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1.
The input of groundwater-borne nutrients to Adelaide's (South Australia) coastal zone is not well known but could contribute to the ongoing decline of seagrass in the area. As a component of the Adelaide Coastal Waters Study (ACWS), the potential for using the radium quartet (223Ra, 224Ra, 226Ra and 228Ra) and 222Rn to evaluate submarine groundwater discharge (SGD) was evaluated. Potential isotopic signatures for SGD were assessed by sampling groundwater from three regional aquifers potentially contributing SGD to the ACWS area. In addition, intertidal groundwater was sampled at two sand beach sites. In general, the regional groundwaters were enriched in long-lived Ra isotopes (226Ra and 228Ra) and in 222Rn relative to intertidal groundwater. Radium activity (but not 222Rn activity) was positively correlated to salinity in groundwater from one of the regional aquifers and in intertidal groundwater. Radium isotope ratios (223Ra/226Ra, 224Ra/226Ra and 228Ra/226Ra) were less variable than individual Ra isotope activities within potential SGD sources. Recirculated seawater (estimated from the intertidal groundwater samples with seawater-like salinities) also had distinctly higher Ra isotope ratios than the regional groundwaters. The activities for all radioisotopes were relatively low in seawater. The activity of the short-lived 223Ra and 224Ra were highest at the shoreline and declined exponentially with distance offshore. In contrast, 228Ra and 226Ra activities had a weak linear declining trend with distance offshore. Rn-222 activity was at or near background in all seawater samples. The pattern of enrichment in short-lived Ra isotopes and the lack of 222Rn in seawater suggest that seawater recirculation is the main contributor to SGD in the ACWS area. Preliminary modeling of the offshore flux of 228Ra and 226Ra suggest that the SGD flux to the ACWS area ranges between 0.2 and 3 · 10− 3 m3 (m of shoreline)− 1 s− 1.  相似文献   

2.
We determined groundwater flow rates shortly after the wet season into an embayment near Ubatuba, Brazil as part of an international intercomparison experiment for submarine groundwater discharge (SGD) assessment techniques. Our estimated rates were determined by the combined use of continuous radon measurements and assessment of radium isotope patterns. The spatial distribution of the short-lived radium isotopes (223Ra and 224Ra) provided the means for independent evaluations of radon losses by mixing and atmospheric evasion. We were thus able to construct a well-constrained mass balance for radon that included a groundwater flux term. Our results showed that the groundwater discharge into this embayment from the fractured crystalline rock aquifer is not steady-state but varies with tidal modulation and rain-induced forcing. Tidally modulated and rain-induced flow rates were comparable during this period. The SGD rates estimated from radon ranged from 1 cm/day to 29 cm/day (cm3/cm2 day) with a mean and standard deviation of 13 ± 6 cm/day. These estimates were mostly similar to a dye-dilution automatic seepage meter (15 ± 19 cm/day) and were within the broad ranges estimated by manual and continuous heat seepage meters but lower than indicated by an artificial tracer test performed nearshore.  相似文献   

3.
海底地下水排放对典型红树林蓝碳收支的影响   总被引：1，自引：0，他引：1  
海底地下水排放(Submarine Groundwater Discharge，SGD)是陆海相互作用的重要表现形式之一，其携带的物质对近岸海域生源要素的收支有重要影响。本文利用222Rn示踪技术估算了我国典型红树林海湾—广西珍珠湾在2019年枯季(1月)SGD携带的碳通量。调查发现，地下水中222Rn活度、溶解无机碳(DIC)和溶解有机碳(DOC)的平均浓度均高于河水和湾内表层海水。利用222Rn质量平衡模型估算得到珍珠湾SGD速率为(0.36±0.36) m/d，SGD输入到珍珠湾的DIC和DOC通量分别为(2.41±2.63)×107 mol/d和(1.96±2.20)×106 mol/d。珍珠湾溶解碳的源汇收支表明，SGD携带的DIC和DOC分别占珍珠湾总DIC和总DOC来源的91%和89%。因此，SGD携带的DIC和DOC是珍珠湾DIC和DOC的主要来源，是海岸带蓝碳收支和生物地球化学循环过程中的重要组成。  相似文献   

