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1.
This paper analyses factors that contributed to the evolution of SO2, NOx and CO2 emissions in Europe from 1960 to 2010. Historical energy balances, along with population and economic growth data, are used to quantify the impacts of major determinants of changing emission levels, including energy intensity, conversion efficiency, fuel mix, and pollution control. Time series of emission levels are compared for countries in Western and Eastern Europe, throwing light on differences in the importance of particular emission-driving forces. Three quarters of the decline in SO2 emissions in Western Europe resulted from a combination of reduced energy intensity and improved fuel mix, while dedicated end-of-pipe abatement measures played a dominant role in the reduction of NOx emissions. The increase in atmospheric emissions in Eastern Europe through the mid-1990s was associated with the growth of energy-intensive industries, which off-setted the positive impact of better fuel quality and changes in fuel mix. A continuous decrease in energy intensity and higher conversion efficiencies have been the main factors responsible for the moderate rate of growth of European CO2 emissions.  相似文献   

2.
中国实施铁路电气化的节能减排量估算   总被引：1，自引：0，他引：1       下载免费PDF全文
基于中国铁路部门逐年统计数据,计算了1975-2007年中国电气化铁路带来的逐年节能量和CO2、烟尘、SO2、CO、NOx与CnHm的直接减排量,并分析了其变化特点.结果表明,33年来电气化铁路使得中国铁路运输行业年均节省123.0万t标准煤的能源消耗,节能量年均增长13.9万t标准煤;CO2、烟尘、SO2、CO、NO...  相似文献   

3.
Substitution of natural gas for coal is one means of reducing carbon dioxide (CO2) emissions. However, natural gas and coal use also results in emissions of other radiatively active substances including methane (CH4), sulfur dioxide (SO2), a sulfate aerosolprecursor, and black carbon (BC) particles. Will switching from coal to gas reduce the net impact of fossil fuel use on global climate? Using the electric utility sector as an example, changes in emissions of CO2, CH4,SO2 and BC resulting from the replacement of coal by natural gas are evaluated, and their modeled net effect on global mean-annual temperature calculated. Coal-to-gas substitution initially produces higher temperatures relative to continued coal use. This warming is due to reduced SO2 emissionsand possible increases in CH4 emissions, and can last from 1 to 30years, depending on the sulfur controls assumed. This is followed by a net decrease in temperature relative to continued coal use, resulting from lower emissions of CO2 and BC. The length of this period and the extent of the warming or cooling expected from coal-to-gas substitution is found to depend on key uncertainties and characteristics of the substitutions, especially those related to: (1) SO2 emissions and consequentsulphate aerosol forcing; and (2) the relative efficiencies of the power plantsinvolved in the switch.  相似文献   

4.
Today's climate policy is based on the assumption that the location of emissions reductions has no impact on the overall climate effect. However, this may not be the case since reductions of greenhouse gases generally will lead to changes in emissions of short-lived gases and aerosols. Abatement measures may be primarily targeted at reducing CO2, but may also simultaneously reduce emissions of NOx, CO, CH4 and SO2 and aerosols. Emissions of these species may cause significant additional radiative forcing. We have used a global 3-D chemical transport model and a radiative transfer model to study the impact on climate in terms of radiative forcing for a realistic change in location of the emissions from large-scale sources. Based on an assumed 10% reduction in CO2 emissions, reductions in the emissions of other species have been estimated. Climate impact for the SRES A1B scenario is compared to two reduction cases, with the main focus on a case with emission reductions between 2010 and 2030, but also a case with sustained emission reductions. The emission reductions are applied to four different regions (Europe, China, South Asia, and South America). In terms of integrated radiative forcing (over 100 yr), the total effect (including only the direct effect of aerosols) is always smaller than for CO2 alone. Large variations between the regions are found (53–86% of the CO2 effect). Inclusion of the indirect effects of sulphate aerosols reduces the net effect of measures towards zero. The global temperature responses, calculated with a simple energy balance model, show an initial additional warming of different magnitude between the regions followed by a more uniform reduction in the warming later. A major part of the regional differences can be attributed to differences related to aerosols, while ozone and changes in methane lifetime make relatively small contributions. Emission reductions in a different sector (e.g. transportation instead of large-scale sources) might change this conclusion since the NOx to SO2 ratio in the emissions is significantly higher for transportation than for large-scale sources. The total climate effect of abatement measures thus depends on (i) which gases and aerosols are affected by the measure, (ii) the lifetime of the measure implemented, (iii) time horizon over which the effects are considered, and (iv) the chemical, physical and meteorological conditions in the region. There are important policy implications of the results. Equal effects of a measure cannot be assumed if the measure is implemented in a different region and if several gases are affected. Thus, the design of emission reduction measures should be considered thoroughly before implementation.  相似文献   

