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BO Husφy 《极地研究(英文版)》2002,13(1)
1 ＩｎｔｒｏｄｕｃｔｉｏｎＡｔｌａｔｉｔｕｄｅｓａｒｏｕｎｄ 80°Ｎａｎｄｉｎｔｈｅｍｅｓｏｓｐｈｅｒｅ /ｌｏｗｅｒｔｈｅｒｍｏｓｐｈｅｒｅ (ＭＬＴ) ,ｔｈｅｒｅｈａｖｅｂｅｅｎｆｅｗｍｅａｓｕｒｅｍｅｎｔｓｏｆｎｅｕｔｒａｌｄｙｎａｍｉｃｓ.ＡｒｅｑｕｉｒｅｍｅｎｔｗａｓｓｅｅｎｆｏｒｌｏｎｇｔｅｒｍｃｏｎｔｉｎｕａｌｍｏｎｉｔｏｒｉｎｇａｎｄａＶＨＦｍｅｔｅｏｒｒａｄａｒｗａｓｉｄｅｎｔｉｆｉｅｄａｓｂｅｉｎｇａｍｏｓｔｓｕｉｔａｂｌｅｉｎｓｔｒｕｍｅｎｔ.ＲａｄａｒｓｌｉｋｅｔｈｅＥＩＳＣＡ… 相似文献
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Molybdenum disulfide (MoS2), a layered transition-metal dichalcogenide, has been of special importance to the research community of geochemistry, materials
and environmental chemistry, and geotechnical engineering. Understanding the oxidation behavior and charge-transfer mechanisms
in MoS2 is important to gain better insight into the degradation of this mineral in the environment. In addition, understanding the
insertion of metals into molybdenite and evaluation of charge-transfer mechanism and dynamics is important to utilize these
minerals in technological applications. Furthermore, a detailed investigation of thermal oxidation behavior and metal-insertion
will provide a basis to further explore and model the mechanism of adsorption of metal ions onto geomedia. 相似文献
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To better constrain sampling strategies for observing biologically sensitive parameters in ground water, we vigorously pumped for 120 h a lightly pumped well completed in a confined glacial aquifer while observing how various physical and chemical parameters evolve in the water produced. The parameters commonly monitored when sampling a well stabilized within about an hour, after 5 wellbore volumes were produced; these parameters include temperature, pH, dissolved oxygen, oxidation-reduction potential (Eh), and electrical conductivity. The concentrations of ferrous iron, sulfide, and sulfate and various biological or biologically sensitive parameters, including the concentrations of dissolved hydrogen and methane, direct cell counts, and the microbial community profile, in contrast, required more than 8 h or 36 well volumes to stabilize. We interpret this result to mean that the zone of influence of the wellbore on biologic processes in the aquifer extends beyond the commonly recognized zone where physical properties are affected. A second period of adjustment of these biologically sensitive parameters began after about 50 h of pumping, following displacement of 230 wellbore volumes, and continued to the end of the experiment. During this period, the cell density and the composition of the microbial community suspended in the water samples changed. This finding indicates that the microbial community in and near the wellbore changed in response to pumping and the changes affected aspects of the composition of water produced from the well. The study demonstrates the importance of allowing adequate pumping time when sampling ground water for the analysis of biologically sensitive parameters. 相似文献
