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1.
Excess 210Pb was determined in six abyssal cores from the Eastern Atlantic, Hatteras Abyssal Plain, and Puerto Rico Trench. A bioturbation rate for each core was evaluated using the mixing model of Guinasso and Schink. The rates were compared to mixing rates evaluated for the same cores using 239,240Pu. In all cases, the excess 210Pb-derived mixing rates were lower than the plutonium-derived mixing rates. 239,240Pu was also present at greater depths than excess 210Pb. One possible explanation for these observations is the association of plutonium with particles of greater food value which are bioturbated at faster rates.  相似文献   

2.
Radionuclide measurements have been conducted on sediment cores collected in 1992 in the south-eastern region of the Barents Sea, known as the Pechora Sea. Cesium-137 and 239,24OPu activities in surface sediments are generally less than 30 Bq/kg, with the highest levels being measured in sediments off the southwestern coastline of the island of Novaya Zemlya. High correlations between both 137Cs and 239,24OPu and the concentration of fine (< 63 μm) particles in surface sediments indicate that much of the variance in radionuclide concentrations throughout the Pechora Sea can be explained by particle size fractionation. However, elevated activities of 137Cs (138 Bq/kg), 60Co (92 Bq/kg), 241Am (433 Bq/kg), and especially 239,24OPu (8.47 × 103 Bq/kg) were measured in one surface sediment sample from the fjord of Chernaya Bay on the southern coast of Novaya Zemlya. The source of radioactive contamination is two underwater nuclear tests conducted in Chernaya Bay in 1955 and 1957.The 238Pu/239,240Vu activity ratio of 0.0245 in Chernaya Bay is equivalent to values measured in global fallout. The 240Pu/239Pu atom ratio (0.0304), measured by mass spectrometry, is much lower than values (0.18) typical of global fallout, but is consistent with ratios measured for fallout from the early (1951–1955) series of weapons tests at the Nevada Test Site. The timing of the Chernaya Bay source term, estimated from the 241Am/241Pu ratio, is consistent with the timing of the 1955 and 1957 underwater nuclear tests. Relatively low initial yields of 241Pu (241Pu/239Pu atom RATIO = 0.00 123) in these tests have resulted in relatively low 241Am/239,240Pu activity ratios (0.05) in recent sediments in Chernaya Bay.Radionuclide tracer profiles in cores from the Pechora Sea can be simulated using a two-layer biodiffusion model with rapid, near-homogeneous mixing in the surface mixed layer and reduced mixing in the deep layer. Lead-210 profiles are consistent with a wide range of sedimentation and mixing rates in the deep sediment layer. However, the 137Cs and 239,240Pu results further constrain the model parameters and indicate that the downward transport of radionuclides in the sediments is governed primarily by sediment mixing, with sediment burial playing a secondary role.  相似文献   

3.
Biologically dominated lower Chesapeake Bay and the physically dominated York River subestuary are contrasted in terms of the dynamics of sediment mixing, strata formation and sea-bed particle residence times. Two lower bay sites were examined; both are located within the bay stem plains and are characterized by muddy sand and an abundance of large, deep-dwelling organisms. X-radiographs indicate extensive biological reworking of sediments, with no long-term preservation of physical stratification.210Pb profiles reveal low sediment accumulation rates at both lower bay sites (<0·1 cm year−1), but significant differences in biological mixing depths (25vs40 cm) and biodiffusivity (>80vs6–30 cm2year−1). In contrast, the York River site, located within a partially-filled palaeochannel, is predominantly mud with a depauperate benthic community dominated by small, short-lived, shallow-dwelling organisms. Although210Pb accumulation rates at the York River site (<0·2 cm year−1) are similar to those measured in the lower bay, there is little bioturbation. In addition, transient bed forms at the York River site form laterally persistent, linear ridges and furrows sub-parallel to the channel, spaced 10–20 m apart. These observations, coupled with evidence of episodic erosion and deposition from radioisotope and porosity profiles, and X-radiographs, suggest that the upper 60–120 cm of the sea-bed are dominated by physical mixing. Deep mixing and low accumulation rates result in long residence times of particles in the mixed upper portion of the sea-bed (102year) at both locations, despite different mixing controls [i.e. biological (diffusive)vsphysical (advective)].  相似文献   

