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为寻找天然抗污损活性化合物,以抗硅藻附着活性为导向,采用有机溶剂萃取、半制备高压液相色谱对分离自海绵的芽孢杆菌UST050418-715代谢产物进行分离,纯化抗硅藻附着活性物质,并利用气相色谱-质谱联用仪、核磁共振波谱分析活性物质结构。从菌株UST050418-715代谢产物中分离得到7种具有抗硅藻附着活性的环二肽类化合物,分别鉴定为:(1)环(L-亮氨酸-反式-8-羟基-L-脯氨酸-)、(2)环(L-缬氨酸-L-脯氨酸)、(3)环(D-脯氨酸-L-亮氨酸)、(4)环(L-脯氨酸-D-亮氨酸)、(5)环(甘氨酸-L-脯氨酸)、(6)环(L-苯丙氨酸-顺式-8-羟基-D-脯氨酸-)、(7)环(L-苯丙氨酸-反式-8-羟基-L-脯氨酸-)。说明海绵附生芽孢杆菌UST050418-715代谢产物中存在大量环二肽类化合物,可以帮助宿主海绵实现对硅藻附着的化学防御。 相似文献
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The unidirectional solidification textures (UST) quartz is generally thought to form from fluids exsolved from shallow intrusions and/or magma chambers, but such an idea is still poorly constrained from the evidence of stable isotopes. In this study, we report for the first time the δ18O of quartz that shows UST from the Qulong Cu–Mo and the Yechangping Mo porphyry deposits in China. The analysis results show that the UST quartz samples from the Qulong deposit have δ18O values ranging from +6.2 ‰ to +7.6 ‰, which are similar to that of quartz phenocrysts (+6.7 ‰ to +7.8 ‰). In contrast, the UST quartz samples from the Yechangping porphyry Mo deposit yield a high δ18O value (+10.0 ‰). The δ18Owater value of Yechangping UST quartz (+8.5 ‰) is also higher than that of Qulong (+4.6 ‰ to +5.8 ‰). Hydrothermal biotite from potassic alteration and sericite from early phyllic alteration at Qulong have similar δ18O values to UST quartz, suggesting the involvement of magmatic fluids during this stage of deposit evolution. 相似文献
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与花岗岩类有关的矿床主要是与其具有时—空及成因联系的岩浆—热液矿床,岩浆能否出溶热液且出溶相当数量热液是花岗岩类成矿的必要前提,直接制约岩浆岩的成矿潜力。基于前人和作者的研究成果得出,与成矿有关的花岗岩中发育的单向固结结构(UST结构)、石英眼、晶洞以及雪球结构等是岩浆挥发分相饱和出溶的标志,岩浆岩组成对于成矿潜力判别的贡献基于元素的地球化学行为以及物理化学条件,挥发组分中卤化物含量的高低和岩石中主量元素的丰度不能作为成矿潜力的判别标志,而微量元素是识别花岗岩类成矿潜力的地球化学指纹。高场强元素以及现出系统地球化学行为变化的稀土元素特征有望成为成矿潜力的最佳判别标志。花岗岩类含矿潜力的评价研究为岩浆热液多金属矿床的成矿预测和勘查评价提供理论指导,本文也指出在研究花岗岩含矿潜力中存在的一些问题及未来的研究方向。 相似文献
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江西永平铜矿花岗质岩石的岩石结构、地球化学特征及其成矿意义 总被引：2，自引：7，他引：2
江西永平铜矿位于华南怀玉山—北武夷山铜铅锌多金属成矿带内,是赣东北地区除了德兴铜矿外的另一个大型铜矿基地。该矿区存在两种类型的花岗质岩石,一种是花岗岩;另一种是英安斑岩。英安斑岩具有典型斑状结构和石英眼结构,而花岗岩则具有单向固结结构。在化学成分上,两者属于高钾的钙碱性系列岩石,英安斑岩贫硅、富Al、Fe、Mg、Ca,以及具有较大的Na_2O/K_2O(0.02～0.64)等特点;而花岗岩富硅、贫Al、Ca,以及富碱和具有较小的Na_2O/K_2O(0.02～0.03)等特点。两种类型的岩石具有一致的REE配分曲线。它们均富集大离子亲石元素(Ba、Rb、K),亏损高场强元素(Th、Nd、Ta、Ti)以及元素Sr和P,显示了与俯冲作用有关的岩浆作用。在结构和化学成分上,花岗岩则类似于美国Climax斑岩钼(铜)矿成矿斑岩的性质(如具有单向固结结构、较高的分异指数、富Si、贫Al、Ca、富Na_2O K_2O以及K_2O>Na_2O)。与英安斑岩有关的蚀变作用主要有夕卡岩化、黑云母化、白云母化、绿泥石化和萤石化,而与花岗岩有关的蚀变作用主要是白云母化和萤石化;相应地,与英安斑岩有关的成矿作用主要为铜,而与花岗岩有关的成矿作用则主要为钼。2件辉钼矿样品的Re-Os年龄分别为156.7±2.8Ma和155.7±3.6Ma,表明与花岗岩有关的钼成矿作用发生在156Ma左右。本文认为,永平铜钼矿的成矿地球动力学背景应是由挤压向伸展的转换环境。 相似文献
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Textural and chemical evolution of a fractionated granitic system: the Podlesí stock, Czech Republic
The Podlesí granite stock (Czech Republic) is a fractionated, peraluminous, F-, Li- and P-rich, and Sn, W, Nb, Ta-bearing rare-metal granite system. Its magmatic evolution involved processes typical of intrusions related to porphyry type deposits (explosive breccia, comb layers), rare-metal granites (stockscheider), and rare metal pegmatites (extreme F–P–Li enrichment, Nb–Ta–Sn minerals, layering). Geological, textural and mineralogical data suggest that the Podlesí granites evolved from fractionated granitic melt progressively enriched in H2O, F, P, Li, etc. Quartz, K-feldspar, Fe–Li mica and topaz bear evidence of multistage crystallization that alternated with episodes of resorption. Changes in chemical composition between individual crystal zones and/or populations provide evidence of chemical evolution of the melt. Variations in rock textures mirror changes in the pressure and temperature conditions of crystallization. Equilibrium crystallization was interrupted several times by opening of the system and the consequent adiabatic decrease of pressure and temperature resulted in episodes of nonequilibrium crystallization. The Podlesí granites demonstrate that adiabatic fluctuation of pressure (“swinging eutectic”) and boundary-layer crystallization of undercooled melt can explain magmatic layering and unidirectional solidification textures (USTs) in highly fractionated granites. 相似文献
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