Vertical structures of PM10 and PM 2.5 and their dynamical character in low atmosphere in Beijing urban areas     

DING Guoan  CHAN Chuenyu  GAO Zhiqiu  YAO Wenqing  LI Yoksheung  CHENG Xinghong  MENG Zhaoyang  YU Haiqing  WONG Kamhang  WANG Shufeng  MIAO Qiuju 《中国科学D辑(英文版)》2005,48(Z2)

The vertical structures and their dynamical character of PM2.5 and PM10 over Beijing urban areas are revealed using the 1 min mean continuous mass concentration data of PM2.5 and PM10 at 8, 100, and 320 m heights of the meteorological observation tower of 325 m at Institute of Atmospheric Physics, Chinese Academy of Sciences (IAP CAS tower hereafter) on 10―26 August, 2003, as well as the daily mean mass concentration data of PM2.5 and PM10 and the continuous data of CO and NO2 at 8, 100 (low layer), 200 (middle layer), and 320 m (high layer) heights, in combination with the same period meteorological field observation data of the meteorological tower. The vertical distributions of aerosols observed on IAP CAS tower in Beijing can be roughly divided into two patterns: gradually and rapidly decreasing patterns, I.e. The vertical distribution of aerosols in calm weather or on pollution day belongs to the gradually decreasing pattern, while one on clean day or weak cold air day belongs to the rapidly decreasing pattern. The vertical distributive characters of aerosols were closely related with the dynamical/thermal structure and turbulence character of the atmosphere boundary layer. On the clean day, the low layer PM2.5 and PM10 concentrations were close to those at 8 m height, while the concentrations rapidly decreased at the high layer, and their values were only one half of those at 8 m, especially, the concentration of PM2.5 dropped even more. On the clean day, there existed stronger turbulence below 150 m, aerosols were well mixed, but blocked by the more stronger inversion layer aloft, and meanwhile, at various heights, especially in the high layer, the horizontal wind speed was larger, resulting in the rapid decrease of aerosol concentration, I.e. Resulting in the obvious vertical difference of aerosol concentrations between the low and high layers. On the pollution day, the concentrations of PM2.5 and PM10 at the low, middle, and high layers dropped successively by, on average, about 10% for each layer in comparison with those at 8 m height. On pollution days, in company with the low wind speed, there existed two shallow inversion layers in the boundary layer, but aerosols might be, to some extent, mixed below the inversion layer, therefore, on the pollution day the concentrations of PM2.5 and PM10 dropped with height slowly; and the observational results also show that the concentrations at 320 m height were obviously high under SW and SE winds, but at other heights, the concentrations were not correlated with wind directions. The computational results of footprint analysis suggest that this was due to the fact that the 320 m height was impacted by the pollutants transfer of southerly flow from the southern peripheral heavier polluted areas, such as Baoding, and Shijiazhuang of Hebei Province, Tianjin, and Shandong Province, etc., while the low layer was only affected by Beijing's local pollution source. The computational results of power spectra and periods preliminarily reveal that under the condition of calm weather, the periods of PM10 concentration at various heights of the tower were on the order of minutes, while in cases of larger wind speed, the concentrations of PM2.5 and PM10 at 320 m height not only had the short periods of minute-order, but also the longer periods of hour order. Consistent with the conclusion previously drawn by Ding et al., that air pollutants at different heights and at different sites in Beijing had the character of "in-phase" variation, was also observed for the diurnal variation and mean diurnal variation of PM2.5 and PM10 at various heights of the tower in this experiment, again confirming the "in-phase" temporal/spatial distributive character of air pollutants in the urban canopy of Beijing. The gentle double-peak character of the mean diurnal variation of PM2.5 and PM10 was closely related with the evident/similar diurnal variation of turbulent momentum fluxes, sensible heat fluxes, and turbulent kinetic energy at various heights in the urban canopy. Besides, under the condition of calm weather, the concentration of PM2.5 and PM10 declined with height slowly, it was 90% of 8 m concentration at the low layer, a little lesser than 90% at the middle layer, and 80% at the high layer, respectively. Under the condition of weak cold air weather, the concentration remarkably dropped with height, it was 70% of 8 m concentration at the low layer, and 20%―30% at the middle and high layers, especially the concentration of PM2.5 was even lower.  相似文献   

Spatial character of the gaseous and particulate state compound correlation of urban atmospheric pollution in winter and summer   总被引：1，自引：0，他引：1  

XU Xiangde  SHI Xiaohui  XIE Lian  DING Guoan  MIAO Qiuju  MA Jianzhong  ZHENG Xiangdong 《中国科学D辑(英文版)》2005,48(Z2)

