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副热带急流对中国南部地区对流层中上层臭氧浓度的影响程度及地理范围目前还研究较少,且缺乏综合使用常规气象资料及卫星资料来判识对流层中上层臭氧浓度增高的方法.本文利用NCEP再分析与最终分析资料、日本GMS-5地球静止卫星水汽云图资料,以2001年3月27~29日中国南部的临安、昆明、香港臭氧探测个例为基础,结合1996年3月29日香港与2001年4月13日临安对流层中上层高浓度臭氧分布个例对副热带急流对中国南部对流层中上层臭氧浓度的影响进行了详细分析,提出根据气象要素场判识春季中国南部对流层中上层臭氧浓度增高的充分条件为根据卫星水汽图像上的暗区、高空急流入口区的左侧辐合区、高空锋区、对流层中上层≥1 PVU的向下伸展的舌状高位涡区来综合判断.本文的分析结果表明,本文个例中对流层中上层高浓度臭氧来自平流层;香港对流层中上层低浓度臭氧来自热带海洋地区.不仅臭氧垂直廓线的多个极小与极大值表明臭氧垂直分布的多尺度变化特征,而且对流层中上层PV分布以及卫星水汽图像分析也表明大气中的多尺度运动对臭氧垂直分布特征有显著影响.本文的结果表明与副热带高空急流相联系的平流层空气侵入不仅发生在中国大陆的较高纬度地区,较低纬度的昆明与香港地区也有平流层空气侵入导致对流层中上层臭氧浓度升高. 相似文献
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东亚一次典型切断低压引起的平流层空气深入侵过程的分析 总被引：2，自引：0，他引：2
利用ERA-Interim再分析资料、卫星资料以及轨迹模式,对2010年6月19-23日东亚夏季一次典型切断低压（COL）过程中的动力、热力及化学结构进行了分析,并详细分析了平流层空气深入侵过程和路径.AIRS臭氧资料与臭氧探空资料分析表明,在COL发展成熟阶段,由极区高位势涡度、高臭氧库区脱离出来的空气在COL的中心形成一个局地高位势涡度与高臭氧浓度区域,并在对流层中上部出现臭氧次峰结构.前向轨迹模式模拟结果表明：COL形成前期,高空槽加深,槽后偏北风急流可以引起极区下平流层空气向中纬度对流层中低层侵入,从而使对流层中低层臭氧浓度升高;COL发展成熟阶段,可以引起平流层空气的＂旋转式＂入侵.最后,应用后向轨迹模式对成熟阶段COL内部及周围空气块源地做进一步模拟分析.结果表明：（1）COL中心高浓度臭氧空气块源地有两个,一是中西伯利亚北部上空的副极地涡旋,这部分气块对COL中心的高臭氧浓度起主要作用;二是90°E以西,50°N附近的温带急流轴左侧的气旋式风速切变区.（2）COL周围低臭氧浓度的气块源地也有两个,一是COL底部臭氧浓度相对较低的空气块主要来自急流轴右侧反气旋式风速切变区,以平流运动为主;二是COL前部及后部的空气块主要来自COL南侧低层暖区,以上升运动为主. 相似文献
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利用1979~1992年卫星TOR对流层臭氧数据库资料,以及同期太阳辐照度数据序列,考察青藏高原对流层臭氧含量变化与太阳辐射周期变化之间的关系.分析表明,青藏高原对流层臭氧分布表现出与太阳辐照度相同的变化趋势,存在着明显的太阳周期变化特征.逐月线性回归分析表明,太阳辐照度增加导致青藏高原对流层臭氧增加的正效应.在太阳周期内,太阳辐射增加可使青藏高原对流层臭氧、平流层臭氧和臭氧总量分别增加1.31、4.97、6.628DU,或4.07%、2.04%、2.28%.该特征与赤道太平洋地区完全相反,分析产生差异的原因,至少应包括两方面因素：一是背景大气NOX和水汽含量的差异;二是青藏高原频繁发生的平流层-对流层大气物质交换和输送. 相似文献
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平流层准两年变化对南海夏季风影响机制的探讨 总被引：2，自引：0，他引：2
利用美国大气研究中心(the National Center for Atmospheric Research, NCAR)的中层大气模式模拟了平流层准两年振荡(Quasi-Biennial Oscillation, QBO)过程对对流层顶和对流层上层的影响, 并结合NCEP(the National Centers for Environmental Prediction)/NCAR、欧洲中期天气预报中心(European Centre for Medium-Range Weather Forecasts, ECMWF)月平均的风场资料和实际的探空观测资料, 分析了平流层QBO对南海夏季风的影响作用. 结果表明: 平流层QBO会引起平流层的异常经向环流并向下传播, 在QBO位相的中后期和位相转换期影响到对流层顶和对流层上层, 使热带和低纬度的对流层上层形成异常的经向气压梯度, 最终在夏季的对流层热带地区激发出不同类型的异常环流—西风位相时, 激发出与南海夏季风环流相反的异常环流, 在南海地区有显著的异常下沉运动, 对南海夏季风有削弱作用; 东风位相时, 激发出反Hadley环流型的异常环流, 在南海地区有明显的异常上升气流, 对南海夏季风有加强的效果. 虽然QBO对南海夏季风经向环流有影响, 但它并不是决定南海夏季风准两年变化的唯一因子. 相似文献
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南极大气臭氧和温度垂直结构及其季节变化的研究 总被引：1，自引：0，他引：1
利用南极中山站2008年2月至2009年2月臭氧和温度探空等资料,对中山站上空大气臭氧和温度的垂直结构及季节变化特征进行了研究.结果表明,在中山站上空热对流层顶和臭氧对流层顶的高度相近,年平均高度分别为7.9和7.4km.对流层顶的气压和温度都存在位相相反一波型季节变化.春季和冬季对流层顶的温度转折没有夏季和秋季明显,而依据臭氧变化恰能更好地确定对流层顶高度.在对流层臭氧垂直分布的季节变化不显著;而平流层却十分明显.春季下平流层臭氧严重耗损,14km处的臭氧最小分压仅为1.57MPa,最大分压出现在上平流层,其他季节下平流层臭氧随高度增加而升高.春季下平流层臭氧的严重损耗,与极夜过后低温条件和平流层冰晶云表面消耗臭氧的光化学过程有密切关系.大气臭氧和温度的垂直结构及季节变化特征,对春季南极臭氧洞的形成和发展具有重要意义. 相似文献
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应用1871-2008年NCEP／NCAR月平均再分析资料,研究了1948-2008年期间全球纬向平均大气环流基本模态的年代际变化.小波凝聚谱的结果表明全球纬向平均大气环流基本模态存在显著的20年左右周期的年代际变化.小波凝聚位相的结果清楚地显示了纬向平均大气环流基本模态的变化顺序.在20年左右的年代际变化时间尺度上,全球纬向平均温度超前纬向平均位势高度2个月,同时超前纬向平均流10个月出现变化;全球纬向平均位势高度又超前纬向平均流8个月出现变化.全球温度上升(下降), 将使高纬度的纬向平均位势高度降低(升高),中低纬度的纬向平均位势高度升高(降低);进而使得中高纬和热带的纬向平均西风加(减)速或东风减(加)速,同时使极地和副热带的西风减(加)速或东风加(减)速.20世纪70年代末期以来全球显著增暖的异常信号最早出现在南半球对流层顶附近,其次出现在南半球对流层低层、北半球对流层顶附近和北半球对流层低层. 相似文献
