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1.
利用卫星资料计算得到的对流层臭氧柱总量数据分析了近20年来全球对流层臭氧柱总量的全球分布特征，并对我国对流层臭氧的季节变化做了研究。利用对流层污染测量仪（MOPITT）的CO和全球臭氧监测仪（GOME）和大气制图扫描成像吸收光谱仪（SCIAMACHY）的NO2数据分析了关于对流层臭氧的分布特征及其原因。得出中高纬度地区对流层臭氧浓度存在规律的年内变化，对流层臭氧高浓度值的分布及变化与人类活动有密切关切。  相似文献   

2.
利用GOME卫星资料分析北京大气NO2污染变化   总被引：11，自引：1，他引：11       下载免费PDF全文
利用GOME (Global Ozone Monitoring Experiment, 全球臭氧监测实验) 1996年1月—2002年12月NO2对流层柱浓度月平均卫星遥感资料以及根据北京市2001年1月1日—2002年12月31日NO2污染指数数据计算出的地面NO2日均质量浓度值, 分析了北京市城市大气NO2污染变化的季节变化特征以及年际变化, 并将2001年1月—2002年12月北京上空GOME NO2对流层柱浓度月平均值变化与北京市地面NO2日均质量浓度月平均值变化进行了比较, 结果表明两者随时间的变化趋势具有较好的一致性, 据此可以利用GOME NO2对流层柱浓度月平均卫星遥感资料来分析特定区域大气NO2的季节变化和年际变化。  相似文献   

3.
Both surface environmental monitoring and satellite remote sensing show that North China is one of the regions that are heavily polluted by NO2. Using the NO2 monitoring data from 18 major cities in the region, the tropospheric NO2 column density data from the Ozone Monitoring Instrument (OMI) on the Aura satellite, and the observations from the China Meteorological Administration network, this paper analyzes a regional NO2 pollution event in February 2007 over North China, examines the convergence of the pollutant, and identifies its correlation with the atmospheric background conditions. The results show that daily mean NO2 concentrations derived from surface observations are consistent with the mean values of the OMI measurements, with their correlation coefficient reaching 0.81. The correlations of NO2 concentration with general weather patterns and sequential changes of temperature structure from 925 hPa down to the surface indicate that the weather fronts, high pressure and low pressure systems in the atmosphere play a role in changing the temporal and spatial evolutions of NO2 through removing, accumulating or converging of the pollutant, respectively. It is also found that the eastern Taihang Mountains is most heavily polluted by NO2 in North China. Based on a model that correlates NO2 column density with surface wind vector, the relation of the NO2 concentrations in six major cities in North China to the surrounding wind field is analyzed. The results show that the maximum wind field is associated with the highest frequency of pollution events, and under certain large-scale atmospheric conditions together with the topographic effect, small- and meso-scale wind fields often act to transport and converge pollutants, and become a major factor in forming the heaviest NO2 pollution event in North China. Analysis of the causes for the severe NO2 pollution event in this study may shed light on understanding, forecasting, and mitigating occurrences of heavy NO2 pollution.  相似文献   

4.
基于中国东部地区（30°—40°N,105°E以东）19个代表站1470—2019年旱涝等级序列、古气候代用资料定量重建的北太平洋海表温度年代际振荡指数以及Nino3.4指数,通过经验正交函数分解、小波分析和集合经验模态分解方法分析了中国东部旱涝年代际变化特征及其与太平洋海温的关系。结果表明,（1）1470年以来中国东部旱涝变化的主模态为全区一致型（方差贡献率为25.2%）,变率中心主要位于黄河中下游,其时间系数的小波分析和集合经验模态分解揭示出全区旱涝存在10—30 a的准周期;该模态长期趋势揭示17—18世纪中国东部整体偏涝,而19世纪以后出现干旱化趋势。（2）寒冷背景下中国东部旱涝一致变化更明显,在17世纪前、中期和19世纪中、后期的小冰期寒冷期全区一致型模态的方差贡献率为35%—40%,且这两个时段10—30 a的年代际变化信号尤为显著;而旱涝的变率中心则表现出冷期偏北,暖期偏南或偏西的特征。（3）中国东部旱涝的年代际变化与北太平洋和赤道中东太平洋海表温度异常有关,表现为偏涝（旱）气候对应于北太平洋海表温度年代际振荡的冷（暖）相位,以及年代际尺度上的冬季Nino3.4区海表温度的异常偏低（高）;在小冰期的寒冷期,旱涝的年代际变化可能与Nino3.4区海表温度异常关系更密切。   相似文献   

