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波 《吉林大学学报(地球科学版)》2014,(2):645-652
计算小流域非点源氮素流失负荷,并以此开展丹江水源区水体污染源解析和控制研究。基于流域断面及小区监测试验,利用平均浓度法对鹦鹉沟流域氮素年均流失模数和不同土地利用类型的非点源污染负荷进行计算分析。结果表明:径流水质中主要是总氮质量浓度超标,且硝氮质量浓度均大于氨氮质量浓度;当坡耕地坡度大于25°时,氮素流失严重,水质极差;农村生产生活污染物排放对水质有很大影响,从断面1到把口站,硝氮质量浓度和总氮质量浓度增加较大;农地、草地和林地的总氮年均径流流失模数分别为0.36、0.22和0.09t/(a·km2);流域出口非点源污染物氨氮、硝氮和总氮的平均质量浓度分别为0.17,4.71和7.55mg/L,点源污染物氨氮、硝氮和总氮的平均质量浓度分别为0.20、2.12和4.08mg/L。总体来说,鹦鹉沟流域径流中总氮的流失模数为0.89t/(a·km2),总氮是影响水质的主要污染物,需加强对坡耕地氮素流失和农村生活垃圾的治理。 相似文献
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以太湖流域雪堰镇为例,通过2009年3月~2010年2月连续12个月及两场次降雨事件的水质监测进行分析,研究不同河流、月份、区域、汛情、土地利用类型下氮素流失规律及形态特性,分析降雨过程中不同尺度3个流域(上涧村、龙泉河、雪堰镇)氮流失特征和不同河段氮流失规律。研究结果表明,雪堰镇氮素为劣Ⅴ类,非汛期污染比汛期严重,变化幅度大,不稳定,氮以溶解态为主,溶解态氮以硝氮为主;镇区硝氮浓度较非镇区低,氨氮比非镇区高,坑塘水面氮流失最严重,有林地(乔木较多)氮流失最少,茶园硝氮占溶解态氮百分比最高,果园氨氮占溶解态氮百分比最高;降雨前期未产流前氮素流失稳定,产流后流失越来越大,不同河段氮沿程变化基本稳定。 相似文献
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降雨强度对植生滤带削减农业面源污染效率的研究 总被引：1，自引：0，他引：1
《地下水》2019,(6)
植生滤带可有效减少农业面源磷污染,并且可以保持水土,被认为是削减农业面源污染最有效的管理措施,并广泛应用于农业面源污染的治理。降雨强度是决定植生滤带拦蓄沉积物和滞留养分的重要因素。本研究选择常见降雨强度范围,根据某中下游流域实际情况设计出模拟实验装置,确定不同降雨强度条件下植生滤带对农业面源污染防治的效果,为某中下游植生滤带的设计和建设提供借鉴依据。结果表明:降雨强度对TP的削减效率的影响主要是通过改变TP的载体即地表径流的流速来实现的,降雨强度越大,径流流速越大,从而导致TP在植生滤带中被吸附的时间和效率降低,导致TP削减效率减少。 相似文献
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云南滇池流域西芹种植区不同施肥条件下的地下水环境氮素污染 总被引：1，自引：1，他引：0
通过野外田间实验,研究了高量施肥处理、低量施肥处理、不施肥处理以及空白对照裸地等不同施肥处理条件下土壤水中各种形态氮的时空分布情况,探讨了地下水环境中氮素在不同施肥处理条件下的迁移转化特征.结果表明,在各种处理条件下,土壤水中硝态氮质量浓度随深度的增大而减小,而亚硝态氮与铵态氮质量浓度在剖面上的变化幅度较大,这种变化主要受土壤水氧化还原电位的影响.硝态氮随时间的变化趋势在4个处理区表现各异:在高量施肥处理区,各层位的土壤水中硝态氮质量浓度总体上呈增大趋势;在低量施肥处理区,硝态氮受作物生长和灌溉的影响呈拍岸浪式向下迁移;在不施肥处理区和空白对照裸地处理区,由于表层土壤中硝态氮背景值较高(0～30 cm处土壤硝态氮平均质量分数达到15.59 g/kg),灌溉水的下渗也导致硝态氮向下迁移.高量施肥处理区和空白对照裸地处理区土壤水的对比表明,施肥可促进0.6～1.5 m深处土壤的反硝化作用,从而增大这些层位土壤水中亚硝态氮和铵态氮的质量浓度. 相似文献
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根据农田坡面氮、磷流失的主要过程,建立了基于次降雨事件的坡面氮、磷迁移模型。模型采用改进的Green-Ampt方程和运动波方程计算下渗与坡面流,土壤侵蚀采用修改的欧洲土壤侵蚀模型计算,用考虑了侵蚀影响与扩散作用的迁移模型计算坡面氮、磷迁移过程,采用一维对流扩散方程计算氮、磷在土壤中的迁移过程。利用室内人工降雨资料对模型进行了率定及验证。结果表明,模型可以较好地模拟地表径流中氮、磷浓度,率定期与验证期模型效率系数均在0.89以上。根据坡地氮、磷流失机理,分析了降雨强度与地表坡度对坡面径流中氮、磷浓度的影响。 相似文献
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干湿交替的回灌方法常被用于解决地面回灌补给地下水的堵塞问题。研究干湿交替条件下地面回灌对地下水的影响对于指导再生水回灌地下水具有重要实际意义。通过室内土柱模拟实验,在入渗强度为10.5 mm/h的条件下,日均进水量3 888 mL;用干湿交替的地面回灌模式持续运行136 d,累计灌入氨氮含量为5 mg/L的模拟再生水23 894 L,研究包气带土柱对氨氮的去除效果及氮素在包气带中的迁移转化规律。研究表明,充分利用包气带的好氧、兼氧和厌氧环境,生物脱氮是地下水回灌过程中脱氮的主要途径。包气带对氨氮的去除机理主要为土壤对氨氮的吸附作用和微生物的降解作用。回灌过程中累积在土颗粒表面的氨氮在干期发生硝化作用,干湿交替会加强氮素在包气带的迁移转化,导致干期后的回灌初期大量硝态氮迁移到饱和带地下水中。 相似文献
