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The electrical aerosol spectrometer (EAS) of the parallel measuring principle at Tartu University is an efficient instrument for rapid measurement of the unstable size spectrum of aerosol particles. The measuring range from 10 nm to 10 μm is achieved by simultaneously using a pair of differential mobility analyzers with two different particle chargers. The particle spectrum is calculated and measurement errors are estimated in real time by using a least-squares method. Experimental calibration ensures reliability of measurement. The instrument is well suited for continuous monitoring of atmospheric aerosol. 相似文献
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Gerrit de Leeuw Lucinda Spokes Tim Jickells Carsten Ambelas Skjth Ole Hertel Elisabetta Vignati Susanne Tamm Michael Schulz Lise-Lotte Srensen Britta Pedersen Laura Klein K. Heinke Schlünzen 《Continental Shelf Research》2003,23(17-19):1743
The ANICE (Atmospheric Nitrogen Inputs into the Coastal Ecosystem) project addressed the atmospheric deposition of nitrogen to the North Sea, with emphasis on coastal effects. ANICE focused on quantifying the deposition of inorganic nitrogen compounds to the North Sea and the governing processes. An overview of the results from modelling and experimental efforts is presented. They serve to identify the role of the atmosphere as a source of biologically essential chemical species to the marine biota. Data from the Weybourne Atmospheric Observatory (UK) are used to evaluate the effect of short episodes with very high atmospheric nitrogen concentrations. One such episode resulted in an average deposition of 0.8 mmol N m−2 day−1, which has the potential to promote primary productivity of 5.3 mmol C m−2 day−1. This value is compared to long-term effects determined from model results. The total calculated atmospheric deposition to the North Sea in 1999 is 948 kg N km−1, i.e. 0.19 mmol N m−2 day−1 which has the potential to promote primary productivity of 1.2 mmol C m−2 day−1. Detailed results for August 1999 show strong gradients across the North Sea due to adjacent areas where emissions of NOx and NH3 are among the highest in Europe. The average atmospheric deposition to the southern part of the North Sea in August 1999 could potentially promote primary production of 2.0 mmol C m−2 day−1, i.e. 5.5% of the total production at this time of the year in this area of the North Sea. For the entire study area the atmospheric contribution to the primary production per m2 is about two-third of this value. Most of the deposition occurs during short periods with high atmospheric concentrations. This atmospheric nitrogen is almost entirely anthropogenic in origin and thus represents a human-induced perturbation of the ecosystem. 相似文献
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Werner Skrotzki Roland Tamm Carl-Georg Oertel Jens Rseberg Heinz-Günter Brokmeier 《Journal of Structural Geology》2000,22(11-12)
Lead sulfide (galena) of different purity and grain size was extruded through a round and rectangular die at temperatures between 773 and 923 K. Global and local lattice preferred orientations (here referred to as textures) were measured by neutron and electron back-scattering diffraction. Tension leads to a <100> <111> double fibre texture. Pure shear deformation yields texture components near the ideal face-centered cubic metal brass, copper, Goss and cube positions. The intensity of the components depends on the purity and/or grain size. The microstructure is partially recrystallized. Electron back-scattering diffraction indicates that in tension the <100> and in pure shear the Goss and cube components are associated with dynamic recrystallization. The deformation texture can be qualitatively explained by the full and relaxed constraints Taylor model using slip on {100}<110>, {110}<110> and {111}<110> systems. The texture formation in lead sulfide compares well with that observed for other ionic crystals with the NaCl-structure as well as for face-centered cubic metals with a high stacking fault energy. 相似文献
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Čeněk Šašinka Zdeněk Stachoň Petr Kubíček Sascha Tamm Aleš Matas Markéta Kukaňová 《The Cartographic journal》2019,56(2):175-191
The form of visual representation affects both the way in which the visual representation is processed and the effectiveness of this processing. Different forms of visual representation may require the employment of different cognitive strategies in order to solve a particular task; at the same time, the different representations vary as to the extent to which they correspond with an individual’s preferred cognitive style. The present study employed a Navon-type task to learn about the occurrence of global/local bias. The research was based on close interdisciplinary cooperation between the domains of both psychology and cartography. Several different types of tasks were made involving avalanche hazard maps with intrinsic/extrinsic visual representations, each of them employing different types of graphic variables representing the level of avalanche hazard and avalanche hazard uncertainty. The research sample consisted of two groups of participants, each of which was provided with a different form of visual representation of identical geographical data, such that the representations could be regarded as ‘informationally equivalent’. The first phase of the research consisted of two correlation studies, the first involving subjects with a high degree of map literacy (students of cartography) (intrinsic method: N?=?35; extrinsic method: N?=?37). The second study was performed after the results of the first study were analyzed. The second group of participants consisted of subjects with a low expected degree of map literacy (students of psychology; intrinsic method: N?