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亚洲地区是物质由对流层向平流层输送的主要通道,在平流层-对流层交换中扮演着积极的角色. 本文主要利用卫星资料和欧洲中心ERA40再分析资料,借助Wei诊断模式研究亚洲地区夏季上对流层-下平流层(UTLS)水汽分布和平流层-对流层水汽交换特征,重点着眼于水汽交换的年际变化,并探讨其与亚洲夏季风的联系. 结果表明,季风区UTLS水汽较赤道地区偏多,且通过磁带记录信号的传播,可穿越对流层顶影响下平流层水汽的多寡. 夏季平流层-对流层水汽交换表现出明显的年际特征,其年际变化与亚洲季风强弱变化有密切联系,尤其与南亚夏季风的关系更为显著. 在亚洲夏季风影响下,亚洲地区出现异常的大气环流和垂直运动,从而影响平流层-对流层之间水汽的交换. 这些结果对认识其它大气成分的输送过程也具有重要的指示意义. 相似文献
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利用中国科学院大气物理研究所9层大气环流模式（IAP9L AGCM）对夏季气候进行了30年（ 1970～1999年）集合回报试验,并采用统计学分析方法对跨季度夏季短期气候的可预测性问 题进行了初步探讨. 结果表明,该模式对对流层中、高层大气环流的预测能力强于低层,位 势高度场和表面气温的可预测性最大,而降水的可预测性则相对较小. 对流层中、高层位势 高度场的可预测性基本呈带状分布,越靠近赤道可预测性越高;而降水的可预测性基本局限 于赤道东太平洋及热带个别区域. 由此可见,降水的预测极为困难和复杂,订正系 统的研究和寻找新的预报物理因子非常重要. 相似文献
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This study demonstrates that ordinary kriging in spherical coordinates using experimental semi-variograms provides highly usable results, especially near the pole in winter and/or where there could be data missing over large areas. In addition, kriging allows display of the spatial variability of daily ozone measurements at different pressure levels. Three satellite data sets were used: Total Ozone Mapping Spectrometer (TOMS) data, Solar Backscattered UltraViolet (SBUV), and the Stratospheric Aerosol and Gas Experiment (SAGE II) ozone profiles. Since SBUV is a nadir-viewing instrument, measurements are only taken along the sun-synchronous polar orbits of the satellite. SAGE II is a limb-viewing solar occultation instrument, and measurements have high vertical resolution but poor daily coverage. TOMS has wider coverage with equidistant distribution of data (resolution 1° × 1.25°) but provides no vertical information. Comparisons of the resulting SBUV-interpolated (column-integrated) ozone field with TOMS data are strongly in agreement, with a global correlation of close to 98%. Comparisons of SBUV-interpolated ozone profiles with daily SAGE II profiles are relatively good, and comparable to those found in the literature. The interpolated ozone layers at different pressure levels are shown. 相似文献
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Arlin J. Krueger Louis S. Walter Charles C. Schnetzler Scott D. Doiron 《Journal of Volcanology and Geothermal Research》1990,41(1-4)
The eruptions of Nevado del Ruiz in 1985 were unusually rich in sulfur dioxide. These eruptions were observed with the Nimbus 7 Total Ozone Mapping Spectrometer (TOMS) which can quantitatively map volcanic sulfur dioxide plumes on a global scale. A small eruption, originally believed to be of phreatic origin, took place on September 11, 1985. However, substantial amounts of sulfur dioxide from this eruption were detected with TOMS on the following day. The total mass of SO2, approximately 9 ± 3 × 104 metric tons, was deposited in two clouds, one in the upper troposphere, the other possibly at 15 km near the stratosphere.The devastating November 13 eruptions were first observed with TOMS at 1150 EST on November 14. Large amounts of sulfur dioxide were found in an arc extending 1100 km from south of Ruiz northeastward to the Gulf of Venezuela and as an isolated cloud centered at 7°N on the Colombia-Venezuela border. On November 15 the plume extended over 2700 km from the Pacific Ocean off the Colombia coast to Barbados, while the isolated mass was located over the Brazil-Guyana border, approximately 1600 km due east of the volcano. Based on wind data from Panama, most of the sulfur dioxide was located at 10–16 km in the troposphere and a small amount was quite likely deposited in the stratosphere at an altitude above 24 km.The total mass of sulfur dioxide in the eruption clouds was approximately 6.6 ± 1.9 × 105 metric tons on November 14. When combined with quiescent sulfur dioxide emissions during this period, the ratio of sulfur dioxide to erupted magma from Ruiz was an order of magnitude greater than in the 1982 eruption of El Chichon or the 1980 eruption of Mount St. Helens. 相似文献
