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1.
《Journal of Asian Earth Sciences》2011,40(6):713-723
Bleaching related to seepage of petroleum fluids and subsurface migration of crude oil and natural gas can alter the chemical and mineralogical properties of rocks, while concurrently depleting hydrocarbon reservoirs. Mud volcanoes constitute one type of petroleum seepage present in several areas on the southern margin of the Junggar Basin in the Xinjiang Uygur Autonomous Region, NW China. The results of XRD, XRF, XANES, and Mössbauer spectroscopy on rock samples collected from areas affected by these mud volcanoes revealed an enrichment of certain minerals and elements, as well changes in mineralogical, molecular, or ionic carrier (“species”). After bleaching, reddish sedimentary rocks showed depletion in silica and enrichment of calcium, magnesium, manganese, and iron. Other elements, including aluminum, potassium, sodium, and titanium, were largely unchanged. Reduced iron and sulfur compounds predominated in the bleached rocks, producing changes in color from the original reddish into green, deep gray, and black. Iron and calcium were associated with carbonates, indicating carbonation of these elements during the bleaching processes. Manganese also appeared to be associated with carbonate, though not with sulfate even though sulfate was present in the bleached rocks. Alkaline conditions were apparently the dominant because reduced manganese would have been absent under acidic condition. The alteration of certain minerals, clay minerals in particular, was also observed in bleached rocks, the alteration of smectite-group minerals to chlorite and muscovite, for example. Mineralogical and geochemical changes in rocks bleached by hydrocarbon fluids could provide a better overall understanding of bleaching processes, and may have applications in surface geochemical exploitation and remote imaging. 相似文献
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青藏高原北缘哈拉湖近800年来 湖泊沉积及其环境意义* 总被引：5，自引：5，他引：5
文章以青藏高原北缘高山祁连山湖泊——哈拉湖作为研究对象,利用放射性核素210 Pb和137 Cs测年资料,通过对此高海拔湖泊沉积碳酸盐氧碳同位素、碳酸盐含量、总有机碳含量、磁化率等环境代用指标的分析,揭示了这一地区近800年来的气候环境变化过程。分析表明哈拉湖记录的气候环境变化经历了3个阶段:1206~1700A.D.环境较为寒冷、湿润,并有持续变湿的趋势;1700~1920A.D.环境由冷湿的状况趋向温暖干旱,1771年之后,环境保持相对稳定;1920~2002A.D.是自1206年以来最为温暖干旱的阶段。 相似文献
3.
We evaluate the exposure during nadir observations with JEM-EUSO, the Extreme Universe Space Observatory, on-board the Japanese Experiment Module of the International Space Station. Designed as a mission to explore the extreme energy Universe from space, JEM-EUSO will monitor the Earth’s nighttime atmosphere to record the ultraviolet light from tracks generated by extensive air showers initiated by ultra-high energy cosmic rays. In the present work, we discuss the particularities of space-based observation and we compute the annual exposure in nadir observation. The results are based on studies of the expected trigger aperture and observational duty cycle, as well as, on the investigations of the effects of clouds and different types of background light. We show that the annual exposure is about one order of magnitude higher than those of the presently operating ground-based observatories. 相似文献
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对QuikSCAT和ASCAT原始轨道10 m反演风场与浮标资料在中国南海北部的统计检验分析结果表明:两套卫星资料在中国南海北部具有较好的适用性,QuickSCAT反演风速偏高0.46 m·s~(-1),ASCAT反演风速在近海偏高0.45 m·s~(-1),在开阔海域偏高0.07 m·s~(-1)。超过半数的QuickSCAT反演风向误差30°。在近岸海域,ASCAT反演风向误差30°的超过56%,在开阔海域,误差绝对值30°的达到64%。小风时卫星反演风速偏大,大风时卫星反演风速明显偏小,且白天的偏差大于夜间;在5~10 m·s~(-1)风速条件下,两者的一致性较好。用WRF模式模拟的近海风能资源存在高估的可能,卫星资料对近海风能资源评估是个有益的补充,本文对卫星反演风场误差的分析结果也可以为卫星反演风场的资料同化提供参考。 相似文献
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6.
《Applied Geochemistry》2002,17(4):353-365
Surprisingly little is known about the relationship between the labile phases removed by sequential extraction procedures and those liberated by single leaches that minimally impact the alumino-silicate matrix of solids. This investigation examines the relationship between the summed concentrations of Al, Co, Cu, Fe, Mn, Ni, Pb and Zn released by an optimized 3-step standardized sequential extraction procedure and those released by a single 0.5 M HCl leach. Thirty-nine representative soil and road deposited sediment samples were examined from an urban watershed, in Honolulu, Hawaii, which has been shown to have a high degree of traffic-associated pollution. Properties of samples analyzed varied widely and exhibited a range in cation exchange capacities from 7 to 59 cmolc/kg, pH values from 3.5 to 7.9, and organic C contents from 1 to 29%. Results indicate that the dilute HCl leach was slightly more aggressive than the sequential procedure as it removed significantly more Al, Cu, Fe, Mn and Ni; though no significant differences were observed between Co, Pb and Zn concentrations liberated by the two approaches. Both approaches showed limited dissolution of the crystal lattice with ⩽9% of the total Al liberated. Regardless of approach, element mobility was the same with the order being: Pb>Mn>Zn>Co≈Cu>Ni>Fe ∼ Al. Regression analysis indicated highly significant (P<0.0001) logarithmic relationships between the two digestion procedures, with coefficients of determination (r2) ⩾92% for all elements except Fe (54%) and Ni (64%). Further support for the strong relationships between elements liberated by both digestions was gained from geochemical contrasts between anomalous and background levels and concentration enrichment ratios. This was particularly true for Pb and Zn, the most anthropogenically enhanced trace metals in the watershed. All data indicated that a dilute HCl leach was a valuable, rapid, and cost-effective analytical tool in contamination assessment. 相似文献
7.
