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21.
Very few studies have conducted long-term observations of methane (CH4) flux over forest canopies. In this study, we continuously measured CH4 fluxes over an evergreen coniferous (Japanese cypress) forest canopy throughout 1?year, using a micrometeorological relaxed eddy accumulation (REA) system with tuneable diode laser spectroscopy (TDLS) detection. The Japanese cypress forest, which is a common forest type in warm-temperate Asian monsoon regions with a wet summer, switched seasonally between a sink and source of CH4 probably because of competition by methanogens and methanotrophs, which are both influenced by soil conditions (e.g., soil temperature and soil moisture). At hourly to daily timescales, the CH4 fluxes were sensitive to rainfall, probably because CH4 emission increased and/or absorption decreased during and after rainfall. The observed canopy-scale fluxes showed complex behaviours beyond those expected from previous plot-scale measurements and the CH4 fluxes changed from sink to source and vice versa.  相似文献   
22.
Food security in China, the world’s most populous country, has long been a concern because of the challenges of population growth, water shortages, and loss of cropland through urbanization, soil degradation, and climate change. Here, we present an integrated analysis of China’s food demand and supply under IPCC Special Report on Emissions Scenarios A1, A2, B1, and B2 in 2020, 2050, and 2080, based on official statistics and future development scenarios. Our analysis accounts for future socioeconomic, technological, and resource developments, as well the impact of climate change. We present a covariant relationship between changes in cereal productivity due to climate change and the cereal harvest area required to satisfy China’s food demand. We also estimated the effects of changing harvested areas on the productivity required to satisfy the food demand; of productivity changes due to climate change on the harvest area required to satisfy food demand; and of productivity and land use changes on the population at risk of undernutrition. China could be able to feed herself without disturbing the global food market in the twenty-first century, but whether the government will choose self-sufficiency or increased food imports may depend on the cost of change, which remains unknown.  相似文献   
23.
In order to assess the contribution of Lyman break galaxies (LBGs) and Lyman α emitters (LAEs) at redshifts  3 < z < 7  to the ionization of intergalactic medium (IGM), we investigate the escape fractions of ionizing photons from supernova-dominated primordial galaxies by solving the three-dimensional (3D) radiative transfer. The model galaxy is employed from an ultra-high-resolution chemodynamic simulation of a primordial galaxy by Mori & Umemura, which well reproduces the observed properties of LAEs and LBGs. The total mass of model galaxy is  1011 M  . We solve not only photoionization but also collisional ionization by shocks. In addition, according to the chemical enrichment, we incorporate the effect of dust extinction, taking the size distributions of dust into account. As a result, we find that dust extinction reduces the escape fractions by a factor of 1.5–8.5 in the LAE phase and by a factor of 2.5–11 in the LBG phase, while the collisional ionization by shocks increases the escape fractions by a factor of  ≈2  . The resultant escape fractions are 0.07–0.47 in the LAE phase and 0.06–0.17 in the LBG phase. These results are well concordant with the recent estimations derived from the flux density ratio at 1500 to 900 Å of LAEs and LBGs. Combining the resultant escape fractions with the luminosity functions of LAEs and LBGs, we find that high- z LAEs and LBGs can ionize the IGM at   z = 3–5  . However, ionizing radiation from LAEs as well as LBGs falls short of ionizing the IGM at   z > 6  . That implies that additional ionization sources may be required at   z > 6  .  相似文献   
24.
The biological and physical controls on microbial processes that produce and consume N2O in soils are highly complex. Isotopomer ratios of N2O, with abundance of 14N15N16O, 15N14N16O, and 14N14N18O relative to 14N14N16O, are promising for elucidation of N2O biogeochemistry in an intact ecosystem. Site preference, the nitrogen isotope ratio of the central nitrogen atom minus that of the terminal nitrogen atom, is useful to distinguish between N2O via hydroxylamine oxidation and N2O via nitrite reduction.We applied this isotopomer analysis to a groundwater system in a temperate coniferous-forested ecosystem. Results of a previous study at this location showed that the N2O concentration in groundwater varied greatly according to groundwater chemistry, i.e. NO3, DOC, and DO, although apportionment of N2O production to nitrification or denitrification was ambiguous. Our isotopic analysis (δ15N and δ18O) of NO3 and N2O implies that denitrification is the dominant production process of N2O, but definitive information is not derived from δ15N and δ18O analysis because of large variations in isotopic fractionations during production and consumption of N2O. However, the N2O site preference and the difference in δ15N between NO3 and N2O indicate that nitrification contributes to total N2O production and that most measured N2O has been subjected to further N2O reduction to N2. The implications of N2O biogeochemistry derived from isotope and isotopomer data differ entirely from those derived from conventional concentration data of DO, NO3, and N2O. That difference underscores the need to reconsider our understanding of the N cycle in the oxic-anoxic interface.  相似文献   
25.
