某矿山天然放射性核素的调查   总被引：1，自引：0，他引：1  

覃国秀  刘庆成  陈宁  徐海峰 《国外铀金地质》2008,(1):54-56

对某矿山工作场所和生活区分别进行了样品采集,并使用ORTEC公司生产的16000道HPGeγ能谱仪进行了测量。结果表明,该矿山工作场所天然放射性核素的比活度大多高于生活区,其中危害最大的为尾矿坝;某些生活区天然放射性核素的比活度比对照点和国家均值要高,但多数都在国家均值范围内,最高值出现在3号生活区的农田土样中,其天然放射性核素的比活度分别为：α（226^Ra）——750．4Bq/kg、α（232^Th）——91．5Bq/kg、α（40^K）——1202Bq/kg。  相似文献   

高放废物处置库天然类比及其有关的地球化学问题     

郭永海  王驹  王志明  刘淑芬  宗自华  周佳 《物探与化探》2008,32(5):574-577

介绍了高放废物处置库天然类比研究的主要内容,重点阐述了类比研究中涉及的地球化学问题,包括核素溶解度和化学形态研究、核素迁移速率研究、核素迁移影响因素研究,并总结相关问题研究取得的成果和认识.  相似文献   

近海核电厂核素地下水释放通量的模型计算方法     

朱君  李婷  陈超  谢添  张艾明 《吉林大学学报(地球科学版)》2021,51(1):201-211

为了定量计算陵区近海核电站排水管线泄漏情景下核素通过地下水途径向海洋环境的释放通量，以某近海核电站为例进行研究。首先，应用GOCAD软件建立三维地形地质模型，刻画地层的分布、剥蚀以及倾向等特点；然后，运用地下水数值模拟软件FEFLOW精细刻画丘陵区地下水系统的补给、径流和排泄特征；最后，以不被吸附滞留的核素³H和被吸附滞留的核素⁹⁰Sr、¹³⁷Cs为对象，通过实验测定了⁹⁰Sr、¹³⁷Cs在不同岩土介质中的分配系数，模拟计算了排水管线连续渗漏60 a后³H、⁹⁰Sr、¹³⁷Cs在地下水中的放射性分布及释放。结果表明：³H迁移速度基本与地下水流速一致，地下水中的最大放射性浓度为0.285 0 Bq/L，第20 000天时向收纳水域的释放通量达到最大值，约526 Bq/d；⁹⁰Sr吸附性能相对较弱，最大迁移距离约80 m，地下水中的最大放射性浓度为0.032 1 Bq/L；¹³⁷Cs吸附能力较强，相当长的时间内被滞留在管线附近，地下水中最大放射性浓度分别为6.840×10^-3 Bq/L，释放通量为0 Bq/d。由弥散度的不确定分析可知，弥散度越大，地下水中³H的最大放射性浓度越小，向海洋环境的释放通量越多。  相似文献   

Sediment transfer in an extremely low-gradient,low-relief and highly buffered system: Darwin Harbour catchment,northern Australia     

M. Nawaz  R. Wasson 《Australian Journal of Earth Sciences》2020,67(3):351-359

Abstract

Sediment yields from and sediment transfer within catchments of very low relief and gradient, which make up about 50% of Earth’s surface, are poorly documented and their internal sediment dynamics are poorly known. Sediment sources, their proportionate contributions to valley floors and sediment yield, and storage are estimated using fallout radionuclides ²¹⁰Pb_(ex) and ¹³⁷Cs in the catchments that drain into Darwin Harbour, northern Australia, an example of this understudied catchment type that appears to be globally at the extreme end of this category of catchments. Unchannelled grassy valley floors (dambos, or seasonal wetlands) trap ～90% of the sediment delivered from hillslopes by sheet and rill erosion. Further down valley, small channels transport ～10% of the sediment that escapes from the dambos, and the remaining sediment comes from erosion of the channels. In this case, the fractional sediment storage is very high as a result of the existence of dambos, a landform that depends for its existence on low gradients.  相似文献   

