对流层气溶胶的直接气候效应对平流层的影响   总被引：1，自引：1，他引：0       下载免费PDF全文

宋刘明  刘煜  朱彬  李维亮 《应用气象学报》2014,25(1):83-94

通过WACCM-3模式中气溶胶光学厚度与卫星资料的对比发现,模式可以很好地再现全球气溶胶的主要分布特征,但在一些区域还存在数值上的差异。利用数值试验研究对流层气溶胶的直接气候效应对平流层气候的影响,结果表明:对流层气溶胶对平流层气候有明显影响,平流层化学过程在这一影响中起重要作用,而对流层气溶胶对平流层辐射的影响不是其直接气候效应对平流层影响的主要原因。其机制可能是对流层气溶胶改变对流层的辐射平衡,影响对流层的温度和大气环流,进而影响行星波的上传,使得平流层气候发生变化;影响区域主要位于高纬度和极地地区,南半球的变化比北半球大,温度变化最大达10 K,纬向风变化最大可达12 m/s,臭氧体积分数最多减少0.8×10-6。  相似文献   

基于MODIS的春、夏季中国近海气溶胶对于云参数的影响差异研究     

邓学良  邓伟涛  聂肃平 《南京气象学院学报》2014,6(4):349-355

通过分析中国近海MODIS数据中气溶胶参数与云参数的相互关系,讨论了该区域气溶胶的间接效应及其对于云的可能影响.结果表明,在中国近海,气溶胶具有明显的间接效应,而且由于气溶胶种类和水汽的季节变化,使得气溶胶的间接作用具有很强的时间变化特征.在夏季,由于人为气溶胶占主导,它作为有效的云凝结核,使得气溶胶光学厚度（AOT）分别与云凝结核数（CCN）有正相关、与云滴有效半径（CER）有负相关性、与云光学厚度（COT）也存在着正相关,气溶胶的间接效应明显;在春季,由于沙尘气溶胶盛行,同时沙尘并不是很好的云凝结核,使得气溶胶光学厚度（AOT）分别与云凝结核数（CCN）的正相关减弱、与云滴有效半径（CER）则由夏季的负相关变为正相关、与云光学厚度（COT）存在弱的负相关,气溶胶的间接效应不明显.  相似文献   

Effects of meridional sea surface temperature changes on stratospheric temperature and circulation   总被引：4，自引：1，他引：3  

HU Dingzhu  TIAN Wenshou  XIE Fei  SHU Jianchuan  Sandip  DHOMSE 《大气科学进展》2014,31(4):888-900

Using a state-of-the-art chemistry-climate model,we analyzed the atmospheric responses to increases in sea surface temperature （SST）.The results showed that increases in SST and the SST meridional gradient could intensify the subtropical westerly jets and significantly weaken the northern polar vortex.In the model runs,global uniform SST increases produced a more significant impact on the southern stratosphere than the northern stratosphere,while SST gradient increases produced a more significant impact on the northern stratosphere.The asymmetric responses of the northern and southern polar stratosphere to SST meridional gradient changes were found to be mainly due to different wave properties and transmissions in the northern and southern atmosphere.Although SST increases may give rise to stronger waves,the results showed that the effect of SST increases on the vertical propagation of tropospheric waves into the stratosphere will vary with height and latitude and be sensitive to SST meridional gradient changes.Both uniform and non-uniform SST increases accelerated the large-scale Brewer-Dobson circulation （BDC）,but the gradient increases of SST between 60°S and 60°N resulted in younger mean age-of-air in the stratosphere and a larger increase in tropical upwelling,with a much higher tropopause than from a global uniform 1.0 K SST increase.  相似文献   

A Review of Aerosol Optical Properties and Radiative Effects          下载免费PDF全文

LIU Yuzhi  JIA Rui  DAI Tie  XIE Yongkun  SHI Guangyu 《Acta Meteorologica Sinica》2014,28(6):1003-1028

Atmospheric aerosols influence the earth's radiative balance directly through scattering and absorbing solar radiation, and indirectly through affecting cloud properties. An understanding of aerosol optical properties is fundamental to studies of aerosol effects on climate. Although many such studies have been undertaken, large uncertainties in describing aerosol optical characteristics remain, especially regarding the absorption properties of different aerosols. Aerosol radiative effects are considered as either positive or negative perturbations to the radiation balance, and they include direct, indirect (albedo effect and cloud lifetime effect), and semi-direct effects. The total direct effect of anthropogenic aerosols is negative (cooling), although some components may contribute a positive effect (warming). Both the albedo effect and cloud lifetime effect cool the atmosphere by increasing cloud optical depth and cloud cover, respectively. Absorbing aerosols, such as carbonaceous aerosols and dust, exert a positive forcing at the top of atmosphere and a negative forcing at the surface, and they can directly warm the atmosphere. Internally mixed black carbon aerosols produce a stronger warming effect than externally mixed black carbon particles do. The semi-direct effect of absorbing aerosols could amplify this warming effect. Based on observational (ground-and satellite-based) and simulation studies, this paper reviews current progress in research regarding the optical properties and radiative effects of aerosols and also discusses several important issues to be addressed in future studies.  相似文献   