5.
It is still not well understood if subseasonal variability of the local PM2.5 in the Beijing-Tianjin-Hebei (BTH) region is affected by the stratospheric state. Using PM2.5 observations and the ERA5 reanalysis, the evolution of the air quality in BTH during the January 2021 sudden stratospheric warming (SSW) is explored. The subseasonal variability of the PM2.5 concentration after the SSW onset is evidently enhanced. Stratospheric circumpolar easterly anomalies lasted for 53 days during the January–February 2021 SSW with two evident stratospheric pulses arriving at the ground. During the tropospheric wave weakening period and the intermittent period of dormant stratospheric pulses, the East Asian winter monsoon weakened, anomalous temperature inversion developed in the lower troposphere, anomalous surface southerlies prevailed, atmospheric moisture increased, and the boundary layer top height lowered, all of which favor the accumulation of pollutant particulates, leading to two periods of pollution processes in the BTH region. In the phase of strengthened East Asian winter monsoon around the very beginning of the SSW and another two periods when stratospheric pulses had reached the near surface, opposite-signed circulation patterns and meteorological conditions were observed, which helped to dilute and diffuse air pollutants in the BTH region. As a result, the air quality was excellent during the two periods when the stratospheric pulse had reached the near surface. The increased subseasonal variation of the regional pollutant particulates after the SSW onset highlights the important role of the stratosphere in the regional environment and provides implications for the environmental prediction.  相似文献   

6.
中国区域性极端降水事件及人口经济暴露度研究   总被引：4，自引：1，他引：3  
基于中国1960-2014年771个气象站的逐日降水资料,选取有效降水序列95百分位数作为极端降水阈值,将既定持续时间尺度和连续面积上超过阈值的降水事件定义为区域性极端降水事件。采用强度-面积-持续时间（Intensity-Area-Duration,IAD）法,根据极端降水事件空间和时间上的连续性特征,对不同持续时间的区域性极端降水事件演变趋势及暴露于极端降水事件下的人口和国内生产总值进行研究。结果表明:（1）相对强度最大的区域性极端降水事件主要集中在1960-1968、1991-1999和2006-2013年3个时段;（2）区域性极端降水事件最强中心主要分布在长江以南和东北地区,发生在北方的多为单日极端降水,南方多为持续多日的极端降水;（3）1960-2014年区域性极端降水事件影响面积有所增大,相对强度变化不明显;（4）暴露于极端降水事件影响区域内的人口和国内生产总值均呈显著增大趋势,暴露人口最多的年份在1983年,达到2408万人/d,暴露国内生产总值最多的年份在1998年,达到20亿元/d。   相似文献   

7.
根据海南省环境科学研究院提供的海口站2013—2016年逐日空气污染数据,统计分析了海口市空气质量状况。综合应用高低空环流场、AQI指数结合MODIS卫星蓝光气溶胶厚度图,采用HYSPLIT轨迹聚类分析法、潜在源贡献因子法和浓度权重轨迹分析方法,重点分析了2013年12月海口空气污染的的主要输送路径,并探讨了首要污染物PM2.5和O3的潜在源区。结果表明：冬夏季风风向转换是海口发生空气污染的最主要气象原因,且首要污染物为PM2.5,其次是PM10和O3;海口市空气质量达标率在97.1%,总体较好,AQI指数呈逐年下降趋势;值得关注的是,O3呈逐年稳定上升趋势。大气污染物浓度受污染物排放和环流场共同影响,海口污染日对应的地面天气形势主要有3种类型,冷高压、变暖高压脊和台风外围下沉气流。此次污染过程中污染源是来自北方地区污染物长距离输送影响的结果。污染物个例分析中,首要污染物PM2.5潜在源区主要集中在湖南和江西的交界处、广东沿海地区、广西北部、江西和福建的交界处以及浙江中部地区,这些潜在源区气团沿着轨迹1、2和4通过长距离输送到海口。海口O3质量浓度贡献较大的区域主要集中在湖南和江西的交界处、粤西一带,主要沿着轨迹2将内陆地区的污染源输送到海口。  相似文献   

