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1.
青藏高原对全球气候变暖响应敏感,研究青藏高原近千年来环境演化过程、规律与驱动机制对预测其未来气候变化有重要意义。本文通过位于青藏高原东部的苦海沉积物总有机质相关指标(总有机碳(TOC)、总氮(TN)、总有机碳与总氮比值(TOC/TN)和总有机碳同位素(δ13Corg)的研究重建了该区域过去840年来环境演化过程。结果表明,苦海沉积物中的有机质主要来自于内源水生植物。由于暖期(冷期)时黄河上游径流量较高(低),苦海水位随之升高(降低),湖泊水动力增强(减弱),浅水区沉水植物对研究岩芯中的有机质贡献率提高(降低),导致沉积物TOC、TN、TOC/TN升高,δ13Corg值正(负)偏。人类活动导致的青藏高原近50年气候异常变暖可能是~1950 AD之后δ13Corg反映的黄河上游径流量变化与重建的中国温度记录之间的关系发生转变的原因。苦海沉积物δ13Corg记录与万象洞石笋δ18O记录和太阳总辐射强度记录变化特征的相似性说明青藏高原东部地区气候变化的控制因素为太阳辐射驱动下的季风降雨量变化。 相似文献
2.
为了解亚热带泥炭地碳氮磷含量的空间分布模式及其影响因素,在神农架大九湖泥炭地采集147份表层泥炭样品进行总有机碳含量(TOC)、总磷含量(TP)和总氮含量(TN)测试和理化参数分析,探究表层泥炭碳氮磷的空间分布特征及其控制因素。结果表明:大九湖表层泥炭TOC含量变化范围为3.51%~37.93%,TP含量变化范围为0.37~2.75 mg/g,TN含量变化范围为0.59~1.6mg/g。相关性分析表明:TOC含量与含水率(r=0.45,P<0.01)和TP含量(r=0.27,P<0.05)呈显著正相关,TP含量与干容重呈显著正相关(r=0.32,P<0.05),TN含量与各种理化参数的相关性均不显著。通过对比亚热带、热带、北方泥炭地的碳氮磷含量,发现相对于热带和北方泥炭地,亚热带泥炭地的TOC含量和TN含量更低,而TP含量更高。本研究为亚热带泥炭地的生态保护提供了关键的基础数据和参考。 相似文献
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4.
黑河中游不同土地利用类型下土壤碳储量及其空间变化 总被引：6，自引：1，他引：5
通过黑河中游不同土地利用类型下土壤碳密度、碳储量的研究表明:总有机碳(TOC)、活性有机碳(AOC)、非活性有机碳(NOC)碳密度、碳储量从小到大呈不同的变化趋势。其中,NOC与TOC碳密度从大到小的空间分布基本一致,而AOC与NOC、TOC的分布存在差异,说明土地利用类型变化对三类有机碳的影响不同。经计算得到,1m深度TOC、AOC、DOC碳库总量分别为94.72、45.12、49.60Tg,DOC碳库占TOC碳库的比例略高于AOC占TOC碳库的比例。分析发现,引入AOC和NOC指标,更能真实反映出有机碳与影响因素间关系。 相似文献
5.
北部湾北部滨海湿地水体和表层沉积物中营养元素分布与污染评价 总被引：2，自引：0，他引：2
2009年4～5月,对北部湾北部滨海湿地水体和表层沉积物进行了取样调查,研究水体中营养盐和表层沉积物中碳、氮和磷元素含量、分布及其影响因素,并在此基础上评价了滨海湿地水体富营养化水平和表层沉积物的污染状况.研究区水体中的溶解无机氮(dissolved inorganic nitrogen,DIN)、活性磷酸盐PO43-—P和化学需氧量(CODMn)平均含量分别为(211.84±37.44) μg/L、(11.01±12.11) μg/L和(0.92±0.32) mg/L;表层沉积物中总氮(TN)、总磷(TP)和总有机碳(TOC)的平均含量分别为(373±355) μg/g、(232.28±157.34) μg/g和(0.45±0.46)％.北部湾北部滨海湿地水体中的DIN含量和PO43-—P含量在茅尾海和廉州湾东部西场海区都很高,且水体富营养化比较严重,大规模的海水养殖可能是造成该现象的主要原因.研究区水体中CODMn含量空间分布呈近岸高、远岸低的特征.研究区铁山港顶部、南流江口、大风江口、钦江和茅岭江口较细的表层沉积物中的TN、TP和TOC含量较高.研究区表层沉积物的TOC/TN值分布表明,钦江口、钦州港区、防城港、企沙港区和珍珠湾东北部的沉积物有机质含量受到了强烈的陆源影响.根据加拿大安大略省环境质量评价标准,除了钦州湾顶部的龙门港区、大风江口中部和铁山港顶部西北角一小部分区域的表层沉积物中的TOC、TN和TP含量分别略高于1％、550μg/g和600μg/g,已被明显污染,而处于最低级别或严重危害级别,会对部分底栖生物产生影响外,其他绝大部分区域都属安全级别,为清洁或部分已被轻微污染. 相似文献
6.