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喀斯特坡地壤中流与地表径流并存,共同驱动了土壤关键生源物质的迁移,造成该区土壤生产力下降、地下水污染。为揭示喀斯特坡地土壤碳氮流失途径及其水文驱动机制,本研究以喀斯特坡地径流微区(2 m×1.2 m)为研究对象,分析了火烧、轻度砍伐、重度砍伐、人工林、耕地、牧草6种不同土地利用方式对土壤碳氮流失途径、形态及通量的影响。结果表明:降雨是土壤碳氮流失的主要驱动因子,降雨产流阈值为16 mm,55 mm时达到产流峰值。各土地利用方式仅在暴雨下有显著差异,其中,人工林的土壤碳氮流失量较大,而重度砍伐的流失量较小。土地利用方式不改变土壤碳氮的流失途径,各土地利用方式均以地表流失为主(51.29%～75.15%),壤中流为辅,其中壤中流主要通过A层流失(65.20%-89.12%)。氮素流失形态以NO3--N为主(45.84%～56.49%)。研究结果可为揭示喀斯特坡地生源物质流失过程及其水文驱动机制、研发水土流失与面源污染阻控技术提供参考。 相似文献
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Development of regional pollution export coefficients based on artificial rainfall experiments and its application in North China 总被引：1，自引：1，他引：0
R. Liu W. Yu J. Shi J. Wang F. Xu Z. Shen 《International Journal of Environmental Science and Technology》2017,14(4):823-832
The Export Coefficient Model (ECM) has been widely used to estimate nonpoint source (NPS) pollution loads due to its ease of application. Accurate pollution export coefficients are crucial for reducing uncertainties in load estimation. By integrating artificial simulated rainfall experiments with field survey data, we have developed a new method that estimates regional pollution export coefficients. Results showed that the export coefficients calculated using this new method accurately express the regional rainfall–runoff characteristics, as the simulation precision of this method had grown by 30% than the results with traditional ECM and export coefficients which surveyed from the literature. Based on the calculated regional pollutant export coefficient, the annual loads of TN and TP in the plains area of the Baiyangdian basin in 2010 were 25,967.13 t and 4349.29 t, respectively. Among different types of sources, rural livestock had the greatest contribution (over 60%), whereas rural domestic waste represented the smallest contribution (approximately 10%). Of the different sources, pigs contributed almost half of all NPS pollution from livestock, rural residential areas were the main land use pollution source, and rural living garbage was the main source of rural domestic waste. Spatially, NPS was mainly distributed in the Zhulong and Juma watersheds. Other watersheds only contributed approximately 5% NPS per watershed. However, the per-area loads of these lower load watersheds were larger or nearly equal to that of the Zhulong watershed. Therefore, the lower load watersheds should be addressed for the control of NPS pollution. 相似文献
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A comparative study on nitrogen-concentration dynamics in surface water in a heterogeneous landscape 总被引：7，自引：0，他引：7
Liding Chen Bojie Fu Shurong Zhang Jun Qiu Xudong Guo Fulin Yang 《Environmental Geology》2002,42(4):424-432