4.
The four naturally-occurring radium isotopes (223Ra, 224Ra, 226Ra and 228Ra) were used to estimate the submarine groundwater discharge (SGD) in the Isola La Cura marsh area in the northern Venice Lagoon (Italy). By determining the radium contributors to the study area (river, coastal ocean and sediments) the radium excess in the lagoon water was quantified through a mass balance model. This radium excess is attributed to a submarine groundwater discharge source and represents the most important input of radium. Possible endmembers were considered from analysis of groundwater samples (subtidal and marsh piezometers, marsh wells and seepage meters) that were enriched in Ra by one to two orders of magnitude relative to surface waters. In particular, a permeable layer at 80 cm depth in the surrounding marsh is considered to be representative of the most likely SGD source, although similar radium activities were measured in other subtidal porewater samples collected in the Isola La Cura area. The estimated SGD flux to the study area ranged from 1 · 109 to 6 · 109 L·d− 1, the same order of magnitude as the overall riverine input to the lagoon (3 · 109 L·d− 1). A major fraction of this SGD flux is likely recirculated seawater, as evidenced by the endmember salinity. The water residence time of 2 days was estimated by both using the shortest-lived radium isotope and estimating the volume of water exchanged between the lagoon and the open sea during a tidal cycle (tidal prism approach). This SGD flux could be used to estimate the input of other chemical species (metals, nutrients, etc.) via SGD which might affect the Venice Lagoon ecosystem.  相似文献   

5.
Submarine groundwater discharge (SGD) is now recognized as an important pathway for water and chemical species fluxes to the coastal ocean. In order to determinate SGD to the Gulf of Lion (France), we measured the activities of 226Ra and 228Ra by thermal ionization mass spectrometry (TIMS) in coastal waters and in the deep aquifer waters of the Rhone deltaic plain after pre-concentration of radium by MnO2. Compared to conventional counting techniques, TIMS requires lower quantities of water for the analyses, and leads to higher analytical precision. Radium isotopes were thus measured on 0.25–2 L water samples containing as little as 20 fg of 226Ra and 0.2–0.4 fg of 228Ra with precision equal to 2%. We demonstrate that coastal surface waters samples are enriched in 226Ra and 228Ra compared to the samples further offshore. The high precision radium measurements display a small but significant 226Ra and 228Ra enrichment within a strip of circa 30 km from the coast. Radium activities decrease beyond this region, entrained in the northern current along the shelf break or controlled by eddy diffusion. The radium excess in the first 30 km cannot be accounted for by the river nor by the early diagenesis. The primary source of the radium enrichment must therefore be ascribed to the discharge of submarine groundwater. Using a mass-balance model, we estimated the advective fluxes of 226Ra and 228Ra through SGD to be 5.2 × 1010 and 21 × 1010 dpm/d respectively. The 226Ra activities measured in the groundwater from the Rhone deltaic plain aquifer are comparable to those from other coastal groundwater studies throughout the world. By contrast, 228Ra activities are higher by up to one order of magnitude. Taking those groundwater radium activities as typical of the submarine groundwater end-member, a minimum volume of 0.24–4.5 × 1010 l/d is required to support the excess radium isotopes on the inner shelf. This has to be compared with the average rivers water runoff of 15.4 × 1010 l/d during the study period (1.6 to 29% of the river flow).  相似文献   

