Chemical weathering and CO2 consumption in the glaciated Karuxung River catchment,Tibetan Plateau     

Fan Zhang  Xiong Xiao  Lijie Wang  Chen Zeng  Zhengliang Yu  Guanxing Wang  Xiaonan Shi 《水文研究》2021,35(8):e14330

Climate factors play critical roles in controlling chemical weathering, while chemically weathered surface material can regulate climate change. To estimate global chemical weathering fluxes and CO₂ balance, it is important to identify the characteristics and driving factors of chemical weathering and CO₂ consumption on the Tibetan Plateau, especially in glaciated catchments. The analysis of the hydro-geochemical data indicated that silicate weathering in this area was inhibited by low temperatures, while carbonate weathering was promoted by the abundant clastic rocks with fresh surfaces produced by glacial action. Carbonate weathering dominated the riverine solute generation (with a contribution of 58%, 51%, and 43% at the QiangYong Glacier (QYG), the WengGuo Hydrological Station (WGHS), and the lake estuary (LE), respectively). The oxidation of pyrite contributed to 35%, 42%, and 30% of the riverine solutes, while silicate weathering contributed to 5%, 6%, and 26% of the riverine solutes at the QYG, WGHS, and LE, respectively. The alluvial deposit of easily weathering fine silicate minerals, the higher air temperature, plant density, and soil thickness at the downstream LE in comparison to upstream and midstream may lead to longer contact time between pore water and mineral materials, thus enhancing the silicate weathering. Because of the involvement of sulfuric acid produced by the oxidation of pyrite, carbonate weathering in the upstream and midstream did not consume atmospheric CO₂, resulting in the high rate of carbonate weathering (73.9 and 75.6 t km⁻² yr⁻¹, respectively, in maximum) and potential net release of CO₂ (with an upper constraint of 35.6 and 35.2 t km⁻² yr⁻¹, respectively) at the QYG and WGHS. The above results indicate the potential of the glaciated area of the Tibetan Plateau with pyrite deposits being a substantial natural carbon source, which deserves further investigation.  相似文献   

氨氮急性攻毒对水产经济动物棘胸蛙(Paa spinosa)蝌蚪死亡率、排氨率、耗氧率及窒息点的影响     

牛春格  杨程  申屠琰  郑晓静  王志铮 《海洋与湖沼》2019,50(1):188-196

以体长(1.932±0.204)cm、体质量(1.386±0.055)g的棘胸蛙蝌蚪为实验动物,在水温(24±0.2)℃、DO(7.30±0.01)mg/L、pH 7.30±0.01条件下,采用静水停食法开展了氨氮对蝌蚪的急性攻毒实验,并以此为基础,测定了不同氨氮质量浓度胁迫下棘胸蛙蝌蚪的排氨率、耗氧率、氧氮比及窒息点。结果表明:(1)蝌蚪对氨氮急性攻毒具明显的运动避毒行为,濒死个体的背部皮肤和肝脏均具明显的色变症状;(2)氨氮对蝌蚪的急性致死率具明显的剂量—时间效应,24h、48h、72h、96h LC50依次为177.5、151.7、148.6和146.8mg/L,毒性时段蓄积程度系数呈持续下降趋势,24—48h、48—72h、72—96h的时段MAC值分别为84.04%、10.1%和5.86%;(3)蝌蚪夜均、昼均、日均及时段排氨率随氨氮质量浓度增加均呈阶梯式下降趋势,其中时段排氨率与对照组均无显著差异的为9.80mg/L实验组,夜均、昼均、日均及时段排氨率与对照组均无显著差异的仅为2.45mg/L实验组(P0.05);(4)氨氮对蝌蚪呼吸耗氧具低毒兴奋效应,其夜均、昼均和日均耗氧率随氨氮质量浓度增加均呈先升后降趋势,峰值氨氮质量浓度范围均为4.90—7.35mg/L(P0.05),与对照组均无显著差异的仅为14.70mg/L实验组(P0.05),窒息点含氧量随氨氮质量浓度增加呈先降后升趋势,谷底出现于4.90mg/L实验组(P0.05),与对照组无显著差异的仅为9.80mg/L实验组(P0.05);(5)实验期间,蝌蚪氧氮比(O:N)波动于18.87—25.34之间,昼均和日均氧氮比(O:N)随氨氮质量浓度增加均依次呈"上升—稳定—下降—再稳定"之趋势,两者的峰值氨氮质量浓度范围分别为4.90—14.70mg/L和4.90—9.80mg/L,夜均氧氮比(O:N)呈先升后降趋势,峰值出现于7.35mg/L实验组(P0.05)。  相似文献   

