一次霾天气条件下石家庄上空大气气溶胶数浓度的飞行探测与特征分析     

金赛花  濮江平  张瑜 《气象与环境科学》2015,38(1):40-45

利用2010年8月30日河北省石家庄一次霾天气条件下的气溶胶飞行探测资料,分析了石家庄地区上空658—6933 m高度范围内大气气溶胶粒子平均数浓度、平均直径的垂直分布特征和9个水平飞行高度上的谱分布特征。结果表明:轻度霾天气条件下的气溶胶平均数浓度为325个/cm3,平均直径为0.169μm。在约1000 m高度以下,气溶胶平均数浓度随高度的增加呈线性减少趋势。粒径也随高度增加而减小,由0.187μm减小至0.164μm。1000 m高度以上,气溶胶平均数浓度随高度减少趋势变缓,粒子平均直径在0.167~0.171μm范围内波动。9个不同高度上的谱分布都呈单峰型,随着高度增加,谱宽变小,峰值向小尺度方向移动。后向轨迹计算分析表明:污染气团的远距离输送可能是导致大气1500 m高度层气溶胶数浓度突增的原因。  相似文献   

Carbonyl Sulphide (OCS) Variability with Latitude in the Atmosphere     

Gisèle Krysztofiak  Yao Veng Té  Gwenaël Berthet  Geoffrey C. Toon  Fabrice Jégou 《大气与海洋》2015,53(1):89-101

Abstract

Carbonyl sulphide (OCS) is an important precursor of sulphate aerosols and consequently a key species in stratospheric ozone depletion. The SPectromètre InfraRouge d'Absorption à Lasers Embarqués (SPIRALE) and shortwave infrared (SWIR) balloon-borne instruments have flown in the tropics and in the polar Arctic, and ground-based measurements have been performed by the Qualité de l'Air (QualAir) Fourier Transform Spectrometer in Paris. Partial and total columns and vertical profiles have been obtained to study OCS variability with altitude, latitude, and season. The annual total column variation in Paris reveals a seasonal variation with a maximum in April–June and a minimum in November–January. Total column measurements above Paris and from SWIR balloon-borne instrument are compared with several MkIV measurements, several Network for the Detection of Atmospheric Composition Change (NDACC) stations, aircraft, ship, and balloon measurements to highlight the OCS total column decrease from tropical to polar latitudes. OCS high-resolution in situ vertical profiles have been measured for the first time in the altitude range between 14 and 30?km at tropical and polar latitudes. OCS profiles are compared with Atmospheric Chemistry Experiment (ACE) satellite measurements and show good agreement. Using the correlation between OCS and N₂O from SPIRALE, the OCS stratospheric lifetime has been accurately determined. We find a stratospheric lifetime of 68?±?20 years at polar latitudes and 58?±?14 years at tropical latitudes leading to a global stratospheric sink of 49?±?14?Gg?S?y^?1.  相似文献   

一种改进的TSI3563积分浊度误差校正方法          下载免费PDF全文

马楠  周秀骥  颜鹏  赵春生 《应用气象学报》2015,26(1):12-21

TSI3563型积分式浊度计是一种性能出色的气溶胶散射系数观测仪器,然而由于仪器设计所固有的限制,TSI3563型浊度计观测结果包含有角度截断和非朗伯体光源两项系统性误差,会使观测结果较真值偏小10%左右。因此,需要对TSI3563型浊度计的观测结果进行校正才能得到较为精确的散射系数观测值。该研究利用2009年华北平原HaChi气溶胶外场观测数据测试了现有校正方法,结果显示,传统的校正方法在我国华北平原这样的高气溶胶污染地区并不适用。为此,提出一种改进的校正方法,利用同时观测的PM₁和PM₁₀数据,在校正方案中加入超微米粒子体积比这一参量,对于不同体积比采用不同的校正函数。利用实际观测数据检验后发现,改进方法的校正效果相对于传统方法有很大改善。  相似文献   

Aerosol Type Identification Using PARASOL Multichannel Polarized Data   总被引：1，自引：0，他引：1       下载免费PDF全文

