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1.
2.
《Cretaceous Research》2008,29(1):87-99
The first carbon and oxygen isotope curves for the Valanginian to Early Barremian (Early Cretaceous) interval obtained from outcrops in the Southern Hemisphere are presented. They were obtained from well-dated (by ammonites) sediments from the Neuquén Basin, Argentina. Measurements were acquired by the innovative method of analysing fossil oyster laminae. The occurrence of the well-established mid-Valanginian positive carbon isotope excursion is documented, while less well-marked positive events may also correlate with peaks identified in the well-known successions of SE France. The mid-Valanginian positive carbon isotope event in the Neuquén Basin is possibly associated with organic-rich sediments. A similar relationship is seen in the European Alps and in oceanic cores in some areas of the world. 相似文献
3.
Wenjun Yong E. Dachs A. C. Withers E. J. Essene 《Contributions to Mineralogy and Petrology》2008,155(2):137-146
The low-temperature heat capacity (C
p) of Si-wadeite (K2Si4O9) synthesized with a piston cylinder device was measured over the range of 5–303 K using the heat capacity option of a physical
properties measurement system. The entropy of Si-wadeite at standard temperature and pressure calculated from the measured
heat capacity data is 253.8 ± 0.6 J mol−1 K−1, which is considerably larger than some of the previous estimated values. The calculated phase transition boundaries in the
system K2O–Al2O3–SiO2 are generally consistent with previous experimental results. Together with our calculated phase boundaries, seven multi-anvil
experiments at 1,400 K and 6.0–7.7 GPa suggest that no equilibrium stability field of kalsilite + coesite intervenes between
the stability field of sanidine and that of coesite + kyanite + Si-wadeite, in contrast to previous predictions. First-order
approximations were undertaken to calculate the phase diagram in the system K2Si4O9 at lower pressure and temperature. Large discrepancies were shown between the calculated diagram compared with previously
published versions, suggesting that further experimental or/and calorimetric work is needed to better constrain the low-pressure
phase relations of the K2Si4O9 polymorphs.
Electronic supplementary material The online version of this article (doi:) contains supplementary material, which is available to authorized users. 相似文献
4.
Anthony C. Withers Marc M. Hirschmann 《Contributions to Mineralogy and Petrology》2008,156(5):595-605
Olivine crystals were grown in the presence of a hydrous silicate fluid during multi-anvil experiments at 8 GPa and 1,000–1,600°C.
Experiments were conducted both in a simple system (FeO–MgO–SiO2–H2O) and in a more complex system containing additional elements (CaO–Na2O–Al2O3–Cr2O3–TiO2–FeO–MgO–SiO2–H2O). Silica activity was buffered by the presence of either pyroxene (high a
SiO2) or ferropericlase (low a
SiO2), and was buffered by the presence of Ni + NiO or Fe + FeO, or constrained by the presence of Fe2O3. Raman spectroscopy was used to identify pyroxene polymorphs in the run products. Clinoenstatite was present in the 1,000°C
experiment, and enstatite in experiments at 1,400–1,520°C. The H2O content of olivine was measured using secondary ion mass spectroscopy, and infrared spectroscopy was used to investigate
the nature of hydrous defects. The H2O storage capacity of olivine decreases with increasing temperature at 8 GPa. In contrast to previous experimental results
at ≤2 GPa, no significant effect of varying oxygen fugacity is evident, but H2O storage capacity is enhanced under conditions of low silica activity. No significant growth of low wavenumber (<3,400 cm−1) peaks, generally associated with high at low pressure, was observed in the FTIR spectra of olivine from the high experiments. Our experiments show that previous high pressure H2O storage capacity measurements for olivine synthesized under more oxidizing conditions than the Earth’s mantle are not likely
to be compromised by the of the experiments. However, the considerable effect of temperature on H2O storage capacity in olivine must be taken into account to avoid overestimation of the bulk upper mantle H2O storage capacity. 相似文献
5.
