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1.
In this work, we examined the carbonate parameters, i.e. total alkalinity (TA), pH, and partial pressure of CO2 (pCO2), and the air–sea CO2 flux (FCO2) in the continental shelves of the southern Yellow Sea (SYS) and East China Sea (ECS), based on two field surveys conducted in April and August of 2011. Surface pCO2 showed significant spatial variations, ranging from 246 to 686 µatm in spring (average ± standard deviation = 379 ± 95 µatm) and from 178 to 680 µatm in summer (384 ± 114 µatm). During the spring cruise, the central SYS (pCO2 < 240 µatm) and the Changjiang estuary (pCO2 < 300 µatm) were under-saturated with CO2, while the southern SYS and the southwestern ECS were supersaturated (pCO2 = 420–680 µatm). In summer, however, the CO2-supersaturated waters (pCO2 = 380–680 µatm) occupied a relatively wide area, including the nearshore of the SYS and the Changjiang estuary, whereas pCO2-deficient water (pCO2 = 220–380 µatm) was observed only at the offshore ECS. In general, the entire SYS and ECS area behaved as a sustained CO2 sink, with average FCO2 of ?3.9 and ?2.1 mmol m?2 d?1 in spring and summer, respectively. Phytoplankton production was the driving force for CO2 absorption, especially during the spring cruise. In addition, we found that typical water mixing processes and decomposition of terrestrial material were responsible for the release of CO2 in three turbidity maximum regions.  相似文献   

2.
We examined the carbonate system, mainly the partial pressure of CO2 (pCO2), dissolved inorganic carbon (DIC) and total alkalinity (TAlk) in the Changjiang (Yangtze) River Estuary based on four field surveys conducted in Sep.–Oct. 2005, Dec. 2005, Jan. 2006 and Apr. 2006. Together with our reported pCO2 data collected in Aug.–Sep. 2003, this study provides, for the first time, a full seasonal coverage with regards to CO2 outgassing fluxes in this world major river–estuarine system. Surface pCO2 ranged 650–1440 μatm in the upper reach of the Changjiang River Estuary, 1000–4600 μatm in the Huangpujiang River, an urbanized and major tributary of the Changjiang downstream which was characterized by a very high respiration rate, and 200–1000 μatm in the estuarine mixing zone. Both DIC and TAlk overall behaved conservatively during the estuarine mixing, and the seasonal coverage of these carbonate parameters allowed us to estimate the annual DIC export flux from the Changjiang River as ∼ 1.54 × 1012 mol. The highly polluted Huangpujiang River appeared to have a significant impact on DIC, TAlk and pCO2 in the lower reaches of the inner estuary. CO2 emission flux from the main stream of the Changjiang Estuary was at a low level of 15.5–34.2 mol m− 2 yr− 1. Including the Huangpujiang River and the adjacent Shanghai inland waters, CO2 degassing flux from the Changjiang Estuary may have represented only 2.0%–4.6% of the DIC exported from the Changjiang River into the East China Sea.  相似文献   

3.
基于2010 年11 月对长江口外东海中北部海域的综合调查, 系统研究了该海域的无机碳体系参数的分布特征、海?气界面二氧化碳通量及其影响因素。研究结果表明, 该海域秋季溶解无机碳(DIC)高值区主要出现在调查海域东北部及长江口附近海域, 而调查海域南部DIC 含量较少且变化平缓, 其主要是受台湾东部流向东北方向的黑潮支流及长江冲淡水的影响; 表层海水CO2分压(pCO2)值变化范围为40.8~63.5 Pa, 呈现沿黑潮支流流入方向由东南向西北逐渐增高的趋势。秋季表层海水pCO2与温度(T)、盐度(S)有较好的负相关性, 说明海水温度升高和盐度增加, pCO2降低, 反之亦然。另外, 通过估算得出, 秋季CO2海-气交换通量为2.69~33.66 mmol/(m2·d), 平均值为(14.35 ± 7.06 )mmol/(m2·d),其在长江口邻近海域相对较大, 而在调查海域南部相对较小; 2010 年秋季水体向大气释放CO2的量(以碳计)为(2.35 ± 1.16)×104 t/d, 是大气CO2较强的源, 说明东海中北部海域秋季总体上是CO2的源。  相似文献   

