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1.
长江口外海域沉积物中有机物的来源及分布 总被引：10，自引：0，他引：10
通过分析长江口外海域不同区域有机碳和氮的分布特征及其影响因素,了解了底部沉 积物中有机碳和氮同位素的生物地球化学特征,探讨二者对长江口外海域底部沉积物中有机 物来源的指示意义。运用质量混合模型,计算了长江输入的陆源有机物的贡献及其空间变化。结果表明,长江口外海域沉积物中TOC 和TN 的分布和东海陆架的环流体系有着密切关系, 与环流的分布相对应,如果大致沿31oN 和123oE 作为分界线, 整个研究区的TOC 和TN 的分布可划分为4 个具有不同分布特征的区域。TOC、TN、δ13C 和δ15N 分别与沉积物的平均粒 径呈线性相关关系,因此,粒度效应是控制长江口外海域沉积物中有机物分布和稳定同位素 碳、氮的一个重要因素。研究区内的C/N 比值能够在一定程度上体现有机物的来源信息,但δ15N 表现出了与C/N 和δ13C 不同的区域分布和变化特征。陆源有机物来源比重较高的区域与 长江口外海域赤潮突发频率最高的地区相对应。长江口附近沉积物中的陆源有机物来源最高, 超过了50%,且等值线呈舌状向东北方向凸出,表明了长江冲淡水的影响。陆源颗粒态有机物沉海底后,要不断经历早期成岩作用和生物作用,因此在在相同地点,陆源有机物对沉积物中有机物的贡献,要明显小于对悬浮颗粒态有机物的贡献。 相似文献
2.
湖泊沉积物有机地化指标在古气候解释中具有复杂性和多解性。TOC、C/N和δ^13Corg作为3种常用的有机地化指标,现已广泛运用于东、中亚全新世气候变化研究中。以这3种指标为例综述了东、中亚全新世湖泊沉积有机地化指标的变化机制及影响因素。根据数据的综合分析与对比,大部分湖泊全新世沉积物TOC百分含量较高时,C／N比值也较高。这与沉积物有机质的来源有关,因两者TOC和C／N作用机制不同,也存在少数湖泊,其两者对应关系不明显;同一湖泊δ^13Corg与TOC及δ^13Corg与C／N对应关系相似;由于不同区域影响有机地化指标的因素不同,TOC、C／N和δ1^3Corg间的关系存在区域差异,据此可将研究区分为中纬度地区、青藏高原区和低纬度季风区。上述区域规律存在于研究中所选的大部分湖泊,由于有机地化指标作用机理的复杂性,也存在不符合这种规律的湖泊,因而上述结论有待于进一步讨论。 相似文献
3.
滇池流域宝象河水库沉积物中有机碳的来源 总被引：1，自引：0，他引：1
通过对滇池流域宝象河水库沉积物TOC、TN、C/N、δ13C及粒度等指标的测定,分析了沉积物中有机碳的主要来源及其变化趋势。结果表明:水体中不同位置沉积物有机碳来源并不相同,距三岔河入库河口相对较近的沉积柱芯A中C/N比值介于2.93~11.73,δ13C值介于-23.66‰~-21.78‰,有机碳主要来源于水生生物,陆源输入贡献较小,有机碳含量受粒径大小影响显著;距三岔河入库河口相对较远的沉积柱芯B中,其TOC和TN含量较高,分别介于14.62~24.93 g?kg-1和2.11~3.3 g?kg-1,δ13C值变化范围为-28.36‰~-26.36‰,粒度以黏土和细粉砂为主,有机碳主要来源于水库周边陆源输入,受人类活动影响强烈。 相似文献
4.
青藏高原对全球气候变暖响应敏感,研究青藏高原近千年来环境演化过程、规律与驱动机制对预测其未来气候变化有重要意义。本文通过位于青藏高原东部的苦海沉积物总有机质相关指标(总有机碳(TOC)、总氮(TN)、总有机碳与总氮比值(TOC/TN)和总有机碳同位素(δ13Corg)的研究重建了该区域过去840年来环境演化过程。结果表明,苦海沉积物中的有机质主要来自于内源水生植物。由于暖期(冷期)时黄河上游径流量较高(低),苦海水位随之升高(降低),湖泊水动力增强(减弱),浅水区沉水植物对研究岩芯中的有机质贡献率提高(降低),导致沉积物TOC、TN、TOC/TN升高,δ13Corg值正(负)偏。人类活动导致的青藏高原近50年气候异常变暖可能是~1950 AD之后δ13Corg反映的黄河上游径流量变化与重建的中国温度记录之间的关系发生转变的原因。苦海沉积物δ13Corg记录与万象洞石笋δ18O记录和太阳总辐射强度记录变化特征的相似性说明青藏高原东部地区气候变化的控制因素为太阳辐射驱动下的季风降雨量变化。 相似文献
5.