4.
We estimated monthly fluxes of 210Pb in shelf sediments beneath a high productivity area off central-southern Chile (36°S) during 1 year (September 2002-August 2003). Sediment cores were obtained using a multiple corer and were analyzed mainly for 210Pb, total pigments, and macrofauna abundance. The 210Pb inventories and fluxes were estimated for surface sediments (0-5 cm) and bioturbation coefficients were inferred using chlorophyll-a (reactive) profiles. In general, 210Pb content was inversely correlated with phytodetritus fluxes. High photosynthetic pigment contents in surface sediments were consistently associated with lower 210Pb contents. Macrofaunal activity responded to oxygen and organic matter supplies at the sediment surface, generally concentrated in the first centimeters, but particularly so during months of high organic matter fluxes and deficient bottom water oxygen conditions. At this study site, several processes involved in the 210Pb surface distribution make it difficult to accurately estimate ages at the surface. We postulate that the organic fluxes promote changes in the faunal activity, which, in combination with sediment resuspension and water circulation over the shelf, produce seasonal variations in the 210Pb inventories.  相似文献   

5.
Box cores were collected close to river mouths along the eastern Brazilian shelf at water depths of 10–30 m. One core was taken from more than 1000 m depth at the shelf slope. 210Pb and 226Ra activities were measured to establish sediment accumulation rates. Seven of the 10 cores exhibited an exponential decrease with depth of excess 210Pb activities. The sediments from the sheltered Sudeste Channel off Caravelas revealed the highest sediment accumulation rate of 0.81 cm yr−1. The sediments at the shelf slope seaward of the Rio Doce revealed the lowest accumulation rate of 0.13 cm yr−1. Sediment accumulation rates increased towards the Caravelas Bank. Current patterns and the morphology of the seabed favor sediment deposition in this area.  相似文献   

6.
Arctic sea ice can incorporate sediment and associated chemical species during its formation in shallow shelf environments and can also intercept atmospherically transported material during transit. Release of this material in ice ablation areas (e.g. the Fram Strait) enhances fluxes of both sediments and associated species in such areas. We have used a suite of natural (7Be, 210Pb) and anthropogenic (137Cs, 239Pu, 240Pu) radionuclides in sea ice, sea-ice sediments (SIS), sediment trap material and bottom sediments from the Fram Strait to estimate transit times of sea ice from source to ablation areas, calculate radionuclide fluxes to the Fram Strait and investigate the role of sea-ice entrained sediments in sedimentation processes. Sea ice intercepts and transports the atmospherically supplied radionuclides 7Be and 210Pb, which are carried in the ice and are scavenged by any entrained SIS. All of the 7Be and most of the excess 210Pb measured in SIS collected in the Fram Strait are added to the ice during transit through the Arctic Ocean, and we use these radionuclides as chronometers to calculate ice transit times for individual ice floes. Transit times estimated from the 210Pb inventories in two ice cores are 1–3 years. Values estimated from the 7Be/210Pbexcess activity ratio of SIS are about 3–5 years. Finally, equilibrium values of the activity ratio of 210Pb to its granddaughter 210Po in the ice cores indicate transit times of at least 2 years. These transit times are consistent with back-trajectory analyses of the ice floes. The latter, as well as the clay-mineral assemblage of the SIS (low smectite and high illite content), suggest that the sampled sea-ice floes originated from the eastern Siberian Arctic shelf seas such as the eastern Laptev Sea and the East Siberian Sea. This result is in agreement with the relatively low activities of 239,240Pu and 137Cs and the 240Pu/239Pu atom ratios (∼0.18, equivalent to that in global fallout) in SIS, indicating that prior global atmospheric fallout, rather than nuclear fuel reprocessing facilities, forms the main source of these anthropogenic radionuclides reaching the western Fram Strait at the time of sampling (1999). Transport of radionuclides by sea ice through the Arctic Ocean, either associated with entrained SIS or dissolved in the ice, accounts for a significant flux in ablation areas such as the Fram Strait, up to several times larger than the current atmospheric flux in the area. Calculated fluxes derived from sea-ice melting compare well to fluxes obtained from sediment traps deployed in the Fram Strait and are consistent with inventories in bottom sediments. 240Pu/239Pu atomic ratios lower than 0.18 in bottom sediments from the Fram Strait provide evidence that plutonium from a source other than atmospheric fallout has reached the area. Most likely sources of this Pu include tropospheric fallout from atomic weapons testing of the former Soviet Union prior to 1963 and Pu released from nuclear reprocessing facilities, intercepted and transported by sea ice to the ablation areas. Future work is envisaged to more thoroughly understand the actual mechanisms by which radionuclides are incorporated in sea ice, focusing on the quantification of the efficiency of scavenging by SIS and the effect of melting and refreezing processes over the course of several years during transit.  相似文献   