6.
Transport between pore waters and overlying surface waters of Flamengo Bay near Ubatuba, Brazil, was quantified using natural and artificial geochemical tracers, 222Rn, Cl−, and SF6, collected from multi-level piezometers installed along a transect perpendicular to the shore. Eight sampling ports positioned along the length of the piezometers allowed sampling of pore waters at discrete depth intervals from 10 to 230 cmbsf (centimeters below seafloor). Small volume samples were collected from the piezometers using a peristaltic pump to obtain pore water depth profiles. Pore water 222Rn is deficient in shallow sediments, allowing application of a diffusion-corrected 222Rn exchange rate. This model estimates the magnitude of pore water exchange rates to be about 130–419 cm/day. An SF6-saturated fluorescein dye tracer was gently pumped into deep pore waters and exchange rates estimated from this method range from 29 to 185 cm/day. While absolute rates are higher using 222Rn than SF6, rates are of similar magnitudes and the trends with distance from shore are the same – flow is greatest 6 m from shore and decreases by more than 50% further offshore. A Cl− mass balance indicates the greatest fraction of fresh SGD occurs along an apparent preferential flow path in sediments within 5–7 m of the shoreline (87%). Recirculating bay waters through sediments dominate pore water advection at 10 m offshore where only 4% of the flow can be attributed to a freshwater source. Both fresh and marine sources combine to make up submarine groundwater discharge to coastal water bodies. The magnitude of fresh aquifer discharge is often a spatially variable and minor component of the total discharge.  相似文献   

7.
基于223Ra和224Ra的桑沟湾海底地下水排放通量   总被引：1，自引：0，他引：1  
海底地下水排放（SGD）是陆地向海洋输送水量和营养物质的重要通道之一,对沿海物质通量及其生物地球化学循环有重要的影响,对生态环境起着不可忽视的作用。本文运用天然放射性同位素223Ra和224Ra示踪估算了我国北方典型养殖基地桑沟湾的海底地下水排放通量。结果表明,海底地下水样尤其是间隙水中Ra活度[224Ra=（968±31）dpm/（100 L）,223Ra=（31.4±4.9）dpm/（100 L）,n=9]远高于表层海水[224Ra=（38.7±2.0）dpm/（100 L）,223Ra=（1.70±0.50）dpm/（100 L）, n=21]。假设稳态条件下,考虑Ra的各源、汇项,利用Ra平衡模型,估算出桑沟湾SGD排放通量为（0.23~1.03）×107 m3/d。潮周期内的观测结果显示,涨潮时,水力梯度较小,SGD排放变弱,落潮时,水力梯度较大,导致了相对较多的SGD排放。在一个潮周期间,基于223Ra和224Ra得到的SGD排放通量平均为0.39×107 m3/d。潮汐动力下的SGD排放平均占总SGD排放的61%,因此桑沟湾沿岸的地下水排放主要受潮汐动力的影响,并对海水组成及海陆间物质交换有显著贡献。  相似文献   

8.
Coastal waters contain elevated dissolved activities of short-lived radium isotopes, 223Ra and 224Ra, having half-lives of 11.4 and 3.66 days, respectively. The input of these isotopes near the coast must be balanced by decay and mixing into the open ocean, where excess activities are zero. Since the decay rate is known, in the ideal case the mixing rate may be determined from the offshore distribution of these isotopes. This study found that samples collected in June 2000 followed the expected exponential decrease with distance offshore. We assign a dispersion coefficient of 28–39 m2 s−1 for this study. During January 2002 and November 2003, there was not a consistent decrease of activity with distance offshore. This is likely due to the ruggedness of the coastline, where many bays and small islands interrupt simple mixing patterns. To estimate exchange rates during 2002 and 2003, we used a model based on the decrease in the 224Ra/223Ra activity ratio (AR) with time for samples isolated from fresh inputs of Ra. This model yielded residence times of 1–2 weeks for samples collected within 20 km of the coast. We used this residence time to calculate the flux of 228Ra (half-life = 5.7 years) to the study area necessary to maintain the enrichment relative to ocean water. This enrichment is a factor of ten greater than the flux of 228Ra expected from submarine groundwater discharge (SGD) occurring within 50 m of shore.  相似文献   