5.
We estimate the domestic environmental and health benefits of exploiting China's energy-related CDM potential. Exploiting the CDM potential may save between 3,000 and 40,000 lives annually. Additional gains are estimated to reach upwards from 1 billion RMB annually. The key to these gains is the fact that actions and measures to reduce CO2 emissions also reduce emissions of TSP and SO2. In our estimate, exploiting the CDM-potential will cut SO2-emissions by between one-half and three million tons annually. To arrive at these conclusions we synthesize a significant body of recent research on co-benefits of climate abatement in China.  相似文献   

6.
The Chinese government actively follows the low-carbon development pattern and has set the definite targets of reducing carbon emissions by 2030. The industrial sector plays a significant role in China's economic growth and CO2 emissions. This is the first study to present a specific investigation on the retrospective decomposition (1993–2014) and prospective trajectories (2015–2035) of China's industrial CO2 emission intensity (ICEI) and industrial CO2 emissions (ICE), aiming at China Industrial Green Development Plan 2016–2020 targets and China's 2030 CO2 emission-reduction targets. We introduce process carbon intensity, investment and R&D factors into the decomposition model and make a combination of dynamic Monte Carlo simulation and scenario analysis to identify whether and how the targets would be realized from a sector-specific perspective. The results indicate that investment intensity is the primary driver for the increase in ICEI, while R&D intensity and energy intensity are the leading contributors to the reduction in ICEI. Under existing policies, it is very possible for the industrial sector to achieve the 2020 and 2030 intensity-reduction targets. However, the realization of 2030 emission-peak target has some uncertainties and needs extra efforts in efficiency improvement and structural adjustment. All the five scenarios would achieve the 2020 and 2030 intensity-reduction targets, except Scenario N4 for China Industrial Green Development Plan 2016–2020 target. Nonetheless, only three scenarios would realize the 2030 emission-peak target. With strong efficiency improvement and structural adjustment, ICE would hit the peak in 2025. In contrast, with high/low efficiency improvement and weak structural adjustment, ICE would fail to reach the peak before 2035. Both ICEI and ICE have substantial mitigation potentials with the enhancement of efficiency improvement and structural adjustment. Finally, we suggest that the Chinese government should raise the baseline requirements of efficiency improvement and structural adjustment for the industrial sector to achieve China’s 2030 targets.  相似文献   

