Atmospheric input of trace elements to the western Pacific Ocean and the Kuroshio ocean area     

Qian Fenlan  Yu Hongjian  Lan Youchang  Chen Zhi  Zhou Mingyu  Farn Parungo  Wu Peiming 《海洋学报(英文版)》1996,15(1):69-84

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离子色谱分析在黄土和粉尘研究中的应用   总被引：1，自引：0，他引：1  

王丹  屈文军  张小曳  严立文  曹国良 《海洋地质与第四纪地质》2005,25(1):113-118

黄土中存在着大量的碱金属及碱土金属，以往的测试方法多为原子吸收和ICP—MS，离子色谱法在测试黄土样品的碱金属和碱土金属元素含量中应用不多。将黄土地质标准样品进行消解后用离子色谱进行测试，测试效果良好，重复测试的相对标准偏差小于5％，与推荐值的相对误差小于5％，准确度和精密度符舍相关的质量控制要求。本实验方法测试的离子含量都在仪器响应呈线性的最佳测试范围之内，标准曲线经回归后相关系数均达到0．9999。黄土样品的分析结果与粉尘气溶胶样品的离子分析结果对比表明，此方法对于探讨粉尘起源以及沙尘暴天气的研究具有重要意义。  相似文献   

南极中山站大气气溶胶的化学组成及其来源的判别   总被引：1，自引：1，他引：1  

黄自强  暨卫东  杨绪林  黄荣坦  汤荣坤  于涛  张功勋 《台湾海峡》2003,22(3):334-346

从1998年3月7日至1999年11月23日历时21个月，在南极中山站连续采集89个海洋气溶胶样品，本文提供全部样品的13种化学元素Cu、Pb、Zn、Cd、Fe、Al、Mn、Cr、V、K、Na、Ca、Mg含量的实测值．研究表明中山站气溶胶化学成份的含量具有季节性变化的特征．通过相关分析、因子分析、富集因子等方法判别不同时间段中山站气溶胶化学成份的来源。  相似文献   

晚新生代亚洲干旱气候发展与全球变冷联系的风尘沉积证据   总被引：14，自引：8，他引：6       下载免费PDF全文

鹿化煜  王先彦  李郎平 《第四纪研究》2008,28(5):949-956

在干旱气候背景下常常有风尘物质的释放和传输,风尘沉积被认为是干旱环境变化良好的地质记录。在亚洲中部和中国北方,大面积的干旱区被沙漠戈壁覆盖,这些地区是粉尘物质的重要源地,释放的风尘物质影响局地和区域环境,并通过参与生物地球化学循环等影响更大空间尺度的气候变化。因此,亚洲中部干旱气候的形成和演化以及发展趋势一直受到重视。长期以来,关于晚新生代亚洲中部干旱气候发展的驱动机制至少有两种解释:一是青藏高原的隆升控制着亚洲中部的干旱化过程,随着高原的阶段性隆升亚洲干旱气候逐步增强;二是晚新生代全球变冷直接驱动着亚洲变干,全球变冷是主导因素。中国黄土高原及其周边地区堆积的黄土-红粘土序列是指示亚洲干旱化过程良好的地质记录,通过对新获得的风尘堆积记录的分析,发现在晚新生代中国风尘堆积的时空演化与全球变冷有较好的对应,全球变冷可以促使亚洲中部干旱气候发展并加强粉尘活动,而青藏高原隆升的幅度和时间还不清楚,进而认为是全球变冷而不是青藏高原隆升直接驱动亚洲内陆的阶段性变干。基于这些结果,我们认为以前关于青藏高原隆升影响全球气候的结论可能高估了青藏高原在地球环境演化中的作用,关于高原隆升直接驱动亚洲干旱化的结论还需要检验。  相似文献   

Circumstellar dust and circumstellar extinction curves     

N. V. Voshchinnikov  F. J. Molster  P. S. Thé 《Astrophysics and Space Science》1995,224(1-2):223-226

We have calculated the circumstellar extinction curves produced by dust grains which absorb and scatter the stellar radiation in the shells of pre-main-sequence stars. A Monte Carlo method was used to model the radiative transfer in non-spherical shells. The dependence on the particle size distribution and the dust shell parameters has been examined.The application of the theoretical results to explain the extinction and polarization of the Herbig Be star HD 45677 shows that the dust shell is not disk-like and that very small grains are absent in it.  相似文献   

南极长城站地区现代环境地球化学特征          下载免费PDF全文

赵俊琳 《极地研究》1990,2(2):1-12

本文通过环境背景值、风化壳地球化学、对流层(大气气溶胶)地球化学和人为地球化学异常,初步探讨了南极长城站地区的现代环境地球化学特征。分析表明:环境要素固有的地球化学性质、区域环境条件和自然环境演变之间具有深刻的内在联系。  相似文献   

Characterization of polycyclic aromatic hydrocarbons （PAHs） in aerosols around Guiyang City, China     

《中国地球化学学报》2006,25(B08):181-181

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Characterization of microbial communities associated with African desert dust and their implications for human and ecosystem health     

