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1IntroductionThecarbonisotopiccompositionofnaturalgasesisregardedasacontanttracerusedinthegeochemicalresearchofnaturalgases .Basedonthecarbonisotopiccomposition ,thegenetictypesofnaturalgasesarebasicallydividedtodeterminethematurationofnaturalgasesandmakegas sourcecorrelations (Stahl,1 973;StahlandCarey ,1 975;Stahletal.,1 977;James ,1 983;Schoell,1 983,1 988;DaiJinxingetal.,1 992 ;FuJiamoetal.,1 992 ;XuYongchang ,1 994 ) .Theformationofnaturalgasescouldbededucedintermsofcarbonisotopicvar… 相似文献
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深入探究页岩气富集机理是保障勘探开发高效推进的基础。本研究通过对四川盆地五峰组—龙马溪组页岩气勘探开发实践的系统分析,梳理总结前人研究成果,从生成机理、运移机理、赋存机理和保存机理四个方面对海相页岩气富集机理进行了深入分析,并讨论了深层和常压页岩气的勘探开发潜力。结果表明：在生成机理方面,埋藏史和热演化史控制了页岩生排烃史、生排烃量和现今含气量;页岩气运移机理涉及运移动力、运移相态、运移方式和运移通道四方面内容,页岩气运移主要是烃源岩内的初次运移,同时讨论了初次运移的影响因素;在赋存机理方面,甲烷—页岩间表现出单/多分子层吸附和微孔充填等多种赋存机制,组分润湿性和孔隙有效性是决定甲烷吸附赋存和解吸运移的关键;在保存机理方面,盖层和物性自封闭是主要的保存机理,构造运动引起的裂缝—流体活动是页岩气保存条件遭到破坏的主要原因,流体活动时间和期次研究是页岩气保存条件和含气量定量评价的重要内容。页岩气富集机理的系统分析和创新认识为页岩气勘探开发评价提供了重要依据,建议加强页岩气演化历史全过程的动态评价。结合深层和常压页岩气勘探实践,分析了深层和常压页岩气的成因机制及主要特征,指出了下一步攻关内容及勘探方向。 相似文献
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Peng Weilong Liu Quanyou Zhang Ying Jia Huichong Zhu Dongya Meng Qingqiang Wu Xiaoqi Deng Shang Ma Yongsheng 《中国科学:地球科学(英文版)》2022,65(5):874-881
Science China Earth Sciences - Helium gas is a scarce but important strategic resource, which is usually associated with natural gas. Presently, only one extra-large helium-rich gas field has been... 相似文献
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何文渊 崔宝文 王凤兰 王永卓 蒙启安 张金友 邵红梅 王瑞 白云风 林旭东 赵莹 孙宝刚 付秀丽 徐庆霞 崔坤宁 钟建华 高剑波 孙宁亮 毛毳 邵珠福 倪良田 宋全友 薛纯琦 郝兵 圣朋朋 张继震 王宇航 张文鑫 《地质论评》2022,68(2):693-741
松辽盆地古龙凹陷有丰富的页岩油气资源.但是目前对古龙凹陷页岩油储层的岩石学特征和页岩油的状态,尤其是储集空间的类型及其组合关联性认识不清.通过对古龙凹陷白垩系青山口组岩芯的精细描述及其薄片分析和电子显微镜观察及三维CT深入研究,发现古龙青山口组页岩油的储集空间具有多样性和多尺度性.除了纳米孔缝外,还有页理缝.根据页理缝... 相似文献
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Deep fluids in a petroliferous basin generally come from the deep crust or mantle beneath the basin basement, and they transport deep substances(gases and aqueous solutions) as well as heat to sedimentary strata through deep faults. These deep fluids not only lead to large-scale accumulations of CO_2, CH_4, H_2, He and other gases, but also significantly impact hydrocarbon generation and accumulation through organic-inorganic interactions. With the development of deep faults and magmatic-volcanic activities in different periods, most Chinese petroliferous basins have experienced strong impacts associated with deep fluid activity. In the Songliao, Bohai Bay, Northern Jiangsu, Sanshui, Yinggehai and Pearl Mouth Basins in China, a series of CO_2 reservoirs have been discovered. The CO_2 content is up to 99%, with δ~(13)C_(CO2) values ranging from-4.1‰ to-0.37‰ and ~3He/~4He ratios of up to 5.5 Ra. The abiogenic hydrocarbon gas reservoirs with commercial reserves, such as the Changde, Wanjinta, Zhaozhou, and Chaoyanggou reservoirs, are mainly distributed in the Xujiaweizi faulted depression of the Songliao Basin. The δ~(13)CCH4 values of the abiogenic alkane gases are generally -30‰ and exhibit an inverse carbon isotope sequence of δ~(13)C_(CH4)δ~(13)C_(C2H6)δ~(13)C_(C3H8)δ~(13)C_(C4H10). According to laboratory