7.
The Scoping Plan for compliance with California Assembly Bill 32 (Global Warming Solutions Act of 2006; AB 32) proposes a substantial reduction in 2020 greenhouse gas (GHG) emissions from all economic sectors through energy efficiency, renewable energy, and other technological measures. Most of the AB 32 Scoping Plan measures will simultaneously reduce emissions of traditional criteria pollutants along with GHGs leading to a co-benefit of improved air quality in California. The present study quantifies the airborne particulate matter (PM2.5) co-benefits of AB 32 by comparing future air quality under a Business as Usual (BAU) scenario (without AB 32) to AB 32 implementation by sector. AB 32 measures were divided into five levels defined by sector as follows: 1) industrial sources, 2) electric utility and natural gas sources, 3) agricultural sources, 4) on-road mobile sources and 5) other mobile sources. Air quality throughout California was simulated using the UCD source-oriented air quality model during 12 days of severe air pollution and over 108 days of typical meteorology representing an annual average period in the year 2030 (10 years after the AB 32 adoption deadline). The net effect of all AB 32 measures reduced statewide primary PM and NOx emissions by ~1 % and ~15 %, respectively. Air quality simulations predict that these emissions reductions lower population-weighted PM2.5 concentrations by ~6 % for California. The South Coast Air Basin (SoCAB) experienced the greatest reductions in PM2.5 concentrations due to the AB 32 transportation measures while the San Joaquin Valley (SJV) experiences the smallest reductions or even slight increases in PM2.5 concentrations due to the AB 32 measures that called for increased use of dairy biogas for electricity generation. The ~6 % reduction in PM2.5 exposure associated with AB 32 predicted in the current study reduced air pollution mortality in California by 6.2 %, avoiding 880 (560–1100) premature deaths per year for the conditions in 2030. The monetary benefit from this avoided mortality was estimated at $5.4B/yr with a weighted average benefit per tonne of $35 k/tonne ($23 k/tonne–$45 k/tonne) of PM, NOx, SOx, and NH3 emissions reduction.  相似文献   

8.
The relationship between the emission of ozone precursors and the chemical production of tropospheric ozone(O3) in the Pearl River Delta Region(PRD) was studied using numerical simulation.The aim of this study was to examine the volatile organic compound(VOC)-or nitrogen oxide(NOx =NO+NO2)limited conditions at present and when surface temperature is increasing due to global warming,thus to make recommendations for future ozone abatement policies for the PRD region.The model used for this application is the U.S.Environmental Protection Agency’s(EPA’s) third-generation air-quality modeling system;it consists of the mesoscale meteorological model MM5 and the chemical transport model named Community Multi-scale Air Quality(CMAQ).A series of sensitivity tests were conducted to assess the influence of VOC and NOx variations on ozone production.Tropical cyclone was shown to be one of the important synoptic weather patterns leading to ozone pollution.The simulations were based on a tropicalcyclone-related episode that occurred during 14-16 September 2004.The results show that,in the future,the control strategy for emissions should be tightened.To reduce the current level of ozone to meet the Hong Kong Environmental Protection Department(EPD) air-quality objective(hourly average of 120 ppb),emphasis should be put on restricting the increase of NOx emissions.Furthermore,for a wide range of possible changes in precursor emissions,temperature increase will increase the ozone peak in the PRD region;the areas affected by photochemical smog are growing wider,but the locations of the ozone plume are rather invariant.  相似文献   

9.
The Yangtze River Delta (YRD), China’s main cultural and economic center, has become one of the most seriously polluted areas in the world with respect to nitrogen oxides (NOx), owing to its rapid industrialization and urbanization, as well as substantial coal consumption. On the basis of nitrogen dioxide (NO2) density data from ozone monitoring instrument (OMI) and ground-based observations, the effects of industrial fluctuations due to the financial crisis on local NO2 pollution were quantitatively assessed. The results were as follows. (1) A distinct V-shaped fluctuation of major industrial products, thermal generating capacity, electricity consumption, and tropospheric NO2 densities was associated with the global financial crisis from May 2007 to December 2009, with the largest anomalies 1.5 times more than standard deviations at the height of the crisis period from November 2008 to February 2009. (2) Among all industrial sectors, thermal power plants were mainly responsible for fluctuations in local NO2 pollution during the crisis period. Thermal generating capacity had its greatest decrease of 12.10% at the height of the crisis compared with that during November 2007–February 2008, leading to local tropospheric NO2 density decreasing by 16.97%. As the crisis appeased, thermal generating capacity increased by 29.63% from November 2009 to February 2010, and tropospheric NO2 densities correspondingly increased by 30.07%. (3) Among all industrial sectors in the YRD, the thermal power sector has the greatest coal consumption of about 65.96%. A decline in thermal power of about 10% can induce a decrease of about 30% in NOx emissions and NO2 densities, meaning that a relative small fluctuation in industrial production can lead to a large decrease in tropospheric NO2 densities over industrially developed areas like the YRD region. Since electricity is mainly obtained from local coal-burning thermal plants without NOx-processing equipment, installing NOx-removal devices for all thermal power plants is an important and feasible way of controlling local NOx pollution at present.  相似文献   