8.
Both surface environmental monitoring and satellite remote sensing show that North China is one of the regions that are heavily polluted by NO2. Using the NO2 monitoring data from 18 major cities in the region, the tropospheric NO2 column density data from the Ozone Monitoring Instrument (OMI) on the Aura satellite, and the observations from the China Meteorological Administration network, this paper analyzes a regional NO2 pollution event in February 2007 over North China, examines the convergence of the pollutant, and identies its correlation with the atmospheric background conditions. The results show that daily mean NO2 concentrations derived from surface observations are consistent with the mean values of the OMI measurements, with their correlation coeficient reaching 0.81. The correlations of NO2 concentration with general weather patterns and sequential changes of temperature structure from 925 hPa down to the surface indicate that the weather fronts, high pressure and low pressure systems in the atmosphere play a role in changing the temporal and spatial evolutions of NO2 through removing, accumulating or converging of the pollutant, respectively. It is also found that the eastern Taihang Mountains is most heavily polluted by NO2 in North China. Based on a model that correlates NO2 column density with surface wind vector, the relation of the NO2 concentrations in six major cities in North China to the surrounding wind field is analyzed. The results show that the maximum wind field is associated with the highest frequency of pollution events, and under certain large-scale atmospheric conditions together with the topographic effect, small- and meso-scale wind fields often act to transport and converge pollutants, and become a major factor in forming the heaviest NO2 pollution event in North China. Analysis of the causes for the severe NO2 pollution event in this study may shed light on understanding, forecasting, and mitigating occurrences of heavy NO2 pollution.  相似文献   

9.
北京地区气溶胶PM2.5粒子浓度的相关因子及其估算模型   总被引：20，自引：0，他引：20  
文中运用统计分析和气象统计预报的方法 ,使用北京白石桥小区的污染物观测资料和同期北京地区的气象观测资料 ,对影响大气污染的气象因子进行了综合分析 ,并分别建立了气溶胶PM 2 .5粒子浓度与气体污染物、气象要素场的两类统计相关拟合模型。发现气溶胶PM2 .5粒子浓度与气体污染物浓度存在不同程度的相关性 ,且与气象条件亦存在显著的相关关系 ,此类时空变化及其量化估算模型具有一定实际应用价值。通过确定气象要素场和气溶胶浓度的关系可进一步研究不同地区的污染物输送和污染源扩散影响的问题。  相似文献   

10.
基于集合卡尔曼滤波的源反演方法是估计排放源、提高空气质量模拟和预报精度的有效方法。为构建排放源与污染物浓度之间的误差协方差矩阵,该方法通常需要运行几十次大气化学传输模式。庞大的计算量限制了该方法的应用,使其无法为实时预报系统快速更新排放源。本研究发展了一种基于集合最优插值的排放源反演方法。该方法使用历史集合数据构建误差协方差矩阵,仅需一次常规的空气质量模拟便可根据观测模拟差异反演排放源,从而显著降低计算量。本文使用该方法同化2015年1月全国1107个地面站点观测的CO小时浓度数据,结合2014年1月的历史集合数据集,估计2015年1月全国15 km分辨率的CO排放源。该方案反演的全国CO排放总量仅比使用2015年1月集合数据集的反演量高1%,表明历史时段与反演时段的气象条件差异对月均CO排放的影响有限。使用历史集合数据集更新的排放源再次模拟可将全国349个独立验证站点的平均低估从0.74 mg m?3降至0.01 mg m?3,均方根误差降低18%,表明该方法可快速更新排放源并降低其不确定性。  相似文献   

11.
利用行业经济活动数据、1 580个地面监测站和6套卫星反演数据,分析了我国新冠肺炎疫情期间人为碳排放和主要大气污染物的变化。与2019年第一季度相比,2020年同期我国碳排放降低9.8%,其中交通部门降幅最大达到43.4%。与2019年2-3月相比,疫情期间全国地表臭氧浓度同比升高1.9 nL/L(5%),其中华北平原以降低为主,东南部地区以上升为主。PM2.5浓度同比下降12.6μg·m^-3(24.9%),其中长三角降幅最大。二氧化氮(NO2)的地面浓度和对流层柱浓度在京津冀、珠三角和长三角都降低20%~30%,体现了高低层的一致性。地面一氧化碳(CO)浓度同比降低17%,而对流层CO柱浓度升高2.5%,可能原因是境外生物质燃烧输送提升了我国南方高层大气的CO浓度。中东部地区气溶胶光学厚度显著降低,导致地表晴空短波辐射同比升高11.6 W·m^-2(9.6%)。  相似文献   