基于分光光度法的多量程海水营养盐原位传感器检测系统设计     

綦声波  任军博  马然  张述伟 《海洋科学》2019,43(11):76-83

针对传统海水营养盐检测方法不能满足海水营养盐长期原位监测需求的问题,研制了一种基于分光光度法的多量程海水营养盐原位传感器检测系统,通过对系统的高度集成及对多量程检测、低功耗技术、漏液保护技术的应用,实现了对海水5项营养盐参数快速、宽范围、高精度的原位测量。经过实验室和青岛中苑码头现场测试,表明本营养盐传感器检测系统具有低功耗、高可靠性能,可满足对5项营养盐参数的快速精确测量要求,实现了对海水营养盐参数的原位监测,为相关部门及时了解海洋生态环境和水体富营养化程度提供了数据支持,具有重大现实意义。  相似文献   

新冠病毒疫情期间复工复产卫星遥感监测     

陶金花  范萌  顾坚斌  陈良富 《遥感学报》2020,24(7):824-836

本文利用美国新一代极轨卫星NPP搭载的VIIRS载荷数据反演获得的热点数据，以及美国NASA的Aura卫星搭载的OMI载荷的二氧化氮对流层柱浓度资料，对中国地区2020-01—02及2019年同期，以及抗击疫情期间和后期复工复产的情况进行监测。监测结果表明：（1）2020-02较1月份及2019年同期相比，工业企业的耗能水平却出现显著降低，NO₂浓度呈现显著下降趋势。（2）全国工业热源点数和分布范围及密度自2020-02-03正式复工后稳步提升。湖北省除武汉、黄石和鄂州地区仍可监测到少数热点外，其他地区2月份均未再监测到任何热点，也证明了湖北基本没有复工迹象。（3）疫情得到基本控制之后，京津冀地区工业热源点有显著增加，但新增区域一般仍处于低能耗水平。从全国大气NO₂柱浓度监测来看，复工开始前后与2019年同期相比，污染物浓度均呈现明显下降趋势，说明复工强度有限。（4）到3月初工业热源点及其能耗水平出现显著升高，中国大部分地区的热源企业虽已逐步复工生产，说明工业产能较2月有显著提升，但生产规模或产能并未完全恢复。  相似文献   

南美洲鳗鲡(Anguilla rostrata)的耗氧率(ROC)、窒息点(AP)和适温范围(RT)及对非离子氨(NIA)、NO2-的LC50和SC的研究     

杨小东  江兴龙  乐普敏  龚铭杰 《海洋与湖沼》2019,50(2):455-464

为研究南美洲鳗鲡(Anguillarostrata)的耗氧率及其对水温、低溶氧、非离子氨和亚硝酸盐耐受性,本研究采用自制的鱼类呼吸装置测定其耗氧率和窒息点,以黑仔鳗为试验材料,探索其对水温、非离子氨、亚硝酸盐耐受性。结果表明,南美洲鳗鲡耗氧率存在昼夜变化,其昼间耗氧率为(86.46±37.77)mg/(kgh),夜间耗氧率为(123.58±22.56)mg/(kgh),二者存在显著性差异(P0.05);在15—30°C范围内,耗氧率随温度升高逐渐增大,耗氧率和水温的回归方程y=–0.1316x2+9.4507x–13.712(R2=0.9993);南美洲鳗鲡的耗氧率随体质量增大而降低,耗氧量随体质量增加而增大,耗氧量和体重的回归方程为y=0.2321x0.8334(R2=0.9979);在水温25°C时其窒息点随鱼体质量的增大而降低,均重10g、40g和160g的鳗鲡窒息点溶解氧浓度分别为(0.98±0.25)、(0.46±0.06)和(0.32±0.02)mg/L;13—29°C为南美洲鳗鲡的适温范围,25—29°C为其生长适宜水温,在一定范围内的短时低水温或高水温环境对其损伤是可逆的;水中非离子氨对南美洲鳗鲡的LC50和SC分别为12.22mg/L和1.22mg/L,亚硝酸盐氮对南美洲鳗鲡的LC50和SC分别为61.68mg/L和6.17mg/L。  相似文献   