对2003年7月-9月第二次北极科学考察期间在楚科奇海及其邻近海域所采集四个站位的沉积物柱状样的生源物质含量进行分析,并对沉积物TC、TOC、TN和TP的空间分布和垂直剖面分布进行讨论。四个站位的TC含量为0.89%-2.17%,TN含量为0.24-1.66mg/g,TP含量为0.15-0.96mg/g,其中C21、S11和M07的总碳中均以有机碳为主,分析结果证实了楚科奇海区是一个高效的有机碳“汇”区的结论。四个站位的有机质主要来源于海洋,其中P24站和M07站的TN随着TOC增加而增加,两者呈极显著的正相关关系,说明这两个站位所在区域的沉积物中氮和有机碳之间的关系密切,氮主要以有机氮形式存在。 相似文献
7.
排灌系统底泥特征是反映土地利用变化生态影响的重要途径,为此对内蒙古河套灌区永济灌域灌排系统底泥有机碳和总氮含量进行了系统研究。结果表明:灌域内永济给水干渠(简称永济干渠)与四号、五号排水干沟(简称四排干、五排干)表层底泥的有机质(OM)及总氮(TN)含量特征分布有所差异。其中均以五排干上游底泥中含量最高,OM与TN平均值分别为3.60%和0.35%,超出河套地区平均值的4.82倍和2.94倍;其底泥有机指数也达到重污染水平,富营养化程度较高;永济干渠底泥OM与TN含量最低,分别为1.41%和0.03%,属于清洁贫营养化级别;四排干底泥OM与TN含量介于五排干和永济干渠之间,其上游较为清洁,基本接近平均值,C/N平均在17左右。排干底泥有机质与总氮含量之间显著相关,y(TN)=0.141x(OM)-0.180(r=0.978;P<0.001)。 相似文献
8.
半干旱生态系统土壤呼吸(Rs)对氮添加的响应机制仍有待探索。本研究在中国半干旱草原设置不同氮添加水平(0、2、4、8、16、32 gN m-2 yr-1),测定土壤呼吸速率、土壤温湿度、微生物磷脂脂肪酸、土壤理化性质与地上生物量等指标,探讨氮添加对土壤呼吸及其温度敏感性(Q10)的影响。结果表明:氮添加显著增加了土壤可溶性有机碳(DOC)和无机氮(IN)的含量,降低了土壤pH值,对地上生物量(ABM)无显著影响。氮添加降低了磷脂脂肪酸(PLFAs)的总量,降低了真菌细菌比(F:B),提高了革兰氏阳性阴性菌比(G+:G–)。氮添加显著降低了土壤呼吸,N2、N4、N8、N16和N32处理下的土壤呼吸分别比对照N0变化了–2.58%、14.86%、22.62%、23.97%和19.87%,结构方程模型表明,氮添加通过降低PLFAs总量和改变微生物组成降低土壤呼吸。氮添加对温度敏感性(Q10)、土壤总有机碳(TOC)和总氮(TN)的影响均不显著,表明氮添加减轻了土壤碳的损失,且不会改变全球变暖背景下土壤有机碳矿化的潜力。 相似文献
9.
