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1.
The interaction of the Aretic winter aerosol (Arctic haze) with solar radiation produces changes in the radiation field that result in the enhancement of scattering and absorption processes which alter the energy balance and solar energy distribution in the Arctic atmosphere-surface system. During the second Arctic Gas and Aerosols Sampling Project (AGASP II) field experiment, we measured radiation parameters using the NOAA WP-3D research aircraft as a platform. State-of-the-art instrumentation was used to measure in situ the absorption of solar radiation by the Arctic atmosphere during severe haze events. Simultaneously with the absorption measurements, we determined optical depths, and total, direct, and scattered radiation fields. All optical measurements were made at spectral bands centered at 412, 500, 675, and 778 nm and with a bandpass of 10 nm. With this selection of spectral regions we concentrated on the measurement of the radiative effects of the aerosol excluding most of the contributions by the gaseous components of the atmosphere. An additional measurement performed during these experiments was the determination of total solar spectrum fluxes. The experimentally determined parameters were used to define an aerosol model that was employed to deduce the absorption by the aerosols over the full solar spectrum and to calculate atmospheric heating rate profiles. The analyses summarized above allowed us to deduce the magnitude of the change in some important parameters. For example, we found changes in instantaneous heating rate of up to about 0.6 K/day. Besides the increased absorption (30 to 40%) and scattering of radiation by the atmosphere, the haze reduces the surface absorption of solar energy by 6 to 10% and the effective planetary albedo over ice surfaces by 3 to 6%. The vertical distribution of the absorbing aerosol is inferred from the flux measurements. Values for the specific absorption of carbon are found to be around 6 m2/g for externally mixed aerosol and about 11.7 m2/g for internally mixed aerosol. A complete study of the radiative effects of the Arctic haze should include infrared measurements and calculations as well as physics of the ice, snow, and water surfaces.  相似文献   

2.
The paper describes the results of the field experiment on studying solar radiation transmission in the visible wavelength range through model aerosol media formed in the lower troposphere with the help of generators installed aboard helicopters. The refractive index and the average size of the aerosol particles formed are close to those characteristic of the natural stratospheric aerosol. The composition of the equipment complex used to control aerosol optical and microphysical aerosol parameters is considered. The measurement results are in satisfactory agreement with the results of theoretical and experimental studies in simulation chambers.  相似文献   

3.
The results of numerical simulation of downward solar radiation fluxes for background and smoke-contaminated atmospheric conditions are discussed. Vertical profiles of aerosol characteristics are obtained from the empirical model based on the data of aircraft sounding of profiles of angular scattering coefficients and content of absorbing particles in the lower troposphere. The background model was created using the results of measurements obtained under cloudless and mostly cloudless atmospheric conditions in 1999–2011. Optical parameters of smoke aerosol are determined from the data of aircraft measurements in the period of long-term wildfires in Siberia in the summer 2012. It is demonstrated that deficiency in diurnal values of total solar radiation at the surface level caused by the formation of the optically dense smoke layer as compared to background conditions, is more than 13 MJ/m2.  相似文献   

4.
Aircraft observations of solar radiative fluxes (including the downward diffuse component) made in cloud-free conditions in the lowest 8 km of the atmosphere, have been interpreted using simultaneous measurements of aerosol characteristics. Measured flux profiles have been compared with those derived from a two-stream model of radiative transfer which can incorporate both gaseous and aerosol effects. In one of the four cases examined, sufficient aerosol data were available to estimate the radiative properties of the aerosol which could then be included in the model calculations. The findings are shown to be broadly consistent with the observations when a realistic aerosol refractive index is used. The measurement of the downward diffuse radiation enabled the radiative properties of the aerosol to be calculated directly from the flux measurements. In particular, the average single-scattering albedo of aerosol within the boundary layer in continental air masses was estimated to be about 0.7.The implications of having a highly absorbing aerosol present within the boundary layer are also considered. In one case a heating rate of about 5 K day-1 was observed across the aerosol layer, which suggests that on occasions, aerosol heating will be a significant term in the heat budget for the boundary layer.  相似文献   