7.
《Marine Chemistry》2001,73(2):125-152
We report here bioturbation and sediment accumulation rates determined from replicate sediment cores at four different sampling sites on the Palos Verdes shelf, Southern California, using bomb fallout and natural radionuclides (137Cs, 239,240Pu, 210Pb, 234Th, and 14C), along with supporting measurements of organic carbon (OC), porosity and granulometry. Present-day particle reworking, on time scales of several months, is restricted to the upper 3 cm, with rates ranging from 13 to 200 cm2/year, as deduced from 234Thxs profiles. There is little evidence that particle reworking reached depths significantly greater than 5 cm. Post-1963 (or post-1971) sediment accumulation rates ranged from 0.7 to 1.4 g/cm2/year (equivalent to 1.1–1.8 cm/year for surficial sediments), as calculated from Pu and Cs isotope profiles, with little change over time or distance from the outfall. Lateral transport of older sediment and multiple sediment sources on the Palos Verdes shelf is suggested from radiocarbon measurements on foraminifera and bulk sedimentary organic matter at two sampling sites, which showed variable, old and refractory sources of OC. Pre-1953 sediments accumulated at rates that were at least 0.4 g/cm2/year (≥0.3 cm/year), based on 210Pbxs dating. Given the abundance of sediment sources to the Palos Verdes shelf, the high sedimentation rates, and shallow particle mixed layers, contaminant-enriched layers should continue to move deeper into the sediments.  相似文献   

8.
Abstract. Two sediment cores were collected in the southern Baltic Sea and sliced into 1.0cm-thick layers. Sediments of each layer were analysed for activities of 210Pb, 137Cs, 134Cs and for the density of meiobenthic organisms (meiofauna). Zones with the rapid mixing occur in the uppermost layers (0–3 cm) of the cores based on I34Cs profiles. The extent and density of meiofauna confirmed the rapid mixing and revealed layers with slow mixing (4–8 cm). Sedimentation rates were derived from 210Pb profiles below the mixing zones (1.21 and 1.72 mm a-I) and were confumed by 137Cs distribution. Of twenty-one major meiofauna taxa commonly found in the Baltic sediments, three were present in the cores.  相似文献   

9.
The distribution and inventory of artificial radionuclides,239,240Pu and137Cs were determined in the East China and the Yellow Seas in 1987. Almost all of239,240Pu and 50 to 80% of137Cs in the continental shelf area are retained in the sediment column.239,240Pu sediment inventory in the sea area is larger than the fallout input and tends to increase southwardly. This excess239,240Pu and the lateral distribution are attributable to the supply of239,240Pu by the Yangtze River discharge. On the contrary,137Cs sediment inventory shows a decrease to the south, and the fact can be accounted for by the southward dispersion of fine silt particles discharged from the Yellow River. Total137Cs inventory is smaller than the estimated fallout input, and the fact seems to indicate dispersion of137Cs out of the shelf region. Vertical profiles of239,240Pu and137Cs contents in sediments differ from that of natural210Pb, implying the effect of varied accumulation rates of the artificial radionuclides over the sediment particle mixing by benthic organisms. Apparent maximum sediment particle mixing coefficient (D B ) calculated from the excess210Pb profiles in stations located between the inner and outer shelves ranged from 1.4 to 8.3 cm2y–1. ThisD B value is higher than that in the Okinawa Trough (1.0 cm2y–1), but lower than previously estimatedD B value (26 cm2y–1) in the outer shelf mud.  相似文献   

