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1.
硼的地球化学性质及其在俯冲带的循环与成矿初探 总被引:2,自引:1,他引:1
硼是广泛应用于化工、农业、材料科学及核工业领域的重要元素。硼与氢的核聚变反应是未来具备运用潜力的清洁能源。硼作为典型的亲石元素,是高度不相容元素。硼元素容易富集于蚀变洋壳及蛇纹石化地幔橄榄岩中。而在板块俯冲过程中,由于硼具有强的流体活动性,会优先赋存于流体中。因此,当蛇纹石化的大洋岩石圈及覆于其上的沉积物在俯冲过程中发生脱水,这使得弧前地幔楔发生大规模的蛇纹石化。此时大量硼元素很可能随俯冲流体释放并封存于弧前地幔楔中。目前已发现的超大型硼矿床主要位于聚合型板块边缘,尤其土耳其拥有世界上最大的硼酸盐储量。我们推测这些矿床的形成基础条件之一可能与弧前高度蛇纹石化的地幔楔有关。尤其是在洋 陆俯冲环境,弧前蛇纹岩或蛇绿混杂岩首先通过俯冲侵蚀再循环到火山弧岩浆中,使得岩浆更富集硼。随后弧火山喷发大量富硼的火山岩、岩浆热液及水气。在岩浆冷却过程中,硼元素析出、沉淀于火山表面,并伴随风化、侵蚀过程汇聚至碰撞造山带的封闭湖盆之中。此外,干冷的气候条件下也进一步促进了硼的成矿。我国具有形成大型、超大型硼矿的地质条件,应加大研究及探勘力度,并适当购买硼作为战略储备。 相似文献
2.
沉积物硼(B)同位素组成可以反映其地质成因及经历的地质过程,因此在许多领域的研究中都有较为广泛的应用。通过对位于柴达木盆地碱山背斜顶部的SG-1b钻孔沉积物(7.3~1.6 Ma)水溶组分的B同位素研究,发现钻孔沉积物B含量在38.55~172.3μg/g之间,平均含量为87.6μg/g;δ~(11)B值的变化范围在3.61‰~16.26‰之间,平均值为10.65‰,B含量与δ~(11)B值具有一定的正相关关系。进一步分析表明,受到碱山背斜构造隆升以及晚新生代以来气候干旱化的影响,柴西古湖逐渐咸化萎缩,沉积环境以及碳酸盐含量、粘土矿物含量及其矿物组合等也在发生变化,B含量和δ~(11)B值自钻孔底部向上的逐步增加以及后期的急剧增加,与水溶离子含量以及矿物和粒度等的变化一致,这说明柴达木盆地晚中新世以来湖泊沉积物的B含量和δ~(11)B值可以很好地反映研究区气候和湖水的演化过程,共同指示了研究区自7.3 Ma以来气候的持续干旱化和湖水盐度的逐步增加,以及3.3Ma以来干旱化和湖水浓缩过程的加剧。 相似文献
3.
4.
Alexandre Raphael Cabral Bernd Lehmann Miguel Tupinambá Michael Wiedenbeck Michael Brauns 《Journal of Geochemical Exploration》2011
The Palaeo-Mesoproterozoic metasiliciclastic rocks of the southern Serra do Espinhaço, Minas Gerais, Brazil, are host to historically important alluvial deposits of diamonds and gold. Detrital gold grains often comprise Au–Pd–Pt intermetallic compounds, with low Ag contents, which contain inclusions of tourmaline and titaniferous hematite (up to ~ 6 wt.% TiO2). The latter minerals connect the alluvial mineralisation to the rutile–hematite–quartz veins and tourmalinisation observed in the quartzitic country rocks of the alluvial gravel. The quartzite (Sopa-Brumadinho Formation of lacustrine to fan-deltaic origin) is affected by pervasive B metasomatism with F-bearing tourmaline replacing the recrystallised quartz fabric. The tourmaline belongs to the alkali group, with Mg/(Mg + Fe) and X/(X + Na) ratios in the ranges from 0.5 to 0.7 and 0.18 to 0.29, respectively, where X represents vacancies in the X site. Boron-isotopic values of tourmaline vary from ~ 1 to − 10.4‰ δ11B. The B-isotope range, in conjunction with the Na–Mg-rich tourmaline composition, and the widespread occurrence of tourmalinite in the Sopa-Brumadinho Formation suggest a derivation from non-marine evaporitic brines. Brines are capable of transporting otherwise immobile Ti and explain, under oxidising conditions, the fractionation of Ag from Pd to precipitate palladiferous gold with extremely high Pd/Ag ratios. Zirconium-in-rutile and Ti-in-quartz temperatures for a variety of hematite-rich veins suggest episodic vein emplacement over a temperature range from around 500 °C to ~ 350 °C. Cross-cutting relationships and episodic vein emplacement indicate a late-Brasiliano age. 相似文献
5.
6.