Radiometric dating of lake sediments from Signy Island (maritime Antarctic): evidence of recent climatic change   总被引：4，自引：0，他引：4  

P. G. Appleby  V. J. Jones  J. C. Ellis-Evans 《Journal of Paleolimnology》1995,13(2):179-191

Sediment cores from three lakes (Moss, Sombre and Heywood) in the maritime Antarctic (Signy Island, South Orkney Islands) have been successfully dated radiometrically by²¹⁰Pb and¹³⁷Cs. The core inventories of both fallout radionuclides are an order of magnitude higher than that which can be supported by the direct atmospheric flux at this latitude. The elevated values may be explained by fallout onto the catchment during the winter being delivered directly to the lakes during the annual thaw. Two of the lakes (Sombre and Heywood) show marked increases in sediment accumulation afterc. 1950. This appears to be associated with a documented rise in temperature in the South Orkney Islands, which has caused extensive deglaciation at Signy Island.This is the tenth of a series of papers to be published by this journal following the 20 ^th anniversary of the first application of²¹⁰Pb dating of lake sediments. Dr P.G. Appleby is guest editing this series.  相似文献   

Interpretation of210Pb profiles and verification of the CRS dating model in PIRLA project lake sediment cores     

Michael W. Binford  Jeffrey S. Kahl  Stephen A. Norton 《Journal of Paleolimnology》1993,9(3):275-296

This paper reports results and analysis of²¹⁰Pb-activity measurements in 51 lake-sediment cores from 32 lakes in the four PIRLA (Paleoecological Investigations of Recent Lake Acidification) project regions (Adirondack Mountains [New York], Northern New England, Northern Florida, and the Northern Great Lakes States). General application of the Constant Rate of Supply (Constant Flux) model for²¹⁰Pb dating is valid for lakes in the PIRLA study, although application of the model is equivocal in a few lakes.²¹⁰Pb inventories and profiles are replicable among closely spaced cores within a lake. Specific²¹⁰Pb activity in surface sediments is negatively correlated with bulk sediment accumulation rate in seepage lakes, but not in drainage lakes. Drainage lakes with lower pH have lower unsupported²¹⁰Pb inventories in sediments, but the relationship does not occur in seepage lakes.²¹⁰Pb profiles in only seven of the cores, all from either the Adirondacks or the northern Great Lakes states, exhibit exponential decay curves. Deviations from an exponential profile include a flattening of the profile in the top few cm or excursions of one or a few measurements away from an exponential curve.²¹⁰Pb dates typically agree with other chronostratigraphic markers, most of which are subject to greater uncertainty. Several hypotheses, including sediment mixing, hydrologic regime, sediment focusing, and acidification, are proposed to explain variation of²¹⁰Pb distribution among lakes and regions. Hydrologic factors exert control on unsupported²¹⁰Pb inventories in PIRLA lakes, and there is a strong focusing effect in drainage lakes but a weak focusing effect in seepage lakes.This is the third of a series of papers to be published by this journal following the 20^th anniversary of the first application of²¹⁰Pb dating of lake sediments. Dr P. G. Appleby is guest editing this series.  相似文献   

水－岩反应的铀系不平衡判别   总被引：1，自引：0，他引：1       下载免费PDF全文

罗兴章  闵茂中 《地球科学》1998,23(5):537-541

天然体系中水－岩反应的铀系不平衡判别,是基于水－岩反应使岩石中天然铀衰变系子体核素＾２３４Ｕ,＾２２６Ｒｂ和六价铀的选择性溶失,造成原始放射性平衡遭到不同程度破坏,因而可利用现今测得的岩石中３组核素放射性活度比值Ａ（＾２３４Ｕ）／Ａ（＾２３８Ｕ）,Ａ（＾２３０Ｔｈ）／Ａ（＾２３４Ｕ）和Ａ（＾２２６Ｒａ）／Ａ（＾２３０Ｔｈ）反演判别该岩石曾经历了近代水－岩反应的大致强度和出现,持续时间,这是近十余年  相似文献   

STUDY ON ~(210) Po IN MARINE ORGANISMS IN NORTH CHINA WATERS     

邹本川  秦学祥 《中国海洋湖沼学报》1999,(4)

