Gamma Emitters on Micro-Becquerel Activity Level in Air at Kraków (Poland)     

Sylwia Grabowska  Jerzy W. Mietelski  Krzysztof Kozak  Paweł Gaca 《Journal of Atmospheric Chemistry》2003,46(2):103-116

The Petryanov air filters combined into half-year sets were analyzed for the presence of ⁴⁰K, ¹³⁷Cs and ²²Na by means of low-background gamma rays spectrometry. Each sample contains aerosols from more than 1 Mm³ of air. Samples were collected in ground level air at Kraków (Southern Poland) from 1996 to 2002. Activity concentrations of ⁴⁰K are almost constant with the mean of 14.7± 4.5 Bq m^–3. Activity concentrations of ¹³⁷Cs, which are on the level of single Bq m^{– 3} show exponential decrease with effective half-life time of 7.07± 0.77 years. The cosmogenic ²²Na shows a strong seasonal variation with significant different mean values activity concentration between 0.333± 0.095 Bq m^–3 and 0.137± 0.045 Bq m^–3, for summer and winter, respectively. Moreover, the activity ratio for two cosmogenic radionuclides: ²²Na and measured previously ⁷Be show also changes with statistically significant seasonal differences. The lower values were found during winters. The mechanisms which might govern this ratio are discussed. The conclusion is that transport of ²²Na during summer seems to be so much effective, that results in kind of relative depletion of stratosphere of this nuclide.  相似文献   

历次核试验进入海洋的~(137)Cs对中国近海影响的模拟研究   总被引：1，自引：0，他引：1  

赵昌  乔方利  王关锁  舒启  夏长水 《海洋学报》2015,37(3):15-24

1945年以来,世界各主要核国家进行了数千次核试验,这些核试验产生的绝大部分放射性物质通过多种途径进入海洋,对海洋环境造成放射性污染。本文建立了一个准全球海洋的放射性物质输运和扩散数值模式,通过数值模拟手段评估了历史核试验释放的放射性物质137 Cs对中国近海海洋环境的影响。本文借助前人工作评估了核试验释放137Cs进入海洋的途径和总量;通过比较模拟结果与观测资料,表明本文建立的放射性物质模式能够较好地模拟出137Cs在中国近海及其邻近海域的分布情况和随时间演变特征;模拟结果表明中国近海里的137Cs浓度在20世纪50年代中期达到最大,其中吕宋海峡海域137Cs浓度最高,达80.99Bq/m3;进一步分析了2011年3月份日本福岛核事故前中国近海137Cs浓度分布状况,2011年整个中国近海137Cs浓度介于1.0~1.6Bq/m3间,且其浓度垂向分布较均匀,相对封闭的南海浓度略高于其他海域。  相似文献   

Quantitative assessment of dissolved radiotracers in the English Channel: Sources, average impact of la Hague reprocessing plant and conservative behaviour (1983, 1986, 1988, 1994)     

P. Bailly du Bois  P. Guguniat 《Continental Shelf Research》1999,19(15-16)

Knowledge of long-term movements of water-masses in the English Channel has been substantially improved using hydrodynamic modelling coupled with radio-tracers studies; nevertheless, the precision of results so obtained is still largely dependent on measurement precision. New tools are now available to make more accurate determinations of radio-tracer distribution: (1) Repositioning of station locations at the same tide reference-time, giving a homogeneous spatial data set, coupled with the possibility of interpolating and quantifying the amounts of dissolved radioactivity flowing through the English Channel; (2) the first measurements of tritium (³H) in seawater on a large scale in the English Channel demonstrate that this fully conservative radionuclide is a clearly identifiable marker of industrial releases; (3) recent campaigns carried out during the FLUXMANCHE II CCE (1994) programme show the general distribution of dissolved radionuclides ¹³⁷Cs, ¹³⁴Cs, ⁶⁰Co, ¹²⁵Sb, ¹⁰⁶Ru and ³H in the English Channel and the Irish Sea; and (4) the re-utilisation of data from previous campaigns (1983, 1986, 1988) provides indications, at any given location in the English Channel, about the average dilution and distribution of releases derived from the La Hague reprocessing plant. Excesses and losses of radionuclides are now quantified with respect to known source terms; estimates of losses are provided for non-conservative radionuclides, while an excess of ¹³⁷Cs was observed in the English Channel during the period 1983–1994. This excess, which has the same order of magnitude as the quantities released from La Hague plant in the English Channel, could be explained by about 1% of the Sellafield reprocessing plant releases entering the Channel. These results confirm and give a more detailed picture of the previously known distribution of water masses in the English Channel. They lead to clear information about transit times and dilution at this scale, and provide directly comparable data for the validation of hydrodynamic models.  相似文献   

