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Seepage of hydrocarbon-rich fluids out of the marine sedimentary column is characterized by temporal changes of flow intensity and resultant spatially variable redox conditions. Authigenic carbonates at marine hydrocarbon seeps provide excellent geological and geochemical archives that serve to explore seepage dynamics over time. In this study, we investigated the potential of Mössbuaer spectroscopy and Fe contents of seep-related authigenic carbonates from the Congo Fan, the Gulf of Mexico, and the Black Sea for reconstructing past redox conditions and fluid seepage activity at cold seeps. The Fe speciation observed by Mössbauer spectroscopy and Fe contents suggest that (1) the Congo Fan carbonates precipitated in a sulfidic environment, (2) the formation conditions of seep carbonates were variable at the Gulf of Mexico seep site, ranging from oxic to suboxic and anoxic and even spanning into the methanogenic zone, and (3) the stratified water column of the Black Sea or suboxic condition resulted in low Fe contents of Black Sea carbonates. The study reveals that Fe speciation can provide constraints on the wide range of redox conditions that imprinted seep carbonates during the life span of seepage. Similarly, Mössbauer spectroscopy – particularly when used in combination with the analysis of redox-sensitive elements – is a promising tool to trace variable redox conditions in marine paleoenvironments other than seeps. 相似文献
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This study is an attempt of a semi-automatic geomorphological GIS analysis based on morphometric indices. In the study, 10-m-resolution Digital Elevation Models (DEMs) are used to assess the neotectonic signals regarding the recent topographic developments and to attach additional significance to active tectonics in the Bingöl basin area. The methodology incorporates the determination of the structural similarities of the faults in the basins using fractal concepts and the application of four morphometric indices (Stream Power Index (SP), Multi-resolution Index of Valley Bottom Flatness (MRVBF), Terrain Ruggedness Index (TRI) and Valley Width-to-Height Ratio (Vf)). In order to detect the deviation from spatial randomness of the applied indices, the weighted correlation coefficient Moran’s I is used and the results are interpreted at a confidence interval of 99%. The spatial distribution of integrated index values is evaluated with the tectonically active fault zones in order to determine the probable activity and the structural deformation in the basin.The applied methodology reveals that the fractal analysis of the fault lines and the spatial analysis of the morphometric indices proved to be effective tools in analyzing the tectonic influence of the fault system on the basin area. Within the basin area, a relatively lesser degree of tectonic activity is observed, in contrast with the high tectonic activity outside the basin. 相似文献
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Radiometric and palynological data of the Upper Oligocene–Lower Miocene Soma Formation from the Kalk?m-Gönen Basin yield new results related to age and palynological contents. In this study, Upper Oligocene strata from the Dani?ment and Linfa areas and Lower Miocene strata from the Bengiler area were sampled palynologically and for radiometric dating. The Dani?ment assemblage, which is older than the Linfa assemblages, mainly contains coniferous and evergreen to deciduous mixed mesophytic forest elements. Relatively high quantities of the altitudinal plants Picea and Abies, indicate a cooler palaeoclimate. The Linfa associations mainly include coniferous and riparian elements. Pollen of the riparian plant Alnus and Taxodiaceae indicative for the swamp forest community was predominant, probably as a result of a high lake level. There is a hiatus during the Oligocene–Miocene transition, probably showing a non-depositional phase and sea-level fall indicating the Mi-1 glaciation event. Higher in the sequence, the Aquitanian Bengiler sediments include high amounts of coniferous forest elements as well as components indicative for the evergreen and deciduous mesophytic forest and also riparian forest and swamp forest. Due to presence of thermophilous taxa Reveesia, Mastixiaceae and Arecaceae, a warm and humid palaeoclimate is inferred according to quantitative analyses using the Coexistence Approach. 相似文献
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主要研究了分数阶混合随机泛函微分方程的能控性.在无限维空间下,假设所考虑方程线性部分生成半群不是紧的,使用非紧性测度技术和Mönch不动点定理,给出了方程能控性充分条件,并通过一个例子说明了结论的有效性. 相似文献
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N. C. Hambly S. J. Smartt S. T. Hodgkin R. F. Jameson S. N. Kemp W. R. J. Rolleston I. A. Steele 《Monthly notices of the Royal Astronomical Society》1999,309(4):L33-L36