10.
以武汉市为研究区域,基于实地调查获得典型行业污染源活动水平,以大气污染物排放清单编制技术指南为参考,利用排放因子法建立2014年武汉市大气污染源排放清单,并结合经纬度、人口密度分布、土地利用类型、道路长度等数据将排放清单进行了3 km×3 km网格化处理.结果表明,2014年武汉市SO2、NOx、PM10、PM2.5、CO、BC、OC、VOCs和NH3排放量分别为10.3、17.0、16.3、7.1、63.1、0.6、0.4、19.8和1.6万t.固定燃烧源为SO2排放的主要来源,其贡献率约64%;移动源为NOx的主要来源,其贡献率约51%;颗粒物排放主要来源于扬尘源和工艺过程源;CO和VOCs主要来源于工艺过程源,BC和OC排放均以移动源和生物质燃烧源为主,NH3排放主要来自农业源.污染物排放主要集中在青山区至新洲区一带.  相似文献   

11.
A combination of linear response models is used to estimate the transient changes in the global means of carbon dioxide (CO2) concentration, surface temperature, and sea level due to aviation. Apart from CO2, the forcing caused by ozone (O3) changes due to nitrogen oxide (NOx) emissions from aircraft is also considered. The model is applied to aviation using several CO2 emissions scenarios, based on reported fuel consumption in the past and scenarios for the future, and corresponding NOx emissions. Aviation CO2 emissions from the past until 1995 enlarged the atmospheric CO2 concentration by 1.4 ppmv (1.7% of the anthropogenic CO2 increase since 1800). By 1995, the global mean surface temperature had increased by about 0.004 K, and the sea level had risen by 0.045 cm. In one scenario (Fa1), which assumes a threefold increase in aviation fuel consumption until 2050 and an annual increase rate of 1% thereafter until 2100, the model predicts a CO2 concentration change of 13 ppmv by 2100, causing temperature increases of 0.01, 0.025, 0.05 K and sea level increases of 0.1, 0.3, and 0.5 cm in the years 2015, 2050, and 2100, respectively. For other recently published scenarios, the results range from 5 to 17 ppmv for CO2 concentration increase in the year 2050, and 0.02 to 0.05 K for temperature increase. Under the assumption that present-day aircraft-induced O3 changes cause an equilibrium surface warming of 0.05 K, the transient responses amount to 0.03 K in surface temperature for scenario Fa1 in 1995. The radiative forcing due to an aircraft-induced O3 increase causes a larger temperature change than aircraft CO2 forcing. Also, climate reacts more promptly to changes in O3 than to changes in CO2 emissions from aviation. Finally, even under the assumption of a rather small equilibrium temperature change from aircraft-induced O3 (0.01 K for the 1992 NOx emissions), a proposed new combustor technology which reduces specific NOx emissions will cause a smaller temperature change during the next century than the standard technology does, despite a slightly enhanced fuel consumption. Regional effects are not considered here, but may be larger than the global mean responses.  相似文献   

12.
Combining policies to remove carbon dioxide (CO2) from the atmosphere with policies to reduce emissions could decrease CO2 concentrations faster than possible via natural processes. We model the optimal selection of a dynamic portfolio of abatement, research and development (R&D), and negative emission policies under an exogenous CO2 constraint and with stochastic technological change. We find that near-term abatement is not sensitive to the availability of R&D policies, but the anticipated availability of negative emission strategies can reduce the near-term abatement optimally undertaken to meet 2°C temperature limits. Further, planning to deploy negative emission technologies shifts optimal R&D funding from ??carbon-free?? technologies into ??emission intensity?? technologies. Making negative emission strategies available enables an 80% reduction in the cost of keeping year 2100 CO2 concentrations near their current level. However, negative emission strategies are less important if the possibility of tipping points rules out using late-century net negative emissions to temporarily overshoot the CO2 constraint earlier in the century.  相似文献   