10.
Radionuclide activities of 210Pb and 226Ra were measured to determine bioturbation coefficients (Db) in seven sediment cores from the Korean licensed block for polymetallic nodules in the Clarion–Clipperton Fracture Zone. Variability in Db is considered in the context of the sedimentological, geochemical, and geotechnical properties of the sediments. Db values in the studied cores were estimated using a steady-state diffusion model and varied over a wide range from 1.1 to 293 cm2/yr with corresponding mixing depths (L) of 26 to 144 cm. When excepting for spurious results obtained from cores where diffusive mixing does not apply, Db values range from 1.1 to 9.0 cm2/yr with corresponding mixing depths (L) of 26 to 63 cm. Such wide variability in Db and L values is exceptional in sites with water depths of ～5000 m and is attributed in this study to an uneven distribution of sediment layers with different shear strengths and total organic carbon (TOC) contents, caused by erosion events. The studied cores can be grouped into two categories based on lithologic associations: layers with high maximum shear strength (MSS) and low TOC content, showing a narrow range of Db values (1.1–9.0 cm2/yr); and layers with low MSS and high TOC content, yielding much higher Db values of over 30 cm2/yr. The distribution of different lithologies, and the resultant spatial variability in MSS and labile organic matter content, controls the presence and maximum burrowing depth of infauna by affecting their mobility and the availability of food. This study provides a unique case showing that shear strength, which relates to the degree of sediment consolidation, might be an important factor in controlling rates of bioturbation and sediment mixing depths.  相似文献   

11.
Sedimentary records of naturally occurring and fallout-derived radionuclides are widely used as tools for estimating both the ages of recent sediments and rates of sedimentation and bioturbation. Developing these records to the point of data interpretation requires careful sample collection, processing, analysis and data modeling. In this work, we document a number of potential pitfalls that can impact sediment core records and their interpretation. This paper is not intended as an exhaustive treatment of these potential problems. Rather, the emphasis is on potential problems that are not well documented in the literature, as follows: (1) the mere sampling of sediment cores at a resolution that is too coarse can result in an apparent diffusive mixing of the sedimentary record at rates comparable to diffusive bioturbation rates observed in many locations; (2) 210Pb profiles in slowly accumulating sediments can easily be misinterpreted to be driven by sedimentation, when in fact bioturbation is the dominant control. Multiple isotopes of different half lives and/or origin may help to distinguish between these two possible interpretations; (3) apparent mixing can occur due simply to numerical artifacts inherent in the finite difference approximations of the advection diffusion equation used to model sedimentation and bioturbation. Model users need to be aware of this potential problem. Solutions to each of these potential pitfalls are offered to ensure the best possible sediment age estimates and/or sedimentation and bioturbation rates can be obtained.  相似文献   

12.
 Recent sediment accumulation rates are 18–230 mg cm-2 yr-1 (0.02–0.2 cm yr-1) based on excess 210Pb activity profiles in the southwestern part of the East Sea (Sea of Japan). Assuming no mixing beneath surface mixed layers, 210Pb-derived sediment accumulation rates are 18–32 mg cm-2 yr-1 in the northern part of the Yamato Ridge and the Ulleung Basin, 29–136 mg cm-2 yr-1 in the Korea Plateau, and 230 mg cm-2 yr-1 in the southern shelf. These values generally agree with long-term sedimentation rates estimated from dated ash layers. Received: 6 October 1995 / Revision received: 31 May 1996  相似文献   

13.
《Marine Geology》2005,216(3):155-167
A total of 83 cores were collected in the Gulf of Lions continental margins and analysed for 210Pbxs (excess 210Pb) in order to understand sedimentation patterns. Apparent sedimentation rates (ASR) range from 0.65 cm year−1 in the vicinity of the Rhône River mouth to 0.01 cm year−1 in the deep basin. Except for the prodelta area, rates decrease with depth linearly with the water depth. On the slope, ASR do not differ between canyons and open slope, except for the western area where the rates are slightly higher in the Lacaze–Duthiers canyon compared to its adjacent, open slope. In the canyon and open slope areas, mass accumulation rates determined from 210Pbxs profiles (0.10 and 0.08 g cm−2 year−1, respectively) are in good agreement with particulate fluxes calculated from 5 years of near-bottom sediment trap data, even when the trap particle fluxes and the apparent accumulation rates are overestimated in response to resuspension and bioturbation effects.However, differences in sediment trap data, between west and east portion of the slope, are not observed in the sedimentation rates calculated with 210Pbxs. The outer shelf area may have an important role in trapping sediment but it is not sufficiently documented. Sediment surface mixed layer depths decrease with water depth, with a mean value for the whole margin of 8±6 cm.210Pbxs inventories in the sediment are systematically higher than the net 210Pb export flux estimated from the above water column. Over the margin, the ratio between accumulated 210Pb and available 210Pb is about 3, suggesting boundary scavenging effects and advective transport.  相似文献   

