北京、郑州和深圳三城市空气中气溶胶单颗粒特征的扫描电镜分析   总被引：1，自引：0，他引：1  

赵承美  邵龙义  侯聪  幸娇萍  胡颖  王文华 《岩石矿物学杂志》2015,34(6):925-931

分别采集北京、深圳和郑州3个城市气溶胶样品,使用场发射扫锚电镜-能谱仪观察气溶胶单颗粒的显微形貌和元素组成,并利用图像分析系统对PM2.5的粒径进行了分析。结果表明,城市气溶胶单颗粒类型以矿物颗粒、烟尘和球形颗粒(飞灰和二次粒子)为主。对比3个城市气溶胶中不同颗粒类型数量百分比发现,矿物颗粒数量最多的城市是北京,飞灰和烟尘数量最多的城市是郑州,而规则矿物颗粒数量最多的城市是深圳。3个城市气溶胶单颗粒的数量-粒径分布均呈单峰分布。深圳气溶胶中颗粒物的粒径相对较小,其次为郑州、北京。3个城市气溶胶中颗粒物来源不同程度上都受到交通污染源影响,而燃煤源对北京和郑州气溶胶中颗粒物来源影响仍然不容忽视。  相似文献   

The Energy Relationship between Ions and Soil Particles based on Wien Effect and Its Application in Soil Science     

《地球科学进展》2015,30(12):1295

The interaction between ions and soil particles plays an important role in the mobilization and bioavailability of ions in soils, which is one of the main research areas of soil chemistry. The new method based on suspension Wien effect has been developed recently to determine the binding energy and adsorption energy between ions and soil particles. Compared with other methods on the basis of adsorption isotherm or ions activity, Wien effect method has more advantages including convenience and direct measurement. The term suspension Wien effect refers to the increase of electrical conductivity of suspension with increasing applied electrical field. In this review paper, we introduced the fundamentals of suspension Wien effect, the apparatus about the Wien effect measurement, and along with demonstrating their application to quantifying the particles-ions interactions for several systems of soils. Our studies indicated that divalent cations have larger binding energies and adsorption energies on soil particles than monovalent because of the electrostatic interaction. However, few studies about the interaction between Cr³⁺ and La³⁺ on soil particles showed that the binding energy and adsorption energy of trivalent cations are lower than those of divalent cations because of hydrolysis. Soil properties such as soil organic matter, soil pH, and iron oxides significantly affected the binding energy and adsorption energy of ions. Our results deepened our understanding about the non specific adsorption of ions in soil chemistry, and enlarged the research area of soil chemistry in fundamental and methodology.  相似文献   

The Cherenkov Telescope Array potential for the study of young supernova remnants     

《Astroparticle Physics》2015

Supernova remnants (SNRs) are among the most important targets for γ-ray observatories. Being prominent non-thermal sources, they are very likely responsible for the acceleration of the bulk of Galactic cosmic rays (CRs). To firmly establish the SNR paradigm for the origin of cosmic rays, it should be confirmed that protons are indeed accelerated in, and released from, SNRs with the appropriate flux and spectrum. This can be done by detailed theoretical models which account for microphysics of acceleration and various radiation processes of hadrons and leptons. The current generation of Cherenkov telescopes has insufficient sensitivity to constrain theoretical models. A new facility, the Cherenkov Telescope Array (CTA), will have superior capabilities and may finally resolve this long standing issue of high-energy astrophysics. We want to assess the capabilities of CTA to reveal the physics of various types of SNRs in the initial 2000 years of their evolution. During this time, the efficiency to accelerate cosmic rays is highest. We perform time-dependent simulations of the hydrodynamics, the magnetic fields, the cosmic-ray acceleration, and the non-thermal emission for type Ia, Ic and IIP SNRs. We calculate the CTA response to the γ-ray emission from these SNRs for various ages and distances, and we perform a realistic analysis of the simulated data. We derive distance limits for the detectability and resolvability of these SNR types at several ages. We test the ability of CTA to reconstruct their morphological and spectral parameters as a function of their distance. Finally, we estimate how well CTA data will constrain the theoretical models.  相似文献   

TeV γ-ray fluxes from the long campaigns on Mrk 421 as constraints on the emission of TeV–PeV neutrinos and UHECRs     

