerlies (206Pb/207Pb=1.195–1.205). The phasing out of leaded gasoline has been invoked to explain the decrease of the 206Pb/207Pb ratios from 1.22 to 1.20 for the past 10 years in North America. Based on trajectory analyses, intermediate 206Pb/207Pb ratios are explained by a mixing of pure US westerlies with Canadian air masses (206Pb/207Pb=1.190–1.195) or Mediterranean air masses (206Pb/207Pb=1.18–1.19). Isentropic trajectories are very useful in explaining the variability of trace metal concentrations, a result of the fluctuating transport range of anthropogenic aerosols to remote marine areas of the North Atlantic. Lead concentrations appear to be closely correlated to the air mass transport patterns as defined from the meteorological analyses. For instance oceanic air masses transported over remote marine areas for more than three days were characterized by lead concentrations 2 to 10 times lower (Pb=0.5 to 2 ng/scm) than coastal air masses (Pb=3 to 10 ng/scm).Anthropogenic trace metal concentrations are generally in good agreement with the air mass signatures which display Pb and Cu, Ni, Zn concentrations higher than 2 and 10 ng/scm respectively in aerosol samples for the US source. Trace metal elemental ratios and soil enrichment factors were used to define industrial sources. Aerosol originating from the US exhibits the distinct industrial signature of Cu/Ni production and coal-oil combustion, while steel metallurgy could account for more than 50% of the overall Mn input into the Northwest Atlantic ocean. 相似文献
12.
吕俊梅张庆云陶诗言琚建华 《应用气象学报》2007,18(4):442-451
根据黄刚等定义的东亚夏季风指数, 对强、弱东亚夏季风年大气环流、大气热源和外强迫源SST的差异进行分析, 结果表明:强 (弱) 东亚夏季风年前期冬季到夏季, 太平洋SSTA为La Ni?a (El Ni?o) 型分布, 西太平洋暖池SST暖 (冷), 使得暖池附近对流活动较强 (较弱)。与此同时, 南亚大陆从印度半岛、青藏高原南部、中南半岛至华南大气异常加热 (变冷), 并且海陆热力对比加强 (减弱), 有利于出现强 (弱) 的东亚夏季风。此外, 由于暖池附近对流活动强 (弱), 该地区上升气流较强 (弱), Walker环流增强 (减弱), 当强 (弱) 的东亚夏季风向北推进时, 副热带西风急流北撤位置偏北 (南), 副热带高压位置也偏北 (南), 7月至8月华北 (江淮流域) 位于副热带西风急流南侧, 降水偏多, 江淮流域 (华北) 降水偏少。并给出与东亚夏季风年际变异有关的大气环流和SST异常的物理图像。 相似文献
13.
Trace Metal Solid State Speciation in Aerosols of the Northern Levantine Basin,East Mediterranean 总被引：3，自引：0，他引：3
Mustafa Koçak Nilgun Kubilay Barak Herut Malcolm Nimmo 《Journal of Atmospheric Chemistry》2007,56(3):239-257
An established three stage sequential leach scheme was applied to a series of selected high volume aerosol samples (n = 35) collected from the Turkish Eastern Mediterranean coastline (Erdemli). Samples were selected according to their air
mass back trajectory history to reflect the contrasting mixtures of aerosol material present in the Eastern Mediterranean
marine aerosol. Two populations were adopted, those samples which were classed as “anthropogenic” and those which were “Saharan”
dominated aerosol populations. Applying the three stage leach it was possible to define the proportion for each of the considered
metals (Al, Fe, Cu, Pb, Cd, Zn and Mn) present in the (a) “exchangeable” (b) “carbonate / oxide” and (c) “refractory” phases,
representing novel solid state aerosol speciation data for this marine system. Clear trends were established, conforming with
data from previous studies with mainly crustal derived metals (Al and Fe) being present in the refractory phases (Al > 88%;
Fe > 84%) and those influenced by anthropogenic sources being dominating in the exchangeable phase, although for these metals
the variability was comparatively high (12–64%; 19–85%; 40–100% for Zn, Pb and Cd, respectively). For the majority, greater
exchangeable fractions were present the lower the crustal source contribution to the aerosol population, whereas the “refractory”
fraction exhibited contrasting behaviour. This was illustrated by the novel application of the mixing diagram, presenting
each of the three speciation stages against the corresponding percent anthropogenic contribution to each collected sample.
Zn, Pb and Cd all illustrated progressive decrease in the percent exchangeable with increasing crustal contribution to the
aerosol population. The percent exchangeable was discussed in terms of its use to represent the upper limit of the bioavailable
fraction of metal associated with the aerosol, post deposition. The mixing diagram approach enabled the prediction of the
residual fractions for Cd, Pb and Zn (41 ± 4%; 62 ± 4% and 82 ± 5%, respectively,) in Saharan end-member material. 相似文献
14.