13.
Study of a high SO2 event observed over an urban site in western India   总被引：1，自引：0，他引：1  
Continuous measurements of SO2, NOx and O3 along with sampling based measurements of CO, CH4, NMHCs and CO2 were carried out during May, 2010 at Ahmedabad. The diurnal variations of SO2 in ambient air exhibited elevated values during the night and lower levels during the sunlit hours. The mean concentration of SO2 during the study period was 0.95 ± 0.88 ppbv. However, the ambient SO2 exceeded 17 ppbv in the night of 20 May, 2010. On the same day, tropospheric columnar SO2 from OMI showed almost 350% increase corroborating the surface observations over an extended height regime. This was also the highest columnar value of SO2 during the summer of 2010. Columnar loadings were also found to be high for formaldehyde, precipitable water vapor and aerosol optical depth on 20 May. Elevated concentrations were also recorded for other trace gases like NO2 and O3. Analysis of related data of trace gases indicated characteristics of fresh emissions with dominant contributions from mobile sources during the study period. However, SO2/NO2 ratio of 0.36 during the event period on 20th May connotes non-local influences. Analyses of meteorological parameters suggest combined impacts of transport and inversion causing higher levels of SO2 and other pollutants during 20?C21 May. Episodes of such enhancements may perturb chemical and radiative balance of the atmosphere.  相似文献   

14.
This paper synthesizes results of the multi-model Energy Modeling Forum 27 (EMF27) with a focus on climate policy scenarios. The study included two harmonized long-term climate targets of 450 ppm CO2-e (enforced in 2100) and 550 pm CO2-e (not-to-exceed) as well as two more fragmented policies based on national and regional emissions targets. Stabilizing atmospheric GHG concentrations at 450 and 550 ppm CO2-e requires a dramatic reduction of carbon emissions compared to baseline levels. Mitigation pathways for the 450 CO2-e target are largely overlapping with the 550 CO2-e pathways in the first half of the century, and the lower level is achieved through rapid reductions in atmospheric concentrations in the second half of the century aided by negative anthropogenic carbon flows. A fragmented scenario designed to extrapolate current levels of ambition into the future falls short of the emissions reductions required under the harmonized targets. In a more aggressive scenario intended to capture a break from observed levels of stringency, emissions are still somewhat higher in the second half due to unabated emissions from non-participating countries, emphasizing that a phase-out of global emissions in the long term can only be reached with full global participation. A key finding is that a large range of energy-related CO2 emissions can be compatible with a given long-term target, depending on assumptions about carbon cycle response, non-CO2 and land use CO2 emissions abatement, partly explaining the spread in mitigation costs.  相似文献   

15.
APEC blue was coined to describe the impact of short-term curbs on air pollution during the Asian-Pacific Economic Cooperation (APEC) Summit organized in Beijing in November 2014 and has been a hot topic among both general public and scientific sector in China. The consensus that gaseous agents NO2 and SO2 are greatly reduced in response to the control and restriction strategies implemented during the Summit period is shared by earlier literature. However, the re-examination of APEC blue conducted in the present study comes to a more contrasted conclusion. The remarkable drop in NO2 abundances is confirmed in terms of both surface concentration and vertical column, whereas corresponding SO2 changes are found to be marginal and not statistically significant, indicating that the decline of SO2 was more tied to natural or random variability rather than externally forced. To explain the contrasted responses of NO2 and SO2 during the APEC summit, short-term variations of these species are further placed in the context of a longer term perspective, which reveals a striking contrast in the pathways of the secular tendency in NO2 and SO2 emissions and corresponding measured abundances of both pollutants. On the one hand, NO2 emissions exhibit a sharp rise by 30–50% from 2006-2010 to 2011–2014; on the other hand, SO2 emissions have undergone a gradual decrease in the last decade and have currently returned to their pre-2000 level. Therefore, short-term control measures are expected to be more effective in reducing the levels of NO2 than SO2.  相似文献   