The accurate detection of heavy metal-induced stress on crop growth is important for food security and agricultural, ecological and environmental protection. Spectral sensing offers an efficient and undamaged observation tool to monitor soil and vegetation contamination. This study proposed a methodology for dynamically estimating the total cadmium (Cd) accumulation in rice tissues by assimilating spectral information into WOFOST (World Food Study) model. Based on the differences among ground hyperspectral data of rice in three experiments fields under different Cd concentration levels, the spectral indices MCARI1, NREP and RH were selected to reflect the rice stress condition and dry matter production of rice. With assimilating these sensitive spectral indices into the WOFOST + PROSPECT + SAIL model to optimize the Cd pollution stress factor fwi, the dynamic dry matter production processes of rice were adjusted. Based on the relation between dry matter production and Cd accumulation, we dynamically simulating the Cd accumulation in rice tissues. The results showed that the method performed well in dynamically estimating the total amount of Cd accumulation in rice tissues with R2 over 85%. This study suggests that the proposed method of integrating the spectral information and the crop growth model could successfully dynamically simulate the Cd accumulation in rice tissues. 相似文献
8.
《Atmospheric Science Letters》2000,1(2):89-100
The extent to which the North Atlantic Oscillation (NAO) is influenced by changes in the ocean state is an issue that has attracted much recent attention. Although there have been counter claims, the weight of evidence clearly suggests that forcing by the ocean of year-to-year changes in the NAO is a weak influence by comparison with atmospheric internal variability. The NAO is thus very different in character to the Southern Oscillation (SO), and its predictability—at least on seasonal-to-interannual timescales—is almost certainly much lower.Although weak, the influence of the ocean on the NAO is not negligible. In a previous study we found that wintertime North Atlantic climate, including the NAO, was significantly influenced by a tripole pattern of North Atlantic SST anomalies. Here we report the results of experiments to further elucidate the nature of this influence. We show that the tripole pattern induces a significant response both in the tropical Atlantic and at mid-to-high latitudes. The low latitude response is forced by the low latitude SST anomalies, but the high latitude response is influenced by the extratropical SST anomalies as well as those in the tropics. Furthermore, we find evidence of nonlinear interaction between the influence of the tropical and extratropical SST anomalies. Lastly, we investigate the feedback from the atmosphere onto the SST tripole. We find that the expected negative feedback is significantly modified at low latitudes by the dynamical response of the atmosphere. 相似文献
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基于风廓线雷达数据产品的垂直速度资料和地面气象观测站2014年分钟降雨记录,采用多项式非线性拟合方法,探讨了各季节特征高度层垂直速度与地面降雨之间的相关关系;并根据场次降雨过程的分钟数据分析了垂直速度阈值对降雨开始、结束时间以及降雨强度的指示性。结果表明,垂直速度能够反映雨滴的下落速度特征,综合各个高度层来看,700 m高度层垂直速度与小时雨量回归方程拟合优度较为稳定,其他高度层在不同季节拟合优度差别略大;垂直速度的大小虽不能完全定量地预报降雨强度,但对于整个过程的雨强波动变化有着明显的指示性作用,700 m高度层垂直速度对于降雨的预报指示效果最为稳定。垂直速度对降水的指示性可用于灾害性天气,如暴雨、冰雹、降雪等的预警及临近预报,其阈值的确定受降水相态、降水类型、气温、湿度、湍流等影响,且并非唯一指标。 相似文献
10.
Previous studies have suggested that coal from the 1891 shipwreck of a collier off Victoria, BC, Canada is responsible for elevated parent (unsubstituted) PAH concentrations in sediments near deep marine outfalls from Esquimalt and Victoria in the Strait of Juan de Fuca. To resolve this question, we analysed a comprehensive suite of resolved and unresolved complex mixture (UCM) alkanes, tricyclic terpane, hopane and sterane biomarkers, and parent and alkyl polycyclic aromatic hydrocarbons (PAHs) in samples of coal, wastewater and sediments. Composition patterns, principal components analysis (PCA) models and PAH and biomarker ratios all indicate that coal from the collier does not make a dominant contribution to any sediment sample. Mass balance calculations based on the n-C24 content and 24/4 tetracyclic terpane to 26/3R tricyclic terpane ratio in coal provide a particularly good match between predicted and observed alkyl PAH concentrations for sediments with high alkyl naphthalenes and phenanthrene/anthracenes and low UCM, but the predicted coal contribution substantially underestimates the measured parent PAHs for all sediment samples. Methylbenz[a]anthracene/chrysene profiles for sediments with a dominance of parent PAHs are very close to coal tar, with a marked predominance of methylbenz[a]anthracenes and the possible 10-methylbenz[a]anthracene as a major constituent, while the methylchrysenes predominate in coal. Hence, coal from the collier could account for most alkyl PAHs in the sediments, but dredged sediment containing pyrolised coal waste from a former coal gas plant in Victoria Harbour is a more likely source for the samples with elevated parent PAHs. PAH ratios indicate that these sources are superimposed on combustion PAHs introduced by a combination of atmospheric deposition and delivery via stormwater and the outfalls. Parent PAH distributions also suggest that PAHs in wastewater that originate from oils and soot in liquid fossil fuel combustion are dispersed and degraded, while the larger wood char particles (containing PAHs more protected from degradation) settle closer to the outfalls. Overall, results suggest that PAHs have predominant sources in wood combustion, coal and possibly coke, with a likelihood of much lower bioavailability than would be expected from wastewater dominated by oils and soot from vehicle combustion. 相似文献