《地理科学进展》2015,(7)
湖沼沉积物地球化学元素对地球气候环境变化敏感性强。本文以江西定南大湖湖沼沉积物地球化学元素为研究对象,使用主成分分析法,并结合总有机碳(TOC)、有机碳同位素(δ13Corg)、中值粒径(Md)、化学蚀变指数(CIA)等相关气候代用指标,以元素组对的形式阐释不同地化元素响应不同气候环境下的地球化学行为和迁移规律。研究结果显示:第一主成分(PC1)包括Al2O3、Ti O2、Si O2、Nb、Rb、Ga、Ba、S等元素,曲线变化与CIA相似,指示湖泊流域的化学风化强度,气候暧湿,PC1含量高;第二主成分(PC2)包括Co、Zr、Hf元素,曲线变化与中值粒径较为一致,指示湖泊流域的水动力条件,气候冷干,PC2含量高;第三主成分(PC3)包括Sc、Cu、U、V元素,曲线变化与TOC、δ13Corg含量变化一致。大湖沉积物的物质来源为:在气候暧湿、流域化学风化作用强的条件下,地表径流冲刷流域周边花岗岩风化壳物质并搬运至湖盆沉积,但不排除在冷干时期,风力携带粉尘物质堆积的影响,粉尘物质可能主要源于周边的风化碎屑物。 相似文献
10.
塔克拉玛干沙漠南缘红柳沙包有机质碳氮含量与气候环境变化 总被引：1，自引：1，他引：0
《干旱区地理》2016,(3)
干旱区红柳沙包沉积纹层具有计年和气候环境指示意义。以塔克拉玛干沙漠南缘策勒和安迪尔地区的红柳沙包为研究对象,通过TOC、TN和C/N分析,探讨气候环境变化。研究表明:红柳落叶C/N变化受到TN和TOC共同影响,但TN是主要因素。虽然受地理位置和人类活动影响,区域间的气候环境变化存在差异,但整个塔克拉玛干沙漠南缘地区,近400多年来,随大气CO_2浓度增加,气温持续升高,气候经历了1600-1690年(冷湿)、1691-1770年(冷干偏暖)、1771-1900年(冷湿偏暖)、1901-1990年(暖干)和1991-2010年(暖湿)等5个阶段。 相似文献
11.
Assessment of nutrient sources and paleoproductivity during the past century in Longgan Lake,middle reaches of the Yangtze River,China 总被引：3，自引：0，他引：3
Total organic carbon (TOC), total nitrogen (TN) and total phosphorus (TP) were determined in combination with stable isotope
ratios of carbon and nitrogen (δ13COrg, δ15N) in a 63 cm sediment core from Longgan Lake, located in the middle reaches of the Yangtze River, China. These geochemical
and isotopic records provide a continuous history of lake productivity and trophic state of Longgan Lake since 1890. Variations
of δ13COrg, TOC, TN and TP indicate that primary productivity of Longgan Lake increased continuously during the last century and that
the trophic state of the lake shifted from oligotrophic to mestrotrophic conditions accordingly. Anthropogenic sources of
organic carbon (OC), nitrogen (N) and phosphorus (P) were distinguished from their natural background in the sediments using
mass accumulation rates. Element mass accumulation rates suggested increased human activities in the lake’s catchment since
1950s, were especially the utilization of artificial fertilizers amplified the anthropogenic input of N and P into the lake.
In the course of the improved availability of dissolved nutrients also primary productivity of Longgan Lake increased, resulting
in an increase of the Suess-effect corrected organic carbon isotope ratios. δ15N of bulk sediments show a marked shift towards lower values around 1950 that has been attributed to the input of nitrogen
from chemical fertilizers characterized by relatively depleted isotopic signatures into the lake. 相似文献
12.
湖泊沉积物有机地化指标在古气候解释中具有复杂性和多解性。TOC、C/N和δ^13Corg作为3种常用的有机地化指标,现已广泛运用于东、中亚全新世气候变化研究中。以这3种指标为例综述了东、中亚全新世湖泊沉积有机地化指标的变化机制及影响因素。根据数据的综合分析与对比,大部分湖泊全新世沉积物TOC百分含量较高时,C／N比值也较高。这与沉积物有机质的来源有关,因两者TOC和C／N作用机制不同,也存在少数湖泊,其两者对应关系不明显;同一湖泊δ^13Corg与TOC及δ^13Corg与C／N对应关系相似;由于不同区域影响有机地化指标的因素不同,TOC、C／N和δ1^3Corg间的关系存在区域差异,据此可将研究区分为中纬度地区、青藏高原区和低纬度季风区。上述区域规律存在于研究中所选的大部分湖泊,由于有机地化指标作用机理的复杂性,也存在不符合这种规律的湖泊,因而上述结论有待于进一步讨论。 相似文献
13.