16.
应用大气化学模式WRF-Chem(Weather Research and Forecast-Chemistry),分别选用亚洲排放源清单INTEX-B(Intercontinental Chemical Transport Experiment-Phase B)、REASv2.1(Regional Emission inventory in Asia version 2.1)以及全球排放源清单HTAP_v2(Hemispheric Transport of Air Pollution version 2),对浙江省2013年12月进行模拟,分别记为IN、RE和HT试验,研究人为源排放清单对大气污染物浓度数值模拟的影响。结果表明,3组试验合理的反映出PM2.5(空气动力学当量直径小于等于2.5μm的颗粒物,即细颗粒物)、PM10(空气动力学当量直径小于等于10μm的颗粒物,即可吸入颗粒物)和NO_2近地面浓度的时空分布特征,相关系数为0.5~0.8,85%以上的模拟值落在观测值的0.5~2倍范围内,但对SO_2近地面浓度模拟较差。IN、RE、HT试验对PM2.5和PM10的模拟偏差均成递减趋势,约为30%、16%和6%,HT试验的模拟值更加接近观测。INTEX-B清单中PM2.5的一次排放与二次气溶胶前提物SO_2均高于REAS与HTAP清单,因此会导致更多的硫酸盐生成,从而进一步增加PM2.5浓度。HTAP_v2清单中较低的NH3排放会抑制硝酸盐的生成,从而有助于降低PM2.5浓度。3个清单的基准年与模拟年的差异对SO_2浓度模拟的准确性影响更大,INTEX-B清单中SO_2排放量明显高于REASv2.1与HTAP_v2清单,尤其在浙北和沿海工业发达地区,导致IN试验模拟的SO_2在这些地区存在明显高估。3组试验模拟的NO_2浓度偏差最小且更为接近(-8%~4%),主要原因是3个清单在浙江省的NOx排放十分一致。从3组试验结果之间的差异程度来看,浙江省范围内PM2.5、PM10、SO_2和NO_2逐日浓度模拟值之间的平均差异程度分别约为14%、15%、51%和16%,最大差异程度分别为69%、78%、137%和132%。月均浓度与逐日浓度的平均差异程度基本一致,但最大差异程度明显更低。总体来看3组试验模拟的PM2.5、PM10与NO_2的差异程度明显低于SO_2。  相似文献   

17.
Uncertainties in climate stabilization   总被引：1，自引：1，他引：0  
The atmospheric composition, temperature and sea level implications out to 2300 of new reference and cost-optimized stabilization emissions scenarios produced using three different Integrated Assessment (IA) models are described and assessed. Stabilization is defined in terms of radiative forcing targets for the sum of gases potentially controlled under the Kyoto Protocol. For the most stringent stabilization case (“Level 1” with CO2 concentration stabilizing at about 450 ppm), peak CO2 emissions occur close to today, implying (in the absence of a substantial CO2 concentration overshoot) a need for immediate CO2 emissions abatement if we wish to stabilize at this level. In the extended reference case, CO2 stabilizes at about 1,000 ppm in 2200—but even to achieve this target requires large and rapid CO2 emissions reductions over the twenty-second century. Future temperature changes for the Level 1 stabilization case differ noticeably between the IA models even when a common set of climate model parameters is used (largely a result of different assumptions for non-Kyoto gases). For the Level 1 stabilization case, there is a probability of approximately 50% that warming from pre-industrial times will be less than (or more than) 2°C. For one of the IA models, warming in the Level 1 case is actually greater out to 2040 than in the reference case due to the effect of decreasing SO2 emissions that occur as a side effect of the policy-driven reduction in CO2 emissions. This effect is less noticeable for the other stabilization cases, but still leads to policies having virtually no effect on global-mean temperatures out to around 2060. Sea level rise uncertainties are very large. For example, for the Level 1 stabilization case, increases range from 8 to 120 cm for changes over 2000 to 2300.  相似文献   

