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1.
A detailed investigation of the fluvial geochemistry of the Han River system allows to estimate the rates of chemical weathering and the consumption of CO2. The Han River drains approximately 26,000 km2 and is the largest river system in South Korea in terms of both water discharge and total river length. It consists of two major tributaries: the North Han River (NHR) and the South Han River (SHR). Distinct differences in basin lithology (silicate vs. carbonate) between the NHR and SHR provide a good natural laboratory in which to examine weathering processes and the influence of basin geology on water quality. The concentrations of major elements and the Sr isotopic compositions were obtained from 58 samples collected in both summer and winter along the Han River system in both 2000 and 2006. The concentrations of dissolved loads differed considerably between the NHR and SHR; compared with the SHR, the NHR had much lower total dissolved solids (TDS), Sr, and major ion concentrations but a higher Si concentration and 87Sr/86Sr ratio. A forward model showed that the dissolved loads in the NHR came primarily from silicate weathering (55 ± 11%), with a relatively small portion from carbonates (30 ± 14%), whereas the main contribution to the dissolved loads in the SHR was carbonate weathering (82 ± 3%), with only 11 ± 4% from silicates. These results are consistent with the different lithologies of the two drainage basins: silicate rocks in the NHR versus carbonate rocks in the SHR. Sulfuric acid derived from sulfide dissolution in coal-containing sedimentary strata has played an important role in carbonate weathering in the SHR basin, unlike in the NHR basin. The silicate weathering rate (SWR) was similar between the NHR and SHR basins, but the rate of CO2 consumption in the SHR basin was lower than in the NHR basin due to an important role of sulfuric acid derived from pyrite oxidation.  相似文献   
2.
The purpose of this study is to apply time series analysis to investigate whether the groundwater quality in the coastal area is affected by the tide. Continuous and regular in situ monitoring data of electrical conductivity (EC) and groundwater level, and tidal level data measured by the National Oceanographic Research Institute were used for the time series analysis. Through the time series analysis, it is known that EC and groundwater level conspicuously fluctuate with two periodicities (15.4 and 0.52-day), which is very similar to those of the tide. Also the behaviors of their fluctuations vary in accordance with the tidal period. These indicate that the groundwater quality has been mainly controlled by the tidal level, and the strength of tidal effect on the groundwater quality is different according to the tidal period.  相似文献   
3.
Geochemical processes were identified as controlling factors of groundwater chemistry, including chemical weathering, salinization from seawater and dry sea-salt deposition, nitrate contamination, and rainfall recharge. These geochemical processes were identified using principal component analysis of major element chemistry of groundwater from basaltic aquifers in Jeju Island, South Korea, a volcanic island with intense agricultural activities. The contribution of the geochemical processes to groundwater chemistry was quantified by a simple mass-balance approach. The geochemical effects due to seawater were considered based on Cl contributions, whereas the effects due to natural chemical weathering were based on alkalinity. Nitrogenous fertilizers, and especially the associated nitrification processes, appear to significantly affect groundwater chemistry. A strong correlation was observed between Na, Mg, Ca, SO4 and Cl, and nitrate concentrations in groundwater. Correspondingly, the total major cations, Cl, and SO4 in groundwater were assessed to estimate relative effect of N-fertilizer use on groundwater chemistry. Cl originates more from nitrate sources than from seawater, whereas SO4 originates mostly from rainwater. N-fertilizer use has shown the greatest effect on groundwater chemistry, particularly when nitrate concentrations exceed 6–7 mg/L NO3–N. Nitrate contamination significantly affects groundwater quality and 18% of groundwater samples have contamination-dominated chemistry.  相似文献   
4.