Christina A. Kellogg 《中国地球化学学报》2006,25(B08):218-219

Desert winds aerosolize several billion tons of soil-derived dust each year, including concentrated seasonal pulses from Africa and Asia. Huge dust events create an atmospheric bridge over continents and oceans, and eject a large pulse of soil-associated microorganisms into the atmosphere. These dust events might therefore have a role in expanding the biogeographical range of some microorganisms by facilitating rare long-distance dispersal events. The goal of this study is to characterize the microbes associated with African dust events and determine if they pose a risk to humans or downwind ecosystems. Air samples were collected by vacuum filtration in a source region （Mali, West Africa） during dust events and plated on R2A media to culture microorganisms. These organisms were compared to those in similar samples collected in the Caribbean during Saharan/Sahelian dust events. A high-volume liquid impinger is currently being tested in Barbados, collecting aerosol samples during African dust events. Over 100 bacteria and fungi （19 genera of bacteria and three genera of fungi） have been characterized from source region dust events.  相似文献   

Natural siliceous dust and human health： Pathways, toxicity, and impact     

Edward Derbyshire 《中国地球化学学报》2006,25(B08):219-219

Fine atmospheric dust includes mineral particles and aggregates, fibrous minerals and fibrous organic material. Generation, dislodgement and transport （deflation） of natural dust with the finer （〈4 microns） components suspended as silt-size aggregates, is widespread in and adjacent to the world＇s drylands, as well as deriving from volcanic vents. Silica is a highly fibrogenic agent in lung tissue. Long-term inhaling of siliceous dusts can lead to a number of fibrotic lung diseases, including natural （non-occupational） pneumoconioses （notably silicosis, but including asbestosis and others）. Different polymorphs of silica show different levels of toxicity in interaction with lung tissue. Particles with highly active surfaces may release radicals, causing cell damage. Some types of inhaled particulates are degraded by macrophages, but many are highly resistant and persist in the lungs, some stimulating fibroblastic cells to deposit collagen. Silicosis is an inflammation of the lung commonly caused by silicate mineral particles, leading to fibrosis. Three types are recognized： nodular pulmonary fibrosis （simple or chronic silicosis）, acute silicosis, and accelerated silicosis. Generally, finer particulates have greater oxidative capacity than the coarser fractions. They contain more reactive oxygen species, their greater bioreactivity making them more toxic to pulmonary tissue. Nevertheless, inhalation of large dust particles （〉 10μm） may constitute a health risk if the mineralogy is toxic, regardless of where the grains lodge in the respiratory system. Dust may absorb harmful gases, disease-generating bacteria and carcinogenic hydrocarbon compounds. Silica-related respiratory disease may also an exacerbate cardiac problem, and epidemiology suggests a link with tuberculosis. Quantification of dust loading and exposure requires study of spatial and temporal patterns, supported by meteorological analysis, airflow modeling and satellite-borne imagery. Some acute, short-term health impacts have been assessed using atmospheric and health records both before and after a dust storm or by comparison of populations within and outside such events. Analysis of the size, shape, mineralogy and geochemistry of ambient dust particulates provides information on natural dust sources, dust concentrations, and potential particulate toxicity, as well as providing a datum for assessment of human exposure levels.  相似文献   

Factors controlling the spatial and temporal variability of dust emissions     

John A. Gillies William G. Nickling Vicken Etyemezian James King Mark Sweeney 《中国地球化学学报》2006,25(B08):219-220

New field measurement techniques are allowing researchers to better understand how surficial properties affect the temporal and spatial variability of dust emissions. In this paper we review the current understanding of the dust emission process and present new field measurements that examine how three surface properties： roughness, crust strength, and temporal changes of surface properties affect dust emissions. These data were collected using three unique measurement systems developed by our team. Roughness exerts considerable control on the entrainment threshold and emissions of dust from a surface. We have carried out a series of experiments designed to quantify roughness effects on aeolian sediment entrainment and transport in a shear stress partitioning framework. Our results show that the model of Raupach et al. （1993） provides very good agreement with available data to predict the amount of shearing stress on the intervening surface among roughness elements, relatively independent of their size and distribution. However, element size affects the aeolian sediment transport process beyond that attributable only to the reduction of surface shear stress caused by the roughness. Additional interactions of the elements with the saltation cloud appear to reduce the transport efficiency and potentially dust emissions as well. The effect of crust strength on dust emissions was assessed using a newly-developed pin penetrometer, which can measure crust strength in-situ. Previous researchers suggested that variation in crust strength even within a small area could lead to considerable spatial variability in dust emissions. Our measurements showed that crust strength is highly variable over a scale of centimeters. This variability may help to explain some of the observed scatter in field measurements of dust emissions for what appear to be homogeneous surfaces. Variability of dust emissions in time and space was also evaluated using a new instrument, the Portable In-Situ Wind Erosion Lab （PI-SWERL） developed to measure dust emissions from soil surfaces.  相似文献