4.
近50 a来杭州湾冲淤变化规律与机制研究   总被引:6,自引:4,他引:2  
使用杭州湾1959-2010年的水下地形图, 结合过去数十年来长江入海水沙量和钱塘江河口段冲淤变化状况, 分析了近50 a来杭州湾在长江入海泥沙量锐减和治江围涂等人类活动作用下的冲淤变化规律及其物理机理。结果表明, 乍浦以上区域近50 a来处于较显著的淤积状态, 且有自上向下发展的趋势, 这种淤积主要是由于钱塘江河口治江缩窄工程所引起的;湾内地形发生了局部调整, 部分小型潮流槽脊系统趋于消亡, 地形趋于平坦化, 湾口北部2003年以后有转淤为冲的趋势, 这与长江入海泥沙量锐减和该区域围垦工程等因素有关;1959-2003和2003-2010年两个时段, 湾内泥沙淤积的年平均值分别为0.91×108和1.66×108 m3。对于整个钱塘江河口系统而言, 即自杭州湾湾口至钱塘江河口段的闸口断面, 长江入海泥沙量减少所产生的影响尚不明显, 2003年以后泥沙淤积速率甚至有所上升。杭州湾近50 a的冲淤变化是人为强烈干预下的大流域-河口系统响应与中小流域-河口系统响应的调整结果。  相似文献   

5.
《Marine Chemistry》2005,93(1):21-32
We investigated distributions of surface water CO2 partial pressure (pCO2), dissolved oxygen (DO) and associated carbonate parameters in the Pearl River estuary, a large subtropical estuary under increasingly anthropogenic pressure in China, in the summer of 2000 and late spring of 2001. pCO2 levels, measured underway using a continuous measurement system, were high during both seasons, with levels of >4000 μatm at salinity <0.5. pCO2 distribution overall mirrored DO across the salinity gradient. Using the linear relationship between excess CO2 and apparent oxygen utilization (AOU) in surface water, we conclude that aerobic respiration is the most important process in maintaining such high pCO2 measured upstream. The material being respired is likely in a close association with the organic pollutants discharged into the system. Based on the measured excess CO2 vs. AOU plots, we estimate that the upper limit of pCO2 should be ∼7000 μatm in the Pearl River estuary assuming that CO2 was produced solely by aerobic respiration.  相似文献   

6.
根据2004年8月在长江口、杭州湾附近海域获得的调查资料对表层水中Ph值、总碱度和溶解无机碳的分布特征及其与环境参数的关系进行了研究,并由此得到了溶解无机碳的组成情况.结果表明,HCO3-、CO23-;和CO2(T)占溶解无机碳浓度百分比分别为80.33%~97.75%、0.61%~19.42%和0.25%~2.34%,平均值分别为(93.28±3.68)%、(5.58±4.03)%和(1.14±0.43)%.水文、浮游植物等对各参数的分布具有重要影响,但对不同参数的影响程度不同.  相似文献   

7.
The distribution of the fugacity of CO2 ( $ f_{{{\text{CO}}_{ 2} }} $ ) and air–sea CO2 exchange were comprehensively investigated in the outer estuary to offshore shallow water region (lying adjacent to the Sundarban mangrove forest) covering an area of ~2,000 km2 in the northern Bay of Bengal during the winter. A total of ten sampling surveys were conducted between 1 December, 2011 and 21 February, 2012. Physico-chemical variables like sea surface temperature (SST), salinity, pH, total alkalinity (TAlk), dissolved inorganic carbon (DIC) and in vivo chlorophyll-a along with atmospheric variables were measured in order to study their role in controlling the CO2 flux. Surface water $ f_{{{\text{CO}}_{ 2} }} $ ranged between 111 and 459 μatm which correlated significantly with the SST (r = 0.71, p < 0.001, n = 62). Neither DIC nor TAlk showed any linear relationship with varying salinity in the estuarine mixing zone, demonstrating the significant presence of non-carbonate alkalinity. An overall net biological control on the surface $ f_{{{\text{CO}}_{ 2} }} $ distribution was established during the study, although no significant correlation was found between chlorophyll-a and $ f_{{{\text{CO}}_{ 2} }} $ (water). The shallow water region studied was mostly under-saturated with CO2 and acted as a sink for atmospheric CO2. The difference between surface water and atmospheric $ f_{{{\text{CO}}_{ 2} }} $ ( $ \Updelta f_{{{\text{CO}}_{ 2} }} $ ) ranged from ?274 to 69 μatm, with an average seaward flux of ?10.5 ± 12.6 μmol m?2 h?1. The $ \Updelta f_{{{\text{CO}}_{ 2} }} $ and hence the air–sea CO2 exchange was primarily regulated by the variation in sea surface $ f_{{{\text{CO}}_{ 2} }} $ , since atmospheric $ f_{{{\text{CO}}_{ 2} }} $ varied over a comparatively narrow range of 361.23–399.05 μatm.  相似文献   