12.
Satellite measurements of tropospheric column O3 and NO2 in eastern and southeastern Asia are analyzed to study the spatial and seasonal characteristics of pollution in these regions. Tropospheric column O3 is derived from differential measurements of total column ozone from Total Ozone Mapping Spectrometer (TOMS), and stratospheric column ozone from the Microwave Limb Sounder (MLS) instrument on the Upper Atmosphere Research Satellite (UARS). The tropospheric column NO2 is measured by Global Ozone Monitoring Experiment (GOME). A global chemical and transport model (Model of Ozone and Related Chemical Tracers, version 2; MOZART-2) is applied to analyze and interpret the satellite measurements. The study, which is based on spring, summer, and fall months of 1997 shows generally good agreement between the model and satellite data with respect to seasonal and spatial characteristics of O3 and NO2 fields. The analysis of the model results show that the industrial emission of NOx (NO + NO2) contributes about 50%–80% to tropospheric column NO2 in eastern Asia and about 20%–50% in southeastern Asia. The contribution of industrial emission of NOx to tropospheric column O3 ranges from 10% to 30% in eastern Asia. Biomass burning and lightning NOx emissions have a small effect on tropospheric O3 in central and eastern Asia, but they have a significant impact in southeastern Asia. The varying effects of NOx on tropospheric column ozone are attributed to differences in relative abundance of volatile organic compounds (VOCs) with respect to total nitrogen in the two regions.  相似文献   

13.
基于2008年9月—2010年9月河北固城生态与农业气象试验站多轴差分吸收光谱仪 (multi-axis differential optical absorption spectroscopy, MAX-DOAS) 获得的太阳散射光谱观测,反演计算该地区NO2对流层柱浓度,分析其季节、日变化特征以及不同来源输送的影响,并与同期NO2地面观测资料和卫星产品进行对比分析。发现固城站NO2对流层柱浓度冬高 (5.14×1016 cm-2) 夏低 (1.28×1016 cm-2);日变化形态在四季均呈现中午低、傍晚高的特征,且冬季最明显。与北京城市区域同期的观测相比,冬季固城站观测值略低,而在春、夏季则偏低较显著。地面风玫瑰图分析显示,来自SW, SSW, NE方向及ENE方向的污染输送对其贡献最大。与地面、卫星NO2观测的对比表明,MAX-DOAS反演的NO2柱浓度与地面观测浓度具有一致的季节和日变化特征,卫星反演的NO2对流层柱浓度产品在华北平原农村地区存在系统性低估。  相似文献   

14.
The spatial distribution, radiative forcing, and climatic effects of tropospheric ozone in China during summer were investigated by using the regional climate model RegCM4. The results revealed that the tropospheric ozone column concentration was high in East China, Central China, North China, and the Sichuan basin during summer. The increase in tropospheric ozone levels since the industrialization era produced clear-sky shortwave and clear-sky longwave radiative forcing of 0.18 and 0.71 W m–2, respectively, which increased the average surface air temperature by 0.06 K and the average precipitation by 0.22 mm day–1 over eastern China during summer. In addition, tropospheric ozone increased the land–sea thermal contrast, leading to an enhancement of East Asian summer monsoon circulation over southern China and a weakening over northern China. The notable increase in surface air temperature in northwestern China, East China, and North China could be attributed to the absorption of longwave radiation by ozone, negative cloud amount anomaly, and corresponding positive shortwave radiation anomaly. There was a substantial increase in precipitation in the middle and lower reaches of the Yangtze River. It was related to the enhanced upward motion and the increased water vapor brought by strengthened southerly winds in the lower troposphere.  相似文献   

15.
Spatio-temporal distribution characteristics and variation trends of tropospheric NO_2 in Pearl River Delta(PRD) urban group and its adjacent areas were analyze from 2005 to 2013 based on remote sensing data from ozone monitoring instrument(OMI) satellite, and further explored the impact of human activities on NO_2. Compared with the ground observation data, the OMI NO_2 remote sensing data displayed high reliability. Due to active industrial production, high car ownership, great energy and power consumption, the average tropospheric NO_2concentration(7.4×1015molec/cm2) of PRD region is about 3 times of the adjacent areas. At the same time, the regional high pollution NO_2 in PRD region as a whole, the urban group effect is remarkable. Sinusoidal model can well fit the periodic variation of the NO_2 in PRD and adjacent areas. NO_2 concentration was highest in winter while lowest in summer. The concentration of NO_2 in PRD region is decreasing in recent 9 years, which has a significantly negative correlation with the second industry output and car ownership. This suggests that the nitrogen oxide emissions governance in PRD region had achieved initial results. The concentration of NO_2 increased significantly in the eastern and northern Guangdong Province, there are good positive correlations with the second industrial outputs and car ownerships, it is thus clear that industrial emissions and automobile exhausts are important sources of NO_2 in these regions. The concentration of NO_2 in western Guangdong area is stable.  相似文献   