14.
黄亚楠 《海洋学报》2022,44(11):77-87
本文对东海及毗邻海域中239+240Pu比活度、240Pu/239Pu原子比值和239+240Pu累积通量或沉积通量数据进行整理,首次从大气沉降、海水中、生物体中、沉积物捕获器中以及沉积物中的239+240Pu 5个方面阐述了东海及毗邻海域中239+240Pu的地球化学行为。研究结果表明,全球大气沉降和太平洋核试验场输入的239+240Pu是东海海水和沉积物中239+240Pu的两个主要来源;在长江径流、浙闽沿岸流、台湾暖流、黑潮与上升流等水团的混合作用以及清除作用的影响下,东海近岸海水中239+240Pu浓度在时间上呈现被清除而减少的趋势,相应近岸浅水区沉积物中239+240Pu的埋藏深度高于远岸深水海域。在黑潮入侵和上升流的作用下,冲绳海槽区尤其是台湾岛东北部,沉积物中的239+240Pu比活度与沉积通量显著增大。同时,利用东海表层沉积物中239+240Pu比活度和240Pu/239Pu原子比值的相关关系证实了台湾东北部黑潮底层分支流的存在,并指示出台湾暖流与黑潮底层分支流可能交汇的海域位置。  相似文献   

15.
In the Hiuchi-Nada area of the Seto Inland Sea, Japan, sedimentation rates were determined with the Pb-210 technique, and heavy metals in sediments were also analyzed. Sediments were collected in twelve short sediment cores and a long sediment core, using 1-m and 6-m gravity corers.The sedimentation rates vary from 0.14 to 0.31 g cm–2yr–1. The highest sedimentation rate was observed in the central part of the area, while lower sedimentation rates were observed in the eastern part.In Hiuchi-Nada, a remarkable increase in copper and zinc contents is noticeable as early as the 1800's. Over the past 240 years a copper smelter at the south-western side of this area has been causing serious pollution of the sediment. Now, anthropogenic copper and zinc loads into the sediment are 123 and 376 ton yr–1 compared to natural copper and zinc loads of 82 and 401 ton yr–1, respectively. The highest level of copper and zinc pollution was observed in the 1960's, when the relative enrichments above background values (copper; 19 and zinc; 93 mg kg–1) were 5.5 and 2.8, respectively.  相似文献   

16.
Results of the radiochemical determination of 239+240Pu and 238Pu in seawater, plankton, marine organisms and sediment are reported. The samples were collected in the Taranto Gulf, and the data are compared with those obtained from other stations in the Mediterranean Sea. The vertical distribution of plutonium isotopes in sediments is also presented and discussed.  相似文献   

17.
Profiles of the radioisotopes 210Pb and 137Cs were determined in 15 sediment cores collected from Sagami Bay, Japan. The activities of 210Pbex (unsupported) in core top sediments increased with water depth from 25 dpm g−1 on the upper continental slope off the mouth of Tokyo Bay to an average of 283 dpm g−1 at the deep-sea station SB. The high 210Pb trapping efficiency of settling particles expected from the results of the sediment trap experiment near the SB site suggests that effective 210Pb enrichment in surface sediments may occur during resuspension and lateral transportation of particles via the benthic nepheloid layer on the continental slope. In several cores, 137Cs profiles showed an increase, a distinct peak, and then a decrease to an undetectable level downcore. These profiles can be compared with the temporal change of bomb-produced 137Cs fallout.The mean sedimentation rates estimated by the 210Pbex inventory method, rather than using 210Pbex profiles, ranged from 0.06 g cm−2 y−1 to 0.14 g cm−2 y−1. The average value of the rates in SB cores was calculated to be 0.11 g cm−2 y−1, which was similar to that calculated under the assumption that the age of the 137Cs peak corresponds to its maximum fallout year in 1963.Although 137Cs inventories represented one tenth of the anthropogenic fallout of 137Cs until 1997, they correlated with the increase in 210Pbex inventory. This suggests that the scavenging of refractory 137Cs as well as 210Pb by settling particles in the water column can lead to the formation of a time marker layer even in deep-sea sediment core, such as at the SB site.  相似文献   