With point-source pollution controlled effectively, nonpoint-source pollution, especially that resulting from agricultural land, has become the main factor affecting surface water. Much attention has been focused on the impact of fertilizer and pesticide application, wastewater irrigation, and land management on pollutant transport. However, landscape pattern also plays an important role in pollutant transport and detention. Landscape types may be classified into two parts: "source" and "sink" landscapes, based on their functions in pollutant transport and detention. As a major contributor to eutrophication of waterbodies, nitrogen loss with runoff has received particular attention when studying nonpoint-source pollution. In this study, four watersheds in the upper parts of the Yuqiao Reservoir Basin, Zuihua, Hebei Province, China, were chosen in order to study the relationship between landscape pattern and nitrogen-concentration dynamics. The results indicate that (1) nitrogen concentration in surface water within different seasons in the rainfall-normal year is higher than that in the rainfall-deficit year and (2) the variation of nitrogen concentration within different seasons in the rainfall-deficit year is smaller compared with that in the rainfall-normal year in which two types of seasonal variation on nitrogen concentration are presented. The first variation occurs when nitrogen concentration is lowest in the dry season, and rises rapidly from the dry season to rainy season and then declines quickly from the rainy season to mean-flow season. This mainly occurs in those areas where most "source" landscapes are close to the monitored waterbody. The second variation occurs when nitrogen concentration is low in the dry season, increases rapidly in the rainy season but does not reach its peak value until the mean flow season. The second variation occurs in those areas where "source" landscape types are spread over the whole watershed. There is no clear relationship between watershed shape, relative importance of landscape types, and nitrogen concentration; however, the spatial distribution of "source" and "sink" landscape types in the watershed has a strong impact on the nitrogen concentration in surface water. 相似文献
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基于平均浓度法原理,根据黄河中游降雨径流特点,将年内过程分为汛期和非汛期两个阶段,同时将高含沙水流中的污染负荷分为水体中的溶解态污染负荷、泥沙吸附态负荷两部分,提出了多沙河流非点源污染负荷估算模型;根据黄河干流潼关断面1950-2006年实测水沙资料,结合水体、泥沙污染物浓度测定试验,分别计算了潼关断面2006年以及丰水年(P=25%)、平水年(P=50%)、枯水年(P=75%)3种不同代表年型下的非点源污染负荷.结果表明:黄河干流潼关断面年污染负荷以汛期为主,汛期污染负荷以非点源为主;非点源污染负荷中,硝酸盐氮、氨氮以溶解态为主,总磷以吸附态为主;潼关断面非点源污染负荷占全年负荷比例:丰水年时,硝酸盐氮占63.09%,氨氮占61.32%,总氮占87.17%、总磷占89.83%;枯水年时,硝酸盐氮占26.92%,氨氮占24.62%,总氮占67.60%、总磷占71.73%.2006年,硝酸盐氮、氨氮、总氮和总磷非点源污染负荷占全年比例依次为:17%、14%、15%和41%. 相似文献