The spatial/temporal variation information of atmospheric dynamic-chemical processes at observation site points of the "canopy" boundary of Beijing urban building ensemble and over urban area "surface", as well as the seasonal correlation structure of the gaseous and particulate states of urban atmospheric pollution (UAP) and its seasonal conversion feature at observation points are investigated, using the comprehensive observation data of the Beijing City Air Pollution Observation Experiment (BECAPEX) in winter and summer 2003 with a "point-surface" combined research approach. By using "one dimension spatial empirical orthogonal function (EOF)" principal component analysis (PCA) mode, the seasonal change of gaseous and particulate states of atmospheric aerosols and the association feature of pollutant species under the background of the complicated structure of urban boundary layer (UBL) are analyzed. The comprehensive analyses of the principal components of particle concentrations,gaseous pollutant species, and meteorological conditions reveal the seasonal changes of the complex constituent and structure features of the gaseous and particulate states of UAP to further trace the impact feature of urban aerosol pollution surface sources and the seasonal difference of the component structure of UAP. Research results suggest that in the temporal evolution of the gaseous and particulate states of winter/summer UAP, NOx, CO, and SO2 showed an "in-phase" evolution feature, however, O3 showed an "inverse-phase" relation with other species,all possessing distinctive dependent feature. On the whole, summer concentrations of gaseous pollutants CO, SO2, and NOx were obviously lower than winter ones, especially, the reduction in CO concentration was most distinctive, and ones in SO2 and NOx were next. However, the summer O3 concentration was more than twice winter one. Winter/summer differences in PM10and PM2.5 particle concentrations were relatively not obvious, which indicates that responses of PM10 and PM2.5 particle concentrations to the difference of winter/summer heating period emission sources are far less distinctive than those of NOx, SO2, and CO. The correlation feature of winter/summer gaseous and particulate states depicts that both PM10 and PM2.5 particles were significantly correlated with NOx, and their correlations with NOx are more significant than those with other pollutants. Through PCA, it is found that there was a distinctive difference in the principal component combination structure of winter/summer PM10 and PM2.5 particles: SO2 and NOx dominated in the principal component of winter PM10 and PM2.5 particles; while CO and NOx played the major role in the principal component of summer PM10 and PM2.5 particles. For winter/summer PM10 and PM2.5 particles, there might exist the gaseous and particulate states correlation structures of different "combinations" of such dependent pollutant species. Research results also uncover that the interaction processes of gaseous and particulate states were also related with the vertical structure of UBL, that is to say, the low value layer of UBL O3 concentration was associated with the collocation of atmospheric vertical structures of the low level inversion,inverse humidity, and small wind, which depicts summer boundary layer atmospheric character, i.e.the compound impact of the dependent factor "combination" of wind, temperature, and humidity elements and their collocation structure on the variations of different gaseous pollutant concentrations. Such a depth structure of the extremely low value of O3 concentration in the UBL accords with its "inverse-phase" relation with other gaseous pollutant species. The PCA of meteorological factors associated with PM10 and PM2.5 concentrations also reveals the sensitivity of PM10 and PM2.5 concentration to the combinatory feature of local meteorological conditions.  相似文献   

吉林海沟金矿矿山地质环境及其恢复治理方法   总被引：1，自引：0，他引：1  

孙春  赵洪满  程明华 《吉林地质》2005,24(3):61-65

在对海沟金矿矿山地质环境调查基础上，针对矿区存在着的问题，提出了治理与防范措施，对同类矿山有借鉴作用。  相似文献   

惰性气体法测定地下水入渗补给量     

王凤林  毛绪美  程胜高  刘存富 《地球学报》2005,26(Z1):283-285

地下水入渗补给量是重要的水文地质参数。本文介绍了测定地下水入渗补给量的最新方法——惰性气体法的原理与方法，该方法适用于封闭条件下的深层地下水。  相似文献   

生态城市的内涵及建设策略   总被引：7，自引：4，他引：7  

程伟 《云南地理环境研究》2005,17(4):43-45

生态城市是通过倡导生态理念，采用生态技术，建立生态化产业体系，从而达到社会、经济、环境的可持续发展，实现自然生态平衡、人文生态和谐的城乡统一体。从可持续发展的角度出发，利用生态学和社会学的观点，论述生态城市的内涵，提出科学的城市规划、合理的城市评价指标体系、完善的城市管理制度是实现生态城市的前提，强调只有自然生态、人文生态两手抓才能真正实现经济、社会、环境全面发展。  相似文献   