18.
Seabed distributions of 234Th excess (Thxs) were determined in the upper centimetres of 38 sediment cores from the north-western Iberian Margin, sampled from 41–44°N and from 9–12°E during five OMEX II cruises. Three main areas, a northern, and at 42°38 and 42°N, were investigated during representative seasons (winter, spring and summer). Low 234Thxs activities in summer 1998 (18–252 Bq per kg) were similar to those measured in summer 1997. In winter 234Th also showed moderate excess. The highest values were observed in spring with surface 234Thxs values up to 402 Bq kg−1. Maximum penetration depths of 234Thxs ranged from a few mm to 3 cm. 234Thxs activities always showed a smooth decrease with depth, without any evidence of non-local mixing. Thus particle mixing on a short time scale can be described as an eddy diffusive process, and bioturbation rates, calculated on this basis, range from 0.02 to 3.07 cm2 per year. Data (activities, inventories, bioturbation rates) are discussed in order to relate the observed surface and down-core variations to spatial and seasonal trends. Using 234Thxs data in sediment as a substitute for sediment trap estimates, particle fluxes were calculated from 234Thxs inventories. The range of 234Th-derived particle fluxes for the north-western Iberian Margin is 16–1418 mg.m−2.d−1. Mean values indicate a gradual decrease of mass fluxes from the shelf to the open ocean. On a 100-day scale, the northern area (43–44°N) represents a low sedimentation regime. Further south, around 42°–43°N, particle inputs are more important. On the middle slope, around 1000 to 2000 m depth, high inventories and bioturbation rates indicate enhanced, and probably organic-rich, particle fluxes to the seafloor, particularly in spring.  相似文献   

19.
Laboratory experiments were carried out to assess the role of photochemical reactions upon the dissolution of 239 + 240pu and 241Am from marine sediment in sea water. Supplementary information was obtained by comparing their behaviour with that of 54Mn under similar experimental conditions. Irradiation from natural sunlight resulted in more than a ten-fold increase in the extent of 239 + 240Pu desorption relative to that observed in the dark. Remobilisation of 54Mn from sediment was also enhanced by natural sunlight, albeit to a lesser extent than 239 + 240Pu, whilst the behaviour of 241Am was largely unaffected. Data for concentrations of dissolved 239 + 240Pu(IV) and 239 + 240Pu(V) species showed that only the oxidised form was significantly affected by irradiation, indicating remobilisation occurs as a result of photooxidation reactions. Further experiments were carried out using artificial light sources to establish the influence of wavelength. Data from these investigations indicated 239 + 240Pu photooxidation (hence desorption) was a function of both light intensity and wavelength. Remobilisation decreased concomitant with light intensity but increased as the wavelength decreased. Similar trends were observed for photoreduction of 54Mn, although differences were less pronounced than those observed for 239 + 240Pu.  相似文献   

20.
《Marine Geology》2005,216(4):249-263
Bottom sediments collected in the Northwest (NW) Pacific Ocean in 1997 were analysed for 90Sr, 137Cs, 239,240Pu and 241Am contents to determine their distribution patterns, inventories and sources. Enhanced inventories of 239,240Pu and 241Am were observed in the latitudinal belts of 10–20°N and 30–40°N, which correspond to major areas of local (tropospheric) and global (stratospheric) fallout (with a contribution from local fallout), respectively. The sediment inventory of 239,240Pu near the Bikini Atoll exceeded its overlying water inventory, however, in the mid-latitudes, more than 70% of 239,240Pu still remains in the water column. 241Am inventories in sediments exceeded that of the water column for the entire NW Pacific Ocean. Higher 137Cs and 90Sr sediment inventories in the latitudinal belt of 30–40°N are due to global fallout, and they account for about 10% and less than 5% of the water column inventories, respectively. The observed activity ratios of 137Cs/90Sr, 238Pu/239,240Pu and 241Am/239,240Pu in sediment were at some stations higher than the global fallout ratios due to contributions from local fallout and due to specific processes in the water column. Two end-member mixing model based on the 240Pu/239Pu atom ratios observed in global and local fallout yielded ∼60% contribution of the local fallout in the bottom sediments near the Bikini Atoll. The upward decrease in the 240Pu/239Pu atom ratios in the sediment column indicates a decrease in the contribution of local fallout to the Pu inventory with time. 241Am and 241Pu dating of sediment layers was utilized to explain a hiatus in sediment accumulation in the deep seafloor.  相似文献   

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