新元古代大冰期及其诱发因素     

钱迈平  袁训来  肖书海 《江苏地质》2000,24(3):135-139

简要介绍了由美国一些科学家最近提出的,引起国际地球科学、环境科学、生命科学及宇宙科学界广泛关注的新元古代雪球假说,及其近期研究情况。根据我国扬子地层分区和江南地层分区震旦系的沉积特征,对新元古代古气候骤变,大冰期的发生与消亡及其诱发因素作了初步探讨。  相似文献   

Metal Distribution in Different Size Fractions of Natural Organic Matter     

Daniel Schmitt  Margit B. Müller  Fritz H. Frimmel 《洁净——土壤、空气、水》2001,28(7):400-410

In this paper, size‐exclusion chromatography (SEC) was used to determine the metal concentration in different size fractions of a bog lake water. Two methods were applied: (a) preparative SEC with off‐line metal concentration analysis and (b) direct coupling of an analytical SEC system on‐line with an inductively‐coupled plasma mass spectrometer (ICP‐MS). In the preparative SEC measurements, maximum concentrations were found for different metal ions in different size fractions of the natural organic matter (NOM). Normalization of metal concentrations to dissolved organic carbon concentration (DOC) yielded two maxima in the high and in the very low molecular‐weight fractions. Whereas good recoveries were found for Al, Fe, and Ni, only 40% were obtained for Pb. This indicates that Pb formed labile complexes with NOM, and hence could strongly interact with the column material. In the experiments with the analytical SEC‐ICP‐MS system, the same trends were observed, but with even lower recoveries than in the preparative system. Sample preconcentration and storage were also investigated with respect to decrease in metal concentration. During the ultrafiltration preconcentration step Al and Fe were removed only to a small extent, whereas about half of the initial Pb was lost. This indicates that Al and Fe were mainly bound to high molecular‐weight fractions of NOM. In contrast to that, Al and in particular Fe were removed from solution more than proportionally with respect to DOC because of aggregation of the NOM during storage, whereas Pb and Ni were concentrated relative to the DOC.  相似文献   

PROBLEMS IN STUDIES ON CARBON AND OXYGEN STABLE ISOTOPES IN CARBONATES     

LI Xinqing  WAN Guojiang 《地球科学进展》1999,14(3):262-268

Carbon and Oxygen stable isotopes in carbonates have long been the important geochemical tracers. Studies on the isotopic compositions can provide insights into the paleoclimatic processes, the paleoceanic environmental processes and the geological processes as well. Researches of more than four decades in the field, especially from the early 1980s on, during which the analysis of the isotopes in fossil brachiopods and early diagenetic cements has contributed much to the knowledge, achieved appreciable progress. However, problems still remained with how to explain the data that already existed on the isotopic compositions of carbonates, on which there is a dichotomy between those who advocate that the data represent the original characteristics of the isotopes and those who argue that the data have been altered diagenetically; with how to select the samples of carbonate for analysis of the isotopic ratios, which has a set of criteria, namely, the microstructure, the Cathodoluminescence and trace elements, for tests of the sample preservations; with whether the fossil brachiopods′shells have vital effects on the isotopic compositions, on which there is a tendency toward the existence in recent years; with to what extent the living environment variations of the fossil affect their carbon and oxygen isotopic ratios and with the utilization of early diagenetic cement as analyzing samples. Along with the problem raising, this paper reviewed the
methods on, and new developing trends toward, the problem-solvings, as well as the up-to-date advances of studies on each problem.  相似文献   

A preliminary study on benthos food web structure of tidal zone in the Laoshan Bay by using stable carbon isotopes     

Cai Deling  Hong Xuguang  Mao Xinghu  Zhang Shufang  Gao Sulan 《海洋学报(英文版)》2000,19(4):81-89