5.
Abstract

Cloudless‐sky solar fluxes calculated by the radiative transfer algorithm used in the Canadian Climate Centre's general circulation climate model are compared with measurements of upwelling radiation at the top of the atmosphere (TOA) and downwelling radiation at the surface. The 12‐layer model partitions the solar spectrum into two broad wavebands (0.25–0.68 and 0.68–4.00 μm). The comparison utilized TOA fluxes estimated from Nimbus‐ 7 measurements and measured downwelling fluxes at the surface for Kalgoorlie, West Australia, and downwelling fluxes at the surface for Woodbridge, Ontario. Model estimates and measurements agreed to within experimental error for most solar zenith angles. Estimates improved, especially at Woodbridge, when aerosol effects were included. The mean bias error was less than 4% for surface irradiance and less than 6% for upwelling TOA irradiance, which produces a TOA albedo error of about 0.01.  相似文献   

6.
Surface erythemal UV radiation is mainly affected by total column ozone, aerosols, clouds, and solar zenith angle. The effect of ozone on the surface UV radiation has been explored many times in the previous studies due to the decrease of ozone layer. In this study, we calculated the effect of aerosols on the surface UV radiation as well as that of ozone using data acquired from Ozone Monitoring Instrument (OMI). First, ozone, aerosol optical depth (AOD), and surface erythemal UVB radiation measured from satellite are compared with those from ground measurements. The results showed that the comparison for ozone was good with r 2 of 0.92. For aerosol, there was difference between satellite measurements and surface measurements due to the insufficient information on aerosol in the retrieval algorithm. The r 2 for surface erythemal UV radiation was high (～0.94) but satellite measurements showed about 30% larger values than surface measurements on average by not considering the effect of absorbing aerosols in the retrieval process from satellite measurements. Radiative amplification factor (RAF) is used to access the effect of ozone and aerosol quantitatively. RAF for ozone was 0.97～1.49 with solar zenith angle. To evaluate the effect of aerosol on the surface UV radiation, only clear-sky pixel data were used and solar zenith angle and total column amount of ozone were fixed. Also, RAF for aerosol was assessed according to the single scattering albedo (SSA) of aerosols. The results showed that RAF for aerosol with smaller SSA (< 0.90) was larger than that for with larger SSA (> 0.90). The RAF for aerosol was 0.09～0.22 for the given conditions which was relatively small compared to that for ozone. However, considering the fact that aerosol optical depth can change largely in time and space while the total column amount of ozone does not change very much, it needs to include the effect of aerosol to predict the variations of surface UV radiation more correctly.  相似文献   

7.
Data are presented on losses from frosts in the Southern Federal Region of Russia. Problems are considered of optimization for radiation frost protection, based on production of artificial smoke layers and fogs. Studies of infrared radiation attenuation by aerosol of different dispersion and simulation of aerosol turbulent diffusion show that, within the atmospheric transmittance window, a sufficient greenhouse effect can be provided by an artificial aerosol layer, containing not less than 1011m−2 aerosol particles of 1.5–2 μm size. An estimate is presented of economical expediency of the optimized methods for the radiation frost protection.  相似文献   

8.
对气溶胶气候效应开展分类评估并探讨诊断方法的合理性。人为气溶胶辐射效应对计算云辐射强迫的影响为0.38 W·m~(-2)。诊断评估气溶胶对云辐射强迫的影响需要排除这个偏差。两种基于不同试验设计诊断得出的半直接效应分别为0.21和0.09 W·m~(-2),存在显著差异。主要原因可能是人为气溶胶影响云辐射强迫的不同机制之间在模式模拟过程中不断地相互交织,不是简单的线性叠加关系。模式诊断得出的Twomey效应不仅包括Twomey效应本身,还包括Twomey效应引起的部分快速调整。总之,利用模式评估分析人为气溶胶气候效应需要注意审查试验设计和诊断方法的合理性。  相似文献   

9.
邱金桓  杨理权 《大气科学》2002,26(4):449-458
从宽带的太阳直接辐射1天或1小时累计量(曝辐量)气象观测资料反演气溶胶光学厚度的一个有效方法是很有用的.作者把太阳曝辐量与"等效"的瞬时太阳直接辐射关联起来,建立了一个与曝辐量"等效"的瞬时太阳直接辐射的模式;应用该模式和一个"等效"波长模式,发展了一个从太阳直接曝辐量反演气溶胶光学厚度的方法.作者还从试验上比较分析了由某时刻的宽带太阳直接辐射、每小时或1天的太阳直接辐射曝辐量反演得到的气溶胶光学厚度以及由太阳光度计探测的气溶胶光学厚度.试验结果表明,由日太阳直接辐射曝辐量反演得到的气溶胶光学厚度可理解为辐射加权的日平均光学厚度.  相似文献   