《Astroparticle Physics》2015

Long TeV γ-ray campaigns have been carried out to study the spectrum, variability and duty cycle of the BL Lac object Markarian 421. These campaigns have given some evidence of the presence of protons in the jet: (i) Its spectral energy distribution which shows two main peaks; one at low energies (∼1 keV) and the other at high energies (hundreds of GeV), has been described by using synchrotron proton blazar model. (ii) The study of the variability at GeV γ-rays and X-rays has indicated no significant correlation. (iii) TeV γ-ray detections without activity in X-rays, called “orphan flares” have been observed in this object.Recently, The Telescope Array Collaboration reported the arrival of 72 ultra-high-energy cosmic rays with some of them possibly related to the direction of Markarian 421. The IceCube Collaboration reported the detection of 37 extraterrestrial neutrinos in the TeV–PeV energy range collected during three consecutive years. In particular, no neutrino track events were associated with this source. In this paper, we consider the proton–photon interactions to correlate the TeV γ-ray fluxes reported by long campaigns with the neutrino and ultra-high-energy cosmic ray observations around this blazar. Considering the results reported by The IceCube and Telescope Array Collaborations, we found that only from ∼25% to 70% of TeV fluxes described with a power law function with exponential cutoff can come from the proton–photon interactions.  相似文献   

Astrophysical ZeV acceleration in the relativistic jet from an accreting supermassive blackhole     

《Astroparticle Physics》2014

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Effects of continuous flow centrifugation on measurements of trace elements in river water: intrinsic contamination and particle fragmentation     

Patrick Ross  Davide Vignati  Janusz Dominik 《水文研究》2006,20(13):2745-2754

Continuous flow centrifugation (CFC) is a well‐established technique used in natural surface water studies to collect large amounts of suspended solids, thus allowing a broad spectrum of measurements. However, a potential contamination or changes in the particle size distribution during the centrifugation may restrain the use of CFC effluents for element analysis in the colloidal and dissolved fractions. In this paper we evaluate the possibility of using the effluent of a Westfalia centrifuge (type KA2‐06‐075, 9700 rpm) for such analysis. This evaluation is based on two laboratory experiments with deionized and tap water and two field experiments in rivers. Elemental concentration changes across the CFC were assessed from the CFC influent and effluent after a filtration at 0·45 µm. Significant increases were found, mainly in the field experiments at a high suspended solids level and a slightly acid pH. A hypothesis was made on the origin of these increases as a superposition of a centrifuge intrinsic contamination and a particle fragmentation effect. A numerical model based on elemental concentration measurements (inductively coupled plasma mass spectrometry) gave a particle fragmentation level of 0·55% (mass percentage of particles broken up into smaller fragments during centrifugation). In another experiment, a direct particle counting (single particle counter) shows an excess of particles smaller than 500 nm in the CFC effluent, corresponding to a fragmentation level of 0·11%. In consequence, the use of CFC effluent for element analysis is possible in low‐turbidity river or lake waters, but should be carefully considered in waters with high suspended matter contents. Copyright © 2006 John Wiley & Sons, Ltd.  相似文献   

The interaction of cosmic rays and magnetized plasma     

A. R. Bell 《Monthly notices of the Royal Astronomical Society》2005,358(1):181-187

A large flux of cosmic rays streaming through a magnetized plasma creates cavities of low plasma density and low magnetic field. The magnetic field focuses the cosmic ray trajectories into the cavities with the possible formation of filaments or beams of high-energy cosmic rays.  相似文献   

Some observations on the effect of ozone treatment on suspended particulate matter in seawater     

Hasong Pak  James Kitchen  Percy Donaghay  J. Ronald  V. Zaneveld 《Estuarine, Coastal and Shelf Science》1981,13(3):327-336

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Contribution of domain rotation to the magnetic susceptibility of spherical two-domain particles of magnetite     

R. J. Veitch 《Geophysical Journal International》1986,86(2):229-240

Summary. Starting with a simplified picture of the presumed magnetization configuration in a two-domain sphere of magnetite, the initial susceptibility due to rotation of the magnetization in the domains has been calculated. In particles between 100 and 300 nm in diameter the calculated susceptibility for randomly oriented particles drops rapidly from about 6 to a little over 3, which is the value to be expected for large multidomain particles. The results agree well with the available experimental results and imply that in magnetite particles in this size range the low field susceptibility is dominated by the domain rotation and that wall motion is effectively inhibited.  相似文献   

Thermosolutal-convective instability in a stellar atmosphere     

R. C. Sharma  Bakshis Singh 《Journal of Astrophysics and Astronomy》1987,8(4):305-314

The thermosolutal-convective instability of a stellar atomsphere is studied in the presence of suspended particles. The criteria for monotonic instability are derived and are found to hold good also in the presence of uniform rotation and uniform magnetic field on the thermosolutal-convective instability. The thermosolutal-convective instability of a stellar atmosphere is also studied in the presence of suspended particles and radiative transfer effects and the criteria for monotonic instability are obtained in terms of source function.  相似文献