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选取甘肃省境内11个典型小流域的水文站实测资料,在分析资料可靠性、一致性、代表性及暴雨洪水特性的基础上,综合利用水文学、数理统计学等理论和方法,建立了小流域最大暴雨量-暴雨历时关系模型、最大洪峰流量-流域特征关系模型。结果表明:各时段最大暴雨量较大值主要分布在泾河流域和嘉陵江流域东南部,较小值主要分布在渭河流域、洮河流域、嘉陵江流域的北峪河;绘制了各代表站最大暴雨量-暴雨历时关系曲线,嘉陵江流域以90min为转折点,其他流域均以180min为转折点,小于转折点时,暴雨量随暴雨历时增长而急剧增加,大于转折点后,变化趋于平缓稳定。重点选取危害较大、难以防范的330场次短历时暴雨洪水,建立各小流域暴雨洪水概化模型,短历时洪水发生时间很短,洪水起涨时间约2～5h,洪峰出现时间约5～7h。研究典型小流域水文要素变化规律,分析局地短历时暴雨洪水特性,并模拟其变化过程,对区域抗旱防汛减灾、水资源管理、小流域治理及生态环境保护具有重要意义。 相似文献
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氮氧同位素在河流硝酸盐研究中的应用 总被引：9，自引：0，他引：9
多年来，世界各地河流普遍存在硝酸盐污染问题。为控制河流的硝酸盐污染，确定河水中硝酸盐的来源以及研究氮的循环过程就显得尤为重要。由于在不同成因下，硝酸盐的δ15N和δ18O存在着较大差异，因此利用氮、氧同位素方法研究河流硝酸盐问题正日益受到国内外研究人员的重视。综述了用硝酸盐中氮、氧同位素来研究河流硝酸盐的不同来源(大气沉降、化肥、牲畜粪、土壤硝酸盐等)和示踪其地球化学循环过程，特别是反硝化过程，这两方面的研究进展，并对我国河流硝酸盐研究现状进行了讨论及提出今后的研究方向。 相似文献
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为了研究关中盆地浅层地下水氮污染对人体产生的潜在健康危害风险,在研究区采集和测试了232个水样,采用单因子污染指数法和健康风险评价模型对浅层地下水氮污染进行了评价。结果表明,在浅层地下水中硝态氮污染程度相对较重,呈面状分布;而铵态氮和亚硝态氮污染程度较轻,以点状存在。浅层地下水中硝态氮对人体健康的慢性毒害指数较高,高风险区占研究区面积的78.2%,主要分布在农业活动强烈的灌区和人口居住密集、工业相对发达的城镇区;硝态氮含量大于12.6mg/L的三类地下水对人体健康也是高风险的,即传统意义上可以饮用的三类水对人体健康并不都是安全的。上述成果对地下水资源管理和保护具有重要的参考价值。 相似文献
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Two numerical models, one for the vadose zone and the other for the aquifer system, are utilized to predict nitrate pollution
potential in groundwater. Transport by dispersion and convection of mobile species of nitrogen, ammonium ion exchange, first
order nitrogen transformations, and nitrogen plant uptake are included in the formulation for the vadose zone. Transport of
nitrate in the aquifer is assumed to be affected only by dispersion-convection phenomena. Justifications for one-dimensional
conceptualization of flow in the vadose zone and two-dimensional representation for the aquifer, under various field conditions,
are presented. To illustrate the concept, a simple hypothetical problem is solved. The approach presented here provides an
efficient means of long-term simulation of large-scale field problems. 相似文献
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Agricultural nonpoint source (NPS) pollution at the Three Gorges reservoir area in China has been increasingly recognized as a threat to aquatic environment in recent years due to the serious eutrophication problem. Adsorbed NPS pollution is one of the major forms of NPS pollution in mountainous regions, the essential of the adsorbed NPS pollution is soil loss. Thus, simple, highly sensitive and continuous methods are required to simulate and quantify sediments yield at watershed scales. It is imperative to construct an integrated model to estimate the sediment yield and adsorbed NPS pollution load. According to the characteristics of climate, hydrology, topography, geology, geomorphology