8.
厘清河口-陆架连续体的碳源/汇机制是认识海洋在“碳中和”中作用的重要基础。本研究基于2017年春季长江口-东海的走航CO2分压(pCO2)及温、盐等资料,分区域阐述春季长江口-东海连续体pCO2的空间分布格局,半定量解析水团分配、有机质生产及降解等过程对pCO2的控制作用。结果表明:水团来源是决定春季长江口-东海连续体pCO2分布及碳源/汇格局的主要因素,而有机质生产或者降解可强烈影响长江口-东海连续体碳源/汇格局。春季长江口门及浙江沿岸受长江径流影响而具有较高的pCO2,碳源强度可达5.36mmol·m-2·d-1;研究区域北部和东部分别受冲淡水及黑潮表层水的影响,表现为大气碳汇,北部碳汇强度为-15.44mmol·m-2·d-1。2017年春季研究区域平均碳通量为-6.73mmol·m-2·d-1。端元混合模型结果表明陆源有机质降解导致河口pCO2增加了约200μatm,促使春季河口由大气CO2的弱汇转变为碳源;陆架区域在仅考虑水团分配下同样为碳汇,而藻华过程进一步降低了pCO2(下降144μatm),增强了其碳汇能力。  相似文献   

9.
Marginal seas play important roles in regulating the global carbon budget, but there are great uncertainties in estimating carbon sources and sinks in the continental margins. A Pacific basin-wide physical-biogeochemical model is used to estimate primary productivity and air-sea CO_2 flux in the South China Sea(SCS), the East China Sea(ECS), and the Yellow Sea(YS). The model is forced with daily air-sea fluxes which are derived from the NCEP2 reanalysis from 1982 to 2005. During the period of time, the modeled monthly-mean air-sea CO_2 fluxes in these three marginal seas altered from an atmospheric carbon sink in winter to a source in summer. On annualmean basis, the SCS acts as a source of carbon to the atmosphere(16 Tg/a, calculated by carbon, released to the atmosphere), and the ECS and the YS are sinks for atmospheric carbon(–6.73 Tg/a and –5.23 Tg/a, respectively,absorbed by the ocean). The model results suggest that the sea surface temperature(SST) controls the spatial and temporal variations of the oceanic pCO_2 in the SCS and ECS, and biological removal of carbon plays a compensating role in modulating the variability of the oceanic pCO_2 and determining its strength in each sea,especially in the ECS and the SCS. However, the biological activity is the dominating factor for controlling the oceanic pCO_2 in the YS. The modeled depth-integrated primary production(IPP) over the euphotic zone shows seasonal variation features with annual-mean values of 293, 297, and 315 mg/(m~2·d) in the SCS, the ECS, and the YS, respectively. The model-integrated annual-mean new production(uptake of nitrate) values, as in carbon units, are 103, 109, and 139 mg/(m~2·d), which yield the f-ratios of 0.35, 0.37, and 0.45 for the SCS, the ECS, and the YS, respectively. Compared to the productivity in the ECS and the YS, the seasonal variation of biological productivity in the SCS is rather weak. The atmospheric pCO_2 increases from 1982 to 2005, which is consistent with the anthropogenic CO_2 input to the atmosphere. The oceanic pCO_2 increases in responses to the atmospheric pCO_2 that drives air-sea CO_2 flux in the model. The modeled increase rate of oceanic pCO_2 is0.91 μatm/a in the YS, 1.04 μatm/a in the ECS, and 1.66 μatm/a in the SCS, respectively.  相似文献   

