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1.
Pittichovâ J. Sekenina Z. Birkle K. Boehnhardt J. Engels D. Keller P. 《Earth, Moon, and Planets》1997,78(1-3):329-338
The Sekanina-Farrell particle fragmentation model for the striated tails of dust comets is successfully applied to two images
of comet Hale-Bopp to study the motions of 12 striae in a time span of March 12–15, 1997. There is evidence for recurring
outbursts with a periodicity of 11h21m, consistent with results based on analysis of dust jets. The ejecta in all the striae appear to have been released from one
source on the nucleus between the end of January and the second half of February 1997, some 60 to 40 days before perihelion.
The parent particles were subjected to a radiation pressure acceleration of βp ≃ 0.55 and their fragmentation lifetimes in 11 of the 12 striae were practically constant and equal to 13–15 days, when normalized
to 1 AU from the Sun. Brief analysis of Watanabe et al.'s measurements of striae on their images from March 5–9, 1997 shows
even shorter fragmentation lifetimes for the parent particles, mostly about 7–11 days at1 AU.
This revised version was published online in July 2006 with corrections to the Cover Date. 相似文献
2.
Rate constants for the reaction of OH radicals with some branched alkyl nitrates have been measured applying a competitive technique. Methyl nitrite photolysis in synthetic air was used as OH radical source at 295±2 K and 1000 mbar total pressure. Using a rate constant of 2.53×10-12 cm3 s-1 for the reaction of OH radicals with n-butane as reference, the following rate constants were obtained (units: 10-12 cm3 s-1): isopropyl nitrate, 0.59±0.22; isobutyl nitrate, 1.63±0.20; 3-methyl-2-butyl nitrate, 1.95±0.15; 2-methyl-1-butyl nitrate, 2.50±0.15; 3-methyl-1-butyl nitrate, 2.55±0.35. These values have been combined with the literature data to recalculate the substituent factors F(X) for the different nitrate groups which can be used to predict OH rate constants for organic nitrates for which experimental data are not available.Preliminary measurements of the photolysis frequency of isopropyl nitrate have shown that for this nitrate as a model substance, OH reactions and direct photolysis are of equal importance under tropospheric conditions. 相似文献
3.
A statistically relevant correlation between the reaction rate coefficient, k
OH, for the OH radical reaction with 161 organic compounds in the gas phase at 300 K, and the corresponding vertical ionisation energies E
i,v, reveals two classes of compounds: aromatics where –log(k
OH/cm3s-1)3/2E
i,v(eV)–2 and aliphatics where –log(k
OH/cm3s-1)4/5E
i,v(eV)+3. The prediction of the rate coefficient, k
OH, for the reaction of OH with organic molecules from the above equations has a probability of about 90%. Assuming a global diurnal mean of the OH radical concentration of 5×105 cm3, the upper limit of the tropospheric half-life of organic compounds and their persistence can be estimated. 相似文献
4.
The mechanical denudation rates of 81 large lake basins (lake area > 500 km2) were determined from long-term river loads and erosion maps. Using the drainage area/lake area ratios the mean sedimentation rates of the lakes were calculated for a porosity of 0.3. The mean sedimentation rates of different lake types vary between 0.1 mm/a (glacial lakes, lowland) and 5.4 mm/a (mostly sag basin lakes). The calculated lifetimes of the lakes are based on the lake volumes and mean sedimentation rates, assuming steady-state conditions and solely clastic material. On average, glacial lakes in highlands and fault-related lakes show the shortest lifetimes (c. 70 ka), glacial lakes in lowlands and rift lakes have the longest lifetimes (c. 1 Ma). Some lakes remain unfilled for very long time spans due to rapid subsidence of their basin floors. The calculated lifetimes are compared with those derived from sediment core studies. Most core studies indicate lower mechanical sedimentation rates than the calculated ones because a major part of the incoming sediment is trapped in deltas. However, a number of lakes (e.g., the Great Lakes of North America) show the opposite tendency which is largely caused by extensive shoreline erosion and resuspension. The lifetimes of large glacial lakes often exceed the duration of interglacials. Hence, their lifetimes are restricted by glaciation and not by sediment infill. Rift lakes persist for long time periods which exceed the calculated lifetimes in some cases. Time-dependent subsidence, basin extension, as well as the impact of climate change are briefly described. 相似文献
5.