Gilles Tedeschi Alexander M. J. van Eijk Jacques Piazzola Jolanta T. Kusmierczyk-Michulec 《Boundary-Layer Meteorology》2017,163(2):327-350
Sea-salt aerosol concentrations in the coastal zone are assessed with the numerical aerosol-transport model MACMod that applies separate aerosol source functions for open ocean and the surf zone near the sea–land transition. Numerical simulations of the aerosol concentration as a function of offshore distance from the surf zone compare favourably with experimental data obtained during a surf-zone aerosol experiment in Duck, North Carolina in autumn 2007. Based on numerical simulations, the effect of variations in aerosol production (source strength) and transport conditions (wind speed, air–sea temperature difference), we show that the surf-zone aerosols are replaced by aerosols generated over the open ocean as the airmass advects out to sea. The contribution from the surf-generated aerosol is significant during high wind speeds and high wave events, and is significant up to 30 km away from the production zone. At low wind speeds, the oceanic component dominates, except within 1–5 km of the surf zone. Similar results are obtained for onshore flow, where no further sea-salt aerosol production occurs as the airmass advects out over land. The oceanic aerosols that are well-mixed throughout the boundary layer are then more efficiently transported inland than are the surf-generated aerosols, which are confined to the first few tens of metres above the surface, and are therefore also more susceptible to the type of surface (trees or grass) that determines the deposition velocity. 相似文献
15.
Data on aerosol optical thickness(AOT) and single scattering albedo(SSA) derived from Moderate Resolution Imaging Spectrometer(MODIS) and Ozone Monitoring Instrument(OMI) measurements,respectively,are used jointly to examine the seasonal variations of aerosols over East Asia.The seasonal signals of the total AOT are well defined and nearly similar over the land and over the ocean.These findings indicate a natural cycle of aerosols that originate primarily from natural emissions. In contrast,the small-sized aerosols represented by the fine-mode AOT,which are primarily generated over the land by human activities,do not have evident seasonalscale fluctuations.A persistent maximum of aerosol loadings centered over the Sichuan basin is associated with considerable amounts of fine-mode aerosols throughout the year.Most regions exhibit a general spring maximum. During the summer,however,the aerosol loadings are the most marked over north central China.This occurrence may result from anthropogenic fine particles,such as sulfate and nitrate.Four typical regions were selected to perform a covariation analysis of the monthly gridded AOT and SSA.Over southwestern and southeastern China,if the aerosol loadings are small to moderate they are composed primarily of the highly absorptive aerosols. However,more substantial aerosol loadings probably represent less-absorptive aerosols.The opposite covariation pattern occurring over the coastal-adjacent oceans suggests that the polluted oceanic atmosphere is closely correlated with the windward terrestrial aerosols.North central China is strongly affected by dust aerosols that show moderate absorption.This finding may explain the lower variability in the SSA that accompanies increasing aerosol loadings in this region. 相似文献
16.
北太平洋冬季年代际尺度海气相互作用 总被引：2，自引：2，他引：0
为了更深了解北太平洋年代际尺度海气相互作用,本文通过对湍流热通量和SST的相关关系进行了研究。当热通量和SSTA正相关时,代表海洋影响大气,而当二者相关系数为负时,表示大气强迫海洋。将整个北太平洋SSTA求平均和把北太平洋分成3个区域求SSTA平均,分别对热通量和SST的关系进行研究。结果表明,北太平洋冬季年代际尺度上的海气相互作用主要表现为海洋强迫大气,而在日本附近海域以及北太平洋中东部,海洋对大气的强迫作用最明显,因此这两个区域是北太平洋冬季年代际尺度上海气相互作用的关键区。 相似文献
17.
D. W. Pierce T. P. Barnett N. Schneider R. Saravanan D. Dommenget M. Latif 《Climate Dynamics》2001,18(1-2):51-70
Decadal time scale climate variability in the North Pacific has implications for climate both locally and over North America.
A crucial question is the degree to which this variability arises from coupled ocean/atmosphere interactions over the North
Pacific that involve ocean dynamics, as opposed to either purely thermodynamic effects of the oceanic mixed layer integrating
in situ the stochastic atmospheric forcing, or the teleconnected response to tropical variability. The part of the variability
that is coming from local coupled ocean/atmosphere interactions involving ocean dynamics is potentially predictable by an
ocean/atmosphere general circulation model (O/A GCM), and such predictions could (depending on the achievable lead time) have
distinct societal benefits. This question is examined using the results of fully coupled O/A GCMs, as well as targeted numerical
experiments with stand-alone ocean and atmosphere models individually. It is found that coupled ocean/atmosphere interactions
that involve ocean dynamics are important to determining the strength and frequency of a decadal-time scale peak in the spectra
of several oceanic variables in the Kuroshio extension region off Japan. Local stochastic atmospheric heat flux forcing, integrated
by the oceanic mixed layer into a red spectrum, provides a noise background from which the signal must be extracted. Although
teleconnected ENSO responses influence the North Pacific in the 2–7 years/cycle frequency band, it is shown that some decadal-time
scale processes in the North Pacific proceed without ENSO. Likewise, although the effects of stochastic atmospheric forcing
on ocean dynamics are discernible, a feedback path from the ocean to the atmosphere is suggested by the results.