and land use types in Three Gorges reservoir area, a GIS-based dynamic-integrated-distributed model of annual adsorbed NPS load was presented in view of impacts of the rainfall intensity, sediment delivery ratio (SDR) and land management, where the temporally dynamic-continuous model of annual sediment yield was established by modifying the revised Universal Soil Loss Equation (RUSLE), and the spatially integrated-distributed model of annual adsorbed NPS load was then developed via the correlation between sediment yield and adsorbed NPS load. Furthermore, a case study of the Jialing River basin in China was applied to validate the integrated model, the dynamic-distributed coupling among GIS technology, sediment yield model, and adsorbed NPS load model was achieved successfully. The simulation results demonstrate the following: (1) runoff and sediment are influenced greatly by rainfall intensity, SDR and vegetation cover; rainfall and land management show high sensitivities to the integrated model; the average annual adsorbed TN and TP pollution loads from 2006 to 2010 decreased by 76 and 74 % compared with the previous treatment (1990), respectively. (2) Spatio-temporal variations of adsorbed NPS nitrogen and phosphorus load are mainly related to different land use types and the background level of nutriments in topsoil; different land use types have different contribution rates; the largest contribution rates of adsorbed total nitrogen (TN, 58.9 %) and total phosphorus (TP, 53 %) loads are both from the dryland cropland. (3) The identification of critical source areas can help to implement the prevention and control measures aiming at the reduction of water environmental pollution. These results will provide useful and valuable information for decision makers and planners to take sustainable land use management and soil conservation measures for the control of sediment pollution in the Three Gorges reservoir area. The application of this model in the catchment shows that the integrated model may be used as a major tool to assess sediment yield risks and adsorbed NPS pollution load at mountainous watersheds. 相似文献
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桂林甑皮岩岩溶地下水硝酸盐来源与转化 总被引：1，自引：0，他引：1
峰林平原是人类活动和居住的密集区，也是岩溶地下水系统的主要径流、排泄地段，地下水资源丰富。随着城市化的发展，地下水硝酸盐污染问题日渐突出。为研究桂林甑皮岩岩溶地下水硝酸盐来源与转化，分别于2018年10月、2019年2月、3月和4月采集地下水样，利用常规水化学及氮氧同位素技术识别硝酸盐来源与转化。结果表明:甑皮岩地下水中NO3-浓度在0~19.523 mg?L-1，δ15N-NO3-和δ18O-NO3-分别在-0.17‰～45.12‰和-5.82‰~16.47‰。硝酸盐氮氧同位素数据表明，甑皮岩地下水硝酸盐来源主要为粪便及污废水，少量来自降雨中的NH4+和土壤有机氮。受岩溶介质不均一性的控制，甑皮岩地下水中NO3-浓度、δ15N-NO3-和δ18O-NO3-均表现出明显的空间变异性。甑皮岩地下水硝酸盐的转化过程复杂，受控于季节和岩溶介质不均一性，表现为旱季以反硝化为主，雨季则以硝化过程为主。厘清硝酸盐来源与转化为治理甑皮岩地下水硝酸盐污染提供一定的科学依据。 相似文献