近百年来东平湖沉积通量变化与环境   总被引：5，自引：0，他引：5  

陈影影  陈诗越  姚敏  刘加珍  张菊 《沉积学报》2010,28(4):783-789

根据210Pb、137Cs法建立的东平湖现代沉积年代序列,结合沉积物粒度与烧失量变化特征以及黄河变迁与流域人类活动的特点,分析探讨了1889年以来东平湖沉积通量的变化。研究表明,百年来东平湖沉积环境不稳定,沉积通量变化较大:1889~1938年,沉积通量较高且基本稳定,1938~1965年,沉积通量逐年下降,1965~2000年,沉积通量整体较低且基本稳定,2000年以来,沉积通量呈逐年上升趋势。早期的高沉积通量与东平湖作为黄河自然滞蓄洪区有关,后期由于人类活动（湖区治理、黄河水利工程建设等）控制了黄河水的自然倒灌,导致了沉积通量的下降并趋于稳定,近期沉积通量的上升是湖区经济活动增强的反映。  相似文献   

内蒙古高原中东部地区137Cs背景值的确定方法(英文)     

胡云锋  刘纪远  巴图娜存  甄霖 《地理学报(英文版)》2014,(6)

In isotope 137 Cs tracing studies, it is a premise to determine suitable 137 Cs reference inventory(CRI) plots and the CRI values. Owing to the heterogeneous spatial distribution of 137 Cs deposition in the ground and diverse, or even irregular, operations in sampling and testing procedures, CRI determination is usually faced with many difficulties and uncertainties. In addition, more difficulties occur in an investigation of a large-scale region because of time constraints and measurement cost limitations. In this study, traditional CRI acquiring methods were summarized first, and then a new complex scheme was established, involving seven core steps and coupling the model estimate and sample measurement. The above CRI determination methodology was implemented in the central-eastern Inner Mongolia Plateau. The case study results showed that the CRI in the dark chestnut soil sub-region, located in the east and south of Xing'an City, exhibited 2447 Bq·m–2; the CRI in the aeolian sandy soil sub-region, positioned in the south central Tongliao City and central Chifeng City, showed 2430 Bq·m–2; the CRI in the sandy chernozem soil sub-region, situated in the northwestern Chifeng City, presented 2384 Bq·m–2; and the CRI in the chestnut soil sub-region, in the southern Xilin Gol City, was 2368 Bq·m–2. The newly proposed CRI determination scheme was proved effective, and the determined CRI plots and CRI values were convincing. The methodology offered a framework for 137 Cs tracing studies in large-scale regions or long-distance transects.  相似文献   

P–T–t evidence for mechanisms of vertical tectonic motion in a contractional orogen: north-western US and Canadian Cordillera     

Whitney  Miller  & Paterson 《Journal of Metamorphic Geology》1999,17(1):75-90

The >1800 km long Coast Mountains–North Cascades orogen of the Canadian Cordillera and north-western US developed as a continental magmatic arc. Metamorphic rocks in the orogen contain widespread evidence for burial of supracrustal rocks to depths of c. 40 km, followed by nearly isothermal decompression to depths of <10 km. Near many shallowly-emplaced, mid-Cretaceous plutons, low-pressure contact metamorphic effects were overprinted by high-pressure regional metamorphic minerals and textures, as evidenced by kyanite±staurolite pseudomorphs after andalusite in metapelitic rocks. Therefore, near-pluton rocks record the loading history of the orogen. Metapelitic rocks not associated with plutons only preserve evidence for high-pressure conditions and/or high-temperature decompression, as indicated, for example, by sillimanite and cordierite after kyanite and garnet, respectively. Petrological evidence for burial and decompression is therefore recorded in different rocks. Various regions of the orogen differ in timing of metamorphism, the overall shape of P–T paths and the relative timing and regional extent of the high-pressure event, but most of these data and observations are consistent with thrusting and/or pure shear thickening as primary loading mechanisms throughout the orogen, as opposed to magma-dominated loading. This interpretation is further supported by comparison with thermal models, which demonstrate that the P–T paths are consistent with simultaneous thrusting and folding at a high initial geothermal gradient (35–40 °C km^?1) in much of the orogen. A high geothermal gradient supports tectonic models invoking intra-arc contraction and suggests that magmatism played an important role in regional temperature-time paths. This tectonic-thermal history may be typical of other contractional orogens and illustrates the importance of large vertical displacement of crust in magmatic arcs.  相似文献   