FAN Xue-Hua  CHEN Hong-Bin 《大气和海洋科学快报》2014,(3):224-229

PARASOL （Polarization ＆ Anisotropy of Reflectances for Atmospheric Sciences coupled with Ob- servations from a Lidar） multi-channel and mul- ti-directional polarized data for different aerosol types were compared. The PARASOL polarized radiance data at 490 nm, 670 nm, and 865 nm increased with aerosol optical thickness （AOT） for fine-mode aerosols; however, the polarized radiances at 490 nm and 670 nm decreased as AOT increased for coarse dust aerosols. Thus, the vari- ation of the polarized radiance with AOT can be used to identify fine or coarse particle-dominated aerosols. Polar- ized radiances at three wavelengths for fine- and coarse-mode aerosols were analyzed and fitted by linear regression. The slope of the line for 670 nm and 490 nm wavelength pairs is less than 0.35 for dust aerosols. However, the value for fine-mode aerosols is greater than 0.60. The Support Vector Machine method （SVM） based on 12 vector features was used to discriminate clear sky, coarse dust aerosols, fine-mode aerosols, and cloud. Two cases were given and validated by AErosol RObotic NETwork （AERONET） measurements, MODIS （Mod- erate Resolution Imaging Spectroradiometer） FMF （Fine Mode Fraction at 550 nm） images, PARASOL RGB （Red Green Blue） images, and CALIOP （Cloud-Aerosol Lidar with Orthogonal Polarization） VFM （Vertical Feature Mask） data.  相似文献   

Real-Time Observation on Water-Soluble Ions of PM_(2.5)in Beijing under the Influences of Different Air Masses in Summer          下载免费PDF全文

CHENG Meng-Tian  SUN Yang  ZHU Xiao-Wan  CHAO Na 《大气和海洋科学快报》2014,(1)

To further understand the variations of water-soluble ions in PM2.5 in Beijing,the authors observed their concentrations continuously and in high temporal resolution by the system for rapid collection of fine particles and ion chromatography(RCFP-IC) during 12–18 July 2010.These results combined with those of earlier backward trajectory research are used analyzed to determine the causes of concentration changes in water-soluble ions under the influences of two kinds of air masses in summer.The results indicate that concentrations of NO3-,SO42-,and NH4+ were influenced strongly by the continental air mass than by the marine air mass.Cl- and Na+ were not changed significantly.Because the sources of K+,Mg2+,and Ca2+ are mainly concentrated on land,their concentration levels were slightly higher under the control of continental air mass than that of the marine air mass.Variations of NO2- during the observation differed from those of other ions;its concentration was significantly higher under the influence of marine air mass.Moreover,the authors obtain the diurnal variations of eight water-soluble inorganic ions including NH4+,K+,Mg2+,Ca2+,Cl-,NO2-,NO3-,and SO42-.Diurnal variations of NH4+,NO3-,and Cl- showed single peak,which appeared before noon,while SO42- showed two peaks that appeared during rush hours.Those of Mg2+,Ca2+,and K+ showed single peak that appeared in the afternoon.That of NO2- showed with a peak appearing at sunrise and a valley appearing at sunset.  相似文献   

湛江地区一次冷锋型海雾微物理特征   总被引：1，自引：1，他引：0       下载免费PDF全文

吕晶晶  牛生杰  赵丽娟  张羽  徐峰 《大气科学学报》2014,37(2):208-215

利用2010年3月31日—4月2日冷锋天气系统影响下湛江海雾综合观测资料,分析了海雾的微物理特征及海雾过程中气溶胶粒子谱的演变特征。结果表明,海雾的生消与风场密切相关,海雾生成和发展与较强的ESE气流相联系,而弱的NE气流则会促使海雾减弱或消散。湛江海雾的雾滴数浓度为100~102cm-3,液态含水量为0.001~0.232 g·m-3,雾滴平均半径小于10μm,雾滴峰值半径多位于1.4μm。海雾雾滴谱分布以单调递减谱为主,谱宽超过20μm,且雾发展过程中雾滴谱谱宽存在突然增宽和迅速减小的现象。海雾过程中雾滴数浓度的变化主要是由半径小于5μm的雾滴数密度变化引起的。海雾过程对气溶胶粒子的湿清除效果并不显著,雾过程中粒径小于0.1μm和大于4μm的气溶胶粒子数密度显著减少,但在雾消散后又迅速恢复到雾发生前的水平。  相似文献   

The Role of the Aerosol Indirect Effect in the Northern Indian Ocean Warming Simulated by CMIP5 Models          下载免费PDF全文