16.
Aircraft campaigns for the meteorological and environmental research have been conducted in regional and global scales. The aircraft is increasingly considered as one of the best platforms to get the atmospheric three-dimensional information, especially over sea. We discuss the airborne observation plan and payloads designed for the aircraft campaigns over the Korean Peninsula. The main goals of the campaigns are to (i) conduct precipitation (snow) enhancement experiments with observations of the microphysical properties of clouds, dominantly in winter, (ii) monitor the severe weather generally in summer, (iii) characterize the climate change composition and the outflow of pollution from the Asian continent of the troposphere over the Korean Peninsula generally in spring or fall, and (iv) validate satellite and ground-based remote measurements of tropospheric composition generally in spring or fall.  相似文献   

17.
In this paper we present a review of atmospheric chemistry research in China over the period 2006-2010, focusing on tropospheric ozone, aerosol chemistry, and the interactions between trace gases and aerosols in the polluted areas of China. Over the past decade, China has suffered severe photochemical smog and haze pollution, especially in North China, the Yangtze River Delta, and the Pearl River Delta. Much scientific work on atmospheric chemistry and physics has been done to address this large-scale, complex environmental problem. Intensive field experiments, satellite data analyses, and model simulations have shown that air pollution is significantly changing the chemical and physical characters of the natural atmosphere over these parts of China. In addition to strong emissions of primary pollutants, photochemical and heterogeneous reactions play key roles in the formation of complex pollution. More in-depth research is recommended to reveal the formation mechanism of photochemical smog and haze pollution and their climatic effects at the urban, regional, and global scales.  相似文献   

18.
2013年1—3月北京及周边地区雾、霾高发,气候特征异于常年。利用2013年1—3月北京及周边地区6个地面观测站观测资料,研究PM2.5和黑碳 (BC) 的质量浓度、区域分布特征及气象要素的影响情况。结果表明:北京及周边地区PM2.5污染呈区域性高值、污染局地积累以及由南向北输送的特征。北京上甸子站在雾、霾与清洁期间BC与PM2.5质量浓度的比值分别为7.1%和10.3%,雾、霾期间低于清洁期间;而河北固城站在雾、霾与清洁期间BC与PM2.5质量浓度的比值分别为17.5%和11.9%,雾、霾期间明显高于清洁期间。二者相反的比值特征反映在清洁的下游地区雾、霾过程中二次生成的气溶胶所占比例较污染的上游地区偏高。  相似文献   

19.
北京冬季雾霾事件的气象特征分析   总被引：4，自引：3，他引：1  
利用观测的气象要素和细颗粒物(即PM2.5)浓度资料,并结合中尺度数值天气模式WRF(Weather Research and Forecasting Model),对2013年1月北京地区雾霾污染期间天气条件和边界层气象特征进行了分析。模拟与观测对比表明,WRF模式可以较好地反映北京—天津—河北地区地面和高空主要气象要素的时空分布。对1月10~14日、27~31日两次重雾霾天气的分析表明,雾霾的形成是高浓度的大气颗粒物和特殊的气象条件共同作用的结果。小风或静风、稳定的大气层结,使大气扩散能力减弱,造成污染物堆积,偏南气流将周边污染物和水汽输送到北京,不仅增加了污染物浓度,而且有利于气溶胶吸湿增长,消光增强,使能见度下降,进而形成雾霾。  相似文献   

20.
综合运用了多元资料（环境空气质量监测资料、地面气象观测资料、L波段雷达探空资料、风廓线雷达探空资料和再分析资料）和多种方法（后向轨迹追踪、聚类分析、潜在源区贡献法和数值模拟）,研究了武汉地区特殊气象条件对重污染过程的影响,揭示了偏东小风所带来的外源污染物对形成严重污染日的贡献.主要研究结论如下：1）后向轨迹追踪分析表明,武汉地区严重污染日气流主要为来自安徽南部（47.5%）的偏东小风,模拟结果也显示偏东气流、偏北气流与局地环流共同作用,在武汉地区形成一个局地涡旋,成为反复污染带,加重了武汉地区的污染程度;2）利用潜在源区贡献法（PSCF）分析发现,武汉市秋冬季的潜在源区主要是安徽、江苏、山东、河南、湖南、江西以及武汉周边地区,因此在冬季大范围污染背景下,跨区域的联防联控（尤其是安徽南部地区）才能有效地减少武汉市秋冬季的重污染日.  相似文献   

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