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31.
Using an Atmospheric Global Circulation Model, we assess the relevance of selected atmospheric mechanisms for climate evolution of Saharan and sub-Saharan regions since the Miocene. First, we test the influence of the East-African Rift System uplift on atmospheric dynamics. Although the uplift played an important role in triggering East-African rainfall, no significant impact over central and western Africa has been detected. We also analyse the feedbacks of a giant lake on the climate of Chad basin. First results infer a negative feedback of the giant lake on the water balance, as convection is weakened by the cold water surface and as water evaporated from the lake does not feed the basin hydrological cycle. Lastly, we suggest that colder than present sea surface temperatures over the Gulf of Guinea reinforce the West-African monsoon, by enhancing the moisture advection engine via stronger thermal contrast between the ocean and the continent. 相似文献
32.
Determination of Rare Earth Elements, Sc, Y, Zr, Ba, Hf and Th in Geological Samples by ICP-MS after Tm Addition and Alkaline Fusion 总被引:2,自引:0,他引:2
Germain Bayon Jean Alix Barrat Joël Etoubleau Mathieu Benoit Claire Bollinger Sidonie Révillon 《Geostandards and Geoanalytical Research》2009,33(1):51-62
We present a revised method for the determination of concentrations of rare earth (REE) and other trace elements (Y, Sc, Zr, Ba, Hf, Th) in geological samples. Our analytical procedure involves sample digestion using alkaline fusion (NaOH-Na2 O2 ) after addition of a Tm spike, co-precipitation on iron hydroxides, and measurement by sector field-inductively coupled plasma-mass spectrometry (SF-ICP-MS). The procedure was tested successfully for various rock types (i.e., basalt, ultramafic rock, sediment, soil, granite), including rocks with low trace element abundances (sub ng g−1 ). Results obtained for a series of nine geological reference materials (BIR-1, BCR-2, UB-N, JP-1, AC-E, MA-N, MAG-1, GSMS-2, GSS-4) are in reasonable agreement with published working values. 相似文献
33.
Pierre Polsenaere Nicolas Savoye Henri Etcheber Mathieu Canton Dominique Poirier Steven Bouillon Gwenaël Abril 《Aquatic Sciences - Research Across Boundaries》2013,75(2):299-319
We measured spatial and temporal variations in carbon concentrations, isotopic compositions and exports during a complete hydrological cycle in nine watercourses draining a lowland forested podzolized catchment, flowing into the Arcachon lagoon (France). In addition, integrated fluxes of CO2 across the water-atmosphere interface were estimated to assess the relative importance of CO2 evasion versus lateral carbon transport at the catchment scale. Watercourse similarities and specificities linked to the local catchment characteristics are discussed and compared with other riverine systems. Low concentrations of suspended particulate matter and particulate organic carbon (POC) were generally measured in all the watercourses (8.4 ± 3.4 and 1.6 ± 0.6 mg L?1, respectively), reflecting limited mechanical soil erosion. The generally high POC content in the suspended matter (20 %), low Chl a concentrations (1.3 ± 1.4 μg L?1) and the relatively constant δ13C-POC value (near ?28 ‰) throughout the year reveal this POC originates from terrestrial C3 plant and soil detritus. The presence of podzols leads to high levels of dissolved organic carbon (DOC; 6.6 ± 2.2 mg L?1). Similarly, high dissolved inorganic carbon (DIC) concentrations were measured in the Arcachon lagoon catchment (5.9 ± 2.2 mg L?1). The δ13C-DIC value around ?20 ‰ throughout the year in many small watercourses reveals the predominance of terrestrial carbon mineralisation and silicate rock weathering in soils as the major DIC source. With pCO2 between 1,000 and 10,000 ppmv, all watercourses were a source of CO2 to the atmosphere, particularly during the low river stage. Organic carbon parameters remained relatively stable throughout the year, whereas DIC parameters showed strong seasonal contrasts closely linked to the hydrological regime and hyporheic flows. In total, the carbon export from the Arcachon watershed was estimated at 15,870 t C year?1 or 6 t C km?2 year?1, mostly exported to the lagoon as DOC (35 %), DIC (24 %) and lost as CO2 degassing to the atmosphere (34 %). 相似文献
34.
35.