1992-2015年中亚五国土地覆盖与蒸散发变化   总被引：8，自引：0，他引：8  

阮宏威  于静洁 《地理学报》2019,74(7):1292-1304

1991年苏联解体,中亚五国独立使得土地覆盖与蒸散发格局发生深刻变化。以中亚五国为研究区,采用欧空局气候变化项目（CCI）土地覆盖和全球陆地数据同化系统（GLDAS）蒸散发数据,分析1992-2015年土地覆盖与蒸散发时空变化特征,进一步研究耕地蒸散耗水特征。结果表明：① 中亚五国土地覆盖变化具有阶段性特征,耕地扩张引起土地覆盖格局变化。1992-2003年耕地快速增加（1.1万km ²/a）,林地和草地大幅减少。2003-2015年耕地增速趋缓（0.3万km ²/a）,林地和草地有一定恢复,裸地和水体持续减少,城镇用地持续增长。耕地共增加12.3万km ²,林地和草地分别减少4.0万km ²和2.3万km ²,且集中于哈萨克斯坦中北部。裸地减少3.5万km ²,集中于哈萨克斯坦西南部,水体减少3.1万km ²,集中在咸海湖泊。乌兹别克斯坦耕地减少、裸地增加,吉尔吉斯斯坦、塔吉克斯坦和土库曼斯坦土地覆盖变化幅度较小;② 中亚五国蒸散发变化与土地覆盖格局基本一致。蒸散发总体呈增加态势（6 mm/a）,1992-2003年快速增加（11.3 mm/a）,2003-2015年缓慢上升（2.4 mm/a）。中亚五国年蒸散发达到276.8 mm,东南部的吉尔吉斯斯坦（347.3 mm）和塔吉克斯坦（302.9 mm）最高,中北部的哈萨克斯坦（297.9 mm）次之,西南部的乌兹别克斯坦（211.0 mm）和土库曼斯坦（150.0 mm）最低;③ 中亚五国蒸散耗水结构受耕地面积大小的影响。中亚五国耕地蒸散耗水的贡献由24.7%增至27.9%,土库曼斯坦耕地蒸散耗水仅占本国的11%,其他国家均超过25%。草地、林地和裸地的蒸散耗水贡献降低,但哈萨克斯坦、吉尔吉斯斯坦和塔吉克斯坦仍以草地和林地蒸散耗水为主（≥ 50%）,土库曼斯坦（61.3%）和乌兹别克斯坦（46.4%）的裸地蒸散耗水占绝对优势。本文明确了中亚五国土地覆盖连续动态变化过程,细化各国土地覆盖与蒸散发特征及差异,增强对土地覆盖与蒸散发现状的认识,可为水土资源管理和生态环境保护提供数据参考。  相似文献   

青藏高原晚始新世干旱化事件：改则盆地康托组碳酸盐岩碳氧同位素的记录     

姜高磊  徐亚东  宋博文  张克信  罗亮 《地质学报》2016,90(8):2023-2034

改则盆地位于青藏高原腹地,盆地内沉积物记录了高原古环境变化的重要信息。本文对改则盆地康托组碳酸盐岩碳氧同位素进行研究,结果显示改则盆地中-晚始新世的演化分为两个阶段:1中始新世湿润气候下开放湖盆阶段:虽然碳酸盐岩δ~(18)O值在43层处向正值偏移,但整体~(18)O和~(13)C强烈亏损,并且该时期碳酸盐岩δ~(18)O值和δ~(13)C变化相关系数为R~2=0.082。表明该阶段的研究区虽然经历过短期蒸发作用增强或补给水减少,但整体是气候湿润条件下补给水丰富的开放型湖盆。2晚始新世干旱气候下封闭湖盆阶段:经过中新世晚期(63层)气候和湖泊水文状态的过渡,晚始新世~(18)O和~(13)C同位素富集,δ~(18)O值和δ~(13)C值变化相关系数为R~2=0.7762。表明该阶段气候干旱,蒸发作用强烈,湖盆萎缩成为封闭湖盆。综合前人研究,认为青藏高原腹地及北缘、东北缘在晚始新世存在明显的区域性干旱化事件。对比分析青藏高原隆升、全球气候记录、全球海水Sr和大气CO_2记录,认为青藏高原腹地和北部的干旱化事件主要受青藏高原隆升的影响。  相似文献   