We present a parallax measurement for the very cool degenerate WD 0346+246, the serendipitous discovery of which was reported by Hambly et al. We find an absolute parallax of 36±5 mas, yielding a distance estimate of 28±4 pc. The resulting absolute visual magnitude of the object is M V =16.8±0.3, making it the second-lowest luminosity white dwarf currently known. We use the distance estimate and measured proper motion to show that the object has kinematics consistent with membership of the Galactic halo. WD 0346+246 is therefore by far the coolest and least luminous of only a handful of plausible halo white dwarf candidates. As such, the object has relevance to the ongoing debate concerning the results of microlensing experiments and the nature of any baryonic dark matter component to the Galactic halo residing in stellar remnants. 相似文献
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Annealing at 400?T?600 °C (40?P?60 MPa and HM buffer-controlled f(O2)) of tourmalines synthesised at the same T and P with NNO buffer induces an oxidation of Fe2+ into Fe3+ in some Y sites only (Mössbauer Spectroscopy data). Annealing in the same conditions of natural tourmalines is consistent with these results. FTIR spectroscopy shows that oxidation of Fe2+ into Fe3+ is charge-balanced by deprotonation of the external OH(3) groups. To cite this article: Y. Fuchs et al., C. R. Geoscience 334 (2002) 245–249. 相似文献
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Fred Worrall Tim P. Burt Gregory R. Hancock Nicholas J.K. Howden John Wainwright 《地球表面变化过程与地形》2020,45(15):3869-3878
This study has hypothesized that for many rivers the trade-off between flow accumulation and the decrease in slope along channel length means that stream power increases downstream and, moreover, that given the low slope angles in headwater and low-order streams, they would have insufficient stream power to erode let alone transport sediment. The study considered the stream power profile, the particle travel distances and the application of the Hjulström curve based on the velocity profile of nine, large UK catchments. The study showed that:
- Some rivers never showed a maximum in their longitudinal stream power profile, implying that some rivers never develop a deposition zone before they discharge at the tidal limit.
- Particle travel distances during a bankfull discharge event showed that for some rivers 91% of the upper main channel would not be cleared of sediment. Furthermore, while some rivers could transport a 2 mm particle their entire length in one bankfull event, for another river it would take 89 such events.
- The Hjulström curve shows that for three of the study rivers the upper 20 km of the river was not capable of eroding a 2 μm particle.
- The study has shown that for all rivers studied, erosion is focused downstream and deposition upstream. Many UK rivers have a dead zone where, on time scales of the order of centuries, no erosion or transport occurs and erosion only occurs in the lower courses of the channel where discharge rather than slope dominates – we propose these as underpowered rivers.
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Ann Louise Heathwaite Catherine Heppell Andrew Binley Patrick Byrne Katrina Lansdown Mark Trimmer Sami Ullah Hao Zhang 《水文研究》2021,35(4):e14135
We report the complex spatial and temporal dynamics of hyporheic exchange flows (HEFs) and nitrogen exchange in an upwelling reach of a 200 m groundwater-fed river. We show how research combining hydrological measurement, geophysics and isotopes, together with nutrient speciation techniques provides insight on nitrogen pathways and transformations that could not have been captured otherwise, including a zone of vertical preferential discharge of nitrate from deeper groundwater, and a zone of rapid denitrification linking the floodplain with the riverbed. Nitrate attenuation in the reach is dominated by denitrification but is spatially highly variable. This variability is driven by groundwater flow pathways and landscape setting, which influences hyporheic flow, residence time and nitrate removal. We observed the spatial connectivity of the river to the riparian zone is important because zones of horizontal preferential discharge supply organic matter from the floodplain and create anoxic riverbed conditions with overlapping zones of nitrification potential and denitrification activity that peaked 10–20 cm below the riverbed. Our data also show that temporal variability in water pathways in the reach is driven by changes in stage of the order of tens of centimetres and by strength of water flux, which may influence the depth of delivery of dissolved organic carbon. The temporal variability is sensitive to changes to river flows under UK climate projections that anticipate a 14%–15% increase in regional median winter rainfall and a 14%–19% reduction in summer rainfall. Superimposed on seasonal projections is more intensive storm activity that will likely lead to a more dynamic and inherently complex (hydrologically and biogeochemically) hyporheic zone. We recorded direct evidence of suppression of upwelling groundwater (flow reversal) during rainfall events. Such flow reversal may fuel riverbed sediments whereby delivery of organic carbon to depth, and higher denitrification rates in HEFs might act in concert to make nitrate removal in the riverbed more efficient. 相似文献
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