6.
湖沼沉积物地球化学元素对地球气候环境变化敏感性强。本文以江西定南大湖湖沼沉积物地球化学元素为研究对象,使用主成分分析法,并结合总有机碳(TOC)、有机碳同位素(δ13Corg)、中值粒径(Md)、化学蚀变指数(CIA)等相关气候代用指标,以元素组对的形式阐释不同地化元素响应不同气候环境下的地球化学行为和迁移规律。研究结果显示：第一主成分(PC1)包括Al2O3、TiO2、SiO2、Nb、Rb、Ga、Ba、S等元素,曲线变化与CIA相似,指示湖泊流域的化学风化强度,气候暧湿,PC1含量高;第二主成分(PC2)包括Co、Zr、Hf元素,曲线变化与中值粒径较为一致,指示湖泊流域的水动力条件,气候冷干,PC2含量高;第三主成分(PC3)包括Sc、Cu、U、V元素,曲线变化与TOC、δ13Corg含量变化一致。大湖沉积物的物质来源为：在气候暧湿、流域化学风化作用强的条件下,地表径流冲刷流域周边花岗岩风化壳物质并搬运至湖盆沉积,但不排除在冷干时期,风力携带粉尘物质堆积的影响,粉尘物质可能主要源于周边的风化碎屑物。 相似文献
7.
长江中游网湖近代沉积环境演变及其对人类活动的响应 总被引：5，自引：2，他引：3
采用放射性核素210Pb和137Cs计年方法,建立了长江中游网湖近代沉积物的年代序列,并对网湖沉积物的粒度组成、磁性参数、重金属元素、花粉组合以及营养盐含量等指标进行了分析。根据沉积指标垂直分布的综合特征,结合湖区史料,重建了网湖100年来沉积环境的演变过程。通过对沉积指标与湖区人口变化、工农业产值等数据的比对,发现中华人民共和国成立以后沉积物中TOC和TN浓度与人口变化存在较高的相关性,相关系数分别达到0.8892和0.8928(P<0.001);沉积物中重金属元素富集序列、营养盐富集序列与孢粉含量的变化序列与湖区人类活动具有较好的耦合性。表明网湖沉积指标可以敏感地反映湖区的人类活动。 相似文献
8.
全新世中后期开封西郊黄泛沉积序列的孢粉记录 总被引：2，自引：1，他引：1
历史时期以来,黄河在开封市附近多次泛滥形成了相对完整的沉积序列。选取开封市西郊25 m岩芯（ZKjm）为研究对象,通过孢粉分析,结合地层沉积旋回和历史文献资料,探讨了全新世中后期以来大洪水事件的孢粉记录。结果表明：黄泛地层中的孢粉含量及其组成很好地记录了大洪水事件,洪水沉积期的木本植物花粉含量高于其间断期,而人工禾本科花粉含量低于间断期。每个粒度旋回基本上都有与之对应的孢粉亚带,且其上下界限的吻合度较高,表明孢粉可作为划分沉积旋回的代用指标。岩芯孢粉亚带的数目（12个）多于粒度旋回数目（9个）,孢粉组合特征可以识别出规模较小的洪水或者一次洪水事件出现的多个短期洪水间歇期所形成的沉积,孢粉指标划分沉积旋回的精度高于粒度指标。 相似文献
9.
江陵地区全新世早期人类活动的孢粉记录 总被引：6，自引：3，他引：3
江陵剖面沉积物孢粉提供全新世早期人类活动的证据。早期人类活动始于6 200 a B.P.,人类大规模活动始于3 400 a B.P.。随着定居点扩大和人类活动加强,地表土壤侵蚀严重,入湖的陆源粗颗粒物质和营养物质增多。湖泊沉积物表现为粗颗粒含量迅速增加,各粒径波动频繁,TOC、TN和C/N的高值以及有机质δ13C的低值。2 500 a B.P.以后,沉积环境发生了显著变化,由湖泊及湖沼堆积转化为洪水漫滩堆积,气候变干,人类逐渐撤离该地区。 相似文献
10.