Abstract The Ogcheon fold belt and the Ryeongnam massif in the Korean Peninsula are made up of Precambrian igneous and sedimentary rocks that have been metamorphosed, tectonically deformed and extensively intruded by mafic to felsic plutonic rocks of Permian to Jurassic age. In the present study, we report seven new U–Pb zircon ages and Sr‐Nd‐Pb isotopic data for Permian to Jurassic plutons in the Ogcheon belt and the Ryeongnam massif. In the Ogcheon belt, these are: the Cheongsan porphyritic granite (217 ± 3.1 My), the Baegrog foliated granodiorite (206.4 ± 3.6 My), the Sani granite (178.8 ± 2.9 My) and the Yeonggwang foliated granite (173.0 ± 1.7 My). For the Ryeongnam massif, we report on the Yeongdeog foliated granodiorite (252.2 ± 2.9 My), the Sancheong gabbro (203.8 ± 3.3 My) and the Baegseogri foliated granodiorite (177.8 ± 2.4 My). All of these ages are lower concordia intercepts; the upper concordia intercepts indicate derivation from a Precambrian protolith. Sr, Nd and Pb isotopes also reveal that much of the Permian–Jurassic (252–173 Ma) plutonism in Korea was generated by recycling of Precambrian rocks. These new ages, together with other published zircon ages indicate that the plutonism in the Ogcheon fold belt is coeval with that in the Ryeongnam massif, but based on the Sr‐Nd‐Pb isotopic evidence, they are not cogenetic. In addition, zircon ages provide information on the movement along the Honam shear zone, which cuts across the whole Korean Peninsula and along most of its length provides the boundary between the Ogcheon fold belt and the Ryeongnam massif. It has a prolonged history of movement and deformation and appears to have been active from the Precambrian through to the Mesozoic, from before 1924 Ma to at least 180 Ma. The Permian–Jurassic igneous and tectonic activity in Korea is a manifestation of the more extensive orogenic activities that affected the East Asian continent at that time. In China, ultra high‐pressure rocks of the Qinling–Dabie belt formed between 210 and 230 Ma as result of the collision between the South China block and the North China block. In central Japan, corresponding plutonic activity is dated as 175 to 231 Ma. The absence of ultra high‐pressure rocks in Korea and Japan precludes a simple extension of the Qinling–Dabie belt eastwards; however, the effects of the continental collision eastwards are apparent from the igneous and tectonic activity.  相似文献   
5.
The interactive influence between groundwater flow and salinization that occurs in an underground LPG cavern site in Korea was investigated using chemical analysis data and cross-correlation analysis between hydraulic head and operating pressure data. The concentration of the major cations and anions showed a large difference between rainy and dry seasons due to the seasonal intrusion of highly saline water into the cavern area. However, the Cl/Br ratio and '18O-Cl relationship showed that two types of saline water (seawater and halite-dissolved solution) influenced the groundwater salinization of the study area. The cross-correlation results revealed that a positive relationship between hydraulic head and cavern operating pressure was far more conspicuous in the propane cavern area (89-91% of correlation coefficients), and tidal change influenced the head variation in the butane cavern area. That is, continuous intrusion of seawater near the South Sea could bring about a high concentration of major cations and anions in the butane seepage waters and groundwaters near the coastal area, and seasonal variation in the operating pressure at the propane cavern played an important driving force in fast infiltration of halite-dissolved solution from surface halite stock and a subsequent increase in Na and Cl concentration during the dry season.  相似文献   
6.
The uranium (U) content and 234U/238U activity ratio were determined for water samples collected from Korea's Han River in spring, summer, and winter 2006 to provide data that might constrain the origin of U isotope fractionation in river water and the link between U isotope systematics in river waters and the lithological nature of the corresponding bedrock. The large difference in the major dissolved loads between the two major branches of the Han River, the North Han River (NHR) and South Han River (SHR), is reflected in the contrasting U content and 234U/238U activity ratio between the tributaries: low U content (0.08–0.75 nM; average, 0.34 nM) and small 234U/238U activity ratio (1.03–1.22; average, 1.09) in the NHR; and high U content (0.65–1.98 nM; average, 1.44 nM) and large 234U/238U activity ratio (1.05–1.45; average, 1.24) in the SHR. The large spatial differences in U content and 234U/238U activity ratio are closely related to both lithological differences between the two tributaries and groundwater input. The low U content and small 234U/238U activity ratio in the NHR arise mainly from a combination of surface and meteoric weathering of the dominant silicate rocks in this branch and congruent dissolution of already weathered (secular equilibrium) materials. In contrast, the high U content and large 234U/238U activity ratio in the SHR are ascribed to the dissolution of carbonates and black shales along with significant inputs of deep groundwater.  相似文献   
7.
Understanding groundwater flow and chemical transport is crucial for operating underground storage caverns. Groundwater flow in the study area is mainly affected by cavern operating conditions, and groundwater chemistry in the study area is modified by disinfection activities for removing possible biological clogging and by mixing with cement pore water. It is significant to discern these two effects because wells affected by the disinfection activities, in particular, may have hydrological connections with water curtains in which disinfectant water was injected to remove the biological clogging. Concentration of tritium (3H) and helium isotopes (4He), and groundwater chemical compositions were used to confirm that there are hydrological connectivities between the water curtain and the well. Groundwater along the fault areas contains low total dissolved solid (TDS) and high 3H, suggesting that the faults may act as fast flow conduits, which is not inconsistent with previous studies. Certain diagnostic conditions (high concentrations of Na+, Cl− and TDS and high pH) are presumed by the effect of disinfection activity, indicating that there are hydrological connections between the water curtain and the wells. This hypothesis is valid in YK2U and YK2L, but is not in YK12L, implying a closed system or an immobile water to explain the isotopic results.  相似文献   
8.