Franoise Bergerat Pierre-Yves Collin Anne-Cline Ganzhorn Franois Baudin Bruno Galbrun Isabelle Rouget Johann Schnyder 《Journal of Geodynamics》2011,51(5):344-357
Instability structures, synsedimentary faults and turbidites have been studied in the Lower Pliensbachian succession of Saint-Michel-en-Beaumont, belonging to the Taillefer block, an ancient half-graben emplaced during the Liassic Tethyan rifting. Geometrical and mechanical analyses demonstrate that the instability structures occurred thanks to movements along spineless synsedimentary normal faults, when the turbiditic and limestone layers were already case-hardened and partly fractured by tension gashes even when the mudstones were still unlithified. Both the tension gashes and the synsedimentary faults are homogeneous in strike with the major regional faults and are in good agreement with the regional direction of extension for this period. The characters of the turbiditic beds, with erosive base, graded bedding, and incomplete Bouma sequence, are in favour of a seismic origin. Instability structures, spineless synsedimentary faults and turbiditic inflows are thus considered as seismites and interpreted as the result of high seismicity periods including some events with M > 5 in the general extensive ambiance of the Liassic Tethyan rifting. The analysis of the geometrical relationships between all these sedimentary features allows to distinguish the successive stage of occurrence of an instability structure, from the sedimentation of alternating marls and limestones, and sudden turbiditic inflows, then early case-hardening of the turbidites, until the important seismotectonic event generating the spineless normal faults, themselves triggering the fall of indurated blocks and locally the forming of breccias. The Ornon Fault, which constitutes the border of the Taillefer block, 15 km eastward, played a major role during the Liassic sedimentation and may represent the major seismic fault related to the seismites occurrence in the Beaumont basin. 相似文献
36.
The sodium solubility in silicate melts in the CaO-MgO-SiO2 (CMS) system at 1400 °C has been measured by using a closed thermochemical reactor designed to control alkali metal activity. In this reactor, Na(g) evaporation from a Na2O-xSiO2 melt imposes an alkali metal vapor pressure in equilibrium with the molten silicate samples. Because of equilibrium conditions in the reactor, the activity of sodium-metal oxide in the molten samples is the same as that of the source, i.e., aNa2O(sample) = aNa2O(source). This design also allows to determine the sodium oxide activity coefficient in the samples. Thirty-three different CMS compositions were studied. The results show that the amount of sodium entering from the gas phase (i.e., Na2O solubility) is strongly sensitive to silica content of the melt and, to a lesser extent, the relative amounts of CaO and MgO. Despite the large range of tested melt compositions (0 < CaO and MgO < 40; 40 < SiO2 < 100; in wt%), we found that Na2O solubility is conveniently modeled as a linear function of the optical basicity (Λ) calculated on a Na-free basis melt composition. In our experiments, γNa2O(sample) ranges from 7 × 10−7 to 5 × 10−6, indicating a strongly non-ideal behavior of Na2O solubility in the studied CMS melts (γNa2O(sample) ? 1). In addition to showing the effect of sodium on phase relationships in the CMS system, this Na2O solubility study brings valuable new constraints on how melt structure controls the solubility of Na in the CMS silicate melts. Our results suggest that Na2O addition causes depolymerization of the melt by preferential breaking of Si-O-Si bonds of the most polymerized tetrahedral sites, mainly Q4. 相似文献
37.
Julien Mercadier Michel Cuney Michel Cathelineau Mathieu Lacorde 《Mineralium Deposita》2011,46(2):105-135
Proterozoic basement-hosted unconformity-related uranium deposits of the Athabasca Basin (Saskatchewan, Canada) were affected
by significant uranium redistribution along oxidation–reduction redox fronts related to cold and late meteoric fluid infiltration.
These redox fronts exhibit the same mineralogical and geochemical features as the well-studied uranium roll-front deposits
in siliclastic rocks. The primary hydrothermal uranium mineralisation (1.6–1.3 Ga) of basement-hosted deposits is strongly
reworked to new disseminated ores comprising three distinctly coloured zones: a white-green zone corresponding to the previous
clay-rich alteration halo contemporaneous with hydrothermal ores, a uranium front corresponding to the uranium deposition
zone of the redox front (brownish zone, rich in goethite) and a hematite-rich red zone marking the front progression. The
three zones directly reflect the mineralogical zonation related to uranium oxides (pitchblende), sulphides, iron minerals
(hematite and goethite) and alumino-phosphate-sulphate (APS) minerals. The zoning can be explained by processes of dissolution–precipitation
along a redox interface and was produced by the infiltration of cold (<50°C) meteoric fluids to the hydrothermally altered
areas. U, Fe, Ca, Pb, S, REE, V, Y, W, Mo and Se were the main mobile elements in this process, and their distribution within
the three zones was, for most of them, directly dependent on their redox potential. The elements concentrated in the redox
fronts were sourced by the alteration of previously crystallised hydrothermal minerals, such as uranium oxides and light rare
earth element (LREE)-rich APS. The uranium oxides from the redox front are characterised by LREE-enriched patterns, which
differ from those of unconformity-related ores and clearly demonstrate their distinct conditions of formation. Uranium redox
front formation is thought to be linked to fluid circulation episodes initiated during the 400–300 Ma period during uplift
and erosion of the Athabasca Basin when it was near the Equator and to have been still active during the last million years.