experiments, introducing external H_2 can improve the rate of hydrocarbon generation by up to 147% through the kerogen hydrogenation process. During the migration from deep to shallow depth, CO_2 can significantly alter reservoir rocks. In clastic reservoirs, feldspar is easily altered by CO_2-rich fluids, leading to the formation of dawsonite, a typical mineral in high CO_2 partial pressure environments, as well as the creation of secondary porosity. In carbonate reservoirs, CO_2-rich fluids predominately cause dissolution or precipitation of carbonate minerals. The minerals, e.g., calcite and dolomite, show some typical features, such as higher homogenization temperatures than the burial temperature, relatively high concentrations of Fe and Mn, positive Eu anomalies, depletion of 18 O and enrichment of radiogenic ~(87)Sr. Due to CO_2-rich fluids, the development of high-quality carbonate reservoirs is extended to deep strata. For example, the Well TS1 in the northern Tarim Basin revealed a high-quality Cambrian dolomite reservoir with a porosity of 9.1% at 8408 m, and the Well ZS1 C in the central Tarim Basin revealed a large petroleum reserve in a Cambrian dolomite reservoir at ~6900 m. During the upward migration from deep to shallow basin strata, large volumes of supercritical CO_2 may extract petroleum components from hydrocarbon source rocks or deep reservoirs and facilitate their migration to shallow reservoirs, where the petroleum accumulates with the CO_2. Many reservoirs containing both supercritical CO_2 and petroleum have been discovered in the Songliao, Bohaiwan, Northern Jiangsu, Pearl River Mouth and Yinggehai Basins. The components of the petroleum trapped with CO_2 are dominated by low molecular weight saturated hydrocarbons. 相似文献
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XU Huiyuan LIU Quanyou JIN Zhijun ZHU Dongy MENG Qingqiang LI Pengpeng ZHU Biqing 《《地质学报》英文版》2023,97(1):327-336
Continental epithermal ore deposits are commonly associated with sedimentary organic matter, oils or solid bitumen. These organics embedded in mineral deposits can convey valuable information of the ore genesis. However, the extent to which the formation of ore minerals was recorded by organic compounds remains largely unknown, as also is how metal-rich ores interfere with the molecular proxies in the temperature regime envisaged for hydrothermal activity. The molecular compositional changes of ... 相似文献
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以4-硝基苯并-15-冠醚-5(4-NO_2-B15C5)做萃取剂,苯甲醚和1-丁基-3-甲基咪唑双(三氟甲烷磺酰)亚胺盐([C_4mim][NTf_2])作稀释剂和协萃剂,以1 mol/L LiCl溶液作萃取溶剂,构建高效的冠醚—离子液体/锂盐溶液的溶剂萃取体系。重点考察了有机相组成、冠醚浓度和锂盐阴离子等对锂同位素分离的影响。结果表明,4-硝基苯并-15-冠醚-5具有良好的锂同位素分离效果,在萃取CF_3COOLi时最大单级分离系数(α)可达1.043±0.01。 相似文献
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青岛灵山岛南背来石剖面发育了两层大型不规则砂脉。其主要特征如下：上层大型不规则砂脉呈分散团块状顺黄褐色凝灰质泥岩分布,断续延伸约60 m,宽数米;有17个侵入砂团块。砂团块多呈浅灰色,主要岩性为砂岩、砂砾岩;砂团块直径在1~2 m。砂团块的形态非常复杂,侧向极易尖灭或突然中止。边界与围岩多突变,某些地方与节理发育方向相同。下层大型不规则砂脉浅灰色,主要底部为砂岩、顶部为砂砾岩,呈透镜状顺层产于灰黑色薄层砂泥岩中,均一团块状和边缘含大量泥砾;厚18 m,宽度和高度不详;上层砂脉发育在浅湖中;下层大型不规则砂脉发育在三角洲前缘。与此同时还探讨了上层砂脉的形成的动力学机制,建立了顺层砂脉的形成深度与液化层的深度之间的关系式（h=0.29H）。该公式可以用来预测顺层的侵位深度和寻找砂脉,为含油气盆地砂脉储层预测提供理论依据和新方法。通过流化公式计算获得了形成上层砂脉的流体上侵速度为1.26 m/s。通过本文的论述,进一步为理解灵山岛地区下白垩统的沉积环境和沉积动力学特征提供了新的岩石学证据。 相似文献