9.
There is increasing evidence that submarine groundwater discharge (SGD) in many areas represents a major source of dissolved chemical constituents to the coastal ocean. In Great South Bay, NY, previous studies have shown that the discharge of nutrients with SGD may cause harmful algal blooms. This study estimates SGD to Great South Bay during August 2006 by performing a mass balance for each of the dissolved Ra isotopes (224Ra, 223Ra, 228Ra, 226Ra). The budget indicates a major unknown source (between 30 and 60% of the total input) of Ra to the bay. This imbalance can be resolved by a flux of Ra-enriched groundwater on the order of 3.5–4.5 × 109 L d− 1, depending on the Ra isotope. The Ra-estimated SGD rates compare well with those previously estimated by models of flow that decreases exponentially away from shore. Compared to previous reports of fresh groundwater discharge to the bay, the Ra-estimated discharge must comprise approximately 90% recirculated seawater. The good agreement between Ra- and model-estimated flow rates indicates that the primary SGD endmember may be best sampled at shallow depths in the sediments a short distance bayward of the low tide line.  相似文献   

10.
Measurements of electric resistivity of the seabed and of the electric conductivity of submarine groundwater discharge (SGD) collected in seepage meters have been made to evaluate temporal variability of the origin and quality of submarine groundwater discharge in Ubatuba, Brazil. A diurnal variation of SGD conductivity was found under the condition of semi-diurnal tidal changes over a period of 4 days. Both the ground resistivity and the conductivity of the discharged groundwater indicated that the freshwater–saltwater interface moved towards offshore at high tide, i.e. in the direction opposite to commonly made observations. SGD comprised a combination of Submarine Fresh Groundwater Discharge (SFGD) of terrestrial origin, and of Recirculated Saline Groundwater Discharge (RSGD) of marine origin. The maximum of the terrestrially derived fraction SFGD/SGD was found at a distance of 50 m offshore. A lower SFGD/SGD ratio was found closer to shore, where the highest SGD flux was measured. SGD conductivity and ground resistivity displayed a diurnal cyclicity at semi-diurnal tidal water level variations, indicating that tidal water level fluctuations may not be the primary driver of SGD flux, but preferential flow in volcanic hydrogeologic setting at Ubatuba.  相似文献   

11.
The distributions of dissolved organic carbon (DOC), Ba, U, and a suite of naturally occurring radionuclides in the U/Th decay series (222Rn, 223,224,226,228Ra) were studied during high- and low-discharge conditions in the Loxahatchee River estuary, Florida to examine the role of submarine groundwater discharge in estuarine transport. The fresh water endmember of this still relatively pristine estuary may reflect not only river-borne constituents, but also those advected during active groundwater/surface water (hyporheic) exchange. During both discharge conditions, Ba concentrations indicated slight non-conservative mixing. Such Ba excesses could be attributed either to submarine groundwater discharge or particle desorption processes. Estuarine dissolved organic carbon concentrations were highest at salinities closest to zero. Uranium distributions were lowest in the fresh water sites and mixed mostly conservatively with an increase in salinity. Suspended particulate matter (SPM) concentrations were generally lowest (< 5 mg L− 1) close to zero salinity and increased several-fold ( 18 mg L− 1; low discharge) toward the seaward endmember, which may be attributed to dynamic resuspension of bottom sediments within Jupiter Inlet.Surface water-column 222Rn activities were most elevated (> 28 dpm L− 1) at the freshwater endmember of the estuary and appear to identify regions of the river most influenced by the discharge of fresh groundwater. Activities of four naturally occurring isotopes of Ra (223,224,226,228Ra) in this estuary and select adjacent shallow groundwater wells yield mean estuarine water-mass transit times of less than 1 day; these values are in close agreement to those calculated by tidal prism and tidal frequency. Submarine groundwater discharge rates to the Loxahatchee River estuary were calculated using a tidal prism approach, an excess 226Ra mass balance, and an electromagnetic seepage meter. Average SGD rates ranged from 1.0 to 3.8 × 105 m3 d− 1 (20–74 L m− 2 d− 1), depending on river-discharge stage. Such calculated SGD estimates, which must include both a recirculated as well as fresh water component, are in close agreement with results obtained from a first-order watershed mass balance. Average submarine groundwater discharge rates yield NH4+ and PO4− 3 flux estimates to the Loxahatchee River estuary that range from 62.7 to 1063.1 and 69.2 to 378.5 μmol m− 2 d− 1, respectively, depending on river stage. SGD-derived nutrient flux rates are compared to yearly computed riverine total N and total P load estimates.  相似文献   