Klauea historical summit lavas have a wide range in matrix 18OVSMOWvalues (4·9–5·6) with lower values in rockserupted following a major summit collapse or eruptive hiatus.In contrast, 18O values for olivines in most of these lavasare nearly constant (5·1 ± 0·1). The disequilibriumbetween matrix and olivine 18O values in many samples indicatesthat the lower matrix values were acquired by the magma afterolivine growth, probably just before or during eruption. BothMauna Loa and Klauea basement rocks are the likely sources ofthe contamination, based on O, Pb and Sr isotope data. However,the extent of crustal contamination of Klauea historical magmasis probably minor (< 12%, depending on the assumed contaminant)and it is superimposed on a longer-term, cyclic geochemicalvariation that reflects source heterogeneity. Klauea's heterogeneoussource, which is well represented by the historical summit lavas,probably has magma 18O values within the normal mid-ocean ridgebasalt mantle range (5·4–5·8) based on thenew olivine 18O values. KEY WORDS: Hawaii; Klauea; basalt; oxygen isotopes; crustal contamination 相似文献
6.
Katsumi Matsumoto 《Journal of Oceanography》2006,62(6):887-902
Iron fertilization of nutrient-rich surface waters of the ocean is one possible way to help slow the rising levels of atmospheric
CO2 by sequestering it in the oceans via biological carbon export. Here, I use an ocean general circulation model to simulate
a patch of nutrient depletion in the subpolar northwest Pacific under various scenarios. Model results confirm that surface
fertilization is an inefficient way to sequester carbon from the atmosphere (Gnanadesikan et al., 2003), since only about 20% of the exported carbon comes initially from the atmosphere. Fertilization reduces future production
and thus CO2 uptake by utilizing nutrients that would otherwise be available later. Effectively, this can be considered as leakage when
compared to a control run. This “effective” leakage and the actual leakage of sequestered CO2 cause a significant, rapid decrease in carbon retention (only 30–45% retained after 10 years and less than 20% after 50 years).
This contrasts markedly with the almost 100% retention efficiency for the same duration using the same model, when carbon
is disposed directly into the northwest Pacific (Matsumoto and Mignone, 2005). As a consequence, the economic effectiveness
of patch fertilization is poor in two limiting cases of the future price path of carbon. Sequestered carbon in patch fertilization
is lost to the atmosphere at increasingly remote places as time passes, which would make monitoring exceedingly difficult.
If all organic carbon from one-time fertilization reached the ocean bottom and remineralized there, acidification would be
about −0.05 pH unit with O2 depletion about −20 μmol kg−1. These anomalies are probably too small to seriously threaten deep sea biota, but they are underestimated in the model because
of its large grid size. The results from this study offer little to advocate purposeful surface fertilization as a serious
means to address the anthropogenic carbon problem. 相似文献
7.
Svante Björck Hannelore Håkansson Siv Olsson Lena Barnekow Jan Janssens 《Journal of Paleolimnology》1993,8(3):233-272
The hitherto longest found lake sediment sequence on Byers Peninsula, Livingston Island, South Shetland Islands, was analysed with respect to lithology, chronology, diatoms, Pediastrum, pollen and spores, mosses, mineralogy, and sediment chemistry. During the ca. 5000 year long development the sediments were influenced by frequent tephra fall-outs. This volcanic impact played a major role in the lake's history during two periods, 4700–4600 and 2800–2500 BP, but was of importance during the lake's entire history with considerable influence on many of the palaeoenvironmentally significant indicators. The large and complex data set was analysed and zonated with different types of multivariate analysis. This resulted in a subdivision of the sequence into 8 time periods and 21 variables. Redundancy analysis (RDA) of this data set, both without and with the tephra periods, and with 4–6 of the variables as explanatory environmental variables, reveal that climatic/environmental signals are detectable. The palaeoclimatic picture that emerged out of the tephra noise suggests that the first 100 years were characterized by mild, humid conditions. This was followed by a less mild and humid climate until ca. 4000 BP when a gradual warming seems to have started, coupled with increased humidity. These mild and humid conditions seem to have reached an optimum slightly after 3000 BP. At ca. 2500 BP a distinct climatic deterioration occurred with colder and drier conditions and long seasons with ice cover. This arid, cold phase probably reached its optimum conditions at ca. 1500 BP, when slightly warmer conditions might have prevailed for a while. Except for the modern sample with rather mild climate, the last 1400 years seem to have been fairly arid and cold, and the effects of the frequent volcanic activity during this period is only vaguely seen in the records. 相似文献
8.