10.
西安市一次晴空气溶胶粒子的观测分析   总被引：17，自引：0，他引：17  
何绍钦 《气象》1987,13(5):19-22
1982年夏季,我国第一架装有PMS粒子测量系统的气象科研考察飞机在西安市首次进行大气物理科学考察。本文仅对6月8日西安城市晴天大气气溶胶粒子观测。资料进行了初步分析。结果表明:西安市晴天气溶胶粒子(直径0.5-8μm)浓度值范围在4×10~0-3.8×10~1个/cm~3,分布趋势随高度递减,逆温层对粒子垂直输送有阻滞作用。同时对气溶胶粒子谱分布及谱分布函数作了探讨,并对一些参数进行理论计算。  相似文献   

11.
Due to increased aerosol emissions and unfavorable weather conditions, severe haze events have occurred frequently in China in the last 10 years. In addition, the interaction between the boundary layer and the aerosol radiative effect may be another important factor in haze formation. To better understand the effect of this interaction, the aerosol radiative effect on a severe haze episode that took place in December 2013 was investigated by using two WRF-Chem model simulations with different aerosol configurations. The results showed that the maximal reduction of regional average surface shortwave radiation, latent heat, and sensible heat during this event were 88, 12, and 37 W m–2, respectively. The planetary boundary layer height, daytime temperature, and wind speed dropped by 276 m, 1°C, and 0.33 m s–1, respectively. The ventilation coefficient dropped by 8%–24% for in the central and northwestern Yangtze River Delta (YRD). The upper level of the atmosphere was warmed and the lower level was cooled, which stabilized the stratification. In a word, the dispersion ability of the atmosphere was weakened due to the aerosol radiative feedback. Additional results showed that the PM2.5 concentration in the central and northwestern YRD increased by 6–18 μg m–3, which is less than 15% of the average PM2.5 concentration during the severely polluted period in this area. The vertical profile showed that the PM2.5 and PM10 concentrations increased below 950 hPa, with a maximum increase of 7 and 8 μg m–3, respectively. Concentrations reduced between 950 and 800 hPa, however, with a maximum reduction of 3.5 and 4.5 μg m–3, respectively. Generally, the aerosol radiative effect aggravated the level of pollution, but the effect was limited, and this haze event was mainly caused by the stagnant meteorological conditions. The interaction between the boundary layer and the aerosol radiative effect may have been less important than the large-scale static weather conditions for the formation of this haze episode.  相似文献   

12.
北京不同区域气溶胶辐射效应   总被引：1，自引：0，他引：1       下载免费PDF全文
采用大气辐射传输模式SES2以及2013年1月—2015年10月欧洲中期天气预报中心细网格再分析资料计算了北京地区4个观测站地面接收的短波辐射通量,分析了晴天和云天北京城郊气溶胶对总辐射的定量影响时空变化特征。结果表明:北京城区和近郊区气溶胶对总辐射的影响约为远郊区的2倍,北京南部和西部气溶胶对辐射的影响较大,晴天和云天北京城区和近郊区气溶胶对总辐射的削减值分别为146.23~180.99 W·m-2和202.11~217.02 W·m-2,晴天总辐射削减空间差异较大;秋冬季气溶胶对总辐射的影响明显大于春夏季,北京市观象台秋冬季气溶胶对总辐射的削减作用最大可达60%,较春夏季高10%~20%;北京城郊总辐射和直接辐射削减率与气溶胶光学厚度变化均呈线性关系,近地面PM2.5浓度对辐射的影响不容忽视。  相似文献   

13.
Abstract

Temporal variations of the transmission coefficient and aerosol optical depth of the atmosphere are considered using multi‐year observations at the Soviet polar stations in the Arctic. The contribution of atmospheric aerosol to the total extinction of solar radiation is estimated. A decreasing trend of atmospheric transparency due to the increase of aerosol contributing to the extinction of solar radiation during the last 25–30 years is noted. Estimates of the atmospheric aerosol influence on the incoming solar radiation indicate that a further systematic decrease of the transmission coefficient may lead to climatic changes of direct and total radiation in most polluted areas of the Arctic.  相似文献   

14.
We present a microphysical model for the surface layer marine and coastal atmospheric aerosols that is based on long-term observations of size distributions for 0.01–100 µm particles. The fundamental feature of the model is a parameterization of amplitudes and widths for aerosol modes of the aerosol size distribution function (ASDF) as functions of fetch and wind speed. The shape of ASDF and its dependence on meteorological parameters, height above sea level (H), fetch (X), wind speed (U) and relative humidity (RH), are investigated. At present, the model covers the ranges H = 0–25 m, U?=?3–18 km s?1, X?≤?120 km and RH?=?40–98%.