Doaa Hassan Youssef 《Journal of Oceanography》2003,59(5):537-544
Concentrations of boron in seawater (from four regions along the Alexandria coastline, subjected to land disposal), brackish
water (Lake Edku) and drains water (e.g. El-Umum Drain) were determined during the period from February to August 2000. Boron
was determined spectrophotometrically by a modified curcumin method. For Lake Edku, boron concentration fluctuated between
0.023 and 0.105 mmol/l. There are several factors that affect the concentration of B in the Lake water: (a) effect of the
drainage water via El-Khairy and Barsiek Drains, (b) utilization of boron by hydrophytes, and (c) water exchange through the
sea-lake connection. It may be concluded that the level of boron in the Lake water cannot be considered a substantial hazard
to the Lake organisms. Boron concentration varied from 0.392 to 0.522 mmol/l in seawater samples and from 0.141 to 0.458 mmol/l
in the sites where the water from the drains (El-Umum Drain and El-Noubaria Canal) mixed with the seawater. The broader variation
of boron (mmol/l)/salinity ratios for seawater samples (0.0106–0.0138) may be due to that the samples were collected from
the upper seawater layers, where contributions from land run-off, atmospheric precipitation and differences in the biota affect
the concentration.
This revised version was published online in July 2006 with corrections to the Cover Date. 相似文献
7.
Lü Yuanyuan ZHENG Mianping CHEN Wenxi ZHANG Xuefei LIU Xifang WU Qian YU Jiangjiang 《《地质学报》英文版》2014,88(Z1):151-152
正The origin of boron in boron-rich salt lakes in the Tibetan Plateau has long been the subject of debate.The Damzung Co Salt Lake in central Tibet has high boron concentrations(B=276–313 mg/L)and is an ideal site for 相似文献
8.
R. B. Trumbull M.-S. Krienitz B. Gottesmann M. Wiedenbeck 《Contributions to Mineralogy and Petrology》2008,155(1):1-18
Tourmaline is widespread in metapelites and pegmatites from the Neoproterozoic Damara Belt, which form the basement and potential
source rocks of the Cretaceous Erongo granite. This study traces the B-isotope variations in tourmalines from the basement,
from the Erongo granite and from its hydrothermal stage. Tourmalines from the basement are alkali-deficient schorl-dravites,
with B-isotope ratios typical for continental crust (δ11B average −8.4‰ ± 1.4, n = 11; one sample at −13‰, n = 2). Virtually all tourmaline in the Erongo granite occurs in distinctive tourmaline-quartz orbicules. This “main-stage”
tourmaline is alkali-deficient schorl (20–30% X-site vacancy, Fe/(Fe + Mg) 0.8–1), with uniform B-isotope compositions (δ11B −8.7‰ ± 1.5, n = 49) that are indistinguishable from the basement average, suggesting that boron was derived from anatexis of the local
basement rocks with no significant shift in isotopic composition. Secondary, hydrothermal tourmaline in the granite has a
bimodal B-isotope distribution with one peak at about −9‰, like the main-stage tourmaline, and a second at −2‰. We propose
that the tourmaline-rich orbicules formed late in the crystallization history from an immiscible Na–B–Fe-rich hydrous melt.
The massive precipitation of orbicular tourmaline nearly exhausted the melt in boron and the shift of δ11B to −2‰ in secondary tourmaline can be explained by Rayleigh fractionation after about 90% B-depletion in the residual fluid.
Electronic supplementary material The online version of this article (doi:) contains supplementary material, which is available to authorized users. 相似文献
9.
10.
In the eastern Sierras Pampeanas, Central Argentina, tourmalinites and coticules are found in close association with stratabound scheelite deposits in metamorphic terranes. In Sierra Grande (Agua de Ramón and Ambul districts) and Sierra de Altautina, tourmalinites are associated with stratabound scheelite deposits related to orthoamphibolites. In the Pampa del Tamboreo area, tourmalinites are located in biotite schists stratigraphically related to acid to intermediate metavolcanic rocks and scheelite-bearing quartzites.The mineral chemistry and boron isotopic compositions of tourmalinite-hosted and vein-hosted tourmalines are investigated. Overall, the tourmalines belong to the dravite-schorl series and are generally aluminous; Fe/(Fe+Mg) ranges from 0.33 to 0.85, Al/(Al+Fe+Mg) from 0.66 to 0.76 and the amount of X-site vacancy (0.12–0.48) indicates significant foitite components. Their boron isotopic compositions (δ11B) are from −24.0‰ to−15.0‰.Similar mineral chemistries and boron isotopic values for tourmaline in tourmalinites related to stratabound scheelite mineralisation and in tungsten-bearing quartz veins suggest a common source for the boron and probably the tungsten. The field, chemical and isotopic relationships are consistent with tungsten and boron in quartz-vein deposits being remobilised from stratabound scheelite and tourmalinite, dominantly by liquid-state transfer associated with regional shear zones. Tungsten and boron in the original sedimentary sequence (now meta-exhalites) are ascribed to volcanogenic exhalations. 相似文献