A high‐resolution monsoon record of millennial‐scale oscillations during Late MIS 3 from Wulu Cave,south‐west China          下载免费PDF全文

FUCAI DUAN  DIANBING LIU  HAI CHENG  XIANFENG WANG  YONGJIN WANG  XINGGONG KONG  SHITAO CHEN 《第四纪科学杂志》2014,29(1):83-90

  相似文献   

Efficient estimation of flood forecast prediction intervals via single‐ and multi‐objective versions of the LUBE method          下载免费PDF全文

Lei Ye  Jianzhong Zhou  Hoshin V. Gupta  Hairong Zhang  Xiaofan Zeng  Lu Chen 《水文研究》2016,30(15):2703-2716

Prediction intervals (PIs) are commonly used to quantify the accuracy and precision of a forecast. However, traditional ways to construct PIs typically require strong assumptions about data distribution and involve a large computational burden. Here, we improve upon the recent proposed Lower Upper Bound Estimation method and extend it to a multi‐objective framework. The proposed methods are demonstrated using a real‐world flood forecasting case study for the upper Yangtze River Watershed. Results indicate that the proposed methods are able to efficiently construct appropriate PIs, while outperforming other methods including the widely used Generalized Likelihood Uncertainty Estimation approach. Copyright © 2016 John Wiley & Sons, Ltd.  相似文献   

基于等高线隔断线确定DEM适宜分辨率的方法研究     

程德强  高春留  赵牡丹 《测绘科学技术学报》2016,(3):306-312

分辨率是等高线数据插值生成格网DEM数据过程中需要考虑的一个重要参数,适宜的分辨率既能将等高线高程信息尽可能保留,又不会因插值造成数据冗余及误差。基于对格网DEM生成方式的理解,提出了等高线隔断线的相关概念,分析了基于地形图矢量化的等高线数据插值生成格网DEM数据,由不同长度等高线隔断线频率统计来确定格网适宜分辨率参考值的方法。同时,不同长度等高线隔断线的长度与其频率相乘得到标准长度,以及等高线隔断线中心点生成的密度分析图,均可在频率特征决定适宜分辨率参考值时起到一定的参考作用。通过样区实验验证,实现简便,可度量性强,与其他相关研究具有一致性,对确定适宜格网分辨率参考值具有一定的借鉴意义。  相似文献   

利用LA-ICP-MS在16 μm和10 μm激光束斑条件下测定独居石U-Th-Pb年龄     

汪双双  韩延兵  李艳广  魏小燕  靳梦琪  程秀花 《岩矿测试》2016,35(4):349-357

我国锂钾主要矿产资源大多分布在西部偏远地区,其勘查找矿或综合利用迫切需要现场快速分析技术的支持。本文介绍了自行开发的便携式Li-K分析仪的主要性能及其在锂辉石中锂的分析应用。Li-K分析仪是一种基于大气压的液体阴极辉光放电光谱仪,以待测液体为放电阴极,实现样品中Li、K等元素的原子化和激发。该仪器以光纤传导CCD光谱仪作为检测器,其波长范围为345～1015 nm,分辨率3 nm;以Li 670.78 nm和K 769.90 nm分析谱线,在最佳仪器工作条件下测定Li、K的精密度（RSD,n=14）均低于2%,检出限为0.03 μg/mL,检测范围0.1～10 μg/mL。研究表明,不同酸度和酸的类型对谱线强度影响较大,且存在显著的样品基体效应,标准曲线法分析锂辉石中Li的结果偏差高达267%;而标准加入法可克服基体效应的影响,获得与ICP-OES一致性较好的分析结果,为现场开展固体样品中Li的测定奠定了基础。  相似文献   

河北东坪金矿地质地球化学特征     

谭杰  程志中  甄世民  袁琛晖 《地质论评》2016,62(S1):45-46

东坪金矿位于河北省崇礼区,大地构造处于华北地台北缘,燕辽沉降带与内蒙地轴结合处南侧,距尚义-崇礼-赤城深大断裂10km。区内出露地层主要为太古界桑干群变质岩系,岩性以片麻岩为主。区内断裂构造较发育,主要有EW向,NW向和NE向,其中以EW向的最为发育。 区内岩浆岩也比较发育,沿尚义-崇礼-赤城深大断裂分布,主要有小张家口超基性岩、水泉沟碱性杂岩和上水泉花岗岩。水泉沟碱性杂岩体呈EW向展布,向南北两侧倾斜,主要岩性为碱性长石正长岩、辉石角闪碱性长石正长岩、辉石角闪正长岩和角闪碱性长石正长岩等。  相似文献