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Summary Eight vertical profiles compiled from simultaneous measurements of Aitken nuclei and ozone concentrations over Germany in different weather conditions are discussed. The position and shape of the profiles is shown to depend on the prevailing weather conditions and the type of air masses. High aerosol concentrations in smoke plumes correlate in some cases with lower ozone concentrations, indicating that ozone in such cases is destroyed in the presence of high concentrations of pollutants such as aerosols and gases. A layered structure in the profiles was found only in association with temperature inversions and where the air above 2 km was subsiding, and was not found in convective parts of the troposphere. 相似文献
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将TOMS测量的北半球不同纬度各纬向平均逐日O。总量作为无规序列,利用时滞方法重构序列的相空间吸引子,计算其系统状态演化过程中形成的整体结构特征.结果表明,各纬度O3层系统吸引子都具有非整数分维结构；此外,在完整的Lpapunov指数谱中,所有指数分量之和均为负值,且最大指数分量总是正值.反映出O3层系统相空间总体上是收缩的,同时提供了存在奇怪吸引子的证据,表征O3层系统的演化是一种耗散混饨运动.这对于进一步应用非线性动力系统理论和方法,深入研究O3层系统的动力学特征具有重要意义. 相似文献
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The 1982 eruption of El Chichon inspired a new technique for monitoring volcanic clouds. Data from the Total Ozone Mapping Spectrometer (TOMS) instrument on the Nimbus-7 satellite were used to measure sulfur dioxide in addition to ozone. For the first time precise data on the sulfur dioxide mass in even the largest explosive eruption plumes could be determined. The plumes could be tracked globally as they are carried by winds. Magmatic eruptions could be discriminated from phreatic eruptions. The data from El Chichon are reanalyzed in this paper using the latest version of the TOMS instrument calibration (V8). They show the shearing of the eruption cloud into a globe-circling band while still anchored over Mexico in three weeks. The measured sulfur dioxide mass in the initial March 28 eruption was 1.6 Tg; the April 3 eruption produced 0.3 Tg more, and the April 4 eruptions added 5.6 Tg, for a cumulative total of 7.5 Tg, in substantial agreement with estimates from prior data versions. TOMS Aerosol Index (absorbing aerosol) data show rapid fallout of dense ash east and south of the volcano in agreement with Advanced Very High Resolution Radiometer (AVHRR) ash cloud positions. 相似文献
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K. Petzoldt 《Annales Geophysicae》1999,17(2):231-241