=?35; extrinsic method: N?=?27).The first study revealed a statistically significant moderate correlation between the students’ response times in extrinsic visualization tasks and their response times in a global subtest (r?=?0.384, p?<?0.05); likewise, a statistically significant moderate correlation was found between the students’ response times in intrinsic visualization tasks and their response times in the local subtest (r?=?0.387, p?<?0.05). At the same time, no correlation was found between the students’ performance in the local subtest and their performance in extrinsic visualization tasks, or between their scores in the global subtest and their performance in intrinsic visualization tasks. The second correlation study did not confirm the results of the first correlation study (intrinsic visualization/‘small figures test’: r?=?0.221; extrinsic visualization/‘large figures test’: r?=?0.135). The first phase of the research, where the data was subjected to statistical analysis, was followed by a comparative eye-tracking study, whose aim was to provide more detailed insight into the cognitive strategies employed when solving map-related tasks. More specifically, the eye-tracking study was expected to be able to detect possible differences between the cognitive patterns employed when solving extrinsic- as opposed to intrinsic visualization tasks. The results of an exploratory eye-tracking data analysis support the hypothesis of different strategies of visual information processing being used in reaction to different types of visualization. 相似文献
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Locally computed statistics of image texture and a case-based reasoning (CBR) system were evaluated for mapping of forest attributes. Cluster analysis was preferred to regression models, as a pre-selection method of features. The best stand-based accuracy using satellite sensor images was 74.64 m−3 ha−1 (36%) RMSE for stand volume, 1.98 m−3 ha−1 a−1 (49%) for annual increase in stand volume, where κ = 0.23 for stand growth classes and κ = 0.41 for dominant tree species in stands. The top pixel-based accuracy using orthophotos was 76.54 m−3 ha−1 (41%) RMSE for stand volume, 1.87 m−3 ha−1 a−1 (44%) for annual increase in stand volume, where κ = 0.24 for stand growth classes and κ = 0.38 for dominant tree species in stands. Mean saturation in 30 m radius was the most useful feature when orthophotos were used, and standard deviation of Landsat ETM 6.2 values in 80 m radius was the best when satellite sensor images were used. The most valuable feature components (radii, channels and local statistics) for orthophotos were: 30 m kernel radius, lightness and the mean of pixel values; for satellite sensor images: 80 m kernel radius, near-infrared channel (ETM 4) and the mean of pixel values. Locally computed statistics. 相似文献
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Aerosol size spectra (d=10 nm–10 μm) were measured with an electrical aerosol spectrometer (EAS) at Mace Head on the west coast of Ireland. Several small aerosol particle (diameter 10–32 nm) concentration bursts were observed during the measurement period. Relationships between the events, air mass trajectories, tide height, and meteorological parameters are examined. Series of bursts were observed when a spectral transformation due to subsequent particle growth from 10 to 56–100 nm can be identified in an Eulerian experiment. Particle growth rates of between 1 and 3 nm/h were determined. These bursts appear in cold and comparatively clean arctic or polar air masses with temperature and relative humidity fluctuations, and do not correlate with low tide in some cases. These episodes, similar to those frequently found in the continental boundary layer, are thought to occur over a wide area and, for clear detection, require stable airflow for a few days. Elevated small-particle concentration events are more common during low tide or shortly after, and are typically associated with low wind speeds. Here, the increased shore exposure during low tide is thought to influence the nucleation and the subsequent growth of these aerosol particles. The occurrences of the bursts are found to depend on local wind direction. The highest d=10–32 nm particle concentrations appeared for wind sectors furthest from the tidal regions when the wind direction was 150–160°(south-easterly). Most of the events occurred during daytime when solar irradiation is most intense. 相似文献
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M. Vana E. Tamm U. Hrrak A. Mirme H. Tammet L. Laakso P.P. Aalto M. Kulmala 《Atmospheric Research》2006,82(3-4):536
In this work, the charging state of atmospheric nanoparticles was estimated through simultaneous measurements of aerosol size distribution and air ions mobility distribution with the aim to elucidate the formation mechanisms of atmospheric aerosols. The measurements were performed as a part of the QUEST 2 campaign at a boreal forest station in Finland. The overlapping part of the measurement ranges of the particle size spectrometers and air ion mobility spectrometers in the mass diameter interval of 2.6–40 nm was used to assess the percentage of charged particles (charging probability). This parameter was obtained as the slope of the linear regression line on the scatterplot of the measured concentrations of total (neutral + charged) and charged particles for the same diameter interval. Charging probabilities as a function of particle diameter were calculated for different days and were compared with the steady state charging probabilities of the particles in the bipolar ion atmosphere. For the smallest particles detectable by the particle size spectrometers (2.6–5 nm), the high percentages of negatively charged particles were found during the nanometer particle concentration