10.
This article presents the results of long-term studies of the dynamics of carbonate parameters and air–sea carbon dioxide fluxes on the Chukchi Sea shelf during the summer. As a result of the interaction of physical and biological factors, the surface waters on the west of Chukchi Sea were undersaturated with carbon dioxide when compared with atmospheric air; the partial pressure of CO2 varied in the range from 134 to 359 μatm. The average value of CO2 flux in the Chukchi Sea per unit area varied in the range from–2.4 to–22.0 mmol /(m2 day), which is significantly higher than the average value of CO2 flux in the World Ocean. It has been estimated that the minimal mass of C absorbed by the surface of Chukchi Sea from the atmosphere during ice-free season is 13 × 1012 g; a great part of this carbon is transported to the deeper layers of sea and isolated from the atmosphere for a long period of time. The studies of the carbonate system of the Chukchi Sea, especially of its western part, will provide some new data on the fluxes of carbon dioxide in the Arctic Ocean and their changes. Our analysis can be used for an interpretation of the satellite assessment of CO2 fluxes and dissolved CO2 distribution in the upper layers of the ocean.  相似文献   

11.
于2009年4月15~23日在长江口及其邻近海域进行了32个站位的浮游动物生态调查,分析了浮游动物的种类组成、优势种、丰度和生物量的空间分布,并利用PRIMER生物统计学软件中的PCA、BIOENV和RELATE程序分析了浮游动物与环境因子的关系.共发现浮游动物成体72种,浮游幼虫9种,合计种类数为81.中华哲水蚤(C...  相似文献   

12.
杭州湾作为典型的高浑浊度海湾,对其水体碳酸盐体系分布特征的研究相对较少。本文基于两个夏季航次(2018年和2019年)获取的调查资料,阐述夏季杭州湾水体中碳酸盐体系参数的空间分布特征,并进一步分析影响溶解无机碳偏离保守混合作用的主要过程及相对贡献。数据结果表明,杭州湾内表层溶解无机碳浓度与总碱度的变化范围分别为1 553~1 964 μmol/kg和1 577~2 101 μmol/kg,略低于长江口(1 407~2 110 μmol/kg和1 752~2 274 μmol/kg),溶解无机碳浓度和总碱度的空间分布受控于淡水与外海水混合的影响,在潮汐作用下,总体呈现出湾内低,向湾外逐渐升高的趋势。影响表层溶解无机碳非保守混合分布的主要过程中,海?气交换降低溶解无机碳浓度,呼吸作用增加溶解无机碳浓度,两个过程对溶解无机碳浓度变化量的贡献分别为(?42.3±11.7)%与(34.2±14.3)%,净效应呈现为相对平衡的状态。通过计算获得表层海水pCO2的平均值为799 μatm (675~932 μatm),海湾总体表现为大气CO2的源。此外,湾内海水碳酸盐缓冲因子的范围为12.8~23.8,对CO2的缓冲能力弱于邻近东海海水(缓冲因子平均值约为11.9),指示其与外部水体的交换可能会降低附近海域的酸化缓冲能力。相对其他河口/海湾而言,杭州湾内高浊度与强潮汐的特点使其湾内水体的碳酸盐体系分布特征具有区域特殊性。  相似文献   

13.
The seasonal variability of the carbon dioxide (CO2) system in the Southern Ocean, south of 50°S, is analysed from observations obtained in January and August 2000 during OISO cruises conducted in the Indian Antarctic sector. In the seasonal ice zone, SIZ (south of 58°S), surface ocean CO2 concentrations are well below equilibrium during austral summer. During this season, when sea-ice is not obstructing gas exchange at the air–sea interface, the oceanic CO2 sink ranges from −2 to −4 mmol/m2/d in the SIZ. In the permanent open ocean zone, POOZ (50–58°S), surface oceanic fugacity fCO2 increases from summer to winter. The seasonal fCO2 variations (from 10 to 30 μatm) are relatively low compared to seasonal amplitudes observed in the subtropics or the subantarctic zones. However, these variations in the POOZ are large enough to cross the atmospheric level from summer to winter. Therefore, this region is neither a permanent CO2 sink nor a permanent CO2 source. In the POOZ, air–sea CO2 fluxes calculated from observations are about −1.1 mmol/m2/d in January (a small sink) and 2.5 mmol/m2/d in August (a source). These estimates obtained for only two periods of the year need to be extrapolated on a monthly scale in order to calculate an integrated air–sea CO2 flux on an annual basis. For doing this, we use a biogeochemical model that creates annual cycles for nitrate, inorganic carbon, total alkalinity and fCO2. The changing pattern of ocean CO2 summer sink and winter source is well reproduced by the model. It is controlled mainly by the balance between summer primary production and winter deep vertical mixing. In the POOZ, the annual air–sea CO2 flux is about −0.5 mol/m2/yr, which is small compared to previous estimates based on oceanic observations but comparable to the small CO2 sink deduced from atmospheric inverse methods. For reducing the uncertainties attached to the global ocean CO2 sink south of the Polar Front the regional results presented here should be synthetized with historical and new observations, especially during winter, in other sectors of the Southern Ocean.  相似文献   