Observed pollutants are of both primary and secondary origins, influenced by local topography and meteorology. Identifying
sources and relative contribution often require vast detailed data collection and complicated models. This study applied a
statistical time series analysis to two selected pollution events, spring and fall, at two sites in northern Taiwan. Vector
moving average representations were used to quantitatively examine relationships among chemical pollutants and estimate their
lifetimes. Results from impulse responses show that wind direction change alters the characteristic of pollution observed
in opposite sites of Taipei City, from chemical dominant system to transport dominant one and vice versa. Chemicals are clearly
separated into photochemical pollutants and primary pollutants. Results pointed out that Taipei City is the major source of
photochemical smog, but not these primary pollutants. Derived chemical lifetimes at same location vary from 20% to four times
under different meteorological condition. Estimated concentrations of hydroxyl radical range between 2 to 8 × 107 cm−3. Photochemical pollutants are responsible for parts of PM10 collected in both station observed. Oxidation of SO2 is only important in PM10 observed at one station. This study provides a simpler tool to derive information usually from
complex models, therefore, is suitable as complement in decision-making process. 相似文献
6.
Gisèle Krysztofiak Yao Veng Té Gwenaël Berthet Geoffrey C. Toon Fabrice Jégou 《大气与海洋》2015,53(1):89-101
AbstractCarbonyl sulphide (OCS) is an important precursor of sulphate aerosols and consequently a key species in stratospheric ozone depletion. The SPectromètre InfraRouge d'Absorption à Lasers Embarqués (SPIRALE) and shortwave infrared (SWIR) balloon-borne instruments have flown in the tropics and in the polar Arctic, and ground-based measurements have been performed by the Qualité de l'Air (QualAir) Fourier Transform Spectrometer in Paris. Partial and total columns and vertical profiles have been obtained to study OCS variability with altitude, latitude, and season. The annual total column variation in Paris reveals a seasonal variation with a maximum in April–June and a minimum in November–January. Total column measurements above Paris and from SWIR balloon-borne instrument are compared with several MkIV measurements, several Network for the Detection of Atmospheric Composition Change (NDACC) stations, aircraft, ship, and balloon measurements to highlight the OCS total column decrease from tropical to polar latitudes. OCS high-resolution in situ vertical profiles have been measured for the first time in the altitude range between 14 and 30?km at tropical and polar latitudes. OCS profiles are compared with Atmospheric Chemistry Experiment (ACE) satellite measurements and show good agreement. Using the correlation between OCS and N2O from SPIRALE, the OCS stratospheric lifetime has been accurately determined. We find a stratospheric lifetime of 68?±?20 years at polar latitudes and 58?±?14 years at tropical latitudes leading to a global stratospheric sink of 49?±?14?Gg?S?y?1. 相似文献
7.
Spatial co‐location pattern mining aims to discover a collection of Boolean spatial features, which are frequently located in close geographic proximity to each other. Existing methods for identifying spatial co‐location patterns usually require users to specify two thresholds, i.e. the prevalence threshold for measuring the prevalence of candidate co‐location patterns and distance threshold to search the spatial co‐location patterns. However, these two thresholds are difficult to determine in practice, and improper thresholds may lead to the misidentification of useful patterns and the incorrect reporting of meaningless patterns. The multi‐scale approach proposed in this study overcomes this limitation. Initially, the prevalence of candidate co‐location patterns is measured statistically by using a significance test, and a non‐parametric model is developed to construct the null distribution of features with the consideration of spatial auto‐correlation. Next, the spatial co‐location patterns are explored at multi‐scales instead of single scale (or distance threshold) discovery. The validity of the co‐location patterns is evaluated based on the concept of lifetime. Experiments on both synthetic and ecological datasets show that spatial co‐location patterns are discovered correctly and completely by using the proposed method; on the other hand, the subjectivity in discovery of spatial co‐location patterns is reduced significantly. 相似文献
8.
Rate constants for the reaction of hydroxyl radicals with dibromomethanehave been measured by discharge flow-resonance fluorescence technique(DF-RF) over the temperature range 288–368 K. The derived Arrheniusequation is k1=(1.51 ± 0.37)× 10-12 exp(-(720 ±60)/T) cm3 molec.-1 s-1.The tropospheric lifetime of dibromomethane has been estimated to be 0.29years. An ozone depletion potential (ODP) value of 0.10 for dibromomethanehas been obtained. 相似文献
9.
溶解氧浓度检测在水产养殖和环境监测中具有重要的意义。本文提出了一种基于快速数字锁相的溶解氧检测优化设计,利用快速数字锁相算法与过采样技术,实现了荧光信号和调制信号的快速相位解调,并得到二者相位差,根据Stern-Volmer方程求出溶解氧浓度值。本文分析了调制频率对测量结果的影响,选择合适的调制频率用于测量,并利用最小二乘法对测量结果进行拟合,拟合后的确定系数R-square为0.999 25。实验数据表明,测量结果相对误差(RE)小于±1.5%,相对标准差(RSD)小于4%,稳定时间小于50 s。本文提出的优化设计不仅具有较高的测量精度,还简化了硬件设计,降低了成本。 相似文献
10.