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Hiroshi Nagasawa Douglas P Blanchard Jeffrey W Jacobs Joyce C Brannon John A Philpotts Naoki Onuma 《Geochimica et cosmochimica acta》1977,41(11):1587-1600
Concentrations of the REE, Sc, Co, Fe, Zn, Ir, Na and Cr were determined by instrumental neutron activation and mass spectrometric isotope dilution analysis for mineral separates of the coarseand fine-grained types (group I and II of Martin and Mason's classification) of the Allende inclusions.These data, combined with data on mineral/liquid partition coefficients, oxygen isotope distributions and diffusion calculations, suggest the following: (1) Minerals in the coarse-grained inclusions (group I) crystallized in a closed system with respect to refractory elements. On the other hand, differences in oxygen isotope distributions among minerals preclude a totally molten stage in the history of the inclusion. Group I inclusions were formed by rapid condensation (either to liquid or solid) in a supercooled solar nebula; extrasolar pyroxene and spinel dust were included but not melted in the condensing inclusions, thus preserving their extrasolar oxygen isotope composition. REE were distributed by diffusion during the subsequent heating at subsolidus temperatures; because oxygen diffuses much more slowly at these temperatures, the oxygen isotope anomalies were preserved. (2) The fine-grained (group II) inclusions were also formed by condensation from a super-cooled nebular gas; however, REE-rich clinopyroxene and spinel were formed early and REE-poor sodalite and nepheline were formed later and mechanically mixed with clinopyroxene and spinel to form the inclusions. The REE patterns of the bulk inclusions and the mineral separates are fractionated, indicating that REE abundances in the gaseous phase were already fractionated at the time of condensation of the minerals. (3) Pre-existing Mg isotope anomalies in the coarse-grained inclusions must have been erased during the heating stage thus resetting the 26Al-26Mg chronometer. 相似文献
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依据南海低纬地区SA09-040孔高分辨率的孢粉记录,自下至上划分了4个孢粉组合带。从孢粉成分的变化,重建了22.25ka B P以来的植被与气候变化历史。结果表明:孢粉主要来源于婆罗洲和周围岛屿,孢粉1带(22.25~16.6ka B P),低山雨林植被发育,为暖热气候,从测年时间看,当时为末次冰期晚期。孢粉2带(16.6~10.82ka B P,为末次冰消期),植被以热带低山雨林和低地雨林为主,针叶的松数量较多,当时的气温比现在低。孢粉3带(全新世早期,10.82~6.43ka B P),植被以热带低山雨林和低地雨林为主,针叶松属数量减少,气温比前期升高,海平面也上升。孢粉4带(全新世中晚期,6.43ka B P至今),全新世中期为炎热、湿润的气候环境,全新世晚期可能与婆罗洲现今的植被景观相近,为热、湿的气候环境。 相似文献
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Fish assemblages that included known predators of benthic crustaceans were compared between kelp and barren habitats in northeastern New Zealand using baited underwater video census methods. The benthic-feeding fish were observed in winter, spring/summer and autumn, as well as during night-time in spring/summer. Overall, the fish assemblages varied between barren and kelp habitat, being most marked in winter. Individual benthic-feeding species, such as grey mao mao (Scorpis lineolatus) and leatherjacket (Meuschenia scaber) were associated with barren habitat, while the spotted wrasse (Notolabrus celidotus) was more strongly associated with kelp habitat. The results suggest that changes in habitats on coastal reefs affect populations of species that are benthic predators, which may in turn influence the distribution and abundance of their prey species, such as juvenile spiny lobsters. 相似文献
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ML Camara B Mérigot F Leprieur JA Tomasini I Diallo M Diallo 《African Journal of Marine Science》2016,38(2):189-206
In a context of growing fishing pressures and recommendations for an ecosystem approach to fisheries, there is a need to monitor changes in fish communities over time. In this study, we analysed data from scientific trawl surveys carried out on the continental shelf off Guinea between 1985 and 2012. We performed factorial analyses and calculated biodiversity indices to characterise the changes in the structure and composition of fish communities that occurred over the 28-year period in this area, particularly given intensive fishing activities. We show that, over the study period, fish communities on the Guinean shelf were structured primarily according to spatial factors, with temporal changes being less pronounced than expected. However, a temporal analysis of biodiversity indices and species dominance showed that the intensification of fishing had significant effects on the general ecological features of the fish assemblages under study. There was a decrease in fish density and in mean trophic level. In addition, there were changes in species dominance, whereby large, slow-growing species with high commercial value were gradually replaced by smaller, fast-growing species of lesser commercial interest. These results from field observations are in line with some conclusions from previous modelling studies in the same geographical area, and provide further support for the hypothesis of a progressive ‘ecosystem effect of fishing’ occurring in Guinean waters. 相似文献