14.
Based on the historical evolution of the Hangzhou Bay, by making use of the conclusions made by the previous research workers and the integration of concrete data, five distinct impact indicators of the sediment from the Changjiang Estuary and the East China Sea to the Hangzhou Bay are summarized. Numerical calculation and analysis indicate that the scouring and deposition of seabed in the Hangzhou Bay are subject to the direct impact of the evolution of the Changjiang Estuary, and the growth and decline and the direction of the sandy bar at Nanhuizui give traces to the sediment transport between the Changjiang Estuary and the Hangzhou Bay. The transport of sediment from the Changjiang Estuary to the Hangzhou Bay occurs mainly in winter and spring seasons and the increase of the Changjiang River runoff and the decrease of sediment charge have caused scouring in the northern coast of the Hangzhou Bay and the seabed erosion along the frontal margin of the Changjiang River Delta.  相似文献   

15.
Based on the historical evolution of the Hangzhou Bay, by making use of the conclusions made by the previous research workers and the integration of concrete data, five distinct impact indicators of the sediment from the Changjiang Estuary and the East China Sea to the Hangzhou Bay are summarized. Numerical calculation and analysis indicate that the scouring and deposition of seabed in the Hangzhou Bay are subject to the direct impact of the evolution of the Changjiang Estuary, and the growth and decline and the direction of the sandy bar at Nanhuizui give traces to the sediment transport between the Changjiang Estuary and the Hangzhou Bay. The transport of sediment from the Changjiang Estuary to the Hangzhou Bay occurs mainly in winter and spring seasons and the increase of the Changjiang River runoff and the decrease of sediment charge have caused scouring in the northern coast of the Hangzhou Bay and the seabed erosion along the frontal margin of the Changjiang River Delta.  相似文献   

16.
彭鹏飞  马媛  史荣君  王迪  许欣  颜彬 《海洋科学》2022,46(10):140-149
根据2018年7月、11月和2019年1月、4月对广东考洲洋牡蛎养殖海域进行4个季节调查获得的pH、溶解无机碳(DIC)、水温、盐度、溶解氧(DO)及叶绿素a(Chla)等数据,估算该区域表层海水溶解无机碳体系各分量的浓度、初级生产力(PP)、表层海水CO2分压[p(CO2)]和海-气界面CO2交换通量(FCO2),分析牡蛎养殖活动对养殖区碳循环的影响。结果表明:牡蛎养殖区表层海水中Chla、DIC、HCO3PP显著低于非养殖区;养殖淡季表层海水中pH、DO、DIC、HCO3、和CO32–显著大于养殖旺季,养殖旺季的p(CO2)和FCO2显著大于养殖淡季。牡蛎养殖区表层海水夏季、秋季、冬季和春季的海-气界面CO2交换通量FCO2平均值分别是(42.04±9.56)、(276.14±52.55)、(–11.59±18.15)和(–13.02±6.71)mmol/(m2·d),冬季各站位FCO2值离散度较大,其中位数是–10.73mmol/(m2·d)。在全年尺度,表层海水p(CO2)及FCO2与水温呈显著正相关,与盐度呈显著负相关。在非养殖区,浮游植物光合作用可能对影响表层海水p(CO2)及FCO2起主导作用。养殖牡蛎钙化、呼吸作用等生理因素释放的CO2对表层海水p(CO2)及FCO2未产生显著影响。考洲洋养殖海域养殖旺季为CO2的源,养殖淡季整体为CO2的弱汇。  相似文献   