硫酸参与的长江流域岩石化学风化速率与大气CO2消耗   总被引：4，自引：0，他引：4  

张连凯  覃小群  刘朋雨  黄奇波 《地质学报》2016,90(8):1933-1943

流域的岩石化学风化过程是全球碳循环中的重要环节。以往的流域水化学碳汇通量估算大多是基于碳酸的风化作用。而实际上,硫酸和碳酸一样,也参与了流域碳元素的地球化学循环,从而对全球碳循环过程产生影响。长江流域水体近几年出现酸化现象,大部分河段SO42-和Ca2+含量增高,其对应的岩石风化过程和大气CO2消耗速率也发生变化。文章对长江干流及主要支流2013年不同季节的离子组成进行监测,利用水化学平衡法和Galy估算模型,对长江流域岩石化学风化速率和CO2消耗通量进行了估算,对硫酸参与下的长江流域岩石风化和碳循环过程进行了分析。结果表明,长江流域水体离子主要来源于硅酸盐岩风化和碳酸盐岩风化。其中碳酸盐岩风化对河水离子贡献率为92%。在硅酸盐岩广泛分布的赣江流域,碳酸盐岩风化离子贡献也达85%。分析表明,硫酸参与了长江流域的岩石风化过程,对水体中离子产生一定影响。硫酸的参与加快了碳酸盐岩的化学风化速率,平均提高约30%,但是使流域大气CO2消耗速率降低。在不考虑蒸发岩溶蚀作用下,平均从516×103 mol/km2·a降至356×103 mol/km2·a,降低约31%。在各支流中,硫酸对乌江流域碳酸盐岩的风化和碳循环的影响最大,而对雅砻江的影响最小,这与乌江流域的含煤地层、矿床硫化物及大气酸沉降有关。  相似文献   

Magma associations in Ediacaran granitoids of the Cachoeirinha‒Salgueiro and Alto Pajeú terranes,northeastern Brazil: Forty years of studies     

《Journal of South American Earth Sciences》2016

Granitic magmatism in the Cachoeirinha‒Salgueiro and Alto Pajeú terranes in the Transversal Zone Domain of the Borborema Province, northeastern Brazil, occurred in three main time intervals: 650–620 Ma, 590–560 Ma and 545–520 Ma. The oldest one is characterized by intrusions of magmatic-epidote (mEp) bearing calc-alkalic (some with trondhjemitic affinities) and high-K calc-alkalic plutons, synkinematic to the main regional foliation, under contractional tectonic regime, and exhibits T_DM < 2.0 Ga and ƐNd (0.6 Ga) from −1 to −4, and δ¹⁸O (zircon) values from 7.1 to 10‰_VSMOW. O- and Nd-isotope data for the 650‒620 Ma group of plutons is compatible with partial fusion of subducted oceanic basaltic crust (mEp-bearing calc-alkalic tonalites/granodiorites, equivalent to adakites). Voluminous intrusions in the 590–560 Ma interval are represented by abundant mEp-free high-K calc-alkalic, peralkalic, ultrapotassic, mEp-bearing high-K calc-alkalic, and less abundant shoshonitic magmas. Nd-model ages for this group of plutons vary from 1.5 to 2.5 Ga and ƐNd (0.6 Ga) ranges from −8 to −20; δ¹⁸O (zircon) varies from 6.4 to 7.9‰_VSMOW. Values of δ¹⁸O (zircon) for the 590‒560 Ma old group of plutons coupled with Nd isotope data are compatible with remelting of crustal (negative ƐNd, 1.6 to 2.0 Ga old) source rocks. O- and Nd-isotope data for this group of plutons are compatible with underplating of basaltic magma in the base of the lower crust for the high-K calc-alkalic granitoids, coeval to transcurrent movements along sigmoidal shear zones. Intrusion of one shoshonitic (Serrote do Arapuá), one calc-alkalic (Riacho do Icó) plutons besides the peralkalic Manaíra-Princeza Isabel dike set have witnessed this transition from contractional to transcurrent movements along shear zones, around 610‒600 Ma.  相似文献   

Comparative Study of the Carbon Emission Situation and Goals between China and India     

Yang Zhanhong  Luo Hong  Xue Jie  Zhang Baoliu 《地球科学进展》2016,31(7):764-773

As the two large developing and populous countries, China and India face the dual challenges of economic development and climate change. Both of them are active in carbon emissions reduction, while India also bears the pressure of being “benchmarked” against China. With taking China and India as the sample of a comparative analysis, and the statistical value of a long sequence as the basic analysis data, based on the detailed analysis and comparison of carbon emissions history, the carbon emissions situation of the two countries from various dimensions including economic development, energy reserves and consumption, etc. were comparatively analyzed. The carbon intensity and energy structure after achieving the objectives were measured and compared by focusing on the carbon emissions reduction targets in China and India. The comparative results show that: China’s total carbon emissions are greater than India’s, but the growth rate of emissions, per capita emissions are significantly lower than India’s, while the carbon intensity decreases significantly faster than that of India. China has taken more efforts to make commitments to carbon reduction than India. With India’s energy structure adjustment, the situation will be gradually better than that in China.  相似文献