蒙古国北部Gun Nuur湖20个表层沉积物孢粉组合与数量分析研究揭示,孢粉组合及浓度分布存在显著空间差异。结果表明：双束松型花粉百分含量由湖泊东南向西北降低,桦属、蒿属、藜科以及禾本科百分含量增加,湖泊东南侧赤松林是造成孢粉组合空间分异的主要原因。孢粉浓度分布与湖泊水深具有良好的对应关系,体现了湖水流对孢粉的二次搬运和富集作用。现代森林草原地带Gun Nuur湖表层孢粉组合中松属含量较高,具超代表性;受松属影响蒿属和藜科花粉含量较低,代表性较低。 相似文献
11.
Late Holocene paleoenvironmental changes in subtropical Taiwan inferred from pollen and diatoms in lake sediments 总被引：1，自引：0，他引：1
Su-Hwa Chen Jiunn-Tzong Wu Tien-Nan Yang Pei-Pei Chuang Shu-Yue Huang Yun-Sen Wang 《Journal of Paleolimnology》2009,41(2):315-327
We analyzed pollen, spores, diatoms, organic carbon, nitrogen, and δ13C of organic matter in lake sediments to infer climate changes and reconstruct the paleo-environment of subtropical Taiwan
over the past ∼1300 years. A 31.5-cm sediment core that represents deposition from 650 AD to present was taken from a mountain
lake, Duck Pond, located 760 m a.s.l. We differentiated five zones using cluster analysis on pollen and spore assemblages.
Fluctuations in the relative abundances of arboreal taxa, herbaceous plants, and ferns reflect changes in the relative amounts
of woody versus grassland vegetation. Such shifts are associated with changes in temperature and humidity and are consistent
with climatic periods reported for the temperate region of central China. Climate changes inferred from the pollen assemblages
are also correlated well with changes in the ratios of fern spores to pollen, with organic carbon to nitrogen, and with the
δ13C values in the sediments. Fluctuations in these data throughout the entire core were in good agreement with the changes in
pH inferred from diatom assemblages. This study provides evidence of climate change in northern Taiwan over the past 1.3 millennia,
assuming that climate can be inferred from the ratio of arboreal to non-arboreal pollen and from the pH of the aquatic environment. 相似文献
12.
拜尔斯半岛位于南极利文斯顿岛最西部,是南设得兰群岛中最大的无冰区。对采自拜尔斯半岛的一根长55 cm的企鹅粪土沉积柱P1进行了元素和同位素地球化学分析。通过对沉积物C/N、有机质来源和δ15N的分析,发现P1沉积剖面中有机质主要来源于企鹅粪。利用富集系数、相关性分析、主成分分析等统计分析方法,识别出该沉积剖面中P、F、Cu、Hg、As、S六种元素具有共同的来源,与企鹅粪的输入密切相关,并且这些元素与TOC和δ15N显著正相关,说明沉积剖面中这些元素含量主要受控于企鹅粪的输入程度。通过与长城站区阿德雷岛、东南极戴维斯站加德纳岛企鹅粪土沉积物的标型元素特征比较,发现上述三个地区的标型元素组合大体上一致,反映了整个南极地区企鹅粪土沉积物生物标型元素组合的共性。研究结果为进一步恢复该地区的企鹅种群数量演化,及其对气候变化的响应提供了可能。 相似文献
13.