Abstract   An absolute age has been determined for the Cretaceous Uhangri Formation in which web-footed bird tracks, pterosaur tracks and dinosaur tracks have been discovered recently. This combined track discovery is a first from Asia. There is one other similar find in the world, however, the Uhangri site is greater in abundance and frequency. Moreover, the size of the pterosaur tracks indicates that the track maker had a wingspan of 10 m or more. Well-preserved tuffaceous rocks in the formation made it possible to measure geological age by Rb–Sr and K–Ar methods. Rb–Sr whole rock ages for the volcanic rocks are: 96.0 ± 2.5 Ma (MSWD = 0.354) for lapilli andesitic tuff, 81.0 ± 2.0 Ma (MSWD = 0.296) for felsic tuff and 77.9 ± 4.1 Ma (MSWD = 4.41) for Hwangsan welded tuff. K–Ar ages are younger, 83.2–68.8 Ma. The layer containing fossil tracks of pterosaurs and web-footed birds are preserved in black shale sandwiched by the lapilli andesitic tuff and felsic tuff, and are thus 96–81 Ma in age. Dinosaur footprints are dated at 96–78 Ma. Thus the pterosaurs, web-footed birds and dinosaurs coexisted in the same environment from Cenomanian to Campanian time.  相似文献   
9.
The need for more agricultural or residential land has encouraged reclamation at the coastal areas of Korea since 1200 ad (approximately). The groundwaters of these reclaimed areas could be expected to reveal hydrogeochemical properties different from those of areas directly affected by seawater intrusion. The purpose of this study, therefore, was to examine the salinization of shallow groundwater in a coastal reclaimed area and to identify the effect of land reclamation on groundwater quality. Major cations and anions, iodide, total organic carbon, δD, δ 18O and δ 13C were measured to assist the hydrogeochemical analysis. Chloride, δD and δ 18O data clearly show that the Na–Cl type water results from mixing of groundwater with seawater. In particular, the δD and δ 18O of Ca+Mg–Cl+NO3 type groundwaters are close to the meteoric water line, but Na–Cl type waters enriched in chloride are 18O-enriched with respect to the meteoric water line. Meanwhile, carbon isotopic data and I/Cl ratios strongly suggest that there are various sources of salinity. The δ 13C values of Na–Cl type groundwaters are generally similar to those of Ca+Mg–Cl+NO3 type waters, which are depleted in 13C with respect to seawater. I/Cl ratios of Na–Cl type groundwater are 10–100 times higher than that of seawater. Because the reclamation has incorporated a large amount of organic matter, it provides optimum conditions for the occurrence of redox processes in the groundwater system. Therefore, the salinization of groundwater in the study area seems to be controlled not only by saltwater intrusion but also by other effects, such as those caused by residual salts and organic matter in the reclaimed sediments.  相似文献   
10.
Ji-Hoon  Kim  Myong-Ho  Park  Urumu  Tsunogai  Tae-Jin  Cheong  Byong-Jae  Ryu  Young-Joo  Lee  Hyun-Chul  Han  Jae-Ho  Oh  Ho-Wan  Chang 《Island Arc》2007,16(1):93-104
Abstract Geochemical analyses of sediments, pore water and headspace gas of the piston cores taken from the eastern part of Ulleung Basin of the East Sea (Japan Sea) were carried out to assess the origin of the sedimentary organic matter and interstitial fluid. Several tephra layers within the core are identified as the Ulleung‐Oki (10.1 ka), the Aira‐Tanzawa (23 ka) and the Ulleung‐Yamato (30.9 ka) tephras. With the exception of these volcanic layers, the cores consist predominantly of muddy sediments that contain >0.5% total organic carbon. Atomic C/N ratios and δ13Corg values suggest that the organic matter originated from marine algae rather than from land vascular plants, whereas Rock‐Eval pyrolysis suggests that the organic matter is thermally immature and comes from a land vascular plant (Type III). These conflicting results seem to be caused by the heavy oxidization of the marine organic matter. Sulphate concentration profiles of pore waters show strongly linear depletion (r2 > 0.97) with sediment depth. The estimated sulphate–methane interface (SMI) depth using the sulphate concentration gradient was nearly 3.5 m below seafloor (mbsf) in the southern part of the study area, and deeper than 6 mbsf in the northern part of the area. The difference in SMI depths is likely associated with the amount of the methane flux. The methane concentration below the SMI in the two southern cores increases rapidly, implying the occurrence of methanogenesis and anaerobic methane oxidation (AMO). In contrast, the two northern cores have a low methane concentration below the SMI. values measured from all cores were in the range of −83.5 to −69.5‰, which suggests that the methane derives from a methanogenic microbe. values become decreased toward SMI, but increased below SMI; therefore, has eventually the minimum value near the SMI. The values are also decreased when the methane concentration is increased. These phenomena support the typical occurrence of AMO in the study area.  相似文献   
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