The latest version of the Marine Aerosol Extinction Profiles model (MaexPro) is described and applied to the computation and analysis of the spectral profiles of aerosol extinction coefficients α(λ) in the wavelength band λ?=?0.2–12 µm. MaexPro is based on the aforementioned aerosol model assuming spherically shaped aerosol particles and the well-known Mie theory.

The spectral profiles of α(λ) calculated by MaexPro are in good agreement with observational data and the numerical results obtained from the Navy Aerosol Model (NAM) and the Advanced Navy Aerosol Model (ANAM). Moreover, MaexPro was found to be an accurate and reliable tool for investigating the optical properties of atmospheric aerosols.  相似文献   

15.
The major finding of this study is that aerosols over the tropical Indian Ocean enhance clear sky atmospheric solar heating significantly and decrease the surface solar heating by even a larger amount. The results presented here are based on aerosol chemical, microphysical, and optical and radiometric data collected at the island of Kaashidhoo (4.97°N, 73.47°E) during February and March of 1998, as part of the first field phase of the Indian Ocean experiment (INDOEX). The aerosol optical properties were integrated with a multiple scattering Monte Carlo radiative transfer model which was validated at the surface with broadband flux measurements and at the top of the atmosphere (TOA) with the clouds and earth's radiant energy system (CERES) radiation budget measurements. We consider both externally and internally mixed aerosol models with very little difference between the two models in the estimated forcing. For the February–March period, the aerosols increase the monthly mean clear sky atmospheric solar heating by about 12 W/m2(about 15% of the total atmospheric solar heating) and decrease the sea surface clear sky solar heating by about 16 W/m2 with a daily range from 5 to 23 W/m2. The net aerosol forcing at the top of the atmosphere is about −4 W/m2 with a daily range from −2 to −6 W/m2. Although the soot contributes only about 10% to the aerosol optical thickness, it contributes more than 50% to the aerosol induced atmospheric solar heating. The fundamental conclusion of this study is that anthropogenic aerosols over the tropical Indian Ocean are altering the clear sky radiation budget of the atmosphere and surface in a major manner.  相似文献   

16.
Influences of the mixing treatments of anthropogenic aerosols on their effective radiative forcing (ERF) and global aridity are evaluated by using the BCC_AGCM2.0_CUACE/Aero, an aerosol–climate online coupled model. Simulations show that the negative ERF due to external mixing (EM, a scheme in which all aerosol particles are treated as independent spheres formed by single substance) aerosols is largely reduced by the partial internal mixing (PIM, a scheme in which some of the aerosol particles are formed by one absorptive and one scattering substance) method. Compared to EM, PIM aerosols have much stronger absorptive ability and generally weaker hygroscopicity, which would lead to changes in radiative forcing, hence to climate. For the global mean values, the ERFs due to anthropogenic aerosols since the pre-industrial are–1.02 and–1.68 W m–2 for PIM and EM schemes, respectively. The variables related to aridity such as global mean temperature, net radiation flux at the surface, and the potential evaporation capacity are all decreased by 2.18/1.61 K, 5.06/3.90 W m–2, and 0.21/0.14 mm day–1 since 1850 for EM and PIM schemes, respectively. According to the changes in aridity index, the anthropogenic aerosols have caused general humidification over central Asia, South America, Africa, and Australia, but great aridification over eastern China and the Tibetan Plateau since the pre-industrial in both mixing schemes. However, the aridification is considerably alleviated in China, but intensified in the Arabian Peninsula and East Africa in the PIM scheme.  相似文献   

17.
For the measurement of atmospheric NO2 vertical column density (VCD), Kitt Peak Solar Flux Atlas can be substituted as an extraterrestrial solar radiation. Compared with differential analysis method, the Taylor expansion of integrated transfer equation underestimates the VCD. This underestimation is as large as 35% when the amount of NO2 is 1 × 1017 cm－2 and observation is conducted with an air mass factor of 10. Even when the VCD is 2 × 1016 cm－2 and the air mass factor is 4, the relative error of the retrieved VCD is still no less than 3%. If the observation is restricted under the small air mass factor condition (≤4), with Kitt Peak Solar spectrum as an extraterrestrial solar radiation, only an atmospheric layer of 2 km thick from ground can be studied, which will make the absorption too weak to be detected by normal instruments.The VCD in winter Tokyo area was observed and analyzed by differential method, which shows a good precision even when the absorption is as low as 3%. The largest average VCD was about 1.3 × 1017 cm－2, and the lowest was about 1.3 × 1016 cm－2. The trend of its variation was almost the same as the ground level observation by Saltzman reagent method.  相似文献   

18.