东亚季风区近地面大气气溶胶中OCPs和PCBs纬度分布：以7Be为参照系     

杨永亮  耿存珍  李勇  张干  史双昕  朱晓华  焦杏春  谭科艳  于寒青 《地球化学》2014,(1):20-31

连续一年在北京、青岛、广州以每周3d的时间尺度同步采集近地面大气中气溶胶中7Be的测定数据以及在春、秋季节变换时期我国5个不同纬度城市大气气溶胶中7Be和典型持久性有机污染物（有机氯农药和多氯联苯1的同步观测数据,并对文献上发表的我国其他城市近地面大气中气溶胶中’Be年平均值数据进行了分析。通过对以上数据资料的总结和分析,观察到在东亚季风区近地表大气气溶胶中7Be浓度的年平均值呈现正态分布模式,并且在中纬度北纬40°N附近达到极大值。大气气溶胶中7Be在春、秋季节变换时期我国不同纬度城市的瞬时纬度分布仍呈现正态分布模式,但以30°N为最大值。在秋季大气颗粒相中HCHs和PCBs浓度最大值出现在30°N。气相中PCB-28所占百分比随纬度增高而增大,而颗粒相中PCB-28的纬度变化不大。蒸汽压较低的PCB-180在气相中的浓度基本上不随纬度变化,而颗粒相中PCB-180则基本上集中在纬度36。N左右,表明在东亚季风区大气中挥发性较低的POPs化合物具有某种纬度聚焦作用。以宇宙射线成因核素7Be作为大气环流的参照系,可以得出东亚季风区大气环流可影响持久性有机污染物纬度分布的结论。  相似文献   

乌鲁木齐冬季黑碳气溶胶污染特征初步研究     

钟玉婷  刘新春  何清  陆辉  赵克蕾 《沙漠与绿洲气象(新疆气象)》2014,8(6):36-40

利用2010年2月乌鲁木齐大气成分观测站黒碳仪观测数据,结合散射系数及常规观测资料,对乌鲁木齐冬季黑碳气溶胶浓度变化特征进行了分析,并通过气流后向轨迹进行了来源分析。结果表明：(1)观测期间BC质量浓度日平均值为12707±4673 ng.m-3,浓度变化范围为4916~22997 ng.m-3,散射系数日均值为1086±561Mm-1,变化范围为350~2232 Mm-1。BC质量浓度和散射系数日均值变化趋势基本一致;(2)BC质量浓度日变化具有明显的峰值和谷值,峰值分别出现在9~11时和20~22时,谷值分别出现在4~6时和16~18时,散射系数与BC质量浓度日变化趋势基本一致,相对其有一定的滞后。春节期间燃放烟花爆竹对空气污染物浓度上升有明显作用,显著影响BC质量浓度日变化规律;(3)乌鲁木齐冬季大气层结稳定,污染物不易扩散,风速和降水对黑碳气溶胶浓度具有明显的稀释作用。在乌鲁木齐特殊的地形和气象条件下,本地源排放与来自周边城市群污染物输送的叠加使得污染更加严重。  相似文献   