18.
In this paper we quantify the CH4, CO2 and NO x emissions during routine operations at a major oil and gas production facility, Prudhoe Bay, Alaska, using the concentrations of combustion by products measured at the NOAA-CMDL observatory at Barrow, Alaska and fuel consumption data from Prudhoe Bay. During the 1989 and 1990 measurement campaigns, 10 periods (called events) were unambiguously identified where surface winds carry the Prudhoe Bay emissions to Barrow (approximately 300 km). The events ranged in duration from 8–48 h and bring ambient air masses containing substantially elevated concentrations of CH4, CO2 and NO y to Barrow. Using the slope of the observed CH4 vs CO2 concentrations during the events and the CO2 emissions based on reported fuel consumption data, we calculate annual CH4 emissions of (24+/–8)×103 metric tons from the facility. In a similar manner, the annual NO x emissions are calculated to be (12+/–4)×103 metric tons, which is in agreement with an independently determined value. The calculated CH4 emissions represent the amount released during routine operations including leakage. However this quantity would not include CH4 released during non-routine operations, such as from venting or gas flaring.  相似文献   

19.
本文利用气体组分及大气气溶胶在线监测系统(MARGA ADI 2080)观测武汉市2018年1月9—26日大气气溶胶中的8种水溶性离子(NH+4、NO-3、SO2-4、Cl-、K+、Ca2+、Na+和Mg2+),结合气象要素数据,使用主成分分析(PCA)、正定矩阵因子分析法(PMF)、HYSPLIT后向轨迹模式、潜在源区贡献(PSCF)和浓度权重轨迹(CWT),对霾污染过程中水溶性离子进行了全面的来源解析,探究了霾不同阶段下来源差异和空间分布特征。结果表明:(1)本次霾污染中的8种水溶性离子和4种污染气体,PCA解析出的源和占比分别为二次源和燃煤源的混合源(41.28%)、工业排放和土壤扬尘混合源(27.73%)和机动车排放源(9.63%),PMF解析出的源和占比分别为燃煤与土壤扬尘混合源(18.57%)、机动车排放源(20.74%)、二次源(18.30%)、光化学污染源(22.24%)和燃煤源(20.15%)。(2)霾在不同阶段下水溶性离子和4种污染气体的来源存在差异,在清洁天和霾消散阶段,光化学的贡献最高,占比分别为31.42%和36.07%;在霾发生阶段燃煤与土壤扬尘源的贡献最高,其贡献为40.94%;在霾发展阶段,最大的控制源为二次源,贡献占比为37.51%。(3)此次武汉市霾污染中PM2.5浓度和NH+4、NO-3和SO2-4的潜在源区为皖豫鄂三省和赣湘鄂三省交界处。霾污染中PM2.5的主要影响范围是武汉市南部和北部省份,NO-3、NH+4和SO2-4的主要影响区域为武汉市东北方向的城市、湖南省和江西省。  相似文献   

20.
During 18–23 July 1990, 31 smoke samples were collected from an aircraft flying at low altitudes through the plumes of tropical savanna fires in the Northern Territory, Australia. The excess (above background) mixing ratios of 17 different trace gases including CO2, CO, CH4, several non-methane hydrocarbons (NMHC), CH3CHO, NO x (– NO + NO2), NH3, N2O, HCN and total unspeciated NMHC and sulphur were measured. Emissionratios relative to excess CO2 and CO, and emissionfactors relative to the fuel carbon, nitrogen or sulphur content are determined for each measured species. The emission ratios and factors determined here for carbon-based gases, NO x , and N2O are in good agreement with those reported from other biomass burning studies. The ammonia data represent the first such measurements from savanna fires, and indicate that NH3 emissions are more than half the strength of NO x emissions. The emissions of NO x , NH3, N2O and HCN together represent only 27% of the volatilised fuel N, and are primarily NO x (16%) and NH3 (9%). Similarly, only 56% of the volatilised fuel S is accounted for by our measurements of total unspeciated sulphur.  相似文献   

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