12.
A mass balance for the naturally-occurring radium isotopes (224Ra, 223Ra, 228Ra, and 226Ra) in Jamaica Bay, NY, was conducted by directly estimating the individual Ra contributions of wastewater discharge, diffusion from fine-grained subtidal sediments, water percolation through marshes, desorption from resuspended particles, and water exchange at the inlet. The mass balance revealed a major unknown source term accounting for 19–71% of the total Ra input, which could only be resolved by invoking a source from submarine groundwater. Shallow (< 2 m depth) groundwater from permeable sediments in Jamaica Bay was brackish and enriched in Ra relative to surface bay waters by over two orders of magnitude. To balance Ra fluxes, a submarine groundwater input of 0.8 × 109–9.0 × 109 L d− 1 was required. This flux was similar for all four isotopes, with individual estimates varying by less than a factor of 2. Our calculated groundwater flux was 6- to 70-fold higher than the fresh groundwater discharge to the bay estimated by hydrological methods, but closely matched direct flow rates measured with seepage meters. This suggests that a substantial portion of the discharge consisted of recirculated seawater. The magnitude of submarine groundwater discharge varied seasonally, in the order: summer > autumn > spring. Chemical analyses suggest that the recirculated seawater component of submarine groundwater delivers as much dissolved nitrogen to the bay as the fresh groundwater flux.  相似文献   

13.
This paper reports the initial results of a study of groundwater and coastal waters of southern Brazil adjacent to a 240 km barrier spit separating the Patos Lagoon, the largest coastal lagoon in South America, from the South Atlantic Ocean. The objective of this research is to assess the chemical alteration of freshwater and freshwater–seawater mixtures advecting through coastal permeable sands, and the influence of the submarine discharge of these fluids (SGD) on the chemistry of coastal waters. Here we focus on dissolved iron in this system and use radium isotopic tracers to quantify SGD and cross-shelf fluxes. Iron concentrations in groundwaters vary between 0.6 and 180 μM. The influence of the submarine discharge of these fluids into the surf zone produces dissolved Fe concentrations as high as several micromolar in coastal surface waters. The offshore gradient of dissolved Fe, coupled with results for Ra isotopes, is used to quantify the SGD flux of dissolved Fe from this coastline. We estimate the SGD flux to be 2 × 106 mol day− 1 and the cross-shelf flux to be 3.2 × 105 mol day− 1. This latter flux is equal to about 10% of the soluble atmospheric Fe flux to the entire South Atlantic Ocean. We speculate on the importance of this previously unrecognized iron input to regional ocean production and on the potential significance of this source to understanding variations in glacial–interglacial ocean production.  相似文献   

14.
Measurements of submarine groundwater discharge (SGD) along the South American coast and over fractured rock aquifers are rare. The rate and distribution of SGD was measured using three types of vented benthic chambers on the floor of Flamengo Bay located at the southeast coast of Brazil. Discharge rates were found up to almost 400 cm day−1, although typically less than 100 cm d−1. Large variations in SGD rates were seen over distances of a few meters which are attributed to the geomorphologic features of the fracture rock aquifer underlying a thin blanket of coastal sediments; clustering of fractures and the topography of the rock–sediment interface might be focusing or dispersing the discharge of groundwater. SGD was modulated by the tides with the highest values occurring at times of low tide, but the interaction was non-linear and, the correlation was weak at tidal ranges less than 1 m. The effect was masked by devices that integrated the SGD, but detected on continuously recording devices.  相似文献   