Total ozone anomalies (deviation from the long-term mean) are created by anomalous circulation patterns. The dynamically produced ozone anomalies can be estimated from known circulation parameters in the layer between the tropopause and the middle stratosphere by means of statistics. Satellite observations of ozone anomalies can be compared with those expected from dynamics. Residual negative anomalies may be due to chemical ozone destruction. The statistics are derived from a 14 year data set of TOMS (Total Ozone Mapping Spectrometer January 1979-Dec. 1992) and corresponding 300 hPa geopotential (for the tropopause height) together with 30 hPa temperature (for stratospheric waves) at 60°N. The correlation coefficient for the linear multiple regression between total ozone (dependent variable) and the dynamical parameters (independent variables) is 0.88 for the zonal deviations in the winter of the Northern Hemisphere. Zonal means are also significantly dependent on circulation parameters, besides showing the known negative trend function of total ozone observed by TOMS. The significant linear trend for 60°N is 3 DU/year in the winter months taking into account the dependence on the dynamics between the tropopause region and the mid-stratosphere. The highest correlation coefficient for the monthly mean total ozone anomalies is reached in November with 0.94. 相似文献
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S. P. Smyshlyaev A. I. Pogoreltsev V. Ya. Galin E. A. Drobashevskaya 《Geomagnetism and Aeronomy》2016,56(1):95-109
The planetary wave impact on the polar vortex stability, polar stratosphere temperature, and content of ozone and other gases was simulated with the global chemical–climatic model of the lower and middle atmosphere. It was found that the planetary waves propagating from the troposphere into the stratosphere differently affect the gas content of the Arctic and Antarctic stratosphere. In the Arctic region, the degree of wave activity critically affects the polar vortex formation, the appearance of polar stratospheric clouds, the halogen activation on their surface, and ozone anomaly formation. Ozone anomalies in the Arctic region as a rule are not formed at high wave activity and can be registered at low activity. In the Antarctic Regions, wave activity affects the stability of polar vortex and the depth of ozone holes, which are formed at almost any wave activity, and the minimal ozone values depend on the strong or weak wave activity that is registered in specific years. 相似文献
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Long-term measurements of the ozone concentration in the vicinity of the city of Berlin have been performed with ground based Dobson spectrophotometers and balloon borne systems. The respective experiments cover the past 24 years. All data have been reevaluated and corrected towards uniform calibration standards, leading to the longest European data set of total column density, altitude-dependent ozone partial pressures and the corresponding temperatures. Smoothing algorithms unravel significant long-term trends.The analysis shows an increase of ozone concentration within the middle stratosphere (below 31 km height) as well as in the troposphere over the past 24 years. On the contrary, ongoing ozone depletion in the lower stratosphere has been found.The large scale vertical redistribution of atmospheric ozone in the troposphere and the lower stratosphere seems to be in agreement with model calculations and trend predictions that have their roots in changes of the chemical composition and the ozone photochemistry due to anthropogenically induced trace gas concentrations.Deutscher Wetterdienst, Meteorologisches Observatorium Potsdam.Deutscher Wetterdienst, Meteorologisches Observatorium Lindenberg. 相似文献