Jinglu Wu Long Ma Hong Yu Haiao Zeng Wen Liu Jilili Abuduwaili 《Journal of Paleolimnology》2013,50(2):245-255
We present a paleolimnological record from shallow Lake Wuliangsu in the Yellow River Basin, north China, using a short (56 cm) sediment core. Our objective was to investigate environmental changes in this semi-arid region over the past ~150 years. The sediment core was dated using 137Cs and 210Pb. We examined stratigraphic trends in core lithology, nutrients, stable isotopes (δ13C and δ15N) and trace element concentrations in the Lake Wuliangsu core to discern between natural sediments and those affected by human agency. A lithologic transition from yellow, coarse-grained sediment to grey, fined-grained sediment marked the lake’s formation about 1860. Until ~1950, sediments displayed relatively low and constant heavy metal concentrations, indicating little human influence. In the 1950s, enrichment factors (EFs) increased, reflecting greater impact of human activities. Carbon and nitrogen stable isotopes in organic matter (OM), along with heavy metal concentrations, were used to infer past shifts in trophic state and identify pollutants that came from agriculture, industry and urbanization. In the late 1950s, the first evidence for environmental change is recorded by increases in total organic carbon (TOC), total organic nitrogen (TN), TOC/TN, EFs, δ13C and a decrease in δ15N. After about year 2000, a more rapid increase in trophic status occurred, as indicated by greater total phosphorus (TP), EFs, δ15N and lower δ13C values. Changes in isotope and TOC/TN values in the lake sediments may reflect a shift in lake ecology during this period. The first increase in trophic status during the late 1950s was mainly a result of agricultural development in the catchment. In contrast, the change after ca. AD 2000 was driven largely by urban and industrial development. Agreement between paleolimnologic data from Lake Wuliangsu, and both instrumental and written records, indicates that the lake sediments provide a reliable archive for investigating the formation and environmental history of the lake. 相似文献
14.
在放射性核素137Cs和210Pb精确计年的基础上,建立了长江中游网湖近代沉积物年代序列。通过对沉积物中TOC、TN、TP、孢粉、重金属元素、粒度等指标的测定,结合相关文献资料,分析了百年来网湖沉积物中营养元素的分布特征,物源变化以及主控因子。结果表明:百年来网湖沉积物中TN和TOC含量显著相关,呈不断上升趋势,存在2个明显的演化阶段,主控因子为流域人类活动强度,气候波动对其有影响,但影响不大。TP的变化与TN和TOC明显不同,波动较大,规律不明显,主要受人类活动强度以及径流侵蚀输移入湖物质变化两大因子控制。 相似文献
15.
长江中游网湖近代沉积环境演变及其对人类活动的响应 总被引：5，自引：2，他引：3
采用放射性核素210Pb和137Cs计年方法,建立了长江中游网湖近代沉积物的年代序列,并对网湖沉积物的粒度组成、磁性参数、重金属元素、花粉组合以及营养盐含量等指标进行了分析。根据沉积指标垂直分布的综合特征,结合湖区史料,重建了网湖100年来沉积环境的演变过程。通过对沉积指标与湖区人口变化、工农业产值等数据的比对,发现中华人民共和国成立以后沉积物中TOC和TN浓度与人口变化存在较高的相关性,相关系数分别达到0.8892和0.8928(P<0.001);沉积物中重金属元素富集序列、营养盐富集序列与孢粉含量的变化序列与湖区人类活动具有较好的耦合性。表明网湖沉积指标可以敏感地反映湖区的人类活动。 相似文献
16.
A geochemical record of recent anthropogenic nutrient loading and enhanced productivity in Lake Nansihu, China 总被引：2，自引：0，他引：2
Total organic carbon (TOC), total nitrogen (TN), stable carbon and nitrogen isotopes (δ13C, δ15N), total phosphorus (TP) and organic phosphorus (OP) were measured in surface sediments and two short cores (DU-3 and WS-4) from Lake Nansihu, China to infer historical changes in anthropogenic nutrient inputs and corresponding shifts in lake primary productivity. Results indicate that organic matter preserved in the sediments is mainly autochthonous and that analyzed sediment variables were affected little by post-burial diagenesis. Increasing TOC, TN, OP and TP concentrations since the 1940s reflect increased P loading and elevated lake productivity. The δ13C values varied from ?21.5 to ?26.6‰ in the two sediment cores. Values were relatively more negative before the 1940s, but thereafter increased until the mid-1980s, reflecting elevated lake productivity. Since the mid-1980s, δ13C values remained relatively constant in core WS-4 and decreased in core DU-3, perhaps reflecting a change in the phytoplankton community. The δ15N values ranged from ?0.5 to 1.3‰ in core DU-3 and from 1.2 to 2.5‰ in core WS-4 before the mid-1980s, and increased to between 2.1 and 8.0‰ and 5.2 and 7.8‰, respectively, thereafter. Topmost sediments in the two cores display δ15N values similar to those recorded in the surface sediments (5.5–7.5‰). Higher δ15N values in recent deposits correspond to greater nitrogen concentration in water, and likely indicate anthropogenic nitrogen input, mainly from human and animal wastes. 相似文献
17.