15.
In certain regions,submarine groundwater discharge(SGD) into the ocean plays a significant role in coastal material fluxes and their biogeochemical cycle;therefore,the impact of SGD on the ecosystem cannot be ignored.In this study,SGD was estimated using naturally occurring radium isotopes(~(223)Ra and ~(224)Ra) in a subtropical estuary along the Beibu Gulf,China.The results showed that the Ra activities of submarine groundwater were approximately 10 times higher than those of surface water.By assuming a steady state and using an Ra mass balance model,the SGD flux in May 2018 was estimated to be 5.98×10~6 m~3/d and 3.60×10~6 m~3/d based on ~(224)Ra and ~(223)Ra,respectively.At the same time,the activities of Ra isotopes fluctuated within a tidal cycle;that is,a lower activity was observed at high tide and a higher activity was seen at low tide.Based on these variations,the average tidal pumping fluxes of SGD were 1.15×10~6 m~3/d and 2.44×10~6 m~3/d with ~(224)Ra and ~(223)Ra,respectively.Tidaldriven SGD accounts for 24%-51% of the total SGD.Therefore,tidal pumping is an important driving force of the SGD in the Dafengjiang River(DFJR) Estuary.Furthermore,the SGD of the DFJR Estuary in the coastal zone contributes significantly to the seawater composition of the Beibu Gulf and the material exchange between land and sea.  相似文献   

16.
Algal blooms in Tolo Harbour, Hong Kong have received much attention and submarine groundwater discharge is speculated to be a significant pathway carrying nutrients into the constricted estuary. Plover Cove, a small cove in the Harbour, was selected for SGD analysis using 222Rn budget. The volumetric SGD rates are estimated to be about 8000 m3/day for neap tide and about 17,000 m3/day for spring tide. Result of nutrient analysis of the porewater indicates that the nutrient loading through this pathway is speculated to be crucial for eutrophication in Tolo Harbour. Current practice for the management of algal blooms in Hong Kong, in which nutrient loading through SGD was ignored, has to be reviewed and the control measures of groundwater contamination are obviously required.  相似文献   

17.
We measured the time-series variations in 222Rn activity at a fixed station in the Yeongsan River Estuary (YRE), Korea, where the upstream water is obstructed by an artificial dam, during November 18–24, 2008, and conducted a horizontal 222Rn survey in the Seomjin River Estuary (SRE), Korea, during December 16–18, 2008. In the YRE, we observed constantly low levels of 222Rn activity over the sampling period, relative to the summer in 2008. The 222Rn variations and 222Rn mass-balance modeling results indicate that the submarine groundwater discharge (SGD) in the YRE was relatively low and constant over the sampling period and that the temporal SGD variations were not related to tides or to the water elevation in the dam upstream. This low and constant SGD appears to be due to the lower water level in the dam relative to the local sea level during the study period, resulting in the SGD mostly from the surrounding land areas rather than from the dam. In the SRE, higher 222Rn activities were observed at upstream stations of the river (salinity: <5) and decreased as the salinity increased, but there were marked increases of 222Rn, together with dissolved inorganic silicate (DSi), at stations close to the river mouth (salinity: ～33). This suggests that the river has major groundwater inputs from the two extreme upstream and downstream areas. Because most chemical flux estimations via river discharge do not account for groundwater inputs from the downstream high-salinity zone, our results suggest that there is an important unaccounted source of river-driven chemical fluxes. Overall, our study shows that the continuous 222Rn monitoring system provides high-resolution information on SGD over different locations and times.  相似文献   