Measurement of solar radiation was initiated in Girona, northeast of the Iberian Peninsula, in the late 1980s. Initially, two pyranometers were installed, one of them equipped with a shadowband for measuring the diffuse component. Two other pyranometers currently exist, both ventilated and one of them shadowed, with a sphere, and a pyrheliometer for measuring direct radiation. Additional instruments for other shortwave and longwave components, clouds, and atmospheric aerosols have been installed in recent years. The station is subject to daily inspection, data are saved at high temporal resolution, and instruments are periodically calibrated, all in accordance with the directions of the Baseline Surface Radiation Network. The present paper describes how the entire series of global solar radiation (1987–2014) and diffuse radiation (1994–2014) were built, including the quality control process. Appropriate corrections to the diffuse component were made when a shadowband was employed to make measurements. Analysis of the series reveals that annual mean global irradiance presents a statistically significant increase of 2.5 W m−2 (1.4 %) decade−1 (1988–2014 period), mainly due to what occurs in summer (5.6 W m−2 decade−1). These results constitute the first assessment of solar radiation trends for the northeastern region of the Iberian Peninsula and are consistent with trends observed in the regional surroundings and also by satellite platforms, in agreement with the global brightening phenomenon. Diffuse radiation has decreased at −1.3 W m−2 (−2 %) decade−1 (1994–2014 period), which is a further indication of the reduced cloudiness and/or aerosol load causing the changes.

  相似文献   

19.
Aerosol size spectra (d=10 nm–10 μm) were measured with an electrical aerosol spectrometer (EAS) at Mace Head on the west coast of Ireland. Several small aerosol particle (diameter 10–32 nm) concentration bursts were observed during the measurement period. Relationships between the events, air mass trajectories, tide height, and meteorological parameters are examined. Series of bursts were observed when a spectral transformation due to subsequent particle growth from 10 to 56–100 nm can be identified in an Eulerian experiment. Particle growth rates of between 1 and 3 nm/h were determined. These bursts appear in cold and comparatively clean arctic or polar air masses with temperature and relative humidity fluctuations, and do not correlate with low tide in some cases. These episodes, similar to those frequently found in the continental boundary layer, are thought to occur over a wide area and, for clear detection, require stable airflow for a few days. Elevated small-particle concentration events are more common during low tide or shortly after, and are typically associated with low wind speeds. Here, the increased shore exposure during low tide is thought to influence the nucleation and the subsequent growth of these aerosol particles. The occurrences of the bursts are found to depend on local wind direction. The highest d=10–32 nm particle concentrations appeared for wind sectors furthest from the tidal regions when the wind direction was 150–160°(south-easterly). Most of the events occurred during daytime when solar irradiation is most intense.  相似文献   

20.
Ground-based aerosol instrumentation covering particle size diameters from 25 nm to 32 µm was deployed to determine aerosol concentration and cloud condensation nuclei (CCN)-activation properties at water vapor supersaturations in the range of S = 0.20–1.50 % in the remote Brazilian northeast semi-arid region (NEB) in coastal (maritime) and continental (inland) regimes. The instruments measured aerosol number concentration and activation spectra for CCN and revealed that aerosol properties are sensitive with respect to the sources as a function of the local wind circulation system. The observations show that coastal aerosol total number concentrations are above 3,000 cm?3 on average, exhibiting concentration peaks depending on the time of the day in a consistent daily pattern. The variation on aerosol concentration has also influences on the fraction of particles active as CCN. At 1.0 % water vapor supersaturation, the fraction can reach as high as 80 %. Inland aerosol total concentrations were about 1,800–1,900 cm?3 and did not show much diurnal variation. The fraction of particles active as CCN observed inland depend on the history of the air masses, and was much higher when air masses were originated over the sea. It was found that (NH4)2SO4 and NaCl are the major soluble inorganic fraction of the aerosols at the coast. The major fraction of NaCl was present in the coarse mode, while ammonium sulfate dominates the inorganic fraction at the submicron range, with about 10 % of the total aerosol mass at 0.32 µm. Inorganic compounds are almost absent in particles with sizes around 0.1 μm. The study suggests that the air masses with high concentration of CCN originate at the sea. The feasible explanation lies in the fact that the NEB’s beaches have a particular morphology that produces a wide surf zone and creates a large load of aerosols when combined with strong and permanent winds of the region.  相似文献   

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