bursts. These values considerably exceeded the values for the steady charging state and it was concluded that negative cluster ions preferably act as condensation nuclei. This effect was found to be the highest in the case of comparatively weak nucleation bursts of nanoparticles, when the rate of the homogeneous nucleation and the concentration of freshly nucleated particles were low. The nucleation burst days were classified according to the concentration of the generated smallest detectable new particles (weak and strong bursts). Approximately the same classification was obtained based on the charge asymmetry on particles with respect to the charge sign (polarity). The probabilities of negative and positive charge on the particles with the diameter of 5–20 nm were found to be nearly equal and they approximately agree with the values corresponding to the steady state charge distribution for negative particles known from lab experiments. It means that the steady charging state was reached during the growing time of particles up to 5 nm. The natural charging state of particles with a diameter between 2.5 and 4.5 nm was estimated by means of a special DMPS setup. Results were found to be in good correlation with the data by the particle size spectrometers and air ion mobility spectrometers. 相似文献
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Ülle Kikas Aivo Reinart Anna Pugatshova Eduard Tamm Vidmantas Ulevicius 《Atmospheric Research》2008,90(2-4):211-ICNAA07
The microphysical structure, chemical composition and prehistory of aerosol are related to the aerosol optical properties and radiative effect in the UV spectral range. The aim of this work is the statistical mapping of typical aerosol scenarios and adjustment of regional aerosol parameters. The investigation is based on the in situ measurements in Preila (55.55° N, 21.00° E), Lithuania, and the AERONET data from the Gustav Dalen Tower (58 N, 17 E), Sweden.Clustering of multiple characteristics enabled to distinguish three aerosol types for clear-sky periods: 1) clean maritime–continental aerosol; 2) moderately polluted maritime–continental aerosol; 3) polluted continental aerosol. Differences between these types are due to significant differences in aerosol number and volume concentration, effective radius of volume distribution, content of SO4− ions and Black Carbon, as well as different vertical profiles of atmospheric relative humidity. The UV extinction, aerosol optical depth (AOD) and the Ångstrom coefficient α increased with the increasing pollution. The value α = 1.96 was observed in the polluted continental aerosol that has passed over central and eastern Europe and southern Russia. Reduction of the clear-sky UV index against the aerosol-free atmosphere was of 4.5%, 27% and 41% for the aerosol types 1, 2 and 3, respectively. 相似文献
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Gerrit de Leeuw Leo Cohen Lise Marie Frohn Gary Geernaert Ole Hertel Bjarne Jensen Tim Jickells Laura Klein Gerard J. Kunz Soren Lund Marcel Moerman Frank Müller Britta Pedersen Knut von Salzen K. Heinke Schlünzen Michael Schulz Carsten A. Skjth Lise-Lotte Sorensen Lucinda Spokes Susanne Tamm Elisabetta Vignati 《Continental Shelf Research》2001,21(18-19)
The aim of the atmospheric nitrogen inputs into the coastal ecosystem (ANICE) project is to improve transport–chemistry models that estimate nitrogen deposition to the sea. To achieve this, experimental and modelling work is being conducted which aims to improve understanding of the processes involved in the chemical transformation, transport and deposition of atmospheric nitrogen compounds. Of particular emphasis within ANICE is the influence of coastal zone processes. Both short episodes with high deposition and chronic nitrogen inputs are considered in the project. The improved transport–chemistry models will be used to assess the atmospheric inputs of nitrogen compounds into the European regional seas (the North Sea is studied as a prototype) and evaluate the impact of various emission reduction strategies on the atmospheric nitrogen loads. Assessment of the impact of atmospheric nitrogen on coastal ecosystems will be based on comparisons of phytoplankton nitrogen requirements, other external nitrogen inputs to the ANICE area of interest and the direct nitrogen fluxes provided by ANICE. Selected results from both the experimental and modelling components are presented here. The experimental results show the large spatial and temporal variability in the concentrations of gaseous nitrogen compounds, and their influences on fluxes. Model calculations show the strong variation of both concentrations and gradients of nitric acid at fetches of up to 25 km. Aerosol concentrations also show high temporal variability and experimental evidence for the reaction between nitric acid and sea salt aerosol is provided by size-segregated aerosol composition measured at both sides of the North Sea. In several occasions throughout the experimental period, air mass back trajectory analysis showed connected flow between the two sampling sites (the Weybourne Atmospheric Observatory on the North Norfolk coast of the UK and Meetpost Noordwijk, a research tower at 9 km off the Dutch coast). Results from the METRAS/SEMA mesoscale chemistry transport model system for one of these cases are presented. Measurements of aerosol and rain chemical composition, using equipment mounted on a commercial ferry, show variations in composition across the North Sea. These measurements have been compared to results obtained with the transport–chemistry model ACDEP which calculates the atmospheric inputs into the whole North Sea area. Finally, the results will be made available for the assessment of the impact of atmospheric nitrogen on coastal ecosystems. 相似文献
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