18.
Radium isotopes (223Ra, 224Ra, 226Ra, and 228Ra) and water chemistry were used to identify two chemically distinct sources of submarine groundwater discharge (SGD) in Celestún Lagoon, Yucatán, Mexico. Low salinity groundwater discharging from springs within the lagoon has previously been identified and extensively sampled for nutrient concentrations. However, a second type of groundwater discharging into the lagoon was detected during this study using radium isotope activity measurements. This second type of groundwater is characterized by moderate salinities (within the range of lagoon salinities) and very elevated radium activities in comparison to the low salinity groundwater, mixed lagoon water, and seawater. Further analysis showed that the two types of groundwater also have distinct chloride, strontium, and sulfate ratios, along with slightly different nutrient concentrations. Groundwater discharge occurs through large and small springs scattered throughout the lagoon, and both types of groundwater were detected discharging from one of the larger springs. The relative proportions of low salinity groundwater and brackish high radium groundwater varied over the tidal cycle. In order to better understand the relative contributions of each type of groundwater to the lagoon, a three end-member mixing model based on the distinct chemical and isotopic compositions of both types of groundwater and of seawater was used to estimate the distribution of each water type throughout the lagoon in different seasons. This study suggests that substantial groundwater discharge to the lagoon can occur during both dry and rainy seasons. The presence of two groundwater sources has implications for monitoring and protection of the Celestún Lagoon Biosphere Reserve, since the two sources may have different susceptibilities to anthropogenic contamination depending on their respective recharge area and recharge rates.  相似文献   

19.
Multiple tracers of groundwater input (salinity, Si, 223Ra, 224Ra, and 226Ra) were used together to determine the magnitude, character (meteoric versus seawater), and nutrient contribution associated with submarine groundwater discharge across the leeward shores of the Hawai'ian Islands Maui, Moloka'i, and Hawai'i. Tracer abundances were elevated in the unconfined coastal aquifer and the nearshore zone, decreasing to low levels offshore, indicative of groundwater discharge (near-fresh, brackish, or saline) at all locations. At several sites, we detected evidence of fresh and saline SGD occurring simultaneously. Conservative estimates of SGD fluxes ranged widely, from 0.02–0.65 m3 m− 2 d− 1at the various sites. Groundwater nutrient fluxes of 0.04–40 mmol N m− 2 d− 1 and 0.01–1.6 mmol P m− 2 d− 1 represent a major source of new nutrients to coastal ecosystems along these coasts. Nutrient additions were typically greatest at locations with a substantial meteoric component in groundwater, but the recirculation of seawater through the aquifer may provide a means of transferring terrestrially-derived nutrients to the coastal zone at several sites.  相似文献   

20.
Based on measurements of the 18O isotope composition of 247 samples collected over a 3-year period we have assessed the oxygen isotope composition of water masses in the North Sea. This is the first δ18O data set that covers the entire North Sea basin. The waters lie on a mixing line: δ18O (‰VSMOW) = −9.300 + 0.274(S) with North Atlantic sub-polar mode water (SPMW) and surface waters, and Baltic Sea water representing the saline and freshwater end members respectively. Patterns exhibited in surface and bottom water δ18O distributions are representative of the general circulation of the North Sea. Oxygen-18 enriched waters from the North Atlantic enter the North Sea between Scotland and Norway and to a lesser extent through the English Channel. In contrast, oxygen-18 depleted waters mainly inflow from the Baltic Sea, the rivers Rhine and Elbe, and to a lesser degree, the Norwegian Fjords and other river sources. Locally the δ18O–salinity relationship will be controlled by the isotopic composition of the freshwater inputs. However, the range of local freshwater compositions around the North Sea basin is too narrow to characterise the relative contributions of individual sources to the overall seawater composition. This dataset provides important information for a number of related disciplines including biogeochemical research and oceanographic studies.  相似文献   

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