By analyses of carbon isotopic composition(δ¹³C values) of the benthos collected in the Laoshan Bay in August 1993 and February and May 1994, it is found that the main food sources of the benthos can be divided into four groups in terms of carbon isotope composition: Particulate Organic Matter (POM),benthic diatoms, benthic macroalgae and the organic matter in sediments.The results show that the carbon isotopic composition of the benthic animals has a close relation with that of the food they take in.The carbon isotopic compositions of benthos may be useful in elucidating their food sources.The carbon isotopic data have confirmed that POM is the main food source of the benthic filter feeders such as bivalves; crustaceans have a wide range of δ¹³C values, showing their food source has diversity; benthic diatoms are an important fraction of the food for most of gastropods.A preliminary investigation of the benthic-pelagic coupling in that region using the stable carbon isotopic tracers has confirmed the importance of POM as a food source for benthos in this region,but the organic matter in sediments and benthic diatoms are also relatively important for a lot of benthic animals.The benthic-pelagic coupling in the Laoshan Bay temperate ecosystem is not so tight as that in ecosystems at higher latitudes such as north-eastern water polynya.  相似文献   

The international at-sea intercomparison of fCO₂ systems during the R/V Meteor Cruise 36/1 in the North Atlantic Ocean     

Arne Krtzinger  Ludger Mintrop  Douglas W. R. Wallace  Kenneth M. Johnson  Craig Neill  Bronte Tilbrook  Philip Towler  Hisayuki Y. Inoue  Masao Ishii  Gary Shaffer  Rodrigo F. Torres Saavedra  Eiji Ohtaki  Eiji Yamashita  Alain Poisson  Christian Brunet  Bernard Schauer  Catherine Goyet  Greg Eischeid 《Marine Chemistry》2000,72(2-4)

The ‘International Intercomparison Exercise of fCO₂ Systems’ was carried out in 1996 during the R/V Meteor Cruise 36/1 from Bermuda/UK to Gran Canaria/Spain. Nine groups from six countries (Australia, Denmark, France, Germany, Japan, USA) participated in this exercise, bringing together 15 participants with seven underway fugacity of carbon dioxide (fCO₂) systems, one discrete fCO₂ system, and two underway pH systems, as well as systems for discrete measurement of total alkalinity and total dissolved inorganic carbon. Here, we compare surface seawater fCO₂ measured synchronously by all participating instruments. A common infrastructure (seawater and calibration gas supply), different quality checks (performance of calibration procedures for CO₂, temperature measurements) and a common procedure for calculation of final fCO₂ were provided to reduce the largest possible amount of controllable sources of error. The results show that under such conditions underway measurements of the fCO₂ in surface seawater and overlying air can be made to a high degree of agreement (±1 μatm) with a variety of possible equilibrator and system designs. Also, discrete fCO₂ measurements can be made in good agreement (±3 μatm) with underway fCO₂ data sets. However, even well-designed systems, which are operated without any obvious sign of malfunction, can show significant differences of the order of 10 μatm. Based on our results, no “best choice” for the type of the equilibrator nor specifics on its dimensions and flow rates of seawater and air can be made in regard to the achievable accuracy of the fCO₂ system. Measurements of equilibrator temperature do not seem to be made with the required accuracy resulting in significant errors in fCO₂ results. Calculation of fCO₂ from high-quality total dissolved inorganic carbon (C_T) and total alkalinity (A_T) measurements does not yield results comparable in accuracy and precision to fCO₂ measurements.  相似文献   

A Model to Predict Granular Activated Carbon Backwash Curves     

Wojciech Dabrowski  Marta Spaczyńska  R. Ian Mackie 《洁净——土壤、空气、水》2008,36(1):103-110

A mathematical model that produces curves for predicting the expansion of granular activated carbon (GAC) filter beds has been developed and applied to several widely used commercial GAC products. Initially, the hydraulic load required to produce a given bed expansion was assumed to be inversely proportional to the viscosity. This assumption was then modified by assuming a power law for the dependence on viscosity. The errors were sufficiently small to allow practical application of the formulae presented in this paper. The potential for application of the method was tested and is illustrated by an example.  相似文献   

Ambient Precursor Gaseous Pollutants and Meteorological Conditions Controlling Variations of Particulate Matter Concentrations     

《洁净——土壤、空气、水》2017,45(8)

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Comparing carbon accumulation in restored and natural wetland soils of coastal Louisiana     