Malin E. Kylander Jonatan Klaminder Barbara Wohlfarth Ludvig Löwemark 《Journal of Paleolimnology》2013,50(1):57-70
There is a relatively good understanding of the paleoenvironmental changes that have occurred in southern Sweden since the Late Glacial. A main exception, however, is the sedimentary response of lacustrine systems during this period of rapid climate shifts. To address this, high-resolution X-ray fluorescence core scanning, Total Organic Carbon (TOC), C/N and δ13C analyses were made on a core from Hässeldala Port, a paleolake in the region. Site-specific geochemical analyses documented variations in silicate inputs (Zr/Ti, Si/Ti, K/Ti and K/Rb), productivity (TOC, Ca/Ti and Sr/Ti), as well as redox conditions in the sediment (δ13C, Mn/Ti and Fe/Ti), which were then linked to the regional climatic framework. During the Bølling/Older Dryas sediment accumulation was at its highest, particularly prior to colonization by terrestrial vegetation, and hydrological transport dominated. No clear signal of the Older Dryas was detected in the elemental chemistry. The Allerød was a period of relatively constant sediment accumulation, with the exception of during the Gerzensee oscillation when rates increased. There is evidence for increased within-lake and -catchment productivity and a change in silicate source during parts of the Allerød. As opposed to other records from the region, constant sediment accumulation rates were found during the Younger Dryas. Other proxies also suggest that this was a rather static period at Hässeldala Port. A gradual change in productivity and hydrological activity was observed from 12,000 cal year BP. The Preboreal section is rather short but the geochemical response was similar to that seen during other periods with milder climate conditions. The geochemical record archived in the sediments at Hässeldala Port was found to be the integrated result of physical erosion, landscape and soil development, vegetation changes, basin hydrology and moisture and temperature variations and it fills an important information gap in our understanding of the geochemical response of lake sediments to past climate change. 相似文献
14.
Jinglu Wu Long Ma Hong Yu Haiao Zeng Wen Liu Jilili Abuduwaili 《Journal of Paleolimnology》2013,50(2):245-255
We present a paleolimnological record from shallow Lake Wuliangsu in the Yellow River Basin, north China, using a short (56 cm) sediment core. Our objective was to investigate environmental changes in this semi-arid region over the past ~150 years. The sediment core was dated using 137Cs and 210Pb. We examined stratigraphic trends in core lithology, nutrients, stable isotopes (δ13C and δ15N) and trace element concentrations in the Lake Wuliangsu core to discern between natural sediments and those affected by human agency. A lithologic transition from yellow, coarse-grained sediment to grey, fined-grained sediment marked the lake’s formation about 1860. Until ~1950, sediments displayed relatively low and constant heavy metal concentrations, indicating little human influence. In the 1950s, enrichment factors (EFs) increased, reflecting greater impact of human activities. Carbon and nitrogen stable isotopes in organic matter (OM), along with heavy metal concentrations, were used to infer past shifts in trophic state and identify pollutants that came from agriculture, industry and urbanization. In the late 1950s, the first evidence for environmental change is recorded by increases in total organic carbon (TOC), total organic nitrogen (TN), TOC/TN, EFs, δ13C and a decrease in δ15N. After about year 2000, a more rapid increase in trophic status occurred, as indicated by greater total phosphorus (TP), EFs, δ15N and lower δ13C values. Changes in isotope and TOC/TN values in the lake sediments may reflect a shift in lake ecology during this period. The first increase in trophic status during the late 1950s was mainly a result of agricultural development in the catchment. In contrast, the change after ca. AD 2000 was driven largely by urban and industrial development. Agreement between paleolimnologic data from Lake Wuliangsu, and both instrumental and written records, indicates that the lake sediments provide a reliable archive for investigating the formation and environmental history of the lake. 相似文献
15.
Climatic and environmental change in Yanchi Lake, Northwest China since the Late Glacial: A comprehensive analysis of lake sediments 总被引：1，自引：0，他引：1
Modern climate research has shown that the Asian summer monsoon water vapor transport is limited to the eastern part of the Qilian Mountains. On the Holocene millennial-scale, whether the northwest boundary of the summer monsoon varies according to climate change is a key scientific issue. Yanchi Lake is located in the northern Qilian Mountains and the middle of the Hexi Corridor, where the modern climate is less affected by the Asian summer monsoon. It is a key research area for examining the long-term variations of the Asian summer monsoon. Paleoclimatic data, including AMS ^14C dates of pollen concentrates and bulk organic carbon, lithology, grain-size, mineral composition and geochemical proxies were acquired from sediments of Yanchi Lake. The chronological results show that the lower part of the lacustrine section is formed mainly in the Late Glacial and early Holocene period, while the proxies＇ data indicate the lake expansion is associated with high content of mineral salts. The middle part of this section is formed during the transitional period of the early and middle Holocene. Affected by the reworking effect, the pollen concentrates AMS^14C dates from the middle part of the section are generally older than those from the lower part. Since the mid-Holocene, Yanchi Lake retreated significantly and the deposition rate dropped obvi- ously. The Yanchi Lake record is consistent with the Late Glacial and Holocene lake records in the Qinghai-Tibet Plateau and the climatic records in typical monsoon domain, which indicate the lake expansion and the strong Asian summer monsoon during the Late Glacial and early Holocene. The long-term monsoonal pattern is different from the lake evolution in Central Asia on the Holocene millennial-scale. This study proves the monsoon impacts on the northwestern margin of the summer monsoon, and also proves the fact that the northern boundary of the summer monsoon moves according to millennial-scale climate change. 相似文献
16.