Received: 23 January 2000 / Accepted: 10 January 2001 相似文献
18.
西北太平洋海域风浪、涌浪、混合浪波浪能资源特征 总被引：1，自引：0，他引：1
用ECMWF的ERA-40海浪再分析资料,应用波浪能流密度计算方法,对西北太平洋海域的风浪能、涌浪能、混合浪能展开研究。结果表明:(1)波浪能流密度呈现出显著季节性差异。混合浪能流密度表现为冬高夏低;春、夏、秋季的涌浪能流密度明显大于风浪能流密度,冬季相反;(2)混合浪能流密度的大值区主要分布于阿留申群岛附近海域,高值中心可达60 kW/m以上;近海的大值区主要分布于琉球群岛—巴士海峡—传统的南海大风区一带,年平均值在4 kW/m以上,南海北部可达12 kW/m以上;(3)黄渤海的涌浪和混合浪能流密度峰值出现在8—9月,波谷出现在6月。风浪能流密度峰值出现在11月—次年3月,波谷出现在6—8月,均呈现双峰型月变化特征。东海、南海北部、南海中南部海域能流密度的月变化特征相似,都为双峰型,12月—次年4月的能流密度整体较高,波峰出现在12月,波谷出现在5—7月;(4)2 kW/m以上混合浪能流密度出现的频率较高,近海低于大洋;(5)0.5 m以上有效波高出现的频率都非常高,中国近海稍低于大洋;(6)涌浪能流密度的稳定性明显好于风浪能流密度;大洋的能流密度稳定性明显强于近岸。1月份能流密度的稳定性最好,4月和7月次之,10月的稳定性最差。 相似文献
19.
Guangjian Wu Baiqing Xu Tandong Yao Chenglong Zhang Shaopeng Gao 《Atmospheric Research》2009,93(4):784-792
This study measured the concentration of heavy metal elements in atmospheric aerosol samples collected between July 2004 and April 2006 at a remote site on Mt. Muztagata (38°17'N, 75°01'E, 4430 m), in the Eastern Pamirs. Inductively coupled plasma mass spectroscopy (ICP–MS) results show that the air at Muztagata contains low concentrations of As and heavy metal elements (Cr, Ni, Cu, Zn, Cd, Pb, and Bi), comparable with those in the Arctic — far lower than in heavily populated or industrialized areas. Observed enrichment factor (EF) values greater than 10 for those elements suggest partly anthropogenic sources. Seasonal variations in the concentrations of Zn, Cd, Pb, Bi, and As resemble those of crustal Al, with greater concentrations during the summer but lower ones in winter. Our results reveal that the background atmosphere in remote inner Asia is only weakly affected by anthropogenic pollution, and demonstrate that high heavy metal concentrations occur during summer but with greater EF values during the winter. The air mass back-trajectory analyses suggest that pollution from West Asia, Central Asia, and South Asia are the main possible source areas that contribute to the heavy metals in aerosols at Muztagata. 相似文献
20.
Seasonal prediction skill of ECMWF System 4 and NCEP CFSv2 retrospective forecast for the Northern Hemisphere Winter 总被引：1，自引：1，他引：0
The seasonal prediction skill for the Northern Hemisphere winter is assessed using retrospective predictions (1982–2010) from the ECMWF System 4 (Sys4) and National Center for Environmental Prediction (NCEP) CFS version 2 (CFSv2) coupled atmosphere–ocean seasonal climate prediction systems. Sys4 shows a cold bias in the equatorial Pacific but a warm bias is found in the North Pacific and part of the North Atlantic. The CFSv2 has strong warm bias from the cold tongue region of the eastern Pacific to the equatorial central Pacific and cold bias in broad areas over the North Pacific and the North Atlantic. A cold bias in the Southern Hemisphere is common in both reforecasts. In addition, excessive precipitation is found in the equatorial Pacific, the equatorial Indian Ocean and the western Pacific in Sys4, and in the South Pacific, the southern Indian Ocean and the western Pacific in CFSv2. A dry bias is found for both modeling systems over South America and northern Australia. The mean prediction skill of 2 meter temperature (2mT) and precipitation anomalies are greater over the tropics than the extra-tropics and also greater over ocean than land. The prediction skill of tropical 2mT and precipitation is greater in strong El Nino Southern Oscillation (ENSO) winters than in weak ENSO winters. Both models predict the year-to-year ENSO variation quite accurately, although sea surface temperature trend bias in CFSv2 over the tropical Pacific results in lower prediction skill for the CFSv2 relative to the Sys4. Both models capture the main ENSO teleconnection pattern of strong anomalies over the tropics, the North Pacific and the North America. However, both models have difficulty in forecasting the year-to-year winter temperature variability over the US and northern Europe. 相似文献