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Zooplankton biomass and distribution in the KwaZulu-Natal Bight were investigated in relation to environmental parameters during summer (January–February 2010) and winter (July–August 2010). Mean zooplankton biomass was significantly higher in winter (17.1 mg dry weight [DW] m–3) than in summer (9.5 mg DW m?3). In summer, total biomass was evenly distributed within the central bight, low off the Thukela River mouth and peaked near Durban. In winter, highest biomass was found offshore between Richards Bay and Cape St Lucia. Zooplankton biomass in each size class was significantly, negatively related to sea surface temperature and integrated nitrate, but positively related to surface chlorophyll a and dissolved oxygen. Zooplankton biomass was significantly related to bottom depth, with greatest total biomass located inshore (<50 m). Distribution across the shelf varied with zooplankton size. Seasonal differences in copepod size composition suggest that a smaller, younger community occupied the cool, chlorophyll-rich waters offshore from the St Lucia upwelling cell in winter, and a larger, older community occurred within the relatively warm and chlorophyll-poor central bight in summer. Nutrient enrichment from quasi-permanent upwelling off Durban and Richards Bay appears to have a greater influence on zooplankton biomass and distribution in the bight than the strongly seasonal nutrient input from the Thukela River. 相似文献
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DJ Karoly JA Cohen GA Meehl JFB Mitchell AH Oort RJ Stouffer RT Wetherald 《Climate Dynamics》1994,10(1-2):97-105
As an example of the technique of fingerprint detection of greenhouse climate change, a multivariate signal or fingerprint of the enhanced greenhouse effect is defined using the zonal mean atmospheric temperature change as a function of height and latitude between equilibrium climate model simulations with control and doubled CO2 concentrations. This signal is compared with observed atmospheric temperature variations over the period 1963 to 1988 from radiosonde-based global analyses. There is a significant increase of this greenhouse signal in the observational data over this period.These results must be treated with caution. Upper air data are available for a short period only, possibly too short to be able to resolve any real greenhouse climate change. The greenhouse fingerprint used in this study may not be unique to the enhanced greenhouse effect and may be due to other forcing mechanisms. However, it is shown that the patterns of atmospheric temperature change associated with uniform global increases of sea surface temperature, with El NinoSouthern Oscillation events and with decreases of stratospheric ozone concentrations individually are different from the greenhouse fingerprint used here. 相似文献
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Stephen R. Winzer David F. Nava Shuford Schuhmann Charles W. Kouns R.K.L. Lum John A. Philpotts 《Earth and Planetary Science Letters》1974,23(3):439-444
Apollo 17 station 7 boulder consortia samples were analyzed for major and minor elements by a combined semimicro atomic absorption spectrophotometric and colorimetric procedure. Lithophile trace element abundances were determined by stable isotope dilution mass spectrometry. Three matrix types samples (77135, 77115, and 77075) were found to be KREEP-rich fragment-laden melts with analogues throughout the Apollo 17 landing site. Of the five clasts analyzed, at least one (77115,19, troctolite) is thought to be a cumulate; 77135, 77115, and 77075 are thought to have originated by impact fusion of material with similar composition. This original material may represent a partial melt of a parent material of the composition of an included, shocked norite breccia (77215). 相似文献
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Recently we showed that visible-UV spectra in aqueous solution can be accurately calculated for arsenic (III) bisulfides, such as As(SH)3, As(SH)2S- and their oligomers. The calculated lowest energy transitions for these species were diagnostic of their protonation and oligomerization state. We here extend these studies to As and Sb oxidation state III and v sulfides and to polysulfides S n 2- , n = 2–6, the bisulfide anion, SH-, hydrogen sulfide, H2S and the sulfanes, S n H2, n = 2–5. Many of these calculations are more difficult than those performed for the As(iii) bisulfides, since the As and Sb(v) species are more acidic and therefore exist as highly charged anions in neutral and basic solutions. In general, small and/or highly charged anions are more difficult to describe computationally than larger, monovalent anions or neutral molecules. We have used both Hartree-Fock based (CI Singles and Time-Dependent HF) and density functional based (TD B3LYP) techniques for the calculations of absorption energy and intensity and have used both explicit water molecules and a polarizable continuum to describe the effects of hydration. We correctly reproduce the general trends observed experimentally, with absorption energies increasing from polysulfides to As, Sb sulfides to SH- to H2S. As and Sb(v) species, both monomers and dimers, also absorb at characteristically higher energies than do the analogous As and Sb(III)species. There is also a small reduction in absorption energy from monomeric to dimeric species, for both As and Sb III and v. The polysufides, on the other hand, show no simple systematic changes in UV spectra with chain length, n, or with protonation state. Our results indicate that for the As and Sb sulfides, the oxidation state, degree of protonation and degree of oligomerization can all be determined from the visible-UV absorption spectrum. We have also calculated the aqueous phase energetics for the reaction of S8 with SH- to produce the polysulfides, S n H-, n = 2–6. Our results are in excellent agreement with available experimental data, and support the existence of a S6 species. 相似文献