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We use reactive transport modeling to better understand the kinetics of chemical weathering in the Cretaceous Middendorf aquifer of South Carolina, USA, and the relationship of this process to subsurface microbial activity. We constructed a model accounting for the kinetics of mineral dissolution and precipitation, ion exchange, and the CO2 and bicarbonate produced by iron reducing and sulfate reducing bacteria in the aquifer. We then fit the model to observed trends in the chemical composition of groundwater along the aquifer by adjusting the rate constants for the kinetic reactions considered. The modeling portrays weathering in the Middendorf as a slow process by which groundwater gradually reacts toward equilibrium with minerals in the aquifer. The rate constants predicted are 6 to 7 orders of magnitude smaller than measured in laboratory experiments and 3 to 4 orders of magnitude less than those inferred from weathering rates in soils. The rate constants are smaller even than expected by projecting observed trends with the duration of weathering to the geologic age of the Middendorf. Weathering is driven largely by biological activity: about half the acid consumed is CO2 derived from the recharge area, and about half is supplied by iron reducing bacteria in the aquifer; only about 1% of the acid is of atmospheric origin, from CO2 dissolved in rainwater. 相似文献
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白云鄂博碳酸岩的方解石-白云石地质温度计 总被引：6，自引：2，他引：4
利用方解石-白云石地质温度计对白云鄂博地区碳酸岩的平衡温度进行了测定。出露于东矿下盘的白云岩质火山岩和出露于尖山的方解石-白云石型火山岩获得了较高的温度,分别为681℃和648℃。这些样品中的方解石呈二十微米左右晶形较完整的小片,被稍大粒度的白云石颗粒包裹,未受交代作用影响,推测这种碳酸岩在快速冷却的情况下保存下了其岩浆侵位时的成分特点,从而指示出接近碳酸岩浆侵位时的温度。但本区多数碳酸岩的平衡温度在400～500℃之间,有下列三种情况:(1)具有自形-半自形中粗粒粒状变晶结构的碳酸岩最后的平衡温度为415～496℃;(2)产自东矿的其余样品(火山岩),所测最后平衡温度为431～485℃,在测温的微区范围内可见极细粒白云石方解石与稀土等矿物共生的现象;(3)为交代重结晶结构的碳酸岩明显受到后期热液流体的交代,在流体的作用下共生方解石和白云石在成分上达到新的平衡,平衡温度为432～507℃。本文所分析的样品多数结果(371～507℃)与用白云石(方解石)和磁铁矿氧同位素温度计对白云鄂博碳酸岩的计算结果(360～546℃)十分一致。虽然有研究者对方解石-白云石温度计用于火成碳酸岩表示过质疑,但本文资料表明火成碳酸岩最后的平衡温度是可以运用方解石-白云石温度计法来计算的。 相似文献
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Extremely alkaline ground water has been found underneath many shuttered steel mills and slag dumps and has been an impediment to the cleanup and economic redevelopment of these sites because little is known about the geochemistry. A large number of these sites occur in the Lake Calumet region of Chicago, Illinois, where large-scale infilling of the wetlands with steel slag has created an aquifer with pH values as high as 12.8. To understand the geochemistry of the alkaline ground water system, we analyzed samples of ground water and the associated slag and weathering products from four sites. We also considered several potential remediation schemes to lower the pH and toxicity of the water. The principal cause of the alkaline conditions is the weathering of calcium silicates within the slag. The resulting ground water at most of the sites is dominated by Ca2+ and OH- in equilibrium with Ca(OH)2. Where the alkaline ground water discharges in springs, atmospheric CO2 dissolves into the water and thick layers of calcite form. Iron, manganese, and other metals in the metallic portion of the slag have corroded to form more stable low-temperature oxides and sulfides and have not accumulated in large concentrations in the ground water. Calcite precipitated at the springs is rich in a number of heavy metals, suggesting that metals can move through the system as particulate matter. Air sparging appears to be an effective remediation strategy for reducing the toxicity of discharging alkaline water. 相似文献
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安徽巢湖凤凰山剖面石炭系微相和层序地层特征 总被引：9，自引：1，他引：9
应用露头层序地层学基本原理和方法 ,对巢湖凤凰山石炭系剖面进行重新研究。巢湖凤凰山石炭系总厚度为79.0 2 m ,在这个剖面中可以识别出 6种主要岩相、18种微相和 11个三级沉积层序 ,其中六个三级沉积层序属于 I型沉积层序 ,三个属于 II型沉积层序 ,缺失第 9和第 10沉积层序。三级沉积层序在不同的古地理单元和不同的沉积环境中可以进行对比。根据各微相特征和成因 ,揭示了沉积间断面上存在的多期古岩溶现象。阐述了三级层序及其对应的三级海平面升降旋回的特征 相似文献