Wu Jinglu Huang Chengmin Zeng Haiao Gerhard H. Schleser Rick Battarbee 《Journal of Paleolimnology》2007,38(1):13-23
Environmental change in Lake Taihu and its catchment since the early to middle part of the twentieth century has left a clear
geochemical record in the lake sediments. The human activities in the lake and its catchment responsible for the change include
agriculture, fishery, urbanisation, sewage and industrial waster disposal. Sediment cores were collected from Meilian Bay
of northern Lake Taihu to investigate the record of anthropogenic impacts on the lake’s ecosystem and to assess its natural,
pre-eutrophication baseline state. Two marked stratigraphic sediment units were identified on the basis of total phosphorus
concentration (TP), pigments, total organic carbon (TOC)/total nitrogen (TN), δ13C and δ15N corresponding to stages in the lake history dominated by phytoplankton, and by aquatic macrophytes. Results show that as
TP loading increased from the early 1950s the lake produced sediments with increasing amounts of organic matter derived from
phytoplankton. In the early 1950s, the first evidence for eutrophication at the Meilian Bay site is recorded by an increase
in C/N values and in sediment accumulation rate, but there is little change in phosphorus concentrations, pigments, δ13C and δ15N at this time. After 1990 a more rapid increase in trophic status took place indicated by increased levels of phosphorus,
pigments, δ15N and by decreased δ13C and TOC/TN values in the lake sediments. The first increase in trophic status of the early 1950s results mainly from agricultural
development in the catchment. In contrast, the acceleration from ca. 1990 originates from the recent development of fisheries
and the urbanisation and industrialisation of the catchment. 相似文献
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19.
松嫩平原中西部湖泊底泥营养盐的空间变异特征 总被引：3，自引：0，他引：3
在GIS技术的支持下,利用地统计学方法分析了松嫩平原中西部湖泊底泥营养盐的空间变异特征,并利用Kriging插值方法绘制了研究区营养元素的空间分布图。研究结果表明,通过块金值与基台值的比值C0/(C0+C1)可以得出总有机碳TOC具有较弱的空间相关性,总磷TP和全氮TN具有中等的空间相关性;Kriging插值表明,松嫩平原中西部地区的湖泊底泥营养盐分布格局是西南地区低于北部地区,北部地区的各项指标均超过全区的平均水平。 相似文献
20.
Yaling Su Marieke Lammers Yongdong Zhang Loes van Bree Zhengwen Liu Gert-Jan Reichart Jack J. Middelburg 《Journal of Paleolimnology》2017,58(3):391-402
Determination of carbon sources and microbial activity in lake sediment is important for understanding organic carbon preservation and methane production. This study aimed to determine the organic carbon sources and microbial activity over the last 140 years in sediments of methanotrophic Lake Rotsee (Switzerland). We investigated phospholipid-derived fatty acid biomarkers and their stable carbon isotope signatures in the sediments of this eutrophic lake. Strong bacterial activity in the sediment deposited during the 1920s–1960s could account for the relatively low ratio of long-chain to short-chain fatty acid ((C24 + C26 + C28)/(C14 + C16 + C18), TARFA) values, which is consistent with low TOC/TN ratios in the sediment deposited during that interval. The carbon stable isotope records, both bulk and compound-specific, showed greater values at such times, although the offset between the bulk and fatty acids decreased. This implies that the microbial community residing at sediment depths deposited in the 1960s preferentially utilised the compounds derived from the enhanced surface-water productivity at that time. This observation contrasts with data from the depth intervals before and after, when a major portion of the labile organic matter was derived from methane-sourced production. In sediments deposited before ca. 1964, the overall very low fatty acid δ13C values suggest that labile carbon was primarily derived from methanotrophs. 相似文献