Variations in sediment sources and yields in the Finger Lakes and Catskills regions of New York     

Gregory N. Nagle  Timothy J. Fahey  Jerry C. Ritchie  Peter B. Woodbury 《水文研究》2007,21(6):828-838

The proportional contributions of stream bank and surface sources to fine sediment loads in watersheds in New York State were quantified with uncertainty analysis. Eroding streamside glacial drift, including glaciolacustrine deposits, were examined to help explain variations in the proportional contributions made by bank erosion. Sediment sources were quantified by comparing concentrations of the bomb‐derived radionuclide ¹³⁷Cs in fluvial sediment with sediment from potential source areas such as agricultural soils, forest soils and stream banks. To compare sediment sources in streams containing abundant deposits of fine‐grained glacial drift with watersheds that lacked moderate or extensive streamside deposits, samples were taken from 15 watersheds in the region. The mean contribution of bank erosion to sediment loads in the six streams with glaciolacustrine deposits was 60% (range 46–76%). The proportional contribution of bank erosion was also important in one stream lacking glaciolacustrine deposits (57%) but was less important in the remainder, with contributions ranging from 0 to 46%. Data from this study on the varying contributions of bank erosion and data from past studies of sediment yield in 15 watersheds of New York State suggest that eroding streamside glacial deposits dominate sediment yield in many watersheds. In other watersheds, past impacts to streams, such as channelization, have also resulted in high levels of bank erosion. Copyright © 2007 John Wiley & Sons, Ltd.  相似文献   

The use of 137Cs as a tracer in an erosion study in south limburg (the Netherlands) and the influence of chernobyl fallout     

A. P. J. De Roo 《水文研究》1991,5(2):215-227

The ¹³⁷Cs radioactivity of soils was used as a tracer of soil erosion in a catchment in the Netherlands: 143 samples were analysed to map the ¹³⁷Cs redistribution using geostatistical interpolation methods. Caesium-137 activities on grassland are significantly higher than on arable land. Also, ¹³⁷Cs activities on waning slopes are higher and activities on steep slopes are lower. The soil erosion estimates, derived from the ¹³⁷Cs data, are used to validate the USLE erosion model. The recent Chernobyl nuclear accident also contributed to the ¹³⁷Cs activity. However, the Chernobyl input of ¹³⁷Cs, with a constant ratio of 1.765:1 to ¹³⁴Cs, cannot be used as a tracer of soil erosion. Because of the rapid decay of ¹³⁴Cs, we will not be possible to separate the sources of ¹³⁷Cs in the near future in areas significantly influenced by Chernobyl fallout and in these areas ¹³⁷Cs can no longer be used as a soil erosion tracer.  相似文献   

原子吸收法测定矿石中的锂铷铯     

李绍卿  郭同章  胡文清 《地球科学与环境学报》1987,(2)

本文研究了锂、铷、铯三元素在丙酮有机溶剂中的行为,测定条件,干扰离子的影响及消除,使灵敏度分别比在水相中提高为2.5—3.5倍。方法灵敏度高,干扰少,测定范围为0～5PPM,适用于矿石中微量锂、铷、铯三元素同时测定。  相似文献   

Hillslope erosion in a grassland environment: Calibration and evaluation of the SIBERIA landscape evolution model     

G.R. Hancock  Abraham Gibson  T. Wells 《地球表面变化过程与地形》2021,46(4):728-743

Field measurement and modelling of soil erosion provides insights into landscape systems as well as the potential for enhanced landscape management. There are a number of field and numerical methods by which soil erosion and deposition can be quantified. Here we examine the capability of the SIBERIA landscape evolution model to quantify short-term erosion and deposition on a well-managed cattle grazing landscape on the east coast of Australia. The model is calibrated by two methods (1) a geomorphological approach using a site digital elevation model (DEM) and soil data and (2) a laboratory-scale flume. The two calibration processes resulted in similar model input parameters and estimated erosion rates of 3.1 t ha⁻¹ year⁻¹ and 4.4 t ha⁻¹ year⁻¹, respectively. These were found to closely match erosion rates estimated using the environmental tracer ¹³⁷Cs (2.7–4.8 t ha⁻¹ year⁻¹). However, erosion and deposition estimated at individual points along the hillslope was not well correlated with ¹³⁷Cs at the same position due to the temporal averaging of the model and microtopography. Sensitivity analysis showed the model was more sensitive to parameterisation than sub-DEM-scale topography. This places confidence in the model's ability to estimate erosion and deposition across an entire hillslope and catchment on decadal time scales. We also highlight the robustness and flexibility of the calibration methods.  相似文献