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The partitioning of Fe and Mg between olivine and carbonate and the stability of carbonate under mantle conditions 总被引:4,自引:1,他引:4
We have investigated the effect of Fe on the stabilities of carbonate (carb) in lherzolite assemblages by determining the partitioning of Fe and Mg between silicate (olivine; ol) and carbonates (magnesite, dolomite, magnesian calcite) at high pressures and temperatures. Fe enters olivine preferentially relative to magnesite and ordered dolomite, but Fe and Mg partition almost equally between disordered calcic carbonate and olivine. Measurement of K
d
(X
Fe
carb
X
Mg
ol
/X
Fe
ol
X
Mg
carb
) as a function of Fe/ Mg ratio indicates that Fe–Mg carbonates deviate only slightly from ideality. Using the regular solution parameter for olivine W
FeMg
ol
of 3.7±0.8 kJ/mol (Wiser and Wood 1991) we obtain for (FeMg)CO3 a W
FeMg
carb
of 3.05±1.50 kJ/mol. The effect of Ca–Mg–Fe disordering is to raise K
d
substantially enabling us to calculate W
CaMg
carb
-W
CaFe
carb
of 5.3±2.2 kJ/mol. The activity-composition relationships and partitioning data have been used to calculate the effect of Fe/Mg ratio on mantle decarbonation and exchange reactions. We find that carbonate (dolomite and magnesian calcite) is stable to slightly lower pressures (by 1 kbar) in mantle lherzolitic assemblages than in the CaO–MgO–SiO2(CMS)–CO2 system. The high pressure breakdown of dolomite + orthopyroxene to magnesite + clinopyroxene is displaced to higher pressures (by 2 kbar) in natural compositions relative to CMS. CO2. We also find a stability field of magnesian calcite in lherzolite at 15–25 kbar and 750–1000°C. 相似文献
5.
Pranab K. Roy Chowdhury Jeanette E. Weaver Eric M. Weber Dalton Lunga St. Thomas M. LeDoux Amy N. Rose 《International Journal of Digital Earth》2020,13(1):119-135
ABSTRACTUrban areas presently consume around 75% of global primary energy supply, which is expected to significantly increase in the future due to urban growth. Having sustainable, universal energy access is a pressing challenge for most parts of the globe. Understanding urban energy consumption patterns may help to address the challenges to urban sustainability and energy security. However, urban energy analyses are severely limited by the lack of urban energy data. Such datasets are virtually non-existent for the developing countries. As per current projections, most of the new urban growth is bound to occur in these data-starved regions. Hence, there is an urgent need of research methods for monitoring and quantifying urban energy utilization patterns. Here, we apply a data-driven approach to characterize urban settlements based on their formality, which is then used to assess intra-urban urban energy consumption in Johannesburg, South Africa; Sana’a, Yemen; and Ndola, Zambia. Electricity is the fastest growing energy fuel. By analyzing the relationship between the settlement types and the corresponding nighttime light emission, a proxy of electricity consumption, we assess the differential electricity consumption patterns. Our study presents a simple and scalable solution to fill the present data void to understand intra-city electricity consumption patterns. 相似文献
6.
The rate of sediment supply from erosional catchment to depositional basin depends primarily upon climate, relief, catchment slope and lithology. It varies in both time and space. Spatial changes in erosion rates due to variations in lithology are illustrated by contrasting rates of drainage divide migration away from faults of known ages. Time variations in relative sediment supply are extremely complex and vary widely according to the direction and magnitude of climate change. In many parts of the Great Basin and south-western USA, glacial maximum climates were characterized by higher effective moisture and the altitudinal downward spread of woods and forests. Sparse data from alluvial fans indicate reduced sediment supply, despite the increased runoff evident from higher lake levels. The situation in Mediterranean areas is less clear, with rival climatic scenarios for vegetation ecotypes predicting contrasting runoff. In order to test these latter we run Cumulative Seasonal Erosion Potential [CSEP] experiments for present-day and a variety of full-glacial Mediterranean candidate climates. The results indicate the likelihood of enhanced sediment supply and runoff compared to the present day during full-glacial times for a cool wet winter climate and a reduction in sediment supply and runoff for a full-glacial cool dry winter climate. We then explore the consequences of such phase differences in sediment supply, and sea and lake levels for the stratigraphy of sedimentary basins. Highstands and lowstands of sea or lake may be accompanied by greater or lesser sediment and water supply, as determined by the regional climate and the direction of climatic change. Thus marine lowstands are not necessarily periods of great transfer of coarse clastic sediments to shelves and deep water basinal environments. Unsteady sediment supply has greatest implications for alluvial systems, in particular the effect that changing relative supplies of water and sediment have upon river and fan channel incision. 相似文献