17.
Multiple biotic and abiotic drivers regulate the balance between CO2 assimilation and release in surface waters. In the present study, we compared in situ measurements of plankton carbon metabolism (primary production and respiration) to calculated air–water CO2 fluxes (based on abiotic parameters) during 1 year (2008) in a hypereutrophic tropical estuary (Recife Harbor, NE Brazil – 08°03′S, 34°52′W) to test the hypothesis that high productivity leads to a net CO2 flux from the atmosphere. The calculated CO2 fluxes through the air–water interface (FCO2) were negative throughout the year (FCO2: –2 to –9 mmol C·m?2·day?1), indicating that Recife Harbor is an atmospheric CO2 sink. Respiration rates of the plankton community ranged from 2 to 45 mmol C·m?2·hr?1. Gross primary production ranged from 0.2 to 281 mmol C·m?2·hr?1, exceeding respiration during most of the year (net autotrophy), except for the end of the wet season, when the water column was net heterotrophic. The present results highlight the importance of including eutrophic tropical shallow estuaries in global air–water CO2 flux studies, in order to better understand their role as a sink of atmospheric CO2.  相似文献   

18.
白令海BR断面海-气CO2通量及其参数特征   总被引:1,自引:0,他引:1  
通过对2008年夏季白令海大气和海水pCO2连续观测资料,结合BR断面上站位水体垂直采样测量,对白令海不同海区pCO2的分布特征及其与理化参数的关系进行了初步研究,结果表明,将白令海划分为4个具有不同CO2吸收能力的海区,其中陆坡流区碳通量高达-18.72 mmol/(m2·d),是海盆北区的近2倍,比海盆南区高一个量...  相似文献   

19.
The third Chinese National Arctic Research Expedition(CHINARE) was conducted in the summer of 2008.During the survey,the surface seawater partial pressure of CO_2(pCO_2) was measured,and sea water samples were collected for CO_2 measurement in the Canada Basin.The distribution of pCO_2 in the Canada Basin was determined,the influencing factors were addressed,and the air-sea CO_2 flux in the Canada Basin was evaluated.The Canada Basin was divided into three regions:the ice-free zone(south of 77°N),the partially ice-covered zone(77°–80°N),and the heavily ice-covered zone(north of 80°N).In the ice-free zone,pCO_2 was high(320 to 368μatm,1 μatm=0.101 325 Pa),primarily due to rapid equilibration with atmospheric CO_2 over a short time.In the partially ice-covered zone,the surface pCO_2 was relatively low(250 to 270 μatm) due to ice-edge blooms and icemelt water dilution.In the heavily ice-covered zone,the seawater pCO_2 varied between 270 and 300 μatm due to biological CO_2 removal,the transportation of low pCO_2 water northward,and heavy ice cover.The surface seawater pCO_2 during the survey was undersaturated with respect to the atmosphere in the Canada Basin,and it was a net sink for atmospheric CO_2.The summertime net CO_2 uptake of the ice-free zone,the partially ice-covered zone and the heavily ice-covered zone was(4.14±1.08),(1.79±0.19),and(0.57±0.03) Tg/a(calculated by carbon,1Tg=10~(12) g),respectively.Overall,the net CO_2 sink of the Canada Basin in the summer of 2008 was(6.5±1.3) Tg/a,which accounted for 4%–10% of the Arctic Ocean CO_2 sink.  相似文献   

20.
东海沿岸海域表层海水酸化趋势及影响因素研究   总被引:1,自引:0,他引:1  
根据2002—2011年东海沿岸海域(4个区域,16个站位)春、夏、秋三个季节的表层海水pH、温度、盐度和叶绿素a等监测资料,对该海域pH的年际时空变化及其影响因素进行了探讨。结果表明,东海沿岸海域表层海水十年间pH变化趋势存在明显的季节和区域差异,共有10个站点表层海水pH呈下降趋势,主要集中于长江口和杭州湾海域,而三门湾和椒江口海域的酸化则不明显。环境因子相关性分析显示,杭州湾海域夏季表层海水的pH与叶绿素a浓度呈极显著正相关,其它海域两者间未显示出显著的相关性;杭州湾海域的pH与海表温度也存在显著的相关性,但季节不同趋势不同,呈现出春季正相关而夏季负相关的特征;pH与盐度的关系在各海域表现得更加明显,长江口、杭州湾和三门湾三个调查海区海水的pH变化与盐度都存在显著的正相关。总之,在10年的连续监测内东海沿岸海域存在一定程度的酸化趋势,其影响机制还需进一步研究。  相似文献   

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