Luciane Fontana Ana Luiza S. Albuquerque Mark Brenner Daniel M. Bonotto Tatiani P. P. Sabaris Maria A. F. Pires Marycel E. B. Cotrim Denise C. Bicudo 《Journal of Paleolimnology》2014,51(1):29-43
Guarapiranga Reservoir is the second most important public water supply in São Paulo, Brazil and has been eutrophic for several decades. We inferred the major ecological shifts for the period 1919–2010 related to multiple stressors (forest flooding, hydrological change, use of algicide and eutrophication), using geochemistry (TOC, TN, TP, C/N, δ15N, δ13C) and diatom assemblages in a short (75-cm) sediment core. Thirty-two diatom species were abundant in the core and stratigraphically constrained incremental sum of squares analysis enabled identification of three diatom zones and four subzones, i.e. depths at which marked changes in species composition occurred. Early diatom assemblages were dominated by benthic, oligotrophic taxa, mainly Eunotia, influenced by flooded vegetation after dam construction. A shift to dominance by a planktonic species (Eunotia tukanorum) occurred ca. 1932, during the period of initial physical disturbance and early use of the water body as a public water supply. Diatoms and geochemical variables show that the reservoir was oligotrophic from ~1919 to 1947. Eutrophication began ~1975 and by the early 1980s the reservoir had become eutrophic, in response to an explosive increase in human population in the watershed. Severe cultural eutrophication has persisted since ~1990. Higher concentrations of copper in the sediments, beginning in 1991, reflect the increased use of copper sulfate to control cyanobacteria blooms and provide a chronological marker. Higher δ15N values in recent sediments indicate greater sewage inputs and low C/N values reflect the predominant contribution of algae to sediment organic matter. Eutrophic taxa Cyclotella meneghiniana and Nitzschia sp. dominate recent diatom assemblages, along with Aulacoseira granulata, a species that is tolerant of copper sulfate. Diatom assemblages reflect multiple stressors, however, geochemical information provides a better understanding of the early phase of the reservoir. Paleolimnologically documented trophic state changes in this important drinking water supply are largely attributable to increased urbanization of the drainage basin and inputs of sewage. Management efforts should focus on mitigating this nutrient source. 相似文献
17.
Wu Jinglu Huang Chengmin Zeng Haiao Gerhard H. Schleser Rick Battarbee 《Journal of Paleolimnology》2007,38(1):13-23
Environmental change in Lake Taihu and its catchment since the early to middle part of the twentieth century has left a clear
geochemical record in the lake sediments. The human activities in the lake and its catchment responsible for the change include
agriculture, fishery, urbanisation, sewage and industrial waster disposal. Sediment cores were collected from Meilian Bay
of northern Lake Taihu to investigate the record of anthropogenic impacts on the lake’s ecosystem and to assess its natural,
pre-eutrophication baseline state. Two marked stratigraphic sediment units were identified on the basis of total phosphorus
concentration (TP), pigments, total organic carbon (TOC)/total nitrogen (TN), δ13C and δ15N corresponding to stages in the lake history dominated by phytoplankton, and by aquatic macrophytes. Results show that as
TP loading increased from the early 1950s the lake produced sediments with increasing amounts of organic matter derived from
phytoplankton. In the early 1950s, the first evidence for eutrophication at the Meilian Bay site is recorded by an increase
in C/N values and in sediment accumulation rate, but there is little change in phosphorus concentrations, pigments, δ13C and δ15N at this time. After 1990 a more rapid increase in trophic status took place indicated by increased levels of phosphorus,
pigments, δ15N and by decreased δ13C and TOC/TN values in the lake sediments. The first increase in trophic status of the early 1950s results mainly from agricultural
development in the catchment. In contrast, the acceleration from ca. 1990 originates from the recent development of fisheries
and the urbanisation and industrialisation of the catchment. 相似文献