A major kaolinisation event was caused by changes in the fluid circulation regime, reworking the primary uranium redox fronts
and causing the redistribution of elements originally concentrated in the uranium-enriched meteoric-related redox fronts. 相似文献
38.
Alexandre Forest Jean-Éric Tremblay Yves Gratton Johannie Martin Jonathan Gagnon Gérald Darnis Makoto Sampei Louis Fortier Mathieu Ardyna Michel Gosselin Hiroshi Hattori Dan Nguyen Roxane Maranger Dolors Vaqué Cèlia Marrasé Carlos Pedrós-Alió Amélie Sallon Christine Michel Colleen Kellogg Jody Deming Elizabeth Shadwick Helmuth Thomas Heike Link Philippe Archambault Dieter Piepenburg 《Progress in Oceanography》2011,91(4):410-436
Major pathways of biogenic carbon (C) flow are resolved for the planktonic food web of the flaw lead polynya system of the Amundsen Gulf (southeast Beaufort Sea, Arctic Ocean) in spring-summer 2008. This period was relevant to study the effect of climate change on Arctic marine ecosystems as it was characterized by unusually low ice cover and warm sea surface temperature. Our synthesis relied on a mass balance estimate of gross primary production (GPP) of 52.5 ± 12.5 g C m−2 calculated using the drawdown of nitrate and dissolved inorganic C, and a seasonal f-ratio of 0.64. Based on chlorophyll a biomass, we estimated that GPP was dominated by phytoplankton (93.6%) over ice algae (6.4%) and by large cells (>5 μm, 67.6%) over small cells (<5 μm, 32.4%). Ancillary in situ data on bacterial production, zooplankton biomass and respiration, herbivory, bacterivory, vertical particle fluxes, pools of particulate and dissolved organic carbon (POC, DOC), net community production (NCP), as well as selected variables from the literature were used to evaluate the fate of size-fractionated GPP in the ecosystem. The structure and functioning of the planktonic food web was elucidated through inverse analysis using the mean GPP and the 95% confidence limits of every other field measurement as lower and upper constraints. The model computed a net primary production of 49.2 g C m−2, which was directly channeled toward dominant calanoid copepods (i.e. Calanus hyperboreus 20%, Calanus glacialis 10%, and Metridia longa 10%), other mesozooplankton (12%), microzooplankton (14%), detrital POC (18%), and DOC (16%). Bacteria required 29.9 g C m−2, a demand met entirely by the DOC derived from local biological activities. The ultimate C outflow comprised respiration fluxes (82% of the initial GPP), a small sedimentation (3%), and a modest residual C flow (15%) resulting from NCP, dilution and accumulation. The sinking C flux at the model limit depth (395 m) supplied 60% of the estimated benthic C demand (2.8 g C m−2), suggesting that the benthos relied partly on other C sources within the bottom boundary layer to fuel its activity. In summary, our results illustrate that the ongoing decline in Arctic sea ice promotes the growth of pelagic communities in the Amundsen Gulf, which benefited from a ∼80% increase in GPP in spring-summer 2008 when compared to 2004 – a year of average ice conditions and relatively low GPP. However, 53% of the secondary production was generated within the microbial food web, the net ecological efficiency of zooplankton populations was not particularly high (13.4%), and the quantity of biogenic C available for trophic export remained low (6.6 g C m−2). Hence it is unlikely that the increase in lower food web productivity, such as the one observed in our study, could support new harvestable fishery resources in the offshore Beaufort Sea domain. 相似文献
39.
40.
G. W. Harris D. Klemp T. Zenker J. P. Burrows B. Mathieu 《Journal of Atmospheric Chemistry》1992,15(3-4):315-326
Measurements of NO2, HCHO, and H2O2 were made by the highly specific method of mid infra-red absorption spectroscopy using tunable diode lasers (TDLAS) during the 1988 Polarstern expedition. The TDLAS data are compared to those obtained during the cruise using less direct methods. Southern Hemisphere NO2 levels suggest nett photochemical destruction of O3 in the boundary layer. Northern Hemisphere HCHO averaged 0.47±0.2 ppbv; the HCHO measurements are used in a simple calculation to estimate OH noontime maxima of 3–6×106 cm-3. 相似文献