《国际泥沙研究》2019,34(6):600-607

Louisiana's chronic wetland deterioration has resulted in massive soil organic matter loss and subsequent carbon release through oxidation. To combat these losses, and reestablish ecosystem function, goods, and services, many restoration projects have been constructed or planned throughout coastal Louisiana. There are significant data gaps and conflicting results regarding wetland contributions to global warming, especially related to carbon sequestration in restored wetlands. An exceptionally large data set was used to derive carbon accumulation rates from key soil characteristics and processes. Assessments and comparisons of bulk density, organic matter, total carbon, vertical accretion (short- and longer-term), and carbon accumulation rates were made across time (chronosequence) and space (i.e., coastwide, watershed basins, and vegetation zones). Carbon accumulation rates in the Louisiana coastal zone were generally correlated to hydrogeomorphology, with higher rates occurring in zones of high river connectivity or in swamp or higher salinity tolerant marsh. On average, naturally occurring wetlands had higher carbon accumulation rates than restoration sites. Although some restoration measures were higher, and most showed increasing carbon accumulation rates over time. Results demonstrate that although wetland restoration provides many ecosystem benefits, the associated carbon sequestration may also provide useful measures for climate change management.  相似文献   

Spatiotemporal patterns of carbon sequestration in a large shallow lake,Chaohu Lake: Evidence from multiple-core records     

《Limnologica》2020

Lake sediment can sequestrate large amounts of carbon and this issue has become a research hotspot. However, most of research on carbon burial in lakes is based on a single (or a few) sediment core records and so may underestimate the variability of carbon burial features within a single lake. In this study, therefore, Chaohu Lake, a typical large shallow lake in the middle and lower reaches of the Yangtze River, was selected to conduct multiple, high resolution sediment core studies to elucidate that variability. Overall 18 sediment cores are analyzed according to paleolimnological proxies (including ²¹⁰Pb/¹³⁷Cs for 3 master cores); sediment accumulation rate, total organic carbon, grain size and loss of ignition is measured or estimated for most cores. The spatiotemporal variations of organic carbon burial rate (OCBR), carbon storage and their driving factors were examined. Results show: 1) There was a clear temporal difference in carbon burial during the past 150 years, with OCBR varying from 1.1 g C/m²/y to 25.6 g C/m²/y (mean 9.8 g C/m²/y). OCBR began to increase after around 1900, a rapid increase followed after 1950s and a downward trend after 1970s. Total carbon burial amount (OCBA) in the lake since the 1850s is 1.11 x 10¹⁰ g. 2) The average OCBR of six sediment cores in the northwest lake area is 13.4 g C/m²/y, significantly higher than that for sediment cores in other areas (9.6 g C/m²/y). 3) TOC, OCBR, OCBA in all 18 cores exhibited similar temporal patterns (i.e. marked increase since 1950s in most of the cores) but with significant differences in several lake locations. 4) During the last 150 years, carbon burial in Chaohu Lake appears to be greatly affected by changes in regional temperature and population size, according to their significant correlations. OCBR also has a significant correlation with the average lake level in the past 50 years, indicating human activity (notably dam building). This has imposed an important impact on OCBR in Chaohu Lake. This multi-sediment core study reveals the spatiotemporal characteristics of carbon burial in the lake and provides an important basis for increasing the accuracy of calculating carbon storage in large shallow lakes.  相似文献   

Mapping global forest biomass and its changes over the first decade of the 21st century     

Anping CHEN  Shushi PENG  Songlin FEI 《中国科学:地球科学(英文版)》2019,(3):585-594

Forests played an important role in carbon sequestration during the past two decades. Using a model tree ensemble method(MTE) to regress the seven reflectance bands of EOS-Terra-MODIS satellite data against country level forest biomass carbon density(BCD) of 2001–2005 provided by United Nations' s Forest Resource Assessment(FRA), we developed a global map of forest BCD at 1 km×1 km resolution for both 2001–2005 and 2006–2010. For 2006–2010, the total global forest biomass carbon stock is estimated as 279.6±7.1 Pg C, and the tropical forest biomass carbon stock is estimated as 174.4±5.4 Pg C. During the first decade of the 21 st century, we estimated an increase of global forest biomass of 0.28±0.75 Pg C yr^-1. Tropical forest biomass carbon stock slightly decreased(-0.31±0.60 Pg C yr^-1); by contrast, temperate and boreal forest biomass increased(0.58±0.28 Pg C yr^-1) during the same period. Our estimation of the global forest biomass carbon stock and its changes is subject to uncertainties due to lack of extensive ground measurements in the tropics, spatial heterogeneity in large countries, and different definitions of forest. The continuously monitoring of forest biomass carbon stock with MODIS satellite data will provide useful information for detecting forest changes.  相似文献