HU Ning  LI Li-Juan  WANG Bin 《大气和海洋科学快报》2014,(5):411-416

The northern Indian Ocean （NIO） experienced a decadal-scale persistent warming from 1950 to 2000, which has influenced both regional and global climate. Because the NIO is a region susceptible to aerosols emis- sion changes, and there are still large uncertainties in the representation of the aerosol indirect effect （ALE） in CMIP5 （Coupled Model Intercomparison Project Phase 5） models, it is necessary to investigate the role of the AIE in the NIO warming simulated by these models. In this study, the authors select seven CMIP5 models with both the aerosol direct and indirect effects to investigate their performance in simulating the basin-wide decadal-scale NIO warming. The results show that the decreasing trend of the downwelling shortwave flux （FSDS） at the surface has the major damping effect on the SST increasing trend, which counteracts the warming effect of greenhouse gases （GHGs）. The FSDS decreasing trend is mostly contrib- uted by the decreasing trend of cloudy-sky surface downwelling shortwave flux （FSDSCL）, a metric used to measure the strength of the AIE, and partly by the clear-sky surface downwelling shortwave flux （FSDSC）. Models with a relatively weaker AIE can simulate well the SST increasing trend, as compared to observation. In contrast, models with a relatively stronger AIE produce a much smaller magnitude of the increasing trend, indicat- ing that the strength of the AIE in these models may be overestimated in the NIO.  相似文献   

对流层气溶胶的直接气候效应对平流层的影响   总被引：1，自引：1，他引：0       下载免费PDF全文

宋刘明  刘煜  朱彬  李维亮 《应用气象学报》2014,25(1):83-94

通过WACCM-3模式中气溶胶光学厚度与卫星资料的对比发现,模式可以很好地再现全球气溶胶的主要分布特征,但在一些区域还存在数值上的差异。利用数值试验研究对流层气溶胶的直接气候效应对平流层气候的影响,结果表明:对流层气溶胶对平流层气候有明显影响,平流层化学过程在这一影响中起重要作用,而对流层气溶胶对平流层辐射的影响不是其直接气候效应对平流层影响的主要原因。其机制可能是对流层气溶胶改变对流层的辐射平衡,影响对流层的温度和大气环流,进而影响行星波的上传,使得平流层气候发生变化;影响区域主要位于高纬度和极地地区,南半球的变化比北半球大,温度变化最大达10 K,纬向风变化最大可达12 m/s,臭氧体积分数最多减少0.8×10-6。  相似文献   

基于MODIS的春、夏季中国近海气溶胶对于云参数的影响差异研究     

邓学良  邓伟涛  聂肃平 《南京气象学院学报》2014,6(4):349-355

通过分析中国近海MODIS数据中气溶胶参数与云参数的相互关系,讨论了该区域气溶胶的间接效应及其对于云的可能影响.结果表明,在中国近海,气溶胶具有明显的间接效应,而且由于气溶胶种类和水汽的季节变化,使得气溶胶的间接作用具有很强的时间变化特征.在夏季,由于人为气溶胶占主导,它作为有效的云凝结核,使得气溶胶光学厚度（AOT）分别与云凝结核数（CCN）有正相关、与云滴有效半径（CER）有负相关性、与云光学厚度（COT）也存在着正相关,气溶胶的间接效应明显;在春季,由于沙尘气溶胶盛行,同时沙尘并不是很好的云凝结核,使得气溶胶光学厚度（AOT）分别与云凝结核数（CCN）的正相关减弱、与云滴有效半径（CER）则由夏季的负相关变为正相关、与云光学厚度（COT）存在弱的负相关,气溶胶的间接效应不明显.  相似文献   

A Review of Aerosol Optical Properties and Radiative Effects          下载免费PDF全文

LIU Yuzhi  JIA Rui  DAI Tie  XIE Yongkun  SHI Guangyu 《Acta Meteorologica Sinica》2014,28(6):1003-1028

Atmospheric aerosols influence the earth's radiative balance directly through scattering and absorbing solar radiation, and indirectly through affecting cloud properties. An understanding of aerosol optical properties is fundamental to studies of aerosol effects on climate. Although many such studies have been undertaken, large uncertainties in describing aerosol optical characteristics remain, especially regarding the absorption properties of different aerosols. Aerosol radiative effects are considered as either positive or negative perturbations to the radiation balance, and they include direct, indirect (albedo effect and cloud lifetime effect), and semi-direct effects. The total direct effect of anthropogenic aerosols is negative (cooling), although some components may contribute a positive effect (warming). Both the albedo effect and cloud lifetime effect cool the atmosphere by increasing cloud optical depth and cloud cover, respectively. Absorbing aerosols, such as carbonaceous aerosols and dust, exert a positive forcing at the top of atmosphere and a negative forcing at the surface, and they can directly warm the atmosphere. Internally mixed black carbon aerosols produce a stronger warming effect than externally mixed black carbon particles do. The semi-direct effect of absorbing aerosols could amplify this warming effect. Based on observational (ground-and satellite-based) and simulation studies, this paper reviews current progress in research regarding the optical properties and radiative effects of aerosols and also discusses several important issues to be addressed in future studies.  相似文献