INTRODUCTIONWiththedevelopmentofcoastalnuclearpowerandmarinenuclearestablishments,peoplepaymoreandmoreattentiontothedistribution ,behaviorandpathwaysofsomeman maderadionuclidesinmarineenvironment.Thedischargedartificialradionuclidesoverlieabackgroundofnaturallyoccurringradionu clideswhicheitheralreadyexistedinmarineenvironmentorwasenhancedbysomeotherhumanactivi ties.Goodunderstandingofsomeman incurredradionuclides’impactsonpeopleandmarineorganismsrequiresknowledgeofsomecriticalnaturalradi…  相似文献   

古地下水定年新方法——81Kr法     

凌新颖  马金珠  杨欢  于海超  何建华 《地质与资源》2019,28(1):90-94

由于⁸¹Kr化学性质稳定、半衰期长且在地下水运移过程中没有额外来源的优点,近年来,成为测定古老地下水年龄（10⁵~10⁶ a）的有效手段.国外对于⁸¹Kr的测定方法、地下水定年应用研究已较为深入,而国内应用⁸¹Kr作为水文地质学的研究尚处于起步阶段.本文通过对国内外⁸¹Kr应用于地下水测年的原理以及⁸¹Kr的测定方法进行总结,针对目前研究的问题进行探讨,并对今后放射性氪核素在水文地球化学中的研究进行展望,为国内对于⁸¹Kr的测定与在古地下水定年研究方面提供科学依据.  相似文献   

西伯利亚水库和叶尼塞河中物质及生态系统条件的预测：生物物理方法     

Andrei Degermendzhy  Vladimir Gubanov 《湖泊科学》1998,10(S1):203-228

An avenue to integrate theoretical, experimental and field research methods to forecast water quality in water bodies for different scenarios of water management is proposed. Exploration of the laws of organization, stability and controllability of laboratory "ideal" water microbial communities (model ecosystems) is the basis to build the following biophysical research chain:to formalize with primary field information a conceptual block-diagram of a water ecosystem →to real chemical and other density-dependent and population-growth-controlling factors → to find our limiting factors for natural ecosystems → to conduct experiments with isolated chemical factors and hydrobionts to derive kinetic dependencies and quantitative parameters→ to transfer regularities of operation and kinetic dependencies to the natural ecosystem→ retrospective verification of the model on the base of available field and derived theoretical-experimental data →prognostic calculations for the scenario. Efficiency of the approach is demonstrated in microalgal "blooming" models for Krasnoyarsk and Kantat reservoirs and in prognostication of radioecological state of great Yenisei river:1) radionuclide distribution in the Yenisei''s bottom sediment is nonuniform-"spotty"; 2) it is theoretically shown, that due to biological interactions and tro-phical radioniclide migration there is "spotive" type of space radionuclide distribution. The research is to make use of the novel methods of ecological biophysics:Monitoring:spectral analysis of surface waters (algal pigments), fluorescent techniques to evaluate productivity and condition of algae; rapid bioassays for water toxicity (bioluminescence, chemotaxis techniques). Kinetic experiments:microcosms on evaluating self-purification rates; special cultivators to evaluate the rates of growth of hydrobionts and radioactive engulfing, nutrition spectra; methods of finding growth limiting factors. Models:application of Bellman Principle to optimizing the river water use; theory and peculiarities of microbiological decomposition of pollutants in the river ecosystem. The composition of Prognostication Simulation Model is the next:1) hydrodynamical unit to calculate 2-dimensional space-time rate of stream on any depth; 2) hydrophysical unit to calculate:water temperature and level of solar radiation inside the water body; 3) ecosystem unit to calculate dynamic of concentration of phytoplankton, zooplankton, bacteria, major chemical matters and pollutants in water, content pollutants inside of hydrobionfs cells and dynamic of bentos; 4) radioe-cological unit to forecast the dynamic of radionuclides in the water body and bottom, their hydro-bont''s concentration; 5) database. Reservoirs and river models are provided by monitoring and kinetic experiments data.  相似文献