青藏高原黑碳气溶胶传输及沉降的季节特征模拟分析     

韩永翔  孙海波  刘建慧  赵天良  S.L.Gong 《干旱气象》2014,(3):319-325

根据全球气溶胶气候模式GEM-AQ/EC的1995~2004年模拟,分析了青藏高原大气黑碳气溶胶的来源、传输及沉降季节特征。研究表明:青藏高原黑碳气溶胶主要来自自由对流层和大气边界层的输送。相对于自由对流层的黑碳输送,紧邻青藏高原的南亚、东亚以及东南亚大气边界层的输送更有效,它形成了青藏高原由北向南、自西往东黑碳气溶胶浓度和沉降明显递增的基本分布形态。横跨欧亚大陆自由对流层的黑碳气溶胶由西向东向青藏高原的输送全年不变,夏季输送路径最北但强度最弱,冬季路径最南而强度最强。大气边界层黑碳气溶胶的输送受控于亚洲季风环流变化,来自南亚的黑碳气溶胶在春季越过孟加拉湾传输进入高原东南部,夏季则可翻越喜马拉雅山抵达青藏高原南部腹地;同时我国中部排放的黑碳气溶胶也在东亚夏季风向北扩展中驱动它从东向西往青藏高原东北部传输。从秋季到冬季,随着夏季风撤退,南亚黑碳源区向青藏高原传输衰退,东亚冬季风的反气旋性环流的南侧及西南侧的偏东风携带秋季我国东南部源区和冬季东南亚源区黑碳气溶胶向青藏高原东南部传输。受青藏高原明显的暖湿季和干冷季气候影响,干湿沉降分别主导了青藏高原冬季和夏季黑碳沉降,夏季青藏高原黑碳气溶胶沉降总量大多超过8~10 kg·km-2,在高原东北部的最高值超过40 kg·km-2。冬季青藏高原黑碳气溶胶沉降量最低,大部地区黑碳沉降低于5 kg·km-2。青藏高原黑碳沉降的冬夏季节相差约为2~8倍。  相似文献   

Statistical data fusion of multi-sensor AOD over the Continental United States     

Sweta Jinnagara Puttaswamy  Hai M. Nguyen  Amy Braverman  Xuefei Hu 《国际地球制图》2014,29(1):48-64

This article illustrates two techniques for merging daily aerosol optical depth (AOD) measurements from satellite and ground-based data sources to achieve optimal data quality and spatial coverage. The first technique is a traditional Universal Kriging (UK) approach employed to predict AOD from multi-sensor aerosol products that are aggregated on a reference grid with AERONET as ground truth. The second technique is spatial statistical data fusion (SSDF); a method designed for massive satellite data interpolation. Traditional kriging has computational complexity O(N³), making it impractical for large datasets. Our version of UK accommodates massive data inputs by performing kriging locally, while SSDF accommodates massive data inputs by modelling their covariance structure with a low-rank linear model. In this study, we use aerosol data products from two satellite instruments: the moderate resolution imaging spectrometer and the geostationary operational environmental satellite, covering the Continental United States.  相似文献   

The Seasonal Variabilities in the Concentration of Atmospheric Aerosols over Qingdao, China   总被引：2，自引：0，他引：2  

SHENG Lifang FU Ying QIU Mingyan GAO Huiwang 《中国海洋大学学报(英文版)》2005,4(4):383-390

Mass concentrations of Total Suspended Particles （TSP） and size-segregated particles were obtained from July 2001 to June 2002 in Qingdao to characterize the seasonal variations of atmospheric aerosols and to show the impact of dust events on the air quality in Qingdao. Data on size-segregated aerosols show that 73.74% of the TSP mass concentration is contributed by particles with diameters less than 11 μm. Particles with diameters less than 1.1μm have a higher concentration during the winter. In spring, larger particles tend to have higher mass concentrations. Bimodal particle size distributions have been observed, with maxima around 4.7-7 μand 0.43-0.65 μm in the winter season, and 7-11 μm and 0.65-1.1 μm in the autumn season. Measurements made during the dust events in March 2002 show high concentrations of particles in the size range 2.1-7μm.  相似文献   

Study of Distinctive Regional Features of Surface Solar Radiation in North and East China          下载免费PDF全文

GUAN Fulai  ZHENG Youfei  CAI Ziying  YU Changwen  ZHANG Nan 《Acta Meteorologica Sinica》2011,25(4):494-505

Solar radiation is an important energy source for plants on the earth and also a major component of the global energy balance.Variations in solar radiation incident at the earth's surface profoundly affect the human and terrestrial environment,including the climate change.To provide useful information for predicting the future climate change in China,distinctive regional features in spatial and temporal variations of the surface solar radiation (SSR) and corresponding attributions (such as cloud and aerosol) are analyzed based on SSR observations and other meteorological measurements in North and East China from 1961 to 2007.Multiple models,such as the plane-parallel radiative transfer model,empirical and statistical models,and corrclation and regrcssion analysis methods are used in the study.The results are given as follows.(1) During 1961-2007,the total SSR in North China went through a process from quickly “dimming” to slowly “dimming”,while in East China,a significant transition from “dimming” to “brightening” occurred.Although there are some differences between thc two regional variation trends,long-term variations in SSR in the two regions are basically consistent with the observation worldwide.(2) Between the 1960s and 1980s,in both North and East China,aerosols played a critical rolc in the radiation dimming.However,after 1989,different variation trends of SSR occurred in North and East China,indicating that aerosols were not the dominant factor.(3) Cloud cover contributed less to the variation of SSR in North China,but was thc major attribution in East China and played a promoting role in the reversal of SSR from dimming to brightening,especially in the “remarkable brightening” period,with its contribution as high as 70％.  相似文献