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Dale P. Cruikshank Allan W. Meyer Roger N. Clark Katrin Stephan Scott A. Sandford Gianrico Filacchione Philip D. Nicholson Thomas B. McCord J. Brad Dalton Dennis L. Matson 《Icarus》2010,206(2):561-572
Several of the icy satellites of Saturn show the spectroscopic signature of the asymmetric stretching mode of C-O in carbon dioxide (CO2) at or near the nominal solid-phase laboratory wavelength of 4.2675 μm (2343.3 cm−1), discovered with the Visible-Infrared Mapping Spectrometer (VIMS) on the Cassini spacecraft. We report here on an analysis of the variation in wavelength and width of the CO2 absorption band in the spectra of Phoebe, Iapetus, Hyperion, and Dione. Comparisons are made to laboratory spectra of pure CO2, CO2 clathrates, ternary mixtures of CO2 with other volatiles, implanted and adsorbed CO2 in non-volatile materials, and ab initio theoretical calculations of CO2 * nH2O. At the wavelength resolution of VIMS, the CO2 on Phoebe is indistinguishable from pure CO2 ice (each molecule’s nearby neighbors are also CO2) or type II clathrate of CO2 in H2O. In contrast, the CO2 band on Iapetus, Hyperion, and Dione is shifted to shorter wavelengths (typically ∼4.255 μm (∼2350.2 cm−1)) and broadened. These wavelengths are characteristic of complexes of CO2 with different near-neighbor molecules that are encountered in other volatile mixtures such as with H2O and CH3OH, and non-volatile host materials like silicates, some clays, and zeolites. We suggest that Phoebe’s CO2 is native to the body as part of the initial inventory of condensates and now exposed on the surface, while CO2 on the other three satellites results at least in part from particle or UV irradiation of native H2O plus a source of C, implantation or accretion from external sources, or redistribution of native CO2 from the interior.The analysis presented here depends on an accurate VIMS wavelength scale. In preparation for this work, the baseline wavelength calibration for the Cassini VIMS was found to be distorted around 4.3 μm, apparently as a consequence of telluric CO2 gas absorption in the pre-launch calibration. The effect can be reproduced by convolving a sequence of model detector response profiles with a deep atmospheric CO2 absorption profile, producing distorted detector profile shapes and shifted central positions. In a laboratory blackbody spectrum used for radiance calibration, close examination of the CO2 absorption profile shows a similar deviation from that expected from a model. These modeled effects appear to be sufficient to explain the distortion in the existing wavelength calibration now in use. A modification to the wavelength calibration for 13 adjacent bands is provided. The affected channels span about 0.2 μm centered on 4.28 μm. The maximum wavelength change is about 10 nm toward longer wavelength. This adjustment has implications for interpretation of some of the spectral features observed in the affected wavelength interval, such as from CO2, as discussed in this paper. 相似文献
9.
Manuela Magliocchetti Steve J. Maddox Ed Hawkins John A. Peacock Joss Bland-Hawthorn Terry Bridges Russell Cannon Shaun Cole Matthew Colless Chris Collins Warrick Couch Gavin Dalton Roberto de Propris Simon P. Driver George Efstathiou Richard S. Ellis Carlos S. Frenk Karl Glazebrook Carole A. Jackson Bryn Jones Ofer Lahav Ian Lewis Stuart Lumsden Peder Norberg Bruce A. Peterson Will Sutherland Keith Taylor 《Monthly notices of the Royal Astronomical Society》2004,350(4):1485-1494
10.
The 2dF Galaxy Redshift Survey: the bJ -band galaxy luminosity function and survey selection function
Peder Norberg Shaun Cole Carlton M. Baugh Carlos S. Frenk Ivan Baldry Joss Bland-Hawthorn Terry Bridges Russell Cannon Matthew Colless Chris Collins Warrick Couch Nicholas J. G. Cross Gavin Dalton Roberto De Propris Simon P. Driver George Efstathiou Richard S. Ellis Karl Glazebrook Carole Jackson Ofer Lahav Ian Lewis Stuart Lumsden Steve Maddox Darren Madgwick John A. Peacock Bruce A. Peterson Will Sutherland Keith Taylor 《Monthly notices of the Royal Astronomical Society》2002,336(3):907-931