The mid-Holocene (ca. 8000-4000 cal yr BP) was a time of marked aridity throughout much of Minnesota, and the changes due to mid-Holocene aridity are seen as an analog for future responses to global warming. In this study, we compare the transition into (ca. 9000-7000 yr ago) and out of (ca. 5000-2500 yr ago) the mid-Holocene (MH) period at Kimble Pond and Sharkey Lake, located along the prairie forest ecotone in south-central Minnesota, using high resolution (∼ 5-36 yr) sampling of pollen, charcoal, sediment magnetic and loss-on-ignition properties. Changes in vegetation were asymmetrical with increasing aridity being marked by a pronounced shift from woodland/forest-dominated landscape to a more open mix of grassland and woodland/savanna. In contrast, at the end of the MH, grassland remained an important component of the landscape despite increasing effective moisture, and high charcoal influxes (median 2.7-4.0 vs. 0.6-1.7 mm2 cm− 2 yr− 1 at start of MH) suggest the role of fire in limiting woodland expansion. Asymmetric vegetation responses, variation among and within proxies, and the near-absence of fire today suggest caution in using changes associated with mid-Holocene aridity at the prairie forest boundary as an analog for future responses to global warming. 相似文献
9.
David W. Kelley Stefanie A. Brachfeld Edward A. Nater Herbert E. Wright Jr. 《Journal of Paleolimnology》2006,35(1):193-206
Sediments from Lake Pepin on the Mississippi River, southeastern Minnesota, are used as provenance tracers to assess variations
in hydrology and sediment-transport during the middle Holocene. Three rivers contribute sediment to Lake Pepin, and each catchment
is characterized by a distinctly different geologic terrain. The geochemical fingerprint for each drainage basin was determined
from the elemental composition of heavy minerals in the silt-sized fraction of modern sediment samples. Down-core elemental
abundances were compared with these fingerprints by use of a chemical-mass-balance model that apportions sediment to the source
areas. We observed a decreased contribution from the Minnesota River during the interval ~6700–5500 14C yr BP, which we attribute to decreased discharge of the Minnesota River, likely controlled by a combination of precipitation,
snow melt, and groundwater input to the river. This hydrologic condition coincides with the mid-Holocene prairie period recorded
by fossil pollen data. The occurrence of this feature in a proxy record for hydrologic variations supports the hypothesis
that the mid-Holocene prairie period reflects drier conditions than before or after in midwestern North America. 相似文献
10.
Daniel H. Doctor E. Calvin Alexander Jr Metka Petrič Janja Kogovšek Janko Urbanc Sonja Lojen Willibald Stichler 《Hydrogeology Journal》2006,14(7):1171-1191
Karst aquifer components that contribute to the discharge of a water supply well in the Classical Karst (Kras) region (Italy/Slovenia) were quantitatively estimated during storm events. Results show that water released from storage within the epikarst may comprise as much as two-thirds of conduit flow in a karst aquifer following rainfall. Principal components analysis (PCA) and end-member mixing analysis (EMMA) were performed using major ion chemistry and the stable isotopes of water (δ18O, δ2H) and of dissolved inorganic carbon (δ13CDIC) to estimate mixing proportions among three sources: (1) allogenic river recharge, (2) autogenic recharge, and (3) an anthropogenic component stored within the epikarst. The sinking river most influences the chemical composition of the water-supply well under low-flow conditions; however, this proportion changes rapidly during recharge events. Autogenic recharge water, released from shallow storage in the epikarst, displaces the river water and is observed at the well within hours after the onset of precipitation. The autogenic recharge end member is the second largest component of the well chemistry, and its contribution increases with higher flow. An anthropogenic component derived from epikarstic storage also impacts the well under conditions of elevated hydraulic head, accounting for the majority of the chemical response at the well during the wettest conditions. 相似文献