Abstract– We performed micro‐Raman spectroscopic analyses of the carbon vein in five ureilites: Allan Hills (ALH) A77257, Northwest Africa (NWA) 3140, Shi?r 007, Yamato 790981 (Y‐790981), and Yamato 791538 (Y‐791538). The graphite peaks showed that the graphite structure in ureilite is well developed, especially compared with the carbonaceous material in carbonaceous chondrite. The domain sizes of the graphite were 45–110 Å. We observed shifts in the diamond peak positions to higher wave numbers with a large full width at half maximum (FWHM), especially for NWA 3140. Although the FWHM of a diamond peak is not a crucial diagnostic test for a chemical vapor deposition (CVD) origin of diamond, the shift of the diamond peaks to higher wave numbers could be a strong indicator that supports the CVD origin as these shifts have only been observed in CVD diamonds. We discuss the origin of diamond from various aspects, and confirm that the CVD model is the most plausible. We conclude that all carbon material (graphite, amorphous carbon, diamond, etc.) condensed on the early condensates in the primitive solar nebula.  相似文献   
26.
Chemical compositions of materials used for new sample holders (vertically aligned carbon nanotubes [VACNTs] and polyimide film), which were developed for the analysis of Hayabusa2‐return samples, were determined by instrumental neutron activation analysis and/or instrumental photon activation analysis, to estimate contamination effects from the sample holders. The synthetic quartz plate used for the sample holders was also analyzed. Ten elements (Na, Al, Cr, Mn, Fe, Ni, Eu, W, Au, and Th) and 14 elements (Na, Al, K, Sc, Ti, Cr, Zn, Ga, Br, Sb, La, Eu, Ir, and Au) could be detected in the VACNTs and polyimide film, respectively. The VACNT data show that contamination by this material with respect to the Murchison meteorite is negligible in terms of the elemental ratios (e.g., Fe/Mn, Na/Al, and Mn/Cr) used for the classification of meteorites due to the extremely low density of VACNTs. However, for the Au/Cr ratio, even small degrees (1.7 wt%) of contamination by VACNTs will change the Au/Cr ratio. Elemental ratios used for the classification of meteorites are only influenced by large amounts of contamination (>60 wt%) of polyimide film, which is unlikely to occur. In contrast, detectable effects on Ti isotopic compositions are caused by >0.1 and >0.3 wt% contamination by VACNTs and polyimide film, respectively, and Hf isotopic changes are caused by >0.1 wt% contamination by VACNTs. The new sample holders (VACNTs and polyimide film) are suitable for chemical classification of Hayabusa2‐return samples, because of their ease of use, applicability to multiple analytical instruments, and low contamination levels for most elements.  相似文献   
27.
28.
A numerical simulation of Otsuchi Bay located on the northeast coast of the Honshu, the largest island of Japan, is conducted, using an ocean general circulation model (OGCM) with a nested-grid system in order to illustrate seasonal variability of the circulation in the bay. Through a year, an anticlockwise circulation is dominant in the bay, as observational studies have implied, although it is modified in the bay-mouth-half of the bay in winter. In addition, there is an intense outflow at the surface layer during spring to autumn, influenced by river water discharge. Intrusion of the Pacific water into the bay is influened by mean circulations, but it is also influenced by baroclinic tides from spring to autumn. Pacific water intrusions affected by baroclinic tides may have an impact on the environment in Otsuchi Bay.  相似文献   
29.
Finite element analysis is carried out for a building frame supported by laminated rubber bearings to simultaneously investigate global displacement and local stress responses under seismic excitation. The frame members and the rubber bearings are discretized into hexahedral solid elements with more than 3 million degrees of freedom. The material property of rubber is represented by the Ogden model, and the frame is assumed to remain in elastic range. It is shown that the time histories of non‐uniform stress distribution and rocking behavior of the rubber bearings under a frame subjected to seismic excitation can be successfully evaluated, and detailed responses of base and frame can be evaluated through large‐scale finite element analysis. Copyright © 2015 John Wiley & Sons, Ltd.  相似文献   
30.
60Co were detected in common octopus specimens collected in the East China Sea in 1996-2005. The source of 60Co has remained unclear yet. Stable isotope analyses showed that there was no difference in stable Co concentrations between octopus samples with 60Co and without 60Co. This result showed that the stable Co in the digestive gland of octopus potentially did not include a trace amount of 60Co and the source of 60Co existed independently. Furthermore, investigations of octopus in other area and other species indicated that the origin of the source of 60Co occurred locally in the restricted area in the East China Sea and not in the coastal area of Japan. Concentrations of 60Co have annually decreased with shorter half-life than the physical half-life. This decrease tendency suggests that the sources of 60Co were